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Ben S. Humphries

Publications and source records attributed to Ben S. Humphries.

3 recordsLinked to original sources

Evolving wrinkles: time-dependent buckling of an elastic sheet on a liquid substrate

We model the formation and evolution of wrinkles in a floating elastic sheet under uniaxial compression. This is a canonical setup in the study of wrinkling, and whilst its static equilibrium configuration is well characterised, its dynamics are not. In this work, we focus on modelling the transition from early, inertia-dominated wrinkle growth to late-time gravity-moderated equilibrium. For an initial configuration in which the sheet is flat, an initial disturbance will first grow at the shortest available wavelengths, because this requires the least kinetic energy, but will subsequently transition to a longer preferred wavelength that minimises potential energy. We observe that the evolving wave pattern must be a spectrum, as opposed to a fundamental wrinkle mode whose wavelength evolves in time. Our results demonstrate that changes in the dominant wrinkle wavelength are coupled to a decay in the compressive force, which is to be expected from equilibrium theory.

physics.flu-dyn

Indirect Communication Between Non-Markovian Baths

In this work we develop a model for an undamped vibration in the presence of an overdamped bath. This two-bath model involves a new derivation of the hierarchical equations of motion (HEOM) for an overdamped Lorentz-Drude (LD) environment that is summed together with an undamped oscillator (UO) bath, termed LDUO-HEOM. We show that information transfer occurs between the two baths, even in the absence of a direct coupling between the baths. This bath-system-bath, mediated information transfer leads to intricate non-Markovian dynamics. The model is analysed using expectation values of the bath coordinates and generates 2D electronic spectra that are in qualitative agreement with single-bath models. Furthermore, the model eliminates the additional superfluous damping introduced by the finite spectral width of the underdamped bath in our previous two-bath underdamped-overdamped, `bath vibration model' [J. Chem. Phys. 156, 084103 (2022)].

quant-ph

Phonon Signatures in Photon Correlations

We show that the second-order, two-time correlation functions for phonons and photons emitted from a vibronic molecule in a thermal bath result in bunching and anti-bunching (a purely quantum effect), respectively. Signatures relating to phonon exchange with the environment are revealed in photon-photon correlations. We demonstrate that cross-correlation functions have a strong dependence on the order of detection giving insight into how phonon dynamics influences the emission of light. This work offers new opportunities to investigate quantum effects in condensed-phase molecular systems.

quant-ph