arXiv subjects

Ben Sun

Publications and source records attributed to Ben Sun.

10 recordsLinked to original sources

arXiv2026

Single-photon time-stretch computational ghost spectroscopy

Time-stretch spectroscopy is powerful for capturing transient spectral phenomena but remains fundamentally limited by detector bandwidth or timing jitter, especially under photon-starved conditions. Here, we devise and implement single-photon time-stretch computational ghost spectroscopy, which integrates dispersive wavelength-to-time mapping with programmable temporal encoding and correlation-based reconstruction to overcome these detection limitations. Specifically, temporally stretched ultrashort pulses are modulated by predefined encoding patterns and detected by a low-bandwidth detector, allowing reconstruction of near-infrared spectra with 450 resolvable channels across 1530-1590 nm without direct high-speed waveform acquisition. By further incorporating compressive sensing, accurate spectral recovery is achieved at sub-Nyquist sampling rates, substantially reducing acquisition requirements to facilitate high-speed operation at 210 kHz. In the single-photon regime, computational ghost reconstruction effectively suppresses the intrinsic detector timing jitter, yielding high-fidelity spectra at illumination fluxes down to 0.01 photons/pulse. By jointly enabling broadband coverage, high spectral resolution, high acquisition speed, and single-photon sensitivity, this approach establishes a computation-enhanced paradigm for time-stretch spectroscopy and provides a versatile platform for ultrafast and photon-efficient spectroscopic applications.

physics.optics↗

arXiv2026

High-speed mid-infrared single-photon upconversion spectrometer

Sensitive and fast mid-infrared (MIR) spectroscopy is highly attractive in a variety of applications including astronomical observation, pharmaceutical synthesis, and environmental monitoring. However, the performance of conventional MIR spectrometers has long been hindered by the limited sensitivity of narrow-bandgap detectors and/or the deficient brightness of broadband light sources. Here, we devise and implement an ultra-sensitive and broadband MIR upconversion spectrometer, which integrates a supercontinuum source covering 1.5-4.2 $\mu$m based on a silicon nitride nanophotonic waveguide. High-efficiency and low-noise nonlinear frequency upconversion is realized based on coincidence pulsed pumping with spectro-temporal optimization, which enables to leverage silicon detectors for facilitating MIR single-photon spectroscopy at 0.2 photons/nm/pulse. Furthermore, the upconversion-based array spectrometer is manifested with high-speed spectral acquisition rates beyond 200 kHz, which is about ten-fold faster than the state-of-the-art scan rates for FTIR-based spectrometers at a comparable spectral resolution. The achieved features of broadband spectral coverage, single-photon sensitivity, and sub-MHz refreshing rate might open up new possibilities in infrared transient spectral measurements in combustion analysis, high-throughput sorting and reaction tracking, among others.

physics.optics↗

arXiv2026

Single-photon time-stretch infrared spectroscopy

Sensitive mid-infrared (MIR) spectroscopy is highly demanded in various fields ranging from industrial inspection, biomedical diagnosis to astronomical observation. However, the detection sensitivity of conventional MIR spectrometers has been severely limited by excessive noises for existing infrared sensors, which hinders widespread use in photon-scarce scenarios. Here, we devise and implement a broadband MIR single-photon time-stretch spectrometer based on high-fidelity spectral upconversion and time-correlated coincidence counting. Specifically, a nanophotonic supercontinuum illumination covering 2.4-4.2 $\mu$m is nonlinearly converted to the near-infrared band, where low-loss single-mode fiber and high-performance silicon detector can be leveraged to facilitate dispersive operation and sensitive detection, respectively. The arrival time for the dispersed upconversion photons is precisely registered with a low-timing-jitter photon counter, which enables us to obtain a high spectral resolution about 0.5 cm$^{-1}$ under a low-light-level illumination down to 0.14 photons/nm/pulse. In comparison to previous MIR upconversion spectrometers, the presented time-stretch architecture favors single-pixel simplicity and high-throughput acquisition for the single-photon spectral measurement. The achieved MIR spectroscopic features of broadband spectral coverage, sub-wavenumber resolution, single-photon sensitivity, and room-temperature operation would stimulate immediate applications in material and life sciences.

physics.optics↗

arXiv2026

Highly-sensitive mid-infrared upconversion detection based on external-cavity pump enhancement

Sensitive mid-infrared (MIR) detection is highly demanded in various applications, ranging from remote sensing, infrared surveillance, environmental monitoring to industrial inspection. Among others, upconversion infrared detectors have recently attracted increasing attention due to the advantageous features of high sensitivity, fast response, and room-temperature operation. However, it remains challenging to realize high-performance passive MIR sensing due to the stringent requirement of high-power continuous-wave pumping. Here, we propose and implement a high-efficiency and low-noise MIR upconversion detection system based on pumping enhancement via a low-loss optical cavity. Specifically, a single-longitudinal-mode pump at 1064 nm is significantly enhanced by a factor of 36, thus allowing for a peak conversion efficiency of up to 22\% at an intra-cavity average power of 55 W. The corresponding noise equivalent power is achieved as low as 0.3 fW/Hz$^{1/2}$, which indicates at least a ten-fold improvement over previous results. Notably, the involved single-frequency pumping would facilitate high-fidelity spectral mapping, which is particularly attractive for high-precision MIR upconversion spectroscopy in photon-starved scenarios.

physics.optics↗

arXiv2026

Mid-Infrared Single-Photon Compressive Spectroscopy

Sensitive mid-infrared (MIR) spectroscopy plays an indispensable role in various photon-starved conditions. However, the detection sensitivity of conventional MIR spectrometers is severely limited by excessive noises of the involved infrared sensors, especially for multi-pixel arrays in parallel spectral acquisition. Here, we devise and implement an ultra-sensitive MIR single-pixel spectrometer, which relies on high-fidelity spectral upconversion and wavelength-encoding compressive measurement. Specifically, a MIR nanophotonic supercontinuum from 3.1 to 3.9 $\mu$m is nonlinearly converted to the near-infrared band via synchronous chirped-pulse pumping, which facilitates both the precise spectral mapping and sensitive upconversion detection. The upconverted signal is then spatially dispersed onto a programmable digital micromirror device, before being registered by a single-element silicon detector. Consequently, the spectral information can be deciphered from the correlation between encoded patterns and recorded measurements, which results in a spectral resolution of 0.5 cm$^{-1}$ under an illumination flux down to 0.01 photons/nm/pulse. Moreover, we demonstrate faithful reconstructions at sub-Nyquist sampling rates by using the compressive sensing algorithm, which leads to a 95\% reduction in data acquisition time. The presented single-pixel computational spectrometer features wavelength multiplexing, high throughput, and efficient sampling, which thus paves a new way for sensitive and fast spectroscopic analysis at the single-photon level.

physics.optics↗

arXiv2026

High-speed mid-infrared imaging via nonlinear multiplexed detection

High-speed mid-infrared (MIR) videography constitutes an enabling tool to monitor and analyze various dynamics in scientific research and industrial applications, such as combustion diagnostics, explosion reactions, photosynthetic tracking, and thermal surveillance. However, the frame rate of conventional MIR imagers is typically limited by readout electronics and detection sensitivity, especially for large spatial formats with massive pixels. Here, we devise and implement a high-speed MIR upconversion imaging system based on time-multiplexed nonlinear structured pumping. Specifically, the dynamic infrared scene is optically gated by a sequence of spatially periodical pump patterns in a nonlinear crystal, which facilitates both rapid temporal encryption and sensitive upconversion detection. Then, the upconverted frames are superimposed onto a silicon camera within a single exposure, thus resulting in a multiplexed snapshot in the spatial-frequency domain. Finally, the sub-exposure images, corresponding to distinct transient events, can be computationally deciphered and reconstructed by the frequency recognition algorithm based on band-pass filtering and Fourier transform operations. The achieved frame rate is tenfold boosted to 10,000 frames per second without compromising the megapixel spatial format, which allows continuous real-time MIR videography at high speed and high definition. The presented approach could be readily extended to far-infrared or terahertz spectral regions, with an aim of performing high-throughput and high-sensitivity observation of transient phenomena with high temporal complexity.

physics.optics↗

arXiv2026

High-resolution mid-infrared single-photon upconversion ranging

Single-photon laser ranging has widespread applications in remote sensing and target recognition. However, highly-sensitive light detection and ranging (LiDAR) has long been restricted in visible or near-infrared bands. An appealing quest is to extend the operation wavelength into the mid-infrared (MIR) region, which calls for an infrared photon counting system at high detection sensitivity and precise temporal resolution. Here, we devise and demonstrate a MIR upconversion LiDAR based on nonlinear asynchronous optical sampling. Specifically, the infrared probe is interrogated in a nonlinear crystal by a train of pump pulses at a slightly different repetition rate, which favors for a temporal optical scanning at a picosecond timing resolution and a kilohertz refreshing rate over $\sim$50 ns. Moreover, the cross-correlation upconversion trace is temporally stretched by a factor of 2$\times$10$^4$, which can thus be recorded by a low-bandwidth silicon detector. In combination with time-correlated photon-counting technique, the achieved effective resolution is about two orders of magnitude better than the timing jitter of the detector itself, which facilitates a ranging precision of 4 $\mu$m under a low detected flux of 8$\times$10$^{-5}$ photons per pulse. The presented MIR time-of-flight range finder is featured with single-photon sensitivity and high positioning resolution, which would be particularly useful in infrared sensing and imaging in photon-starved scenarios.

physics.optics↗

arXiv2026

Mid-infrared single-photon computational temporal ghost imaging

The capture of transient optical waveforms is critical to reveal dynamical phenomena in various fields. However, fast and sensitive mid-infrared (MIR) measurements are typically limited by processing bandwidth and detection sensitivity of conventional infrared detectors. Here, we propose and implement a computational temporal ghost imaging system, which favors high-speed and high-sensitivity characterization of MIR temporal objects. The core process relies on high-fidelity nonlinear optical transduction for facilitating both the programmable structured illumination and frequency upconversion detection based on the high-performance near-infrared light modulator and detector, respectively. Consequently, the correlation between the recorded integral upconversion intensity and the designated encoding patterns allows one to reconstruct the MIR profiles with a temporal resolution of 80 ps, well beyond the intrinsic bandwidth or timing jitter of the involved detectors. Moreover, a record-high detection sensitivity is manifested by recovering single-photon MIR waveforms with an incident flux below 0.1 photon/bit. Additionally, faithful reconstructions at sub-Nyquist sampling rates are demonstrated using the compressive sensing algorithm, which can reduce the data acquisition time by over 90\%. The presented paradigm features high timing precision, single-photon sensitivity, and efficient data sampling, which could be extended into far-infrared or terahertz regions to address pressing demands in fast and sensitive sensing.

physics.optics↗

arXiv2026

Infrared Single-Pixel Hyperspectral Imaging via Spatial-Temporal Multiplexing

Near-infrared (NIR) hyperspectral imaging is widely used to reveal morphological and chemical information. However, conventional spectral imagers usually rely on costly focal plane arrays and suffer from data redundancy and inefficiencies in spatial-spectral data acquisition. Here, we devise and implement a single-pixel NIR hyperspectral imaging system based on high-fidelity spectrum-to-time mapping and high-precision spatial-encoding compressive measurements. The system employs a single-mode telecommunication fiber for temporal dispersion and a programmable spatial light modulator to impose structured spatial patterns, with all signals detected by a single InGaAs photodetector. By correlating temporally stretched waveforms with spatial encodings, we reconstruct 64$\times$64 spatially resolved hyperspectral datacubes spanning 50 spectral bands over the 1550-1600 nm range. Furthermore, real-time monitoring of dynamic liquid injection is demonstrated at a datacube refreshing rate of 12 Hz under sub-Nyquist sampling. The presented architecture features single-pixel simplicity, high optical throughput, and efficient data acquisition, which would pave a novel way for NIR spectral imaging in biomedical diagnostics and material characterization.

physics.optics↗

arXiv2026

Wide-field mid-infrared cavity-enhanced upconversion imaging

Mid-infrared (MIR) spectral imaging enables precise target identification and analysis by capturing rich chemical fingerprints, which calls for high-sensitivity broadband MIR imagers at room temperature. Here, we devise and implement a continuous-wave pumping MIR upconversion imaging system based on external-cavity enhancement, which favors a large field of view, a low cavity loss, and a high spectral resolution. The involved optical cavity is constructed in an integrated fashion by utilizing one crystal facet as a cavity mirror, which allows a 43-fold power enhancement for the single-longitudinal-mode pump at 1064 nm. In combination with the chirped-poled crystal design, high-fidelity and wide-field spectral imaging mapping is permitted to facilitate an acceptance angle up to 28.5$^\circ$ over a spectral coverage of 2.5--5 $\mu$m. Moreover, a thermal locking approach is used to stabilize the cavity at the high-power operation, eliminating active feedback and ensuring long-term stability. A proof-of-principle demonstration is presented to showcase real-time observation of CO$_{2}$ gas injection dynamics. The implemented MIR upconversion imager features wide-field operation, high detection sensitivity, and compact footprint, which would benefit subsequent applications including environment monitoring, gas leakage inspection, and medical diagnostics.

physics.optics↗