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Benjamin A. Stickler

Publications and source records attributed to Benjamin A. Stickler.

At least 19 recordsLinked to original sources

Nonlinear dynamics and mechanical frequency combs with a Meissner-levitated micromagnet

Nonlinearities in multimode mechanical systems can give rise to rich dynamical phenomena with great potential for sensing applications and for future quantum experiments. We demonstrate that the coupled center-of-mass and rotational motion of a Meissner-levitated micromagnet offer a promising platform for nonlinear dynamics, combining low dissipation, magnetic tunability, strong intrinsic Duffing nonlinearities, and nonlinear intermodal couplings. We use this tunability to demonstrate the generation of a mechanical frequency comb in the micromagnet dynamics, realized by parametric excitation of two translational modes followed by cascaded nonlinear frequency mixing, which produces a phononic comb with tunable spacing. At large amplitudes, nonlinear coupling to a low-frequency librational mode of the magnet leads to parametric excitation and phase locking of that mode, generating a dense spectral fine structure at subharmonics of the drive. These results establish levitated micromagnets as a platform for nonlinear multimode mechanics, with potential applications in precision sensing and quantum-limited metrology.

quant-ph

Controlling rotations of magnetically levitated superconductors

Magnetically trapped type-I superconductors are promising candidates for precision experiments at the quantum-to-classical borderline, with applications in quantum sensing of forces and accelerations and fundamental tests of quantum physics. Here, we show how the rotational motion of micron-sized superconductors is strongly affected by (i) the diamagnetic torques due to the gradient of the trapping field and by (ii) the gyromagnetic coupling due to Einstein-de Haas and Barnett effects. We show that this allows the three-dimensional alignment of asperhical superconductors in the trap center, as required for future sensing applications and quantum experiments, and determine the resulting librational trapping frequencies. Finally, we propose an experiment to probe gyromagnetic coupling in levitated superconductors and we discuss how it can be used to control the particle rotation.

quant-ph

A Levitated Random Telegraph Noise Spectrometer

Random Telegraph Noise is a ubiquitous process manifesting across technology and the natural world. It is characterized by random jumps between two distinct states with Poissonian waiting times, and is the origin of 1/f noise. Understanding and characterizing this noise is critical for the reliable operation of micro-, nano- and quantum-technologies. In this work we probe random telegraph noise using a levitated microparticle sensor whose dynamics are driven almost entirely by this non-white source of noise. We observe a startling resonant behaviour, characterized by a thousand-fold increase in the underdamped sensor's position fluctuations, enabling us to measure the spectral properties of the noise over six decades of timescale. This work not only provides a unique way to probe random telegraph noise, but also demonstrates a platform for studying non-equilibrium stochastic dynamics in the presence of realistic non-white noise, with applications from biology to social behaviour.

physics.ins-det

Floquet engineering of nonreciprocal light-induced dipolar interactions

Tweezer arrays of polarizable objects are a promising platform for assembling quantum matter and building next-generation quantum sensors. Light-induced dipolar interactions have emerged as a method to couple their motion, thereby establishing a new paradigm for controlling collective mechanical degrees of freedom. Here, we extend these into the regime of Floquet-driven interactions, combined with the intrinsic nonreciprocity of optical forces. We demonstrate beamsplitter, single-, and two-mode squeezing operations, as well as signatures of a negative-mass-like oscillator arising from the nonreciprocity. Moreover, we show that a programmable combination of these operations enables continuous tuning of complex eigenfrequencies. These results establish a toolbox of quantum operations of nonreciprocal interactions that are essential for investigating non-Hermitian many-body physics and collective quantum optomechanics.

quant-ph

Gyroscopically stabilized quantum spin rotors

Recent experiments demonstrate all-electric spinning of levitated nanodiamonds with embedded nitrogen-vacancy spins. Here, we argue that such gyroscopically stabilized spin rotors offer a promising platform for probing and exploiting quantum spin-rotation coupling of particles hosting a single spin degree of freedom. Specifically, we derive the effective Hamiltonian describing how an embedded spin affects the rotation of rapidly revolving quantum rotors due to the Einstein-de Haas and Barnett effects, which we use to devise experimental protocols for observing this coupling in state-of-the-art experiments. This will open the door for future exploitations of quantum spin rotors for superposition experiments with massive objects.

quant-ph

Steady-state entanglement of interacting masses in free space through optimal feedback control

We develop a feedback strategy based on optimal quantum feedback control for Gaussian systems to maximise the likelihood of steady-state entanglement detection between two directly interacting masses. We employ linear quadratic Gaussian (LQG) control to engineer the phase space dynamics of the two masses and propose Einstein-Podolsky-Rosen (EPR)-type variance minimisation constraints for the feedback to facilitate unconditional entanglement generation. This scheme allows for stationary entanglement in parameter regimes where strategies based on total energy minimisation cooling would fail.

quant-ph

Quantum ground-state cooling of two librational modes of a nanorotor

Controlling the motion of nanoscale objects at the quantum limit promises new tests of quantum mechanics and advanced sensors. Rotational motion is of particular interest, as it follows nonlinear dynamics in a compact, closed configuration space, which opens up a plethora of phenomena and applications beyond the possibilities of free or trapped linear motion. A prerequisite for such experiments is the capability to trap nanorotors and initialize them in a quantum ground state of libration. Here, we demonstrate the reliable, repetitive laser-induced loading of silica nanodimers and trimers into an optical tweezer. Coherent scattering in a high-finesse cavity allows us to cool two different librational modes to the quantum ground state with occupation numbers as low as $n_β=0.54\pm0.32$ and $n_α=0.21\pm0.03$. By simultaneously cooling both degrees of freedom ($n_β=0.73\pm0.22$, $n_α=1.02\pm0.08$) we align nanorotors to a space-fixed axis with precision better than 20$\,μ$rad, close to the zero-point amplitude of librations.

quant-ph

Inverse Microparticle Design for Enhanced Optical Trapping and Detection Efficiency in All Six Degrees of Freedom

Achieving quantum-limited motional control of optically trapped particles beyond the sub-micrometer scale is an outstanding problem in levitated optomechanics. A key obstacle is solving the light scattering problem and identifying particle geometries that allow stable trapping and efficient motional detection of their center of mass and rotational motion in three dimensions. Here, we present a computational framework that combines an efficient electromagnetic scattering solver with the adjoint method to inversely design printable microparticles tailored for levitated optomechanics. Our method allows identifying optimized geometries, characterized by enhanced optical trapping and detection efficiencies compared to conventional microspheres. This improves the feasibility of quantum-limited motional control of all translational and rotational degrees of freedom in a standard standing-wave optical trap.

physics.optics

Nonequilibrium entanglement between levitated masses under optimal control

We present a protocol that maximizes unconditional entanglement generation between two masses interacting directly through $1/r^{n}$ potential. The protocol combines optimal quantum control of continuously measured masses with their non-equilibrium dynamics, driven by a time-dependent interaction strength. Applied to a pair of optically trapped sub-micron particles coupled via electrostatic interaction, our protocol enables unconditional entanglement generation at the fundamental limit of the conditional state and with an order of magnitude smaller interaction between the masses compared to the existing steady-state approaches.

quant-ph

Desorption-induced decoherence of nanoparticle motion

We derive the quantum master equation predicting how the translational and rotational dynamics of a nanoparticle is affected by the emission of surface adsorbates. This is motivated by recent experiments which prepared the motion of internally hot silica particles in the deep quantum regime. In the limit of a well localized nanoparticle the ro-translational dynamics can be characterized by diffusion rates in quantitative agreement with classical expectations. The theory is also suited to describe the decoherence effect of outgassing and sublimation.

quant-ph

Probing molecular photophysics in a matter-wave interferometer

We show that matter-wave diffraction off a single standing laser wave can be used as an accurate measurement scheme for photophysical molecular parameters. These include state-dependent optical polarizabilities and photon-absorption cross sections, the relaxation rates for fluorescence, internal conversion, and intersystem crossing, as well as ionization or cleavage probabilities. We discuss how the different photophysical processes manifest as features of the interference pattern, and we determine the accuracy of molecular parameters estimated from a realistic measurement with finite particle numbers. The analysis is based on an analytic calculation in Wigner representation, which accounts for the laser-induced coherent and incoherent dynamics, for the finite longitudinal and transverse coherence in the matter-wave beam, the gravitational and Coriolis acceleration, and an imperfect standing laser wave.

physics.atom-ph

Probing rotational decoherence with a trapped-ion planar rotor

The quantum rotor is one of the simplest model systems in quantum mechanics, but only in recent years has theoretical work revealed general fundamental scaling laws for its decoherence. For example, a superposition of orientations decoheres at a rate proportional to the sine squared of the angle between them. Here we observe scaling laws for rotational decoherence dynamics for the first time, using a 4-micrometer diameter planar rotor composed of two Paul-trapped ions. We prepare the rotational motion of the ion crystal into superpositions of angular momentum with well-defined differences ranging from 1-3 $\hbar$, and measure the rate of decoherence. We also tune the system-environment interaction strength by introducing resonant electric field noise. The observed scaling relationships for decoherence are in excellent agreement with recent theoretical work, and are directly relevant to the growing development of rotor-based quantum applications.

quant-ph

Decoherence of dielectric particles by thermal emission

Levitated nanoparticles are a promising platform for sensing applications and for macroscopic quantum experiments. While the nanoparticles' motional temperatures can be reduced to near absolute zero, their uncontrolled internal degrees of freedom remain much hotter, inevitably leading to the emission of heat radiation. The decoherence and motional heating caused by this thermal emission process is still poorly understood beyond the case of the center-of-mass motion of point particles. Here, we present the master equation describing the impact of heat radiation on the motional quantum state of arbitrarily sized and shaped dielectric rigid rotors. It predicts the localization of spatio-orientational superpositions only based on the bulk material properties and the particle geometry. A counter-intuitive and experimentally relevant implication of the presented theory is that orientational superpositions of optically isotropic bodies are not protected by their symmetry, even in the small-particle limit.

quant-ph

Quantum theory of non-Hermitian optical binding between nanoparticles

Recent experiments demonstrate highly tunable nonreciprocal coupling between levitated nanoparticles due to optical binding [Rieser et al., Science 377, 987 (2022)]. In view of recent experiments cooling nanoparticles to the quantum regime, we here develop the quantum theory of small dielectric objects interacting via the forces and torques induced by scattered tweezer photons. The interaction is fundamentally non-Hermitian and accompanied by correlated quantum noise. We present the corresponding Markovian quantum master equation and show how to reach nonreciprocal and unidirectional coupling. Our work provides the theoretical tools for exploring and exploiting the rich quantum physics of nonreciprocally coupled nanoparticle arrays.

quant-ph

Quantum Optical Binding of Nanoscale Particles

Optical binding refers to the light-induced interaction between two or more objects illuminated by laser fields. The high tunability of the strength, sign, and reciprocity of this interaction renders it highly attractive for controlling nanoscale mechanical motion. Here, we discuss the quantum theory of optical binding and identify unique signatures of this interaction in the quantum regime. We show that these signatures are observable in near-future experiments with levitated nanoparticles. In addition, we prove the impossibility of entanglement induced by far-field optical binding in free space and identify strategies to circumvent this no-go theorem.

quant-ph

Diffracting molecular matter-waves at deep-ultraviolet standing-light waves

Matter-wave interferometry with molecules is intriguing both because it demonstrates a fundamental quantum phenomenon and because it opens avenues to quantum-enhanced measurements in physical chemistry. One great challenge in such experiments is to establish matter-wave beam splitting mechanisms that are efficient and applicable to a wide range of particles. In the past, continuous standing light waves in the visible spectral range were used predominantly as phase gratings, while pulsed vacuum ultraviolet light found applications in photo-ionisation gratings. Here, we explore the regime of continuous, intense deep-ultraviolet ($\rm >1 MW/cm^2$, $\rm 266\,nm$) light masks, where a rich variety of photo-physical and photo-chemical phenomena and relaxation pathways must be considered. The improved understanding of the mechanisms in this interaction opens new potential pathways to protein interferometry and to matter-wave enhanced sensing of molecular properties.

quant-ph

Talbot interference of whispering gallery modes

The Talbot self-imaging phenomenon is a fundamental interference effect that is natural to all waves with a periodic structure. We theoretically and experimentally study the Talbot effect for optical waves in the transverse angular domain using whispering-gallery modes of step-index multimode fibers, which carry a high orbital angular momentum and fulfill the required quadratic dispersion relation. By using the complex interference along the core-cladding interface of these fibers, we experimentally demonstrate that the high-order fractional Talbot effect can be used to implement 9- and 30-port beamsplitters using only off-the-shelf components in a compact arrangement. In addition, we show that the beamsplitters can be efficiently interfaced with single-mode fibers, such that our work not only extends the recent developments on the angular Talbot effect to widely available step-index multimode fibers, but also demonstrates a powerful application as a signal multiplexer, which becomes more compact as the number of channels is increased.

physics.optics

Non-Hermitian dynamics and nonreciprocity of optically coupled nanoparticles

Non-Hermitian dynamics, as observed in photonic, atomic, electrical, and optomechanical platforms, holds great potential for sensing applications and signal processing. Recently, fully tunable nonreciprocal optical interaction has been demonstrated between levitated nanoparticles. Here, we use this tunability to investigate the collective non-Hermitian dynamics of two nonreciprocally and nonlinearly interacting nanoparticles. We observe parity-time symmetry breaking and, for sufficiently strong coupling, a collective mechanical lasing transition, where the particles move along stable limit cycles. This work opens up a research avenue of nonequilibrium multi-particle collective effects, tailored by the dynamic control of individual sites in a tweezer array.

physics.optics