arXiv subjects

Barry Bradlyn

Publications and source records attributed to Barry Bradlyn.

At least 19 recordsLinked to original sources

arXiv2026

Multi-State Geometry of Density Matrices and Rectification Sum Rules

The geometry of quantum states has emerged as a key ingredient in understanding the linear and nonlinear responses of quantum materials. To date, however, the connection between geometry and nonlinear response is best understood for clean, noninteracting systems at zero temperature. In this work, we develop a theory of multi-state geometry for density matrices and use it to derive sum rules for second-order rectification, making no assumptions about the strength of disorder or interactions. We first show that perturbation theory for thermal density matrices gives rise to two dual information-theoretic connections and an almost complex structure. We introduce a complex, quantum generalization of the Amari-Chentsov tensor of classical information theory, the cQAC tensor, which captures the multi-state geometry of the perturbed density matrix. We derive a zero-temperature sum rule for the frequency-integrated DC rectification response of an insulator as a difference between a ground state third cumulant and the complex distortion tensor, a multi-state geometric quantity built from the cQAC tensor. This generalizes known single-particle sum rules for the shift and nonlinear Hall currents to many-body systems and general perturbations. Specializing to the shift current, we resolve the geometric contribution for multiband insulators into particle-like and hole-like terms. We verify the sum rule numerically in a generalized Kane-Mele model, finding that the geometric contribution can dominate the integrated response. Finally, we show that although the splitting of the sum rule into cumulant and geometric contributions does not survive at nonzero temperature, the measured sum rule for insulators differs from its zero-temperature form by corrections exponentially small in the gap, allowing low-temperature rectification measurements to probe the multi-state geometry of insulators.

cond-mat.mes-hall↗

arXiv2026

Stable Real-Space Invariants and Topology Beyond Symmetry Indicators

We introduce stable real-space invariants (SRSIs), topological invariants defined from adiabatic deformations between Wannier states, generalizing previously discovered local and composite real-space invariants. SRSIs are $\mathbb{Z}$- and $\mathbb{Z}_n$-valued ($n=2,4$) linear combinations of Wannier state multiplicities characterizing the stable equivalence of atomic insulators. We enumerate all SRSIs in nonmagnetic space groups with and without spin-orbit coupling. $\mathbb{Z}$SRSIs are in one-to-one correspondence with momentum-space symmetry data and thus determine symmetry indicators of topology (SIs). $\mathbb{Z}_n$SRSIs capture real-space information beyond momentum-space symmetry data and SIs. Applying SRSIs to split elementary band representations (EBRs) whose symmetry data decomposes into positive sums of other EBR symmetry data, we diagnose the topology of all 211 cases across 51 space groups except for 8 exceptions in 5 space groups. Our results solidify Topological Quantum Chemistry beyond SIs and momentum-space symmetry data. Finally, we use SRSIs to diagnose an obstructed atomic insulator in a realistic material.

cond-mat.mes-hall↗

arXiv2026

Imaginary Time Formalism for Causal Nonlinear Response Functions

It is well established that causal linear response functions can be found by computing the much simpler imaginary time-ordered Matsubara functions and performing an analytic continuation. This principle is the basis for much of our understanding of linear response for interacting and disordered systems, via diagrammatic perturbation theory. Similar imaginary-time approaches have recently been introduced for computing nonlinear response functions as well, for example in [Annalen der Physik 536, 2300504 (2024); Physical Review X 11, 041006 (2021)], where the authors analytically continue the Matsubara functions to obtain the Keldysh response functions. In this work, we provide a proof of this connection to all orders in perturbation theory using an equation of motion based approach. We show by induction that causal nonlinear response functions at every order can be obtained from an analytic continuation of an appropriate time-ordered Matsubara function. We demonstrate this connection explicitly for second order response functions in the Lehmann representation. As a byproduct of our approach, we derive an explicit expression for the Lehmann representation of $n$-th order response functions by solving the equations of motion. We also use our result to find an analytic spectral density representation for both causal response functions and Matsubara functions. As an example, we apply our method to derive the non-linear $A^3$ term in the $SU(2)$ spin Hall response of an insulator with spin rotation symmetry. Finally, we show how our results lead to a family of generalized sum rules, focusing explicitly on the asymptotic expression for $n$-th harmonic generation rate. Our work opens the door to using imaginary time approaches to study nonlinear response functions in general condensed matter systems.

cond-mat.mes-hall↗

arXiv2026

Leggett-Garg Inequality Violations Bound Quantum Fisher Information

We prove that a violation of a Leggett-Garg inequality for bounded observables in stationary pure states and thermal states yields a rigorous lower bound on the quantum Fisher information. This turns a qualitative foundations test of realism in quantum systems into a quantitative witness of useful quantum sensitivity and, in the collective setting, into a lower bound on multipartite entanglement depth in many-body systems. We further demonstrate that Leggett-Garg violations are constrained by the same spectral moments, susceptibilities, and $f$-sum-rule bounds that organize many-body response. Our results show that temporal correlations of a single collective observable can serve as an experimentally accessible witness of many-body quantum coherence, without requiring full state reconstruction.

quant-ph↗

arXiv2026

Decomposing momentum scales in the Hubbard Model: From Hatsugai-Kohmoto to Aubry-André

The all-to-all momentum coupling of the Hubbard interaction makes interacting lattice models generically unsolvable. In many settings, however, from Peierls instabilities to Moiré superlattice physics, the low-energy behavior is dominated by scattering at a few characteristic wavevectors. We exploit this by constructing a momentum-space clustering scheme that retains only a chosen subset of interaction channels. Our scheme can be considered a generalization of twist-averaged boundary conditions. In proving this, we also prove that our scheme can be considered as a generalization of Hatsugai-Kohmoto (HK) models, and all versions of the HK model previously considered in the literature arise as special cases. This shows that the surprising phenomenological success of HK models arises from their correspondence to the finite-site Hubbard model. In particular, the recently introduced "Momentum-Mixing HK" model corresponds to a specific choice of clustering limit, which is equal to the original finite-site Hubbard model with twist-averaged boundary conditions. Our scheme becomes particularly powerful when a spatially varying potential selects the dominant momentum channels. We demonstrate this on the one-dimensional analogue of interacting moiré systems: the Aubry-André-Hubbard model. We show that for sufficiently strong onsite potential, clusters as small as two sites can recover the ground state energy to below 1% error relative to DMRG benchmarks. This establishes that physically motivated momentum-space truncations can yield accurate low-energy descriptions at feasible computational cost, opening a path toward tractable interacting models of Moiré systems in two dimensions. Code for reproducing all numerical results is available at https://github.com/chainik1125/decomposing-hubbard.

cond-mat.str-el↗

arXiv2026

Exploring Many-Body Quantum Geometry Beyond the Quantum Metric with Correlation Functions: A Time-Dependent Perspective

The quantum geometric tensor and quantum Fisher information have recently been shown to provide a unified geometric description of the linear response of many-body systems. However, a similar geometric description of higher-order perturbative phenomena including nonlinear response in generic quantum systems is lacking. In this work, we develop a general framework for the time-dependent quantum geometry of many-body systems by treating external perturbing fields as coordinates on the space of density matrices. We use the Bures distance between the initial and time-evolved density matrix to define geometric quantities through a perturbative expansion. To lowest order, we derive a time-dependent generalization of the Bures metric related to the spectral density of linear response functions, unifying previous results for the quantum metric in various limits and providing a geometric interpretation of Fermi's golden rule. At next order in the expansion, we define a time-dependent Bures-Levi-Civita connection for general many-body systems. We show that the connection is the sum of one contribution that is related to a second-order nonlinear response function, and a second contribution that captures the higher geometric structure of first-order perturbation theory. We show that in the quasistatic, zero-temperature limit for noninteracting fermions, this Bures connection reduces to the known expression for band-theoretic Christoffel symbols. Our work provides a systematic framework to explore many-body quantum geometry beyond the quantum metric and highlights how higher-order correlation functions can probe this geometry.

cond-mat.mes-hall↗

arXiv2026

Geometry of Contact Terms in Linear Response: Applications to Elasticity

Employing the Kubo linear response formalism to calculate the elasticity of anisotropic systems has been shown to yield odd elastic moduli. For Hamiltonian systems, this result seems to be contradictory as it would violate energy conservation. To resolve this discrepancy, we examine the predictions of quantum linear response in the context of our expectation from classical elasticity theory. Our framework reveals that the geometry of the space of strain perturbations introduces correction factors to the correspondence between the Kubo formula and the elastic moduli which resolves the contradiction. We use a two-dimensional gas of electrons in a magnetic field as a pedagogical example. We use generalized f-sum rules to demonstrate how contact terms may reveal themselves in experimental measurements. Finally, we discuss the implications of our results for interpreting more general linear response functions.

cond-mat.mes-hall↗

arXiv2026

Dynamic competition between phason and amplitudon observed by ultrafast multimodal scanning tunneling microscopy

The intertwining between two ordered states that arise from the same interactions is reflected in the dynamics of their coupled collective excitations. While the equilibrium phase diagram resulting from such intertwined orders has been extensively studied, the dynamic competition between non-equilibrium modes is a largely unexplored territory. Here, we introduce a multimodal STM-based pump-probe technique, that combines ultrafast tunneling microscopy (USTM), ultrafast point-contact spectroscopy (UPC), and optical pump-probe reflectance (OPPR) on femtosecond timescale, all within a single instrument. Using this platform, we investigate the collective excitations of the unconventional charge density wave insulator (TaSe4)2I. Our UPC measurements reveal charge oscillations at 0.22 THz, with a temperature dependence that matches the theoretically predicted behavior of the long-sought massive phason gaining mass through the Anderson-Higgs mechanism. Unexpectedly, the data also reveals a second mode at 0.11 THz exhibiting similar temperature and polarization dependence with comparable mode intensity. These features, along with the robust 1/2 frequency ratio locking suggest that the 0.11 THz phason is a 'daughter mode' that arises from the splitting of the 0.22 THz massive phason into two massless phasons via parametric amplification, analogous to the decay of a neutral pion into two photons. Strikingly, comparison with OPPR data reveals that the daughter phason competes with and suppresses the amplitudon at proximate frequency. Our studies reveal an unexplored mechanism for the generation and extinction of collective excitations in quantum materials and pave the way for a microscopic understanding of ultrafast phenomena.

cond-mat.str-el↗

arXiv2026

Fundamental Tests of Quantum Geometric Bounds in Ionic and Covalent Insulators using Inelastic X-Ray Scattering

Quantum geometry underlies many fundamental properties of materials, but it has remained largely inaccessible to direct experiment. Here we demonstrate that inelastic x-ray scattering (IXS) provides a direct, quantitative probe of quantum geometry and quantum information in solids. Studying two prototype insulators, covalently bonded diamond and ionically bonded LiF, we measure the density response and experimentally determine the quantum Fisher information, the associated Bures metric, and the electron localization length. These measurements enable a quantitative comparison of quantum geometry for two distinct bonding environments. We find that the dimensionless quantum weight, $aK(q)$, which quantifies the longitudinal localization of quantum information, is constrained by fundamental electrostatic bounds in both materials. Crucially, the quantum weight of diamond exceeds that of LiF, indicating that covalent bonds exhibit a higher degree of delocalization and higher density of quantum information than the ionic bonds. Our results establish a direct experimental relationship between quantum information, electron localization, and chemical bonding, and identify IXS as a powerful tool for measuring quantum geometry in materials.

cond-mat.mes-hall↗

arXiv2026

Building blocks of topological band theory for photonic crystals

We derive a framework for classifying topological bands in three-dimensional photonic band structures, where the zero frequency polarization singularity implied by Maxwell's equations complicates the direct application of existing symmetry-based approaches. Building on recent advances in the regularization of photonic bands, we use the recently introduced concept of stable real-space invariants (SRSIs) to show how photonic band structures can be unambiguously characterized in terms of equivalence classes of band representations. We classify topologically trivial photonic bands using SRSIs, treating them as the fundamental building blocks of 3D photonic band structures. This means that if certain bands cannot be constructed from these building blocks, they are necessarily topological. Furthermore, we distinguish between photonic and electronic band structures by analyzing which SRSI values are allowed in systems with and without polarization singularity. We also explore the impact of the polarization singularity on the behavior of Wilson loops, providing new insights into the topological classification of 3D photonic systems.

physics.optics↗

arXiv2025

Charge Susceptibility and Kubo Response in Hatsugai-Kohmoto-related Models

We study in depth the charge susceptibility for the band Hatsugai-Kohmoto (HK) and orbital (OHK) models. As either of these models describes a Mott insulator, the charge susceptibility takes on the form of a modified density response function with lower and upper Hubbard bands, thereby giving rise to a multi-pole structure. The particle-hole continuum consists of hot spots along the $ω$ vs $q$ axis arising from inter-band transitions. Such transitions, which are strongly suppressed in non-interacting systems, obtain here because of the non-rigidity of the Hubbard bands. This modified density response function gives rise to a plasmon dispersion that is inversely dependent on the momentum, resulting in an additional contribution to the conventional f-sum rule. This extra contribution originates from a long-range diamagnetic contribution to the current. This results in a non-commutativity of the long-wavelength ($q\rightarrow 0$) and thermodynamic ($L\rightarrow\infty$) limits. When the correct limits are taken, we find that the Kubo response computed with either open or periodic boundary conditions yields identical results that are consistent with the continuity equation contrary to recent claims. We also show that the long wavelength pathology of the current noted previously also plagues the Anderson impurity model interpretation of dynamical mean-field theory (DMFT).

cond-mat.str-el↗

arXiv2025

Transversality-Enforced Tight-Binding Models for 3D Photonic Crystals aided by Topological Quantum Chemistry

Tight-binding models can accurately replicate the band structure and topology of crystalline systems. They have been widely used in solid-state physics due to their versatility and low computational cost. It is straightforward to build an accurate tight-binding model of any crystalline system using the crystal's maximally localized Wannier functions as a basis. Unfortunately, in 3D photonic crystals, the transversality condition of Maxwell's equations precludes the construction of a basis of maximally localized Wannier functions via usual techniques. As a result, building reliable tight-binding models of 3D photonic crystals has not been straightforward up to now. In this work, we show how to overcome this problem using topological quantum chemistry, allowing us to express the band structure of the photonic crystal as a difference of band representations. This can be achieved by introducing a set of auxiliary modes, as recently proposed in Christensen et al., Phys. Rev. X 12, 021066 (2022), which regularizes the Gamma-point obstruction arising from the transversality constraint of Maxwell's equations. The decomposition into elementary band representations allows us to isolate a set of pseudo-orbitals that permit us to construct an accurate transversality-enforced tight-binding model that matches the dispersion, symmetry content, and topology of the 3D photonic crystal under study. Moreover, we show how to introduce the effects of a gyrotropic bias in the framework, modeled via non-minimal coupling to a static magnetic field. Our work provides the first systematic method to analytically model the photonic bands of the lowest transverse modes over the entire Brillouin zone via a transversality-enforced tight-binding model.

physics.optics↗

arXiv2025

Computing the $\mathbb{Z}_2$ Invariant in Two-Dimensional Strongly-Correlated Systems

We show that the two-dimensional $\mathbb{Z}_2$ invariant for time-reversal invariant insulators can be formulated in terms of the boundary-condition dependence of the ground state wavefunction for both non-interacting and strongly-correlated insulators. By introducing a family of quasi-single particle states associated to the many-body ground state of an insulator, we show that the $\mathbb{Z}_2$ invariant can be expressed as the integral of a certain Berry connection over half the space of boundary conditions, providing an alternative expression to the formulations that appear in [Lee et al., Phys. Rev. Lett. $\textbf{100}$, 186807 (2008)]. We show the equivalence of the different many-body formulations of the invariant, and show how they reduce to known band-theoretic results for Slater determinant ground states. Finally, we apply our results to analytically calculate the invariant for the Kane-Mele model with nonlocal (orbital) Hatsugai-Kohmoto (HK) interactions. This rigorously establishes the topological nontriviality of the Kane-Mele model with HK interactions, and represents one of the few exact calculations of the $\mathbb{Z}_2$ invariant for a strongly-interacting system.

cond-mat.str-el↗

arXiv2025

Quantum Fisher Information Reveals UV-IR Mixing in the Strange Metal

The density-density response in optimally doped Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$ has recently been shown to exhibit conformal symmetry. Using, the experimentally inferred conformal dynamic susceptibility, we compute the resultant quantum Fisher information (QFI), a witness to multi-partite entanglement. For a Fermi liquid, we find that the QFI grows quadratically as the temperature increases, consistent then with the phase space available for scattering in the standard theory of metals. By contrast, the QFI in a strange metal increases as a power law at as the temperature decreases, but ultimately extrapolates to a constant at $T=0$. The constant is of the form, $ω_g^{2Δ}$, where $Δ$ is the conformal dimension and $ω_g$ is the UV cutoff which is on the order of the pseudogap. As this constant {depends on both UV and IR properties}, it illustrates that multipartite entanglement in a strange metal exhibits UV-IR mixing, a benchmark feature of doped Mott insulators as exemplified by dynamical spectral weight transfer. We conclude with a discussion of the implication of our results for low-energy reductions of the Hubbard model.

cond-mat.str-el↗

arXiv2025

Extrinsic Geometry and Gappable Edges in Rotationally Invariant Topological Phases

Recent work on Abelian topological phases with rotational symmetry has raised the question of whether rotational symmetry can protect gapless propagating edge modes. Here we address this issue by considering the coupling of topological phases to the extrinsic geometry of the background. First, we analyze an effective hydrodynamic theory for an Abelian topological phase with vanishing Hall conductance. After integrating out the bulk hydrodynamic degrees of freedom, we identify charge neutral, rotationally invariant mass terms by coupling the propagating boundary modes to the extrinsic geometry. This allows us to integrate out the edge modes and we find a gapped theory described by a local induced action that depends on the extrinsic geometry of the boundary, regardless of the shift. Finally, we apply these ideas to a microscopic theory and find the explicit bulk terms which respect gauge and rotational symmetry and open a gap in the edge spectrum.

cond-mat.mes-hall↗

arXiv2025

Spectral Density and Sum Rules for Second-Order Response Functions

Sum rules for linear response functions give powerful and experimentally-relevant relations between frequency moments of response functions and ground state properties. In particular, renewed interest has been drawn to optical conductivity and density-density sum rules and their connection to quantum geometry in topological materials. At the same time, recent work has also illustrated the connection between quantum geometry and second-order nonlinear response functions in quantum materials, motivating the search for exact sum rules for second-order response that can provide experimental probes and theoretical constraints for geometry and topology in these systems. Here we begin to address these questions by developing a general formalism for deriving sum rules for second-order response functions. Using generalized Kramers-Kronig relations, we show that the second-order Kubo formula can be expressed in terms of a spectral density that is a sum of Dirac delta functions in frequency. We show that moments of the spectral density can be expressed in terms of averages of equal-time commutators, yielding a family of generalized sum rules; furthermore, these sum rules constrain the large-frequency asymptotic behavior of the second harmonic generation rate. We apply our formalism to study generalized $f$-sum rules for the second-order density-density response function and the longitudinal nonlinear conductivity. We show that for noninteracting electrons in solids, the generalized $f$-sum rule can be written entirely in terms of matrix elements of the Bloch Hamiltonian. Finally, we derive a family of sum rules for rectification response, determining the large-frequency asymptotic behavior of the time-independent response to a harmonic perturbation.

cond-mat.mes-hall↗

arXiv2025

Quantum entanglement and quantum geometry measured with inelastic X-ray scattering

Using inelastic X-ray scattering (IXS), we experimentally investigate the quantum geometry and quantum information in the large-gap insulator, LiF. Using sum rules for the density-density response function measured in IXS, we compute the quantum Fisher information of the equilibrium density matrix of LiF associated with density perturbations. Next, by exploiting universal relations between the quantum Fisher information, the optical conductivity, and the quantum metric tensor, we extrapolate the diagonal $(h,k,l) = (1,0,0)$ component of the quantum metric of LiF, known as the quantum weight. We compare our results to recently-proposed bounds on the quantum weight and find that the quantum weight in LiF comes close to saturating a theoretical upper bound, showing that quantum-mechanical delocalization plays an important role even in ionic insulators. Our work serves as a proof-of-principle that IXS techniques can be used to quantify state-of-the-art quantum geometric quantities of materials, and establishes the quantum Fisher information as an experimentally-accessible generalization of quantum geometry to real materials.

cond-mat.mes-hall↗

arXiv2025

Grokking vs. Learning: Same Features, Different Encodings

Grokking typically achieves similar loss to ordinary, "steady", learning. We ask whether these different learning paths - grokking versus ordinary training - lead to fundamental differences in the learned models. To do so we compare the features, compressibility, and learning dynamics of models trained via each path in two tasks. We find that grokked and steadily trained models learn the same features, but there can be large differences in the efficiency with which these features are encoded. In particular, we find a novel "compressive regime" of steady training in which there emerges a linear trade-off between model loss and compressibility, and which is absent in grokking. In this regime, we can achieve compression factors 25x times the base model, and 5x times the compression achieved in grokking. We then track how model features and compressibility develop through training. We show that model development in grokking is task-dependent, and that peak compressibility is achieved immediately after the grokking plateau. Finally, novel information-geometric measures are introduced which demonstrate that models undergoing grokking follow a straight path in information space.

cs.LG↗