arXiv subjects

Benjamin J. Sussman

Publications and source records attributed to Benjamin J. Sussman.

At least 19 recordsLinked to original sources

arXiv2026

Simultaneous amplitude and phase spectroscopy using two-photon interference

Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin beams of light to reduce the noise sources inherent to absorption spectroscopy. However, measurements of the phase shift imparted by the chemical sample, which provides complementary information to the absorption, continue to be a challenge. Here, we propose and demonstrate a scheme using entangled photon pairs that can simultaneously measure both the absorption and phase shift of a sample with extremely low optical intensities and with relatively fast few-minute acquisition times. This method combines the previous use of intensity correlations with a broadband quantum interferometer utilizing two-photon interference to measure the complete linear optical response of the sample. Our work shows that precise measurements of absorption can also be made phase-sensitive using suitable choices of probe beam and detection scheme. This enables a new class of quantum spectroscopy schemes which measure absorption and phase with a single probe. Our technique is relevant to the characterization of a wide array of chemical and biological samples, such as quantum dots and organic fluorophores, and may be useful for spectroscopic measurements that are otherwise constrained in intensity.

quant-ph↗

arXiv2025

Ultrafast switching of telecom photon-number states

A crucial component of photonic quantum information processing platforms is the ability to modulate, route, convert, and switch quantum states of light noiselessly with low insertion loss. For instance, a high-speed, low-loss optical switch is crucial for scaling quantum photonic systems that rely on measurement-based feed-forward approaches. Such a device will also ideally be capable of operating on photon-number states, which can act as non-Gaussian resources. Here, we demonstrate ultrafast all-optical switching of heralded photon-number states, of up to 6 photons, using the optical Kerr effect in a single-mode fiber. A local birefringence is created by a high-intensity pump pulse at a center wavelength of 1030 nm which overlaps temporally with the 1550 nm photons in the fiber. A switching efficiency of $>$99 % is reached with a resolution of 2.3 ps, an insertion loss of $2.27\pm0.08$ dB, and a signal-to-noise ratio of 32,000.

quant-ph↗

arXiv2025

Broadband spectral manipulation of single photons using cross-phase modulation

Manipulating the frequency and bandwidth of light is crucial in classical and quantum applications including communication, spectroscopy, imaging, and signal processing. Such capabilities also offer potential for interfacing disparate quantum systems in quantum networking and for quantum information processing. We experimentally demonstrate deterministic, broadband frequency control of heralded telecom-band single photons via cross-phase modulation in a short length of single-mode fiber. An intense, ultrafast pump pulse imposes a transient, intensity-dependent refractive-index gradient which imparts a tunable phase shift on the single photons. We present absolute frequency shifts of up to $+6.46\pm0.01$\,THz and $-5.74\pm0.01$\,THz, and bandwidth manipulation ranging from a factor of $0.66\pm0.03$ to $8.4\pm0.3$ times that of the input. Spectral measurements are acquired with a time-of-flight spectrometer and superconducting nanowire detectors. Our scheme offers a compact and scalable route to spectral routing and bandwidth engineering for ultrafast quantum networking and quantum information processing.

quant-ph↗

arXiv2025

Imaging at the quantum limit with convolutional neural networks

Deep neural networks have been shown to achieve exceptional performance for computer vision tasks like image recognition, segmentation, and reconstruction or denoising. Here, we evaluate the ultimate performance limits of deep convolutional neural network models for image reconstruction, by comparing them against the standard quantum limit set by shot-noise and the Heisenberg limit on precision. We train U-Net models on images of natural objects illuminated with coherent states of light, and find that the average mean-squared error of the reconstructions can surpass the standard quantum limit, and in some cases reaches the Heisenberg limit. Further, we train models on well-parameterized images for which we can calculate the quantum Cramér-Rao bound to determine the minimum possible measurable variance of an estimated parameter for a given probe state. We find the mean-squared error of the model predictions reaches these bounds calculated for the parameters, across a variety of parameterized images. These results suggest that deep convolutional neural networks can learn to become the optimal estimators allowed by the laws of physics, performing parameter estimation and image reconstruction at the ultimate possible limits of precision for the case of classical illumination of the object.

cs.LG↗

arXiv2025

Terahertz electro-optic modulation of single photons

The manipulation of visible and near-infrared light at the single-photon level plays a key role in quantum communication systems where information is encoded into photonic degrees of freedom. In practical implementations, it is important to achieve this manipulation with high speeds, low loss, and low noise. In this work, we propose the use of terahertz~(THz) electric fields as a pump source for electro-optic modulation of single photons in bulk media. We demonstrate spectral modulations of single photons in the form of frequency translation and bandwidth manipulations as the terahertz field imparts linear and quadratic phases on the photons at various time delays within 1~ps. Our results show frequency translations exceeding 500~GHz at multi-THz modulation speeds and loss levels of $\approx$1~dB, complementing the current state-of-the-art electro-optic modulation techniques limited to speeds up to 100~GHz. The proposed approach leverages recent developments in terahertz generation techniques, introducing new avenues to manipulate non-classical light in an unexplored regime for quantum photonics.

quant-ph↗

arXiv2024

3D-2D Neural Nets for Phase Retrieval in Noisy Interferometric Imaging

In recent years, neural networks have been used to solve phase retrieval problems in imaging with superior accuracy and speed than traditional techniques, especially in the presence of noise. However, in the context of interferometric imaging, phase noise has been largely unaddressed by existing neural network architectures. Such noise arises naturally in an interferometer due to mechanical instabilities or atmospheric turbulence, limiting measurement acquisition times and posing a challenge in scenarios with limited light intensity, such as remote sensing. Here, we introduce a 3D-2D Phase Retrieval U-Net (PRUNe) that takes noisy and randomly phase-shifted interferograms as inputs, and outputs a single 2D phase image. A 3D downsampling convolutional encoder captures correlations within and between frames to produce a 2D latent space, which is upsampled by a 2D decoder into a phase image. We test our model against a state-of-the-art singular value decomposition algorithm and find PRUNe reconstructions consistently show more accurate and smooth reconstructions, with a x2.5 - 4 lower mean squared error at multiple signal-to-noise ratios for interferograms with low (< 1 photon/pixel) and high (~100 photons/pixel) signal intensity. Our model presents a faster and more accurate approach to perform phase retrieval in extremely low light intensity interferometry in presence of phase noise, and will find application in other multi-frame noisy imaging techniques.

physics.optics↗

arXiv2024

Toward deterministic sources: Photon generation in a fiber-cavity quantum memory

We demonstrate the generation of photons within a fiber-cavity quantum memory, followed by later on-demand readout. Signal photons are generated by spontaneous four-wave mixing in a fiber cavity comprising a birefringent fiber with dichroic reflective end facets. The detection of the partner herald photon indicates the creation of the stored signal photon. After a delay, the signal photon is switched out of resonance with the fiber cavity by intracavity frequency translation using Bragg scattering four-wave mixing, driven by ancillary control pulses. We measure sub-Poissonian statistics in the output signal mode, with $g^{(2)}_{AC}=0.54(1)$ in the first readout bin and a readout frequency translation efficiency of $\approx$80%. The 1/e memory lifetime is $\approx$67 cavity cycles, or 1.68$μ$s. In an alternate fiber cavity, we show a strategy for noise reduction and measure $g^{(2)}_{AC}=0.068(10)$ after one cavity cycle.

quant-ph↗

arXiv2022

Toward a Quantum Memory in a Fiber Cavity Controlled by Intracavity Frequency Translation

We propose a quantum memory protocol based on trapping photons in a fiber-integrated cavity, comprised of a birefringent fiber with dichroic reflective end facets. Photons are switched into resonance with the fiber cavity by intracavity Bragg-scattering frequency translation, driven by ancillary control pulses. After the storage delay, photons are switched out of resonance with the cavity, again by intracavity frequency translation. We demonstrate storage of quantum-level THz-bandwidth coherent states for a lifetime up to 16 cavity round trips, or 200ns, and a maximum overall efficiency of 73%.

quant-ph↗

arXiv2020

Enhancing LIDAR performance metrics using continuous-wave photon-pair sources

In order to enhance LIDAR performance metrics such as target detection sensitivity, noise resilience and ranging accuracy, we exploit the strong temporal correlation within the photon pairs generated in continuous-wave pumped semiconductor waveguides. The enhancement attained through the use of such non-classical sources is measured and compared to a corresponding target detection scheme based on simple photon-counting detection. The performances of both schemes are quantified by the estimation uncertainty and Fisher information of the probe photon transmission, which is a widely adopted sensing figure of merit. The target detection experiments are conducted with high probe channel loss ($\simeq 1-5\times10^{-5}$) and formidable environment noise up to 36 dB stronger than the detected probe power of $1.64\times 10^{-5}$ pW. The experimental result shows significant advantages offered by the enhanced scheme with up to 26.3 dB higher performance in terms of estimation uncertainty, which is equivalent to a reduction of target detection time by a factor of 430 or 146 (21.6 dB) times more resilience to noise. We also experimentally demonstrated ranging with these non-classical photon pairs generated with continuous-wave pump in the presence of strong noise and loss, achieving $\approx$5 cm distance resolution that is limited by the temporal resolution of the detectors.

physics.optics↗

arXiv2020

Underwater quantum communication over a 30-meter flume tank

Underwater quantum communication has recently been explored using polarization and orbital angular momentum. Here, we show that spatially structured modes, e.g., a coherent superposition of beams carrying both polarization and orbital angular momentum, can also be used for underwater quantum cryptography. We also use the polarization degree of freedom for quantum communication in an underwater channel having various lengths, up to $30$ meters. The underwater channel proves to be a difficult environment for establishing quantum communication as underwater optical turbulence results in significant beam wandering and distortions. However, the errors associated to the turbulence do not result in error rates above the threshold for establishing a positive key in a quantum communication link with both the polarization and spatially structured photons. The impact of the underwater channel on the spatially structured modes is also investigated at different distances using polarization tomography.

quant-ph↗

arXiv2019

Theory of Four-Wave Mixing of Cylindrical Vector Beams in Optical Fibers

Cylindrical vector (CV) beams are a set of transverse spatial modes that exhibit a cylindrically symmetric intensity profile and a variable polarization about the beam axis. They are composed of a non-separable superposition of orbital and spin angular momentum. Critically, CV beams are also the eigenmodes of optical fiber and, as such, are of wide-spread practical importance in photonics and have the potential to increase communications bandwidth through spatial multiplexing. Here, we derive the coupled amplitude equations that describe the four-wave mixing (FWM) of CV beams in optical fibers. These equations allow us to determine the selection rules that govern the interconversion of CV modes in FWM processes. With these selection rules, we show that FWM conserves the total angular momentum, the sum of orbital and spin angular momentum, in the conversion of two input photons to two output photons. When applied to spontaneous four-wave mixing, the selection rules show that photon pairs can be generated in CV modes directly and can be entangled in those modes. Such quantum states of light in CV modes could benefit technologies such as quantum key distribution with satellites.

physics.optics↗

arXiv2019

Characterization of an underwater channel for quantum communications in the Ottawa River

We examine the propagation of optical beams possessing different polarization states and spatial modes through the Ottawa River in Canada. A Shack-Hartmann wavefront sensor is used to record the distorted beam's wavefront. The turbulence in the underwater channel is analysed, and associated Zernike coefficients are obtained in real-time. Finally, we explore the feasibility of transmitting polarization states as well as spatial modes through the underwater channel for applications in quantum cryptography.

quant-ph↗

arXiv2018

Quantum-enhanced standoff detection using correlated photon pairs

We investigate the use of correlated photon pair sources for the improved quantum-level detection of a target in the presence of a noise background. Photon pairs are generated by spontaneous four-wave mixing, one photon from each pair (the herald) is measured locally while the other (the signal) is sent to illuminate the target. Following diffuse reflection from the target, the signal photons are detected by a receiver and non-classical timing correlations between the signal and herald are measured in the presence of a configurable background noise source. Quantum correlations from the photon pair source can be used to provide an enhanced signal-to-noise ratio when compared to a classical light source of the same intensity.

quant-ph↗

arXiv2018

THz-bandwidth all-optical switching of heralded single photons

Optically induced ultrafast switching of single photons is demonstrated by rotating the photon polarization via the Kerr effect in a commercially available single mode fiber. A switching efficiency of 97\% is achieved with a $\sim1.7$\,ps switching time, and signal-to-noise ratio of $\sim800$. Preservation of the quantum state is confirmed by measuring no significant increase in the second-order autocorrelation function $g^{(2)}(0)$. These values are attained with only nanojoule level pump energies that are produced by a laser oscillator with 80\,MHz repetition rate. The results highlight a simple switching device capable of both high-bandwidth operations and preservation of single-photon properties for applications in photonic quantum processing and ultrafast time-gating or switching.

quant-ph↗

arXiv2017

Time-bin to Polarization Conversion of Ultrafast Photonic Qubits

The encoding of quantum information in photonic time-bin qubits is apt for long distance quantum communication schemes. In practice, due to technical constraints such as detector response time, or the speed with which co-polarized time-bins can be switched, other encodings, e.g. polarization, are often preferred for operations like state detection. Here, we present the conversion of qubits between polarization and time-bin encodings using a method that is based on an ultrafast optical Kerr shutter and attain efficiencies of 97% and an average fidelity of 0.827+/-0.003 with shutter speeds near 1 ps. Our demonstration delineates an essential requirement for the development of hybrid and high-rate optical quantum networks.

quant-ph↗

arXiv2017

Storage of polarization-entangled THz-bandwidth photons in a diamond quantum memory

Bulk diamond phonons have been shown to be a versatile platform for the generation, storage, and manipulation of high-bandwidth quantum states of light. Here we demonstrate a diamond quantum memory that stores, and releases on demand, an arbitrarily polarized $\sim$250 fs duration photonic qubit. The single-mode nature of the memory is overcome by mapping the two degrees of polarization of the qubit, via Raman transitions, onto two spatially distinct optical phonon modes located in the same diamond crystal. The two modes are coherently recombined upon retrieval and quantum process tomography confirms that the memory faithfully reproduces the input state with average fidelity $0.784\pm0.004$ with a total memory efficiency of $(0.76\pm0.03)\%$. In an additional demonstration, one photon of a polarization-entangled pair is stored in the memory. We report that entanglement persists in the retrieved state for up to 1.3 ps of storage time. These results demonstrate that the diamond phonon platform can be used in concert with polarization qubits, a key requirement for polarization-encoded photonic processing.

quant-ph↗

arXiv2016

Quantum memories: emerging applications and recent advances

Quantum light-matter interfaces are at the heart of photonic quantum technologies. Quantum memories for photons, where non-classical states of photons are mapped onto stationary matter states and preserved for subsequent retrieval, are technical realizations enabled by exquisite control over interactions between light and matter. The ability of quantum memories to synchronize probabilistic events makes them a key component in quantum repeaters and quantum computation based on linear optics. This critical feature has motivated many groups to dedicate theoretical and experimental research to develop quantum memory devices. In recent years, exciting new applications, and more advanced developments of quantum memories, have proliferated. In this review, we outline some of the emerging applications of quantum memories in optical signal processing, quantum computation, and nonlinear optics. We review recent experimental and theoretical developments, and their impacts on more advanced photonic quantum technologies based on quantum memories.

quant-ph↗

arXiv2015

Quantum optical signal processing in diamond

Controlling the properties of single photons is essential for a wide array of emerging optical quantum technologies spanning quantum sensing, quantum computing, and quantum communications. Essential components for these technologies include single photon sources, quantum memories, waveguides, and detectors. The ideal spectral operating parameters (wavelength and bandwidth) of these components are rarely similar; thus, frequency conversion and spectral control are key enabling steps for component hybridization. Here we perform signal processing of single photons by coherently manipulating their spectra via a modified quantum memory. We store 723.5 nm photons, with 4.1 nm bandwidth, in a room-temperature diamond crystal; upon retrieval we demonstrate centre frequency tunability over 4.2 times the input bandwidth, and bandwidth modulation between 0.5 to 1.9 times the input bandwidth. Our results demonstrate the potential for diamond, and Raman memories in general, to be an integrated platform for photon storage and spectral conversion.

quant-ph↗