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Beatriz Jurado

Publications and source records attributed to Beatriz Jurado.

11 recordsLinked to original sources

Precision masses of neutron-rich platinum and gold nuclei reveal enhanced $N=126$ shell strength below doubly-magic $^{208}$Pb

The heaviest stable nuclei in the universe owe their existence to quantum shell structure, the grouping of protons and neutrons into discrete energy levels separated by gaps. The largest known neutron shell gap in stable nuclei, at $N=126$, stabilizes doubly-magic $^{208}$Pb and is responsible for the characteristic abundance peak of heavy elements near gold and platinum produced by the rapid neutron-capture process (r-process). Whether this shell gap persists as protons are removed from lead is a question central to both nuclear structure and the modeling of heavy-element synthesis, yet it has remained unanswered due to the extraordinary difficulty of producing the relevant neutron-rich nuclei. Direct experimental knowledge in this region was essentially absent. Here we report the first precision mass measurements of $^{203,204}$Pt and $^{204,205,206}$Au, performed at GSI using a novel combination of Schottky and isochronous mass spectrometry in a heavy-ion storage ring. The $N=126$ isotones $^{204}$Pt and $^{205}$Au are more strongly bound than the extrapolated trend of the previously known mass surface by 403 and 464~keV, respectively, revealing an unexpectedly enhanced $N=126$ shell strength below doubly-magic $^{208}$Pb. Furthermore, the proton-neutron interaction strength exhibits a hitherto unobserved bifurcation at $N=126$ as protons are removed from $^{208}$Pb. Our results redefine the nuclear mass surface in the neutron-rich heavy-element region and provide direct experimental benchmarks for theoretical models whose extrapolations toward more exotic nuclei are essential for r-process nucleosynthesis calculations.

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Surrogate neutron-capture studies with fission detection in inverse kinematics at the ESR storage ring

The NECTAR (Nuclear rEaCTions At storage Rings) experiment at the ESR heavy-ion storage ring at GSI/FAIR Darmstadt is dedicated to surrogate reaction studies of neutron-induced reactions on heavy nuclei in inverse kinematics. In this work, we report on the implementation and performance of a newly developed fission-fragment detection system integrated into the NECTAR experimental setup. The upgraded detector configuration enables, for the first time in a surrogate experiment, the simultaneous detection ofgamma-decay residues, multi-neutron-emission residues, and fission fragments. The full setup was used for the first time in an experiment where a stored beam of bare 238U92+ ions at 17.24 MeV/u interacted with a gas-jet deuterium target, populating excited 238U and 239U nuclei via the 238U(d,d') and 238U(d,p) reactions. We describe the geometry of the used fission fragment detectors, design constraints, and simulation-based efficiency determination. The target-like particle identification and beam-like residue spectra demonstrating the performance of the complete setup are also shown.

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Development of a gaseous proton-recoil detector for neutron flux measurements between 0.2 and 2 MeV neutron energy

Absolute measurements of neutron fluence are an essential prerequisite of neutron-induced cross section measurements, neutron beam lines characterization and dosimetric investigations. The H(n,p) elastic scattering cross section is a very well known standard used to perform precise neutron flux measurements in high precision measurements. The use of this technique, with proton recoil detectors, is not straightforward below incident neutron energy of 1 MeV, due to a high background in the detected proton spectrum. Experiments have been carried out at the AIFIRA facility to investigate such background and to determine its origin and components. Based on these investigations, a gaseous proton-recoil detector has been designed with a reduced low energy background. A first test of this detector has been carried out at the AIFIRA facility, and first results will be presented.

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Review on the progress in nuclear fission

An overview is given on some of the main advances in experimental methods, experimental results and theoretical models and ideas of the last years in the field of nuclear fission. New experimental approaches extended the availability of fissioning systems considerably and provided a full identification of all fission products in A and Z for the first time. In particular, the transition from symmetric to asymmetric fission around 226Th and some unexpected structure in the mass distributions in the fission of systems around Z = 80 to 84 as well as an extended systematics of the odd-even effect in fission fragment Z distributions have been measured [A. N. Andreyev et al., Rep. Progr. Phys. 81 (2018) 016301]. Three classes of theoretical descriptions of fission presently appear to be the most promising or the most successful ones: Self-consistent quantum-mechanical models fully consider the quantum-mechanical features of the fission process. Intense efforts are presently made to develop suitable theoretical tools [N. Schunck, L. M. Robledo, Rep. Prog. Phys. 79 (2016) 116301] for modeling the non-equilibrium, large-amplitude collective motion leading to fission. Stochastic, essentially classical models provide a fully developed technical framework. The main features of the fission-fragment mass distribution are well reproduced from mercury to fermium and beyond [P. Möller, J. Randrup, Phys. Rev. C 91 (2015) 044316]. In an alternative semi-empirical approach [K.-H. Schmidt et al., Nucl. Data Sheets 131 (2016) 107], considerable progress in describing the fission observables has been achieved by combining several general theoretical concepts. This new approach reveals a high degree of regularity and allows calculating high-quality data with a unique parameter set for a large number of systems and an extended excitation-energy range.

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A spallation-based neutron target for direct studies of neutron-induced reactions in inverse kinematics

We discuss the possibility to build a neutron target for nuclear reaction studies in inverse kinematics utilizing a storage ring and radioactive ion beams. The proposed neutron target is a specially designed spallation target surrounded by a large moderator of heavy water (D$_2$O). We present the resulting neutron spectra and their properties as a target. We discuss possible realizations at different experimental facilities.

physics.ins-det

Influence of complete energy sorting on the characteristics of the odd-even effect in fission-fragment element distributions

The characteristics of the odd-even effect in fission-fragment Z distributions are compared to a model based on statistical mechanics. Special care is taken for using a consistent description for the influence of pairing correlations on the nuclear level density. The variation of the odd-even effect with the mass of the fissioning nucleus and with fission asymmetry is explained by the important statistical weight of configurations where the light nascent fission fragment populates the lowest energy state of an even-even nucleus. This implies that entropy drives excitation energy and unpaired nucleons predominantly to the heavy fragment. Therefore, within our model, the odd-even effect appears as an additional signature of the recently discovered energy-sorting process in nuclear fission.

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Further evidence for energy sorting from the even-odd effect in fission-fragment element distributions

The even-odd effect in fission is explained by a model based on statistical mechanics. It reveals that the variation of the even-odd effect with the mass of the fissioning nucleus and the increase towards asymmetric splits is due to the important statistical weight of configurations where the light fission fragment populates the ground state of an even-even nucleus. This implies that entropy drives excitation energy and unpaired nucleons predominantly to the heavy fragment. Therefore, the even-odd effect is an additional signature of the recently discovered energy-sorting process in fission.

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Inconsistencies in the description of pairing effects in nuclear level densities

Pairing correlations have a strong influence on nuclear level densities. Empirical descriptions and theoretical models have been developed to take these effects into account. The present article discusses cases, where descriptions of nuclear level densities are inconsistent or in conflict with the present understanding of nuclear properties. Phenomenological approaches consider a back-shift parameter. However, the absolute magnitude of the back-shift, which actually corresponds to the pairing condensation energy, is generally not compatible with the observation that stable pairing correlations are present in essentially all nuclei. It is also shown that in the BCS model pairing condensation energies and critical pairing energies are inconsistent for light nuclei. A modification to the composite Gilbert-Cameron level-density description is proposed, and the use of more realistic pairing theories is suggested.

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Final excitation energy of fission fragments

We study how the excitation energy of the fully accelerated fission fragments is built up. It is stressed that only the intrinsic excitation energy available before scission can be exchanged between the fission fragments to achieve thermal equilibrium. This is in contradiction with most models used to calculate prompt neutron emission where it is assumed that the total excitation energy of the final fragments is shared between the fragments by the condition of equal temperatures. We also study the intrinsic excitation-energy partition according to a level density description with a transition from a constant-temperature regime to a Fermi-gas regime. Complete or partial excitation-energy sorting is found at energies well above the transition energy.

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Thermodynamics of nuclei in thermal contact

The behaviour of a di-nuclear system in the regime of strong pairing correlations is studied with the methods of statistical mechanics. It is shown that the thermal averaging is strong enough to assure the application of thermodynamical methods to the energy exchange between the two nuclei in contact. In particular, thermal averaging justifies the definition of a nuclear temperature.

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Entropy-driven excitation-energy sorting in superfluid fission dynamics

We study the consequences of the constant-temperature behaviour of nuclei in the superfluid regime for the exchange of excitation energy between two nuclei in thermal contact. This situation is realized at the scission configuration of fission at moderate excitation energies. It is shown that all available excitation energy is transferred to the colder fragment. This effect explains why an increase of excitation energy is translated into an increase of the number of emitted neutrons for the heavy fission fragments only. This observation remained unexplained up to now.

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