arXiv subjects

Bartholomeus Machielse

Publications and source records attributed to Bartholomeus Machielse.

At least 19 recordsLinked to original sources

arXiv2025

A scalable photonic quantum interconnect platform

Many quantum networking applications require efficient photonic interfaces to quantum memories which can be produced at scale and with high yield. Synthetic diamond offers unique potential for the implementation of this technology as it hosts color centers which retain coherent optical interfaces and long spin coherence times in nanophotonic structures. Here, we report a technique enabling wafer-scale processing of thin-film diamond that combines ion implantation and membrane liftoff, high-quality overgrowth, targeted color center implantation, and serial, high-throughput thermocompression bonding with yields approaching unity. The deterministic deposition of thin diamond membranes onto semiconductor substrates facilitates consistent integration of photonic crystal cavities with silicon-vacancy (SiV) quantum memories. We demonstrate reliable, strong coupling of SiVs to photons with cooperativities approaching 100. Furthermore, we show that photonic crystal cavities can be reliably fabricated across several membranes bonded to the same handling chip. Our platform enables modular fabrication where the photonic layer can be integrated with functionalized substrates featuring electronic control lines such as coplanar waveguides for microwave delivery. Finally, we implement passive optical packaging with sub-decibel insertion loss. Together, these advances pave the way to the scalable assembly of optically addressable quantum memory arrays which are a key building block for modular photonic quantum interconnects.

quant-ph↗

arXiv2025

Collective many-body dynamics in a solid-state quantum sensor controlled through nanoscale magnetic gradients

Coherent collective dynamics of strongly interacting qubits are a central resource in quantum information science, with applications from quantum computing and simulation to metrology. While electronic spins interact strongly via dipolar couplings in dense solid-state ensembles, imperfections and positional disorder pose major obstacles to coherent correlated behavior, limiting their usefulness. Here, we realize collective many-body dynamics by combining time-dependent magnetic field gradients with global coherent control of dense electron spin ensembles in diamond. We control and probe the dynamics of nanometer-scale spin spirals, and, by exploiting Hamiltonian engineering that enhances the microscopic symmetry of the interactions, we observe a disorder-resilient collective spin evolution. Our results establish a pathway to interaction-enhanced quantum metrology and nanoscale imaging of materials and biological systems under ambient conditions.

quant-ph↗

arXiv2025

Purcell-enhanced spin-phonon coupling with a single color center

The radiative properties of atoms are inherently linked to their surrounding environment. Placing an electromagnetic resonator around atoms can enhance spontaneous emission, as shown by Purcell in the 1940s. This approach is now routinely used in quantum computing and communication to channel photons emitted by atoms into well-defined modes and control atom-photon interactions. For solid-state artificial atoms, such as color-centers, the host lattice introduces an acoustic environment, allowing excited atoms to relax by emitting phonons. Here we observe the acoustic Purcell effect by constructing a specially engineered, microwave-frequency nanomechanical resonator around a color-center spin qubit in diamond. Using a co-localized optical mode of the structure that strongly couples to the color-center's excited state, we perform single-photon-level laser spectroscopy at milliKelvin temperatures and observe ten-fold faster spin relaxation when the spin qubit is tuned into resonance with a 12 GHz acoustic mode. Additionally, we use the color-center as an atomic-scale probe to measure the broadband phonon spectrum of the nanostructure up to a frequency of 28 GHz. Our work establishes a new regime of control for quantum defects in solids and paves the way for interconnects between atomic-scale quantum memories and qubits encoded in acoustic and superconducting devices.

quant-ph↗

arXiv2024

Entanglement of Nanophotonic Quantum Memory Nodes in a Telecom Network

A key challenge in realizing practical quantum networks for long-distance quantum communication involves robust entanglement between quantum memory nodes connected via fiber optical infrastructure. Here, we demonstrate a two-node quantum network composed of multi-qubit registers based on silicon-vacancy (SiV) centers in nanophotonic diamond cavities integrated with a telecommunication (telecom) fiber network. Remote entanglement is generated via the cavity-enhanced interactions between the SiV's electron spin qubits and optical photons. Serial, heralded spin-photon entangling gate operations with time-bin qubits are used for robust entanglement of separated nodes. Long-lived nuclear spin qubits are used to provide second-long entanglement storage and integrated error detection. By integrating efficient bi-directional quantum frequency conversion of photonic communication qubits to telecom frequencies (1350 nm), we demonstrate entanglement of two nuclear spin memories through 40 km spools of low-loss fiber and a 35 km long fiber loop deployed in the Boston area urban environment, representing an enabling step towards practical quantum repeaters and large-scale quantum networks.

quant-ph↗

arXiv2024

A Thin Film Lithium Niobate Near-Infrared Platform for Multiplexing Quantum Nodes

Practical quantum networks will require quantum nodes consisting of many memory qubits. This in turn will increase the complexity of the photonic circuits needed to control each qubit and will require strategies to multiplex memories and overcome the inhomogeneous distribution of their transition frequencies. Integrated photonics operating at visible to near-infrared (VNIR) wavelength range, compatible with the transition frequencies of leading quantum memory systems, can provide solutions to these needs. In this work, we realize a VNIR thin-film lithium niobate (TFLN) integrated photonics platform with the key components to meet these requirements. These include low-loss couplers ($<$ 1 dB/facet), switches ($>$ 20 dB extinction), and high-bandwidth electro-optic modulators ($>$ 50 GHz). With these devices we demonstrate high-efficiency and CW-compatible frequency shifting ($>$ 50 $\%$ efficiency at 15 GHz), as well as simultaneous laser amplitude and frequency control through a nested modulator structure. Finally, we highlight an architecture for multiplexing quantum memories using the demonstrated TFLN components, and outline how this platform can enable a 2-order of magnitude improvement in entanglement rates over single memory nodes. Our results demonstrate that TFLN can meet the necessary performance and scalability benchmarks to enable large-scale quantum nodes.

physics.optics↗

arXiv2024

Development of a Boston-area 50-km fiber quantum network testbed

Distributing quantum information between remote systems will necessitate the integration of emerging quantum components with existing communication infrastructure. This requires understanding the channel-induced degradations of the transmitted quantum signals, beyond the typical characterization methods for classical communication systems. Here we report on a comprehensive characterization of a Boston-Area Quantum Network (BARQNET) telecom fiber testbed, measuring the time-of-flight, polarization, and phase noise imparted on transmitted signals. We further design and demonstrate a compensation system that is both resilient to these noise sources and compatible with integration of emerging quantum memory components on the deployed link. These results have utility for future work on the BARQNET as well as other quantum network testbeds in development, enabling near-term quantum networking demonstrations and informing what areas of technology development will be most impactful in advancing future system capabilities.

quant-ph↗

arXiv2023

Deterministic Creation of Strained Color Centers in Nanostructures via High-Stress Thin Films

Color centers have emerged as a leading qubit candidate for realizing hybrid spin-photon quantum information technology. One major limitation of the platform, however, is that the characteristics of individual color-centers are often strain dependent. As an illustrative case, the silicon-vacancy center in diamond typically requires millikelvin temperatures in order to achieve long coherence properties, but strained silicon vacancy centers have been shown to operate at temperatures beyond 1K without phonon-mediated decoherence. In this work we combine high-stress silicon nitride thin films with diamond nanostructures in order to reproducibly create statically strained silicon-vacancy color centers (mean ground state splitting of 608 GHz) with strain magnitudes of $\sim 4 \times 10^{-4}$. Based on modeling, this strain should be sufficient to allow for operation of a majority silicon-vacancy centers within the measured sample at elevated temperatures (1.5K) without any degradation of their spin properties. This method offers a scalable approach to fabricate high-temperature operation quantum memories. Beyond silicon-vacancy centers, this method is sufficiently general that it can be easily extended to other platforms as well.

quant-ph↗

arXiv2023

High Q-factor diamond optomechanical resonators with silicon vacancy centers at millikelvin temperatures

Phonons are envisioned as coherent intermediaries between different types of quantum systems. Engineered nanoscale devices such as optomechanical crystals (OMCs) provide a platform to utilize phonons as quantum information carriers. Here we demonstrate OMCs in diamond designed for strong interactions between phonons and a silicon vacancy (SiV) spin. Using optical measurements at millikelvin temperatures, we measure a linewidth of 13 kHz (Q-factor of ~440,000) for 6 GHz acoustic modes, a record for diamond in the GHz frequency range and within an order of magnitude of state-of-the-art linewidths for OMCs in silicon. We investigate SiV optical and spin properties in these devices and outline a path towards a coherent spin-phonon interface.

physics.optics↗

arXiv2023

Integrated Phononic Waveguides in Diamond

Efficient generation, guiding, and detection of phonons, or mechanical vibrations, are of interest in various fields including radio frequency communication, sensing, and quantum information. Diamond is an important platform for phononics because of the presence of strain-sensitive spin qubits, and its high Young's modulus which allows for low-loss gigahertz devices. We demonstrate a diamond phononic waveguide platform for generating, guiding, and detecting gigahertz-frequency surface acoustic wave (SAW) phonons. We generate SAWs using interdigital transducers integrated on AlN/diamond and observe SAW transmission at 4-5 GHz through both ridge and suspended waveguides, with wavelength-scale cross sections (~1 μm2) to maximize spin-phonon interaction. This work is a crucial step for developing acoustic components for quantum phononic circuits with strain-sensitive color centers in diamond.

physics.app-ph↗

arXiv2023

Telecom networking with a diamond quantum memory

Practical quantum networks require interfacing quantum memories with existing channels and systems that operate in the telecom band. Here we demonstrate low-noise, bidirectional quantum frequency conversion that enables a solid-state quantum memory to directly interface with telecom-band systems. In particular, we demonstrate conversion of visible-band single photons emitted from a silicon-vacancy (SiV) center in diamond to the telecom O-band, maintaining low noise ($g^2(0)<0.1$) and high indistinguishability ($V=89\pm8\%$). We further demonstrate the utility of this system for quantum networking by converting telecom-band time-bin pulses, sent across a lossy and noisy 50 km deployed fiber link, to the visible band and mapping their quantum states onto a diamond quantum memory with fidelity $\mathcal{F}=87\pm 2.5 \% $. These results demonstrate the viability of SiV quantum memories integrated with telecom-band systems for scalable quantum networking applications.

quant-ph↗

arXiv2022

Efficient Source of Shaped Single Photons Based on an Integrated Diamond Nanophotonic System

An efficient, scalable source of shaped single photons that can be directly integrated with optical fiber networks and quantum memories is at the heart of many protocols in quantum information science. We demonstrate a deterministic source of arbitrarily temporally shaped single-photon pulses with high efficiency (detection efficiency = 14.9%) and purity ($g^{(2)}(0) = 0.0168$) and streams of up to 11 consecutively detected single photons using a silicon-vacancy center in a highly directional fiber-integrated diamond nanophotonic cavity. Combined with previously demonstrated spin-photon entangling gates, this system enables on-demand generation of streams of correlated photons such as cluster states and could be used as a resource for robust transmission and processing of quantum information.

quant-ph↗

arXiv2022

Robust multi-qubit quantum network node with integrated error detection

Long-distance quantum communication and networking require quantum memory nodes with efficient optical interfaces and long memory times. We report the realization of an integrated two-qubit network node based on silicon-vacancy centers (SiVs) in diamond nanophotonic cavities. Our qubit register consists of the SiV electron spin acting as a communication qubit and the strongly coupled 29Si nuclear spin acting as a memory qubit with a quantum memory time exceeding two seconds. By using a highly strained SiV with suppressed electron spin-phonon interactions, we realize electron-photon entangling gates at elevated temperatures up to 1.5 K and nucleus-photon entangling gates up to 4.3 K. Finally, we demonstrate efficient error detection in nuclear spin-photon gates by using the electron spin as a flag qubit, making this platform a promising candidate for scalable quantum repeaters.

quant-ph↗

arXiv2022

Development of hard masks for reactive ion beam angled etching of diamond

Diamond offers good optical properties and hosts bright color centers with long spin coherence times. Recent advances in angled-etching of diamond, specifically with reactive ion beam angled etching (RIBAE), have led to successful demonstration of quantum photonic devices operating at visible wavelengths. However, larger devices operating at telecommunication wavelengths have been difficult to fabricate due to the increased mask erosion, arising from the increased size of devices requiring longer etch times. We evaluated different mask materials for RIBAE of diamond photonic crystal nanobeams and waveguides, and how their thickness, selectivity, aspect ratio and sidewall smoothness affected the resultant etch profiles and optical performance. We found that a thick hydrogen silesquioxane (HSQ) layer on a thin alumina adhesion layer provided the best etch profile and optical performance. The techniques explored in this work can also be adapted to other bulk materials that are not available heteroepitaxially or as thin films-on-insulator.

physics.app-ph↗

arXiv2021

Roadmap on Integrated Quantum Photonics

Integrated photonics is at the heart of many classical technologies, from optical communications to biosensors, LIDAR, and data center fiber interconnects. There is strong evidence that these integrated technologies will play a key role in quantum systems as they grow from few-qubit prototypes to tens of thousands of qubits. The underlying laser and optical quantum technologies, with the required functionality and performance, can only be realized through the integration of these components onto quantum photonic integrated circuits (QPICs) with accompanying electronics. In the last decade, remarkable advances in quantum photonic integration and a dramatic reduction in optical losses have enabled benchtop experiments to be scaled down to prototype chips with improvements in efficiency, robustness, and key performance metrics. The reduction in size, weight, power, and improvement in stability that will be enabled by QPICs will play a key role in increasing the degree of complexity and scale in quantum demonstrations. In the next decade, with sustained research, development, and investment in the quantum photonic ecosystem (i.e. PIC-based platforms, devices and circuits, fabrication and integration processes, packaging, and testing and benchmarking), we will witness the transition from single- and few-function prototypes to the large-scale integration of multi-functional and reconfigurable QPICs that will define how information is processed, stored, transmitted, and utilized for quantum computing, communications, metrology, and sensing. This roadmap highlights the current progress in the field of integrated quantum photonics, future challenges, and advances in science and technology needed to meet these challenges.

quant-ph↗

arXiv2021

Optical Entanglement of Distinguishable Quantum Emitters

Solid-state quantum emitters are promising candidates for the realization of quantum networks, owing to their long-lived spin memories, high-fidelity local operations, and optical connectivity for long-range entanglement. However, due to differences in local environment, solid-state emitters typically feature a range of distinct transition frequencies, which makes it challenging to create optically mediated entanglement between arbitrary emitter pairs. We propose and demonstrate an efficient method for entangling emitters with optical transitions separated by many linewidths. In our approach, electro-optic modulators enable a single photon to herald a parity measurement on a pair of spin qubits. We experimentally demonstrate the protocol using two silicon-vacancy center sin a diamond nanophotonic cavity, with optical transitions separated by 7.4 GHz. Working with distinguishable emitters allows for individual qubit addressing and readout, enabling parallel control and entanglement of both co-located and spatially separated emitters, a key step towards scaling up quantum information processing systems

quant-ph↗

arXiv2019

Experimental demonstration of memory-enhanced quantum communication

The ability to communicate quantum information over long distances is of central importance in quantum science and engineering. For example, it enables secure quantum key distribution (QKD) relying on fundamental principles that prohibit the "cloning" of unknown quantum states. While QKD is being successfully deployed, its range is currently limited by photon losses and cannot be extended using straightforward measure-and-repeat strategies without compromising its unconditional security. Alternatively, quantum repeaters, which utilize intermediate quantum memory nodes and error correction techniques, can extend the range of quantum channels. However, their implementation remains an outstanding challenge, requiring a combination of efficient and high-fidelity quantum memories, gate operations, and measurements. Here we report the experimental realization of memory-enhanced quantum communication. We use a single solid-state spin memory integrated in a nanophotonic diamond resonator to implement asynchronous Bell-state measurements. This enables a four-fold increase in the secret key rate of measurement device independent (MDI)-QKD over the loss-equivalent direct-transmission method while operating megahertz clock rates. Our results represent a significant step towards practical quantum repeaters and large-scale quantum networks.

quant-ph↗

arXiv2019

Quantum interference of electromechanically stabilized emitters in nanophotonic devices

Photon-mediated coupling between distant matter qubits may enable secure communication over long distances, the implementation of distributed quantum computing schemes, and the exploration of new regimes of many-body quantum dynamics. Nanophotonic devices coupled to solid-state quantum emitters represent a promising approach towards realization of these goals, as they combine strong light-matter interaction and high photon collection efficiencies. However, the scalability of these approaches is limited by the frequency mismatch between solid-state emitters and the instability of their optical transitions. Here we present a nano-electromechanical platform for stabilization and tuning of optical transitions of silicon-vacancy (SiV) color centers in diamond nanophotonic devices by dynamically controlling their strain environments. This strain-based tuning scheme has sufficient range and bandwidth to alleviate the spectral mismatch between individual SiV centers. Using strain, we ensure overlap between color center optical transitions and observe an entangled superradiant state by measuring correlations of photons collected from the diamond waveguide. This platform for tuning spectrally stable color centers in nanophotonic waveguides and resonators constitutes an important step towards a scalable quantum network.

physics.app-ph↗

arXiv2018

Spectral alignment of single-photon emitters in diamond using strain gradient

Solid-state single-photon emitters are attractive for realization of integrated quantum systems due to their experimental convenience and scalability. Unfortunately, however, their complex mesoscopic environments cause photons from different emitters to be spectrally distinguishable. Here we demonstrate spectral alignment of two solid-state single-photon emitters by utilizing the strain gradient. Multiple germanium vacancy (GeV) color centers in diamond are created in fabricated diamond microcantilevers using focused ion beam implantation. The strain response of the electronic energy levels of the GeV is measured by inducing an electrically controlled strain in the device. Leveraging the large strain gradient, we tune two GeVs in the spot to emit at the same optical wavelength. Simultaneous resonant excitation of two spectrally aligned GeVs is demonstrated using a narrow linewidth laser. This strain gradient tuning can be used to realize spectrally identical quantum emitters for on-chip integrated quantum systems.

cond-mat.mes-hall↗