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Berk Zengin

Publications and source records attributed to Berk Zengin.

6 recordsLinked to original sources

Interlayer interactions reshape charge-density wave through electronic elasticity in 4H$_{\mathrm{b}}$-TaS$_2$

Incommensurate charge-density waves (CDWs) in layered quantum materials frequently exhibit widely varying ordering wave vectors, even among nominally identical samples, obscuring their intrinsic electronic properties. Here we identify an inherent origin of this variability through the electronic elasticity of an incommensurate CDW using the model heterostructure 4H$_{\mathrm{b}}$-TaS$_2$, composed of alternating commensurate CDW on 1T and incommensurate CDW on 1H layers. Low-temperature scanning tunneling microscopy, combined with Fourier and quasiparticle-interference analysis, exploits the lattice-pinned 1T CDW as an internal reference to resolve discrete compressive ($-2.3\%$) and tensile ($+3.2\%$) elastic states of the neighboring 1H CDW selected by the interlayer registry of the adjacent layers. Corresponding few-meV shifts of a flat band demonstrate that weak interlayer interactions reshape the low-energy electronic structure through the intrinsic elasticity of the incommensurate CDW. These findings establish electronic elasticity as a mechanism by which subtle interlayer interactions control correlated electronic states in van der Waals heterostructures.

cond-mat.str-el

Reversible nanoscale patterning of WTe$_2$ with a scanning tunneling microscope

Manipulating the lattice structure of ferroelectric quantum materials enables their use in low-power electronic devices, including field-effect transistors. WTe$_2$ is a Weyl-semimetal candidate and ferroelectric, both properties arising from the reduced crystal symmetry of its T$_\mathrm{d}$ ground state. The T$_\mathrm{d}$ crystal phase results from a Peierls distortion of the 1T parent structure and an interlayer shift. While experiments in WTe$_2$ have established ferroelectric switching and transient control of the predicted topological phase via ultrafast excitations, persistent electronic changes on the nanometer scale remain elusive. Here, we demonstrate that current pulses applied via scanning tunneling microscopy can both write and erase persistent nanometer-scale patterns on the surface of WTe$_2$. These patterns consist of apparent picometer in-plane and out-of-plane atomic displacements, accompanied by changes to the local density of states. The out-of-plane displacements further modulate the Peierls-like distortion present in WTe$_2$, while the in-plane displacements are indicative of ferroelectric switching. The induced patterns can be repositioned and erased, suggesting a nanoscale handle on the ferroelectric properties of WTe$_2$.

cond-mat.mtrl-sci

Vacuum cleaving of superconducting niobium tips to optimize noise filtering and with adjustable gap size for scanning tunneling microscopy

Superconducting (SC) tips for scanning tunneling microscopy (STM) can enhance a wide range of surface science studies because they offer exquisite energy resolution, allow the study of Josephson tunneling, or provide spatial contrast based on the local interaction of the SC tip with the sample. The appeal of a SC tip is also practical. An SC gap can be used to characterize and optimize the noise of a low-temperature apparatus. Unlike typical samples, SC tips can be made with less ordered materials, such as from SC polycrystalline wires or by coating a normal metal tip with a superconductor. Those recipes either require additional laboratory infrastructure or are carried out in ambient conditions, leaving an oxidized tip behind. Here, we revisit the vacuum cleaving of an Nb wire to prepare fully gapped tips in an accessible one-step procedure. To show their utility, we measure the SC gap of Nb on Au(111) to determine the base temperature of our microscope and to optimize its RF filtering. The deliberate coating of the Nb tip with Au fully suppresses the SC gap and we show how sputtering with Ar$^{+}$ ions can be used to gradually recover the gap, promising tunability for tailored SC gaps sizes.

cond-mat.supr-con

A versatile platform for graphene nanoribbon synthesis, electronic decoupling, and spin polarized measurements

The on-surface synthesis of nano-graphenes has led the charge in prototyping structures with perspectives beyond silicon-based technology. Following reports of open-shell systems in graphene-nanoribbons (GNR), a flurry of research activities is directed at investigating their magnetic properties with a keen eye for spintronic applications. Although the synthesis of nano-graphenes is usually straightforward on gold, it is difficult to use it for electronic decoupling and spin-polarized measurements. Using a binary alloy Cu3Au(111), we show how to combine the efficient gold-like nano-graphene formation with spin polarization and electronic decoupling known from copper. We prepare copper oxide layers, demonstrate thermally and tip-assisted synthesis of GNR and grow thermally stable magnetic Co islands. We functionalize the tip of a scanning tunneling microscope with carbon-monoxide, nickelocene, or attach Co clusters for high-resolution imaging, magnetic sensing, or spin-polarized measurements. This versatile platform will be a valuable tool in the advanced study of magnetic nano-graphenes.

cond-mat.mes-hall

Adaptive Sparse Sampling for Quasiparticle Interference Imaging

Quasiparticle interference imaging (QPI) offers insight into the band structure of quantum materials from the Fourier transform of local density of states (LDOS) maps. Their acquisition with a scanning tunneling microscope is traditionally tedious due to the large number of required measurements that may take several days to complete. The recent demonstration of sparse sampling for QPI imaging showed how the effective measurement time could be fundamentally reduced by only sampling a small and random subset of the total LDOS. However, the amount of required sub-sampling to faithfully recover the QPI image remained a recurring question. Here we introduce an adaptive sparse sampling (ASS) approach in which we gradually accumulate sparsely sampled LDOS measurements until a desired quality level is achieved via compressive sensing recovery. The iteratively measured random subset of the LDOS can be interleaved with regular topographic images that are used for image registry and drift correction. These reference topographies also allow to resume interrupted measurements to further improve the QPI quality. Our ASS approach is a convenient extension to quasiparticle interference imaging that should remove further hesitation in the implementation of sparse sampling mapping schemes.

cond-mat.other

Fast spectroscopic mapping of two-dimensional quantum materials

Spectroscopic mapping refers to the massive recording of spectra whilst varying an additional degree of freedom, such as: magnetic field, location, temperature, or charge carrier concentration. As this involves two serial tasks, spectroscopic mapping can become excruciatingly slow. We demonstrate exponentially faster mapping through our combination of sparse sampling and parallel spectroscopy. We exemplify our concept using quasiparticle interference imaging of Au(111) and Bi2Sr2CaCu2O8 (Bi2212), as two well-known model systems. Our method is accessible, straightforward to implement with existing scanning tunneling microscopes, and can be easily extended to enhance gate or field-mapping spectroscopy. In view of a possible four orders of magnitude speed advantage, it is setting the stage to fundamentally promote the discovery of novel quantum materials.

cond-mat.mtrl-sci