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Benedetta Flebus

Publications and source records attributed to Benedetta Flebus.

At least 37 records · Page 2Linked to original sources

Cooperative non-reciprocal emission and quantum sensing of symmetry breaking

Non-reciprocal propagation of energy and information is fundamental to a wide range of quantum technology applications. In this work, we explore the quantum many-body dynamics of a qubit ensemble coupled to a shared bath that mediates coherent and dissipative inter-qubit interactions with both symmetric and anti-symmetric components. We find that the interplay between anti-symmetric (symmetric) coherent and symmetric (anti-symmetric) dissipative interactions results in non-reciprocal couplings, which, in turn, generate a spatially asymmetric emission pattern. We demonstrate that this pattern arises from non-reciprocal interactions coupling different quantum many-body states within a specific excitation manifold. Focusing on solid-state baths, we show that their lack of time-reversal and inversion symmetry is a key ingredient for generating non-reciprocal dynamics in the qubit ensemble. With the plethora of quantum materials that exhibit this symmetry breaking at equilibrium, our approach paves the way for realizing cooperative non-reciprocal transport in qubit ensembles without requiring time-modulated external drives or complex engineering. Using an ensemble of nitrogen-vacancy (NV) centers coupled to a generic non-centrosymmetric ferromagnetic bath as a concrete example, we demonstrate that our predictions can be tested in near-future experiments. As the spatial asymmetry in the relaxation dynamics of the qubit ensemble is a direct probe of symmetry breaking in the solid-state bath, our work also opens the door to developing model-agnostic quantum sensing schemes capable of detecting bath properties invisible to current state-of-the-art protocols, which operate solid-state defects as single-qubit sensors.

quant-ph↗

The role of excitation vector fields and all-polarisation state control of cavity magnonics

Recently the field of cavity magnonics, a field focused on controlling the interaction between magnons and confined microwave photons within microwave resonators, has drawn significant attention as it offers a platform for enabling advancements in quantum- and spin-based technologies. Here, we introduce excitation vector fields, whose polarisation and profile can be easily tuned in a two-port cavity setup, thus acting as an effective experimental knob to explore the coupled dynamics of cavity magnon-polaritons. Moreover, we develop theoretical models that accurately predict and reproduce the experimental results for any polarisation state and field profile within the cavity resonator. This versatile experimental platform offers a new avenue for controlling spin-photon interactions and as such also delivering a mechanism to readily control the exchange of information between hybrid systems.

quant-ph↗

Magnetic structure of EuCd$_2$Sb$_2$ single-crystal thin-film

We investigate the magnetic order in single crystalline EuCd$_2$Sb$_2$ thin films using a combined theoretical and experimental approach. Resonant elastic x-ray scattering experiments reveal a sharp magnetic peak at $q = (0, 0, \frac{1}{2})$ below $T_N = 7.2$ K, indicative of interlayer antiferromagnetic ordering. Additionally, we observe a weak diffuse magnetic signal centered at $q = (0, 0, 1)$ that persists above $T_N$, up to $T_C \sim 11$ K. Our Monte-Carlo simulations of a classical spin model approximation of the Eu magnetic sublattice demonstrate that the diffuse signal can arise from ferromagnetic coupling in the top few layers due to surface oxidation. On the other hand, the bulk of the sample exhibits antiferromagnetic coupling between layers. Finally, our fit of the model parameters to the magnetic ordering temperatures, shed light on the exchange couplings that are key in stabilizing the observed composite magnetic order.

cond-mat.mtrl-sci↗

Magnon-Photon Coupling in an Opto-Electro-Magnonic Oscillator

The opto-electronic oscillators (OEOs) hosting self-sustained oscillations by a time delayed mechanism are of particular interest in long-haul signal transmission and processing. On the other hand, owing to their unique tunability and compatibility, magnons - as elementary excitations of spin waves - are advantageous carriers for coherent signal transduction across different platforms. In this work, we integrated an opto-electronic oscillator with a magnonic oscillator consisting of a microwave waveguide and a yttrium iron garnet sphere. We find that, in the presence of the magnetic sphere, the oscillator power spectrum exhibits sidebands flanking the fundamental OEO modes. The measured waveguide transmission reveals anti-crossing gaps, a hallmark of the coupling between the opto-electronic oscillator modes and the Walker modes of the sphere. Experimental results are well reproduced by a coupled-mode theory that accounts for nonlinear magnetostrictive interactions mediated by the magnetic sphere. Leveraging the advanced fiber-optic technologies in opto-electronics, this work lays out a new, hybrid platform for investigating long distance coupling and nonlinearity in coherent magnonic phenomena.

physics.optics↗

Layer-dependent magnetism and spin fluctuations in atomically thin van der Waals magnet CrPS4

van der Waals (vdW) magnets, an emerging family of two-dimensional (2D) materials, have received tremendous attention due to their rich fundamental physics and significant potential for cutting-edge technological applications. In contrast to the conventional bulk counterparts, vdW magnets exhibit significant tunability of local material properties, such as stacking engineered interlayer coupling and layer-number dependent magnetic and electronic interactions, which promise to deliver previously unavailable merits to develop multifunctional microelectronic devices. As a further ingredient of this emerging topic, here we report nanoscale quantum sensing and imaging of atomically thin vdW magnet chromium thiophosphate CrPS4, revealing its characteristic layer-dependent 2D static magnetism and dynamic spin fluctuations. We also show a large tunneling magnetoresistance in CrPS4-based spin filter vdW heterostructures. The excellent material stability, robust strategy against environmental degradation, in combination with tailored magnetic properties highlight the potential of CrPS4 in developing state-of-the-art 2D spintronic devices for next-generation information technologies.

cond-mat.mes-hall↗

Even-Odd-Layer-Dependent Symmetry Breaking in Synthetic Antiferromagnets

In this work we examine synthetic antiferromagnetic structures consisting of two, three, and four antiferromagnetic coupled layers, i.e., bilayers, trilayers, and tetralayers. We vary the thickness of the ferromagnetic layers across all structures and, using a macrospin formalism, find that the nearest neighbor exchange interaction between layers is consistent across all structures for a given thickness. Our model and experimental results demonstrate significant differences in how the magnetostatic equilibrium states of even and odd-layered structures evolve as a function of the external field. Even layered structures continuously evolve from a collinear antiferromagnetic state to a spin canted non-collinear magnetic configuration that is mirror-symmetric about the external field. In contrast, odd-layered structures begin with a ferrimagnetic ground state; at a critical field, the ferrimagnetic ground state evolves into a non-collinear state with broken symmetry. Specifically, the magnetic moments found in the odd-layered samples possess stable static equilibrium states that are no longer mirror-symmetric about the external field after a critical field is reached. Our results reveal the rich behavior of synthetic antiferromagnets.

cond-mat.mes-hall↗

Oscillatory Edge Modes in Two Dimensional Spin-Torque Oscillator Arrays

Spin torque oscillators (STOs) are dissipative magnetic systems that provide a natural platform for exploring non-Hermitian phenomena. We theoretically study a two-dimensional (2d) array of STOs and show that its dynamics can be mapped to a 2d, non-Hermitian Su-Schrieffer-Heeger (SSH) model. We calculate the energy spectrum and identify the one-dimensional (1d) edge states of our model, corresponding to auto-oscillation of STOs on the boundary of the system while the bulk oscillators do not activate. We show that tuning the Gilbert damping, injected spin current, and coupling between STOs allows for exploring the edge state properties under different parameter regimes. Furthermore, this system admits 1d edge states with non-uniform probability density, and we explore their properties in systems of different sizes. Additional symmetry analysis indicates that these states are not topologically protected but are nevertheless confined to the edge of the system, as the bulk is protected by PT-symmetry. These results indicate that 2d arrays of STOs may be useful to explore novel edge state behavior in dissipative systems.

cond-mat.mes-hall↗

Exceptional points as signatures of dynamical magnetic phase transitions

One of the most fascinating and puzzling aspects of non-Hermitian systems is their spectral degeneracies, i.e., exceptional points (EPs), at which both eigenvalues and eigenvectors coalesce to form a defective state space. While coupled magnetic systems are natural hosts of EPs, the relation between the linear and nonlinear spin dynamics in the proximity of EPs remains relatively unexplored. Here we theoretically investigate the spin dynamics of easy-plane magnetic bilayers in the proximity of exceptional points. We show that the interplay between the intrinsically dissipative spin dynamics and external drives can yield a rich dynamical phase diagram. In particular, we find that, in antiferromagnetically coupled bilayers, a periodic oscillating dynamical phase emerges in the region enclosed by EPs. Our results not only offer a pathway for probing magnetic EPs and engineering magnetic nano-oscillators with large-amplitude oscillations, but also uncover the relation between exceptional points and dynamical phase transitions in systems displaying non-linearities.

cond-mat.mes-hall↗

Magnon-magnon interactions induced by spin pumping-driven symmetry breaking in synthetic antiferromagnets

The richness in both the dispersion and energy of antiferromagnetic magnons has spurred the magnetism community to consider antiferromagnets for future spintronic/magnonic applications. However, the excitation and control of antiferromagnetic magnons remains challenging, especially when compared to ferromagnetic counterparts. A middle ground is found with synthetic antiferromagnet metamaterials, where acoustic and optical magnons exist at GHz frequencies. In these materials, the magnon energy spectrum can be tuned by static symmetry-breaking external fields or dipolar interactions hybridizing optical and acoustic magnon branches. Here, we experimentally measure the magnon energy spectrum of synthetic antiferromagnetic tetralayers, and discover avoided energy level crossings in the energy spectrum that are unexplained by the antiferromagnetic interlayer coupling. We explain our experimental results using a phenomenological model incorporating both fieldlike and dampinglike torques generated by spin pumping in noncollinear magnetic multilayers separated by normal-metal spacers. We show that an asymmetry in the fieldlike torques acting on different magnetic layers can lift the spectral degeneracies of acoustic and optical magnon branches and yield symmetry-breaking induced magnon-magnon interactions. Our work extends the phenomenology of spin pumping to noncollinear magnetization configurations and significantly expands ways of engineering magnon-magnon interactions within antiferromagnets and quantum hybrid magnonic materials.

cond-mat.mes-hall↗

Perspective: non-Hermitian physics in magnetic systems

Non-Hermitian Hamiltonians provide an alternative perspective on the dynamics of quantum and classical systems coupled non-conservatively to an environment. Once primarily an interest of mathematical physicists, the theory of non-Hermitian Hamiltonians has solidified and expanded to describe various physically observable phenomena in optical, photonic, and condensed matter systems. Self-consistent descriptions of quantum mechanics based on non-Hermitian Hamiltonians have been developed and continue to be refined. In particular, non-Hermitian frameworks to describe magnonic and hybrid magnonic systems have gained popularity and utility in recent years, with new insights into the magnon topology, transport properties, and phase transitions coming into view. Magnonic systems are in many ways a natural platform in which to realize non-Hermitian physics because they are always coupled to a surrounding environment and exhibit lossy dynamics. In this perspective we review recent progress in non-Hermitian frameworks to describe magnonic and hybrid magnonic systems, such as cavity magnonic systems and magnon-qubit coupling schemes. We discuss progress in understanding the dynamics of inherently lossy magnetic systems as well as systems with gain induced by externally applied spin currents. We enumerate phenomena observed in both purely magnonic and hybrid magnonic systems which can be understood through the lens of non-Hermitian physics, such as PT and Anti-PT-symmetry breaking, dynamical magnetic phase transitions, non-Hermitian skin effect, and the realization of exceptional points and surfaces. Finally, we comment on some open problems in the field and discuss areas for further exploration.

cond-mat.mes-hall↗

Non-linear dynamics of the non-Hermitian Su-Schrieffer-Heeger model

We numerically determine the robustness of the lasing edge modes in a spin-torque oscillator array that realizes the non-Hermitian Su-Schrieffer-Heeger model. Previous studies found that the linearized dynamics can enter a topological regime in which the edge mode is driven into auto-oscillation, while the bulk dynamics are suppressed. Here we investigate the full non-linear and finite-temperature dynamics, whose understanding is essential for spin-torque oscillators-based applications. Our analysis shows that the lasing edge mode dynamics persist in the non-linear domain for a broad range of parameters and temperatures. We investigate the effects of perturbations relevant to experimental implementations and discuss which ones might be detrimental to the stability of the lasing edge mode. Finally, we map our model onto a photonic model. Our analysis has the potential to shed light onto the dynamics of a plethora of non-Hermitian systems with non-linearities.

cond-mat.mes-hall↗

Multitude of exceptional points in van der Waals magnets

Several works have recently addressed the emergence of exceptional points (EPs), i.e., spectral singularities of non-Hermitian Hamiltonians, in the long-wavelength dynamics of coupled magnetic systems. Here, by focusing on the driven magnetization dynamics of a van der Waals ferromagnetic bilayer, we show that exceptional points can appear over extended portions of the first Brillouin zone as well. Furthermore, we demonstrate that the effective non-Hermitian magnon Hamiltonian, whose eigenvalues are purely real or come in complex-conjugate pairs, respects an unusual wavevector-dependent pseudo-Hermiticity. Finally, for both armchair and zigzag nanoribbon geometries, we discuss both the complex and purely real spectra of the topological edge states and their experimental implications.

cond-mat.mes-hall↗

Topological magnetic phase transition in Eu-based A-type antiferromagnets

Recently, a colossal magnetoresistance (CMR) was observed in EuCd$_2$P$_2$ -- a compound that does not fit the conventional mixed-valence paradigm. Instead, experimental evidence points at a resistance driven by strong magnetic fluctuations within the two-dimensional ($2d$) ferromagnetic (FM) planes of the layered antiferromagnetic (AFM) structure. While the experimental results have not yet been fully understood, a recent theory relates the CMR to a topological vortex-antivortex unbinding, i.e., Berezinskii-Kosterlitz-Thouless (BKT), phase transition. Motivated by these observations, in this work we explore the magnetic phases hosted by a microscopic classical magnetic model for EuCd$_2$P$_2$, which easily generalizes to other Eu A-type antiferromagnetic compounds. Using Monte Carlo techniques to probe the specific heat and the helicity modulus, we show that our model can exhibit a vortex-antivortex unbinding phase transition. We find that this phase transition displays the same sensitivity to in-plane magnetization, interlayer coupling, and easy-plane anisotropy that is observed experimentally in the CMR signal, providing qualitative numerical evidence that the effect is related to a magnetic BKT transition.

cond-mat.mes-hall↗

Non-Hermitian skin effect in magnetic systems

Far from being limited to a trivial generalization of their Hermitian counterparts, non-Hermitian topological phases have gained widespread interest due to their unique properties. One of the most striking non-Hermitian phenomena is the skin effect, i.e., the localization of a macroscopic fraction of bulk eigenstates at a boundary, which underlies the breakdown of the bulk-edge correspondence. Here we investigate the emergence of the skin effect in magnetic insulating systems by developing a phenomenological approach to describing magnetic dissipation within a lattice model. Focusing on a spin-orbit-coupled van der Waals (vdW) ferromagnet with spin-nonconserving magnon-phonon interactions, we find that the magnetic skin effect emerges in an appropriate temperature regime. Our results suggest that the interference between Dzyaloshinskii-Moriya interaction (DMI) and nonlocal magnetic dissipation plays a key role in the accumulation of bulk states at the boundaries.

cond-mat.mes-hall↗

Spin interactions and topological magnonics in chromium trihalide CrClBrI

The discovery of spontaneous magnetism in van der Waal (vdW) magnetic monolayers has opened up an unprecedented platform for investigating magnetism in purely two-dimensional systems. Recently, it has been shown that the magnetic properties of vdW magnets can be easily tuned by adjusting the relative composition of halides. Motivated by these experimental advances, here we derive a model for a trihalide CrClBrI monolayer from symmetry principles and we find that, in contrast to its single-halide counterparts, it can display highly anisotropic nearest- and next-to-nearest neighbor Dzyaloshinskii-Moriya and Heisenberg interactions. Depending on the parameters, the DM interactions are responsible for the formation of exotic chiral spin states, such as skyrmions and spin cycloids, as shown by our Monte Carlo simulations. Focusing on a ground state with a two-sublattice unit cell, we find spin-wave bands with nonvanishing Chern numbers. The resulting magnon edge states yield a magnon thermal Hall conductivity that changes sign as function of temperature and magnetic field, suggesting chromium trihalides as a candidate for testing topological magnon transport in two-dimensional noncollinear spin systems.

cond-mat.mes-hall↗

Magnonics in collinear magnetic insulating systems

In the last decades, collinear magnetic insulating systems have emerged as promising energy-saving information carriers. Their elementary collective spin excitations, i.e., magnons, can propagate for long distances bypassing the Joule heating effects that arise from electron scattering in metal-based devices. This tutorial article provides an introduction to theoretical and experimental advances in the study of magnonics in collinear magnetic insulating systems. We start by outlining the quantum theory of spin waves in ferromagnetic and antiferromagnetic systems and we discuss their quantum statistics. We review the phenomenology of spin and heat transport of the coupled coherent and incoherent spin dynamics and the interplay between magnetic excitations and lattice degrees of freedom. Finally, we introduce the reader to the key ingredients of two experimental probes of magnetization dynamics, spin transport and NV-center relaxometry setups, and discuss experimental findings relevant to the outlined theory.

cond-mat.mes-hall↗

Floquet-engineering topological transitions in a twisted transition metal dichalcogenide homobilayer

Motivated by the recent experimental realization of twisted transition metal dichalcogenide bilayers, we study a simplified model driven by different forms of monochromatic light. As a concrete and representative example we use parameters that correspond to a twisted MoTe$_2$ homobilayer. First, we consider irradiation with circularly polarized light in free space and demonstrate that the corresponding Floquet Hamiltonian takes the same form as the static Hamiltonian, only with a constant overall shift in quasi-energy. This is in stark contrast to twisted bilayer graphene, where new terms are typically generated under an analagous drive. Longitudinal light, on the other hand, which can be generated from the transverse magnetic mode in a waveguide, has a much more dramatic effect--it renormalizes the tunneling strength between the layers, which effectively permits the tuning of the twist angle {\em in-situ}. We find that, by varying the frequency and amplitude of the drive, one can induce a topological transition that cannot be obtained with the traditional form of the Floquet drive in free space. Furthermore, we find that strong drives can have a profound effect on the layer pseudospin texture of the twisted system, which coincides with multiple simultaneous band gap closings in the infinite-frequency limit. Surprisingly, these bandgap closings are not associated with topological transitions. For high but finite drive frequencies near $0.7$eV, the infinite-frequency band crossings become band gap minima of the order of $10^{-6}$ eV or smaller.

cond-mat.mes-hall↗

Quantum Sensing of Spin Transport Properties of an Antiferromagnetic Insulator

Antiferromagnetic insulators (AFIs) are of significant interest due to their potential to develop next-generation spintronic devices. One major effort in this emerging field is to harness AFIs for long-range spin information communication and storage. Here, we report a non-invasive method to optically access the intrinsic spin transport properties of an archetypical AFI α-Fe2O3 via nitrogen-vacancy (NV) quantum spin sensors. By NV relaxometry measurements, we successfully detect the time-dependent fluctuations of the longitudinal spin density of α-Fe2O3. The observed frequency dependence of the NV relaxation rate is in agreement with a theoretical model, from which an intrinsic spin diffusion constant of α-Fe2O3 is experimentally measured in the absence of external spin biases. Our results highlight the significant opportunity offered by NV centers in diagnosing the underlying spin transport properties in a broad range of high-frequency magnetic materials, which are challenging to access by more conventional measurement techniques.

cond-mat.mes-hall↗