arXiv subjects

Benjamin A. Stickler

Publications and source records attributed to Benjamin A. Stickler.

At least 55 records · Page 3Linked to original sources

arXiv2020

Quantum persistent tennis racket dynamics of nanorotors

Classical rotations of asymmetric rigid bodies are unstable around the axis of intermediate momentof inertia, causing a flipping of rotor orientation. This effect, known as the tennis racket effect,quickly averages to zero in classical ensembles since the flipping period varies significantly uponapproaching the separatrix. Here, we explore the quantum rotations of rapidly spinning thermalasymmetric nanorotors and show that classically forbidden tunnelling gives rise to persistent tennisracket dynamics, in stark contrast to the classical expectation. We characterise this effect, demon-strating that quantum coherent flipping dynamics can persist even in the regime where millions ofangular momentum states are occupied. This persistent flipping offers a promising route for observ-ing and exploiting quantum effects in rotational degrees of freedom for molecules and nanoparticles.

quant-ph↗

arXiv2020

Quantum electromechanics with levitated nanoparticles

Preparing and observing quantum states of nanoscale particles is a challenging task with great relevance for quantum technologies and tests of fundamental physics. In contrast to atomic systems with discrete transitions, nanoparticles exhibit a practically continuous absorption spectrum and thus their quantum dynamics cannot be easily manipulated. Here, we demonstrate that charged nanoscale dielectrics can be artificially endowed with a discrete level structure by coherently interfacing their rotational and translational motion with a superconducting qubit. We propose a pulsed scheme for the generation and read-out of motional quantum superpositions and entanglement between several levitated nanoparticles, providing an all-electric platform for networked hybrid quantum devices.

quant-ph↗

arXiv2020

Entangling levitated nanoparticles by coherent scattering

We show how entanglement between two optically levitated nanoparticles can be generated and detected by coherent scattering of tweezer photons into a single cavity mode. Triggered by the detection of a Stokes photon, the tweezer detuning is switched from the blue to the red; entanglement is then verified by the conditioned anti-Stokes photon flux, which oscillates with the mechanical beat frequency. The proposed setup is realizable with near-future technology and opens the door to the first experimental observation of non-classical center-of-mass correlations between two or more levitated nanoscale objects.

quant-ph↗

arXiv2019

Macroscopicity of quantum mechanical superposition tests via hypothesis falsification

We establish an objective scheme to determine the macroscopicity of quantum mechanical superposition tests, which is based on the Bayesian hypothesis falsification of macrorealistic modifications of quantum theory. The measure uses the raw data gathered in an experiment, taking into account all measurement uncertainties, and can be used to directly assess any conceivable quantum test. We determine the resulting macroscopicity for three recent tests of quantum physics: double-well interference of Bose-Einstein condensates, Leggett-Garg tests with atomic random walks, and entanglement generation and read-out of nanomechanical oscillators.

quant-ph↗

arXiv2019

Decoherence of nonrelativistic bosonic quantum fields

We present a generic Markovian master equation inducing the gradual classicalization of a bosonic quantum field. It leads to the decoherence of quantum superpositions of field configurations, while leaving the Ehrenfest equations for both the field and the mode-variables invariant. We characterize the classicalization analytically and numerically, and show that the semiclassical field dynamics is described by a linear Boltzmann equation in the functional phase space of field configurations.

quant-ph↗

arXiv2019

Levitated electromechanics: all-electrical cooling of charged nano- and micro-particles

We show how charged levitated nano- and micro-particles can be cooled by interfacing them with an $RLC$ circuit. All-electrical levitation and cooling is applicable to a wide range of particle sizes and materials, and will enable state-of-the-art force sensing within an electrically networked system. Exploring the cooling limits in the presence of realistic noise we find that the quantum regime of particle motion can be reached in cryogenic environments both for passive resistive cooling and for an active feedback scheme, paving the way to levitated quantum electromechanics.

quant-ph↗

arXiv2018

Probing Macroscopic Quantum Superpositions with Nanorotors

Whether quantum physics is universally valid is an open question with far-reaching implications. Intense research is therefore invested into testing the quantum superposition principle with ever heavier and more complex objects. Here we propose a radically new, experimentally viable route towards studies at the quantum-to-classical borderline by probing the orientational quantum revivals of a nanoscale rigid rotor. The proposed interference experiment testifies a macroscopic superposition of all possible orientations. It requires no diffraction grating, uses only a single levitated particle, and works with moderate motional temperatures under realistic environmental conditions. The first exploitation of quantum rotations of a massive object opens the door to new tests of quantum physics with submicron particles and to quantum gyroscopic torque sensors, holding the potential to improve state-of-the art devices by many orders of magnitude.

quant-ph↗

arXiv2018

Conformer-selection by matter-wave interference

We establish that matter-wave interference at near-resonant ultraviolet optical gratings can be used to spatially separate individual conformers of complex molecules. Our calculations show that the conformational purity of the prepared beam can be close to 100% and that all molecules remain in their electronic ground state. The proposed technique is independent of the dipole moment and the spin of the molecule and thus paves the way for structure-sensitive experiments with hydrocarbons and biomolecules, such as neurotransmitters and hormones, which evaded conformer-pure isolation so far

physics.chem-ph↗

arXiv2018

Rotational friction and diffusion of quantum rotors

We present the Markovian quantum master equation describing rotational decoherence, friction, diffusion, and thermalization of planar, linear, and asymmetric rotors in contact with a thermal environment. It describes how an arbitrary initial rotation state decoheres and evolves toward a Gibbs-like thermal ensemble, as we illustrate numerically for the linear and the planar top, and it yields the expected rotational Fokker-Planck equation of Brownian motion in the semiclassical limit.

quant-ph↗

arXiv2018

Rotational Alignment Decay and Decoherence of Molecular Superrotors

We present the quantum master equation describing the coherent and incoherent dynamics of a rapidly rotating molecule in presence of a thermal background gas. The master equation relates the rate of rotational alignment decay and decoherence to the microscopic scattering amplitudes, which we calculate for anisotropic van der Waals scattering. For large rotational energies, we find excellent agreement of the resulting alignment decay rate with recent superrotor experiments.

quant-ph↗

arXiv2018

Gas-induced friction and diffusion of rigid rotors

We derive the Boltzmann equation for the rotranslational dynamics of an arbitrary convex rigid body in a rarefied gas. It yields as a limiting case the Fokker-Planck equation accounting for friction, diffusion, and nonconservative drift forces and torques. We provide the rotranslational friction and diffusion tensors for specular and diffuse reflection off particles with spherical, cylindrical, and cuboidal shape, and show that the theory describes thermalization, photophoresis, and the inverse Magnus effect in the free molecular regime.

cond-mat.stat-mech↗

arXiv2017

Quantum Angular Momentum Diffusion of Rigid Bodies

We show how to describe the diffusion of the quantized angular momentum vector of an arbitrarily shaped rigid rotor as induced by its collisional interaction with an environment. We present the general form of the Lindblad-type master equation and relate it to the orientational decoherence of an asymmetric nanoparticle in the limit of small anisotropies. The corresponding diffusion coefficients are derived for gas particles scattering off large molecules and for ambient photons scattering off dielectric particles, using the elastic scattering amplitudes.

quant-ph↗

arXiv2017

Optically driven ultra-stable nanomechanical rotor

Nanomechanical devices have attracted the interest of a growing interdisciplinary research community, since they can be used as highly sensitive transducers for various physical quantities. Exquisite control over these systems facilitates experiments on the foundations of physics. Here, we demonstrate that an optically trapped silicon nanorod, set into rotation at MHz frequencies, can be locked to an external clock, transducing the properties of the time standard to the rod's motion with the remarkable frequency stability $f_{\rm r}/Δf_{\rm r}$ of $7.7 \times 10^{11}$. While the dynamics of this periodically driven rotor generally can be chaotic, we derive and verify that stable limit cycles exist over a surprisingly wide parameter range. This robustness should enable, in principle, measurements of external torques with sensitivities better than 0.25zNm, even at room temperature. We show that in a dilute gas, real-time phase measurements on the locked nanorod transduce pressure values with a sensitivity of 0.3%.

quant-ph↗

arXiv2017

Collapse-induced Orientational Localization of Rigid Rotors

We show how the ro-translational motion of anisotropic particles is affected by the model of Continuous Spontaneous Localization (CSL), the most prominent hypothetical modification of the Schrödinger equation restoring realism on the macroscale. We derive the master equation describing collapse-induced spatio-orientational decoherence, and demonstrate how it leads to linear- and angular-momentum diffusion. Since the associated heating rates scale differently with the CSL parameters, the latter can be determined individually by measuring the random motion of a single levitated nanorotor.

quant-ph↗

arXiv2017

Full Rotational Control of Levitated Silicon Nanorods

We study a nanofabricated silicon rod levitated in an optical trap. By manipulating the polarization of the light we gain full control over the ro-translational dynamics of the rod. We are able to trap both its centre-of-mass and align it along the linear polarization of the laser field. The rod can be set into rotation at a tuned frequency by exploiting the radiation pressure exerted by elliptically polarized light. The rotational motion of the rod dynamically modifies the optical potential, which allows tuning of the rotational frequency over hundreds of Kilohertz. This ability to trap and control the motion and alignment of nanoparticles opens up the field of rotational optomechanics, rotational ground state cooling and the study of rotational thermodynamics in the underdamped regime.

quant-ph↗

arXiv2016

Ro-Translational Cavity Cooling of Dielectric Rods and Disks

We study the interaction of dielectric rods and disks with the laser field of a high finesse cavity. The quantum master equation for the coupled particle-cavity dynamics, including Rayleigh scattering, is derived for particle sizes comparable to the laser wavelength. We demonstrate that such anisotropic nanoparticles can be captured from free flight at velocities higher than those required to capture dielectric spheres of the same volume, and that efficient ro-translational cavity cooling into the deep quantum regime is achievable.

quant-ph↗

arXiv2016

Spatio-Orientational Decoherence of Nanoparticles

Motivated by trapping and cooling experiments with non-spherical nanoparticles, we discuss how their combined rotational and translational quantum state is affected by the interaction with a gaseous environment. Based on the quantum master equation in terms of orientation-dependent scattering amplitudes, we evaluate the localization rate for gas collisions off an anisotropic van der Waals-type potential and for photon scattering off an anisotropic dielectric. We also show how pure angular momentum diffusion arises from these open quantum dynamics in the limit of weak anisotropies.

quant-ph↗

arXiv2015

Molecular Rotations in Matter-Wave Interferometry

We extend the theory of matter-wave interferometry of point-like particles to non-spherical objects by taking the orientational degrees of freedom into account. In particular, we derive the grating transformation operator, that maps the impinging state onto the outgoing state, for a general, orientation-dependent interaction potential between the grating and the molecule. The grating operator is then worked out for the diffraction of symmetric top molecules from standing light waves, and the resulting interference pattern is calculated in the near-field. This allows us to identify a signature of the orientational degrees of freedom in near-field matter-wave experiments.

quant-ph↗