arXiv subjects

Benjamin Dollet

Publications and source records attributed to Benjamin Dollet.

27 records · Page 2Linked to original sources

arXiv2011

Dynamical thickening transition in plate coating with concentrated surfactant solutions

We present a large range of experimental data concerning the influence of surfactants on the well-known Landau-Levich-Derjaguin experiment where a liquid film is generated by pulling a solid plate out of a bath. The thickness h of the film was measured as a function of the pulling velocity V for different kind of surfactant and at various concentrations. Measuring the thickening factor $α=h/h_{LLD}$, where hLLD is obtained for a pure liquid, in a wide range of capillary ($Ca=ηV/γ$), two regimes of constant thickening can be identified: at small capillary number, $α$ is large due to a confinement and surface elasticity (or Marangoni) effects and at large Ca, $α$ is slightly higher than unity, due to surface viscous effects. At intermediate Ca, $α$ decreases as Ca increases along a "dynamic transition". In the case of non-ionic surfactants, the dynamic transition occurs at a fixed Ca, independently of the surfactant concentration, while for ionic surfactants, the dynamic transition depends on the concentration due to the existence of an electrostatic barrier. The control of physico-chemical parameters allowed us to elucidate the nature of the dynamic transition and to relate it to surface rheology.

cond-mat.soft↗

arXiv2011

Bubble size prediction in co-flowing streams

In this paper, the size of bubbles formed through the breakup of a gaseous jet in a co-axial microfluidic device is derived. The gaseous jet surrounded by a co-flowing liquid stream breaks up into monodisperse microbubbles and the size of the bubbles is determined by the radius of the inner gas jet and the bubble formation frequency. We obtain the radius of the gas jet by solving the Navier-Stokes equations for low Reynolds number flows and by minimization of the dissipation energy. The prediction of the bubble size is based on the system's control parameters only, i.e. the inner gas flow rate $Q_i$, the outer liquid flow rate $Q_o$, and the tube radius $R$. For a very low gas-to-liquid flow rate ratio ($Q_i / Q_o \rightarrow 0$) the bubble radius scales as $r_b / R \propto \sqrt{Q_i / Q_o}$, independently of the inner to outer viscosity ratio $η_i/η_o$ and of the type of the velocity profile in the gas, which can be either flat or parabolic, depending on whether high-molecular-weight surfactants cover the gas-liquid interface or not. However, in the case in which the gas velocity profiles are parabolic and the viscosity ratio is sufficiently low, i.e. $η_i/η_o \ll 1$, the bubble diameter scales as $r_b \propto (Q_i/Q_o)^β$, with $β$ smaller than 1/2.

physics.flu-dyn↗

arXiv2011

Microbubble formation and pinch-off scaling exponent in flow-focusing devices

We investigate the gas jet breakup and the resulting microbubble formation in a microfluidic flow-focusing device using ultra high-speed imaging at 1 million frames/s. In recent experiments [Dollet et al., Phys. Rev. Lett. 100, 034504 (2008)] it was found that in the final stage of the collapse the radius of the neck scales with time with a 1/3 power-law exponent, which suggested that gas inertia and the Bernoulli suction effect become important. Here, ultra high-speed imaging was used to capture the complete bubble contour and quantify the gas flow through the neck. It revealed that the resulting decrease in pressure, due to Bernoulli suction, is too low to account for an accelerated pinch-off. The high temporal resolution images enable us to approach the final moment of pinch-off to within 1 μs. We observe that the final moment of bubble pinch-off is characterized by a scaling exponent of 0.41 +/- 0.01. This exponent is approximately 2/5, which can be derived, based on the observation that during the collapse the neck becomes less slender, due to the exclusive driving through liquid inertia.

physics.flu-dyn↗

arXiv2009

Local description of the two-dimensional flow of foam through a contraction

The 2D flow of a foam confined in a Hele-Shaw cell through a contraction is investigated. Its rheological features are quantified using image analysis, with measurements of the elastic stress, rate of plasticity, and velocity. The behavior of the velocity strongly differs at the contraction entrance, where the flow is purely convergent, and at the contraction exit, where a velocity undershoot and a re-focussing of the streamlines are unraveled. The yielded region, characterized by a significant rate of plasticity and a maximal stress amplitude, is concentrated close to the contraction. These qualitative generic trends do not vary significantly with the flow rate, bubble area and contraction geometry, which is characteristic of a robust quasistatic regime. Using surfactants with a high surface viscoelasticity, a marked dependence of the elastic stress on the velocity is exhibited. The results show that the rate of plasticity does not only depend on the local magnitude of the deformation rate, but also crucially on the orientation of both elastic stresses and deformation rate. It is also discussed how the viscous friction controls the departure from the quasistatic regime.

cond-mat.soft↗

arXiv2009

Preferred sizes and ordering in surface nanobubble populations

Two types of homogeneous surface nanobubble populations, created by different means, are analyzed statistically on both their sizes and spatial positions. In the first type (created by droplet-deposition, case A) the bubble size R is found to be distributed according to a generalized gamma law with a preferred radius R*=20 nm. The radial distribution function shows a preferred spacing at ~5.5 R*. These characteristics do not show up in comparable Monte-Carlo simulations of random packings of hard disks with the same size distribution and the same density, suggesting a structuring effect in the nanobubble formation process. The nanobubble size distribution of the second population type (created by ethanol-water exchange, case B) is a mixture of two clearly separated distributions, hence, with two preferred radii. The local ordering is less significant, due to the looser packing of the nanobubbles.

physics.flu-dyn↗

arXiv2006

Two-dimensional flow of foam around a circular obstacle: local measurements of elasticity, plasticity and flow

We investigate the two-dimensional flow of a liquid foam around circular obstacles by measuring all the local fields necessary to describe this flow: velocity, pressure, bubble deformations and rearrangements. We show how our experimental setup, a quasi-2D "liquid pool" system, is adapted to the determination of these fields: the velocity and bubble deformations are easy to measure from 2D movies, and the pressure can be measured by exploiting a specific feature of this system, a 2D effective compressibility. To describe accurately bubble rearrangements, we propose a new, tensorial descriptor. All these quantities are evaluated via an averaging procedure that we justify showing that the fluctuations of the fields are essentially random. The flow is extensively studied in a reference experimental case; the velocity presents an overshoot in the wake of the obstacle, the pressure is maximum at the leading side and minimal at the trailing side. The study of the elastic deformations and of the velocity gradients shows that the transition between plug flow and yielded regions is smooth. Our tensorial description of T1s highlight their correlation both with the bubble deformations and the velocity gradients. A salient feature of the flow, notably on the velocity and T1 repartition, is a marked asymmetry upstream/downstream, signature of the elastic behaviour of the foam. We show that the results do not change qualitatively when various control parameters vary, identifying a robust quasistatic regime. These results are discussed in the frame of the actual foam rheology literature, and we argue that they constitute a severe test for existing rheological models, since they capture both the elastic, plastic and fluid behaviour of the foam.

physics.flu-dyn↗

arXiv2005

Inverse lift: a signature of the elasticity of complex fluids?

To understand the mechanics of a complex fluid such as a foam we propose a model experiment (a bidimensional flow around an obstacle) for which an external sollicitation is applied, and a local response is measured, simultaneously. We observe that an asymmetric obstacle (cambered airfoil profile) experiences a downards lift, opposite to the lift usually known (in a different context) in aerodynamics. Correlations of velocity, deformations and pressure fields yield a clear explanation of this inverse lift, involving the elasticity of the foam. We argue that such an inverse lift is likely common to complex fluids with elasticity.

cond-mat.soft↗

arXiv2005

Two-dimensional flow of foam around an obstacle: force measurements

A Stokes experiment for foams is proposed. It consists in a two-dimensional flow of a foam, confined between a water subphase and a top plate, around a fixed circular obstacle. We present systematic measurements of the drag exerted by the flowing foam on the obstacle, \emph{versus} various separately controlled parameters: flow rate, bubble volume, bulk viscosity, obstacle size, shape and boundary conditions. We separate the drag into two contributions, an elastic one (yield drag) at vanishing flow rate, and a fluid one (viscous coefficient) increasing with flow rate. We quantify the influence of each control parameter on the drag. The results exhibit in particular a power-law dependence of the drag as a function of the bulk viscosity and the flow rate with two different exponents. Moreover, we show that the drag decreases with bubble size, and increases proportionally to the obstacle size. We quantify the effect of shape through a dimensioned drag coefficient, and we show that the effect of boundary conditions is small.

cond-mat.soft↗

arXiv2004

Two-dimensional flows of foam: drag exerted on circular obstacles and dissipation

A Stokes experiment for foams is proposed. It consists in a two-dimensional flow of a foam, confined between a water subphase and a top plate, around a fixed circular obstacle. We present systematic measurements of the drag exerted by the flowing foam on the obstacle, \emph{versus} various separately controlled parameters: flow rate, bubble volume, solution viscosity, obstacle size and boundary conditions. We separate the drag into two contributions, an elastic one (yield drag) at vanishing flow rate, and a fluid one (viscous coefficient) increasing with flow rate. We quantify the influence of each control parameter on the drag. The results exhibit in particular a power-law dependence of the drag as a function of the solution viscosity and the flow rate with two different exponents. Moreover, we show that the drag decreases with bubble size, increases with obstacle size, and that the effect of boundary conditions is small. Measurements of the streamwise pressure gradient, associated to the dissipation along the flow of foam, are also presented: they show no dependence on the presence of an obstacle, and pressure gradient depends on flow rate, bubble volume and solution viscosity with three independent power laws.

cond-mat.soft↗