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Bernard Doudin

Publications and source records attributed to Bernard Doudin.

12 recordsLinked to original sources

Wavelength-Resolved Control of Photovoltaic Screening and Defect-Mediated Doping in Photo-Ferroelectric/Graphene Devices

Ferroelectrics enable large charge doping of two-dimensional overlayers, but the coexistence of switching and nonswitching charge dynamics complicate electro-optical analysis. Here, we investigate the optoelectronic response of a ferroelectric/graphene device under 365 and 530 nm illumination, disentangling effects on ferroelectric dipole alignment from extrinsic current pathways. Graphene acts as a high-gain sensor, amplifying subtle polarization dynamics into a pronounced resistance difference. By resolving switching and nonswitching channels in dark and illuminated conditions, we reveal a competition between photovoltaic charge screening and defect-assisted excitation that governs device electrostatics. Above-band gap illumination generates free carriers that induce leaky ferroelectric hysteresis and suppress the graphene resistance ratio between opposite remanent polarization states from 290% to 15% due to dynamic photovoltaic charge screening. In contrast, 530 nm illumination primarily induces charge redistribution in ferroelectrics via defect-state excitation, leading to a significantly weaker suppression of the resistance variation of graphene. These results establish practical guidelines for selecting photon energy and intensity to either preserve remanent polarization while tuning channel doping or deliberately reconfigure polarization through optical programming.

cond-mat.other

Lubrication-Induced Newtonianization Enables Passive Transport of Non-Newtonian materials

Non Newtonian flows are typically governed by intrinsic bulk rheology, which imposes strong constraints on transport through confined geometries. Here, we show that stable boundary lubrication can fundamentally alter this behavior by localizing shear within a thin, low-viscosity interfacial layer. As a result, the nonlinear rheological response of a broad class of complex materials, including yield-stress, shear-dependent, and thixotropic materials, is strongly suppressed during flow. Using analytical solutions of Stokes flow and numerical simulations, we demonstrate that lubrication-induced shear localization leads to an apparent Newtonianization of transport, in which the macroscopic flow response becomes primarily controlled by the lubricating layer and geometric confinement rather than the intrinsic material properties. In this regime, materials that would otherwise require large pressure gradients can be transported at substantially lower driving forces. Notably, this boundary-dominated transport enables gravity-driven passive flow with orders-of-magnitude enhancement in throughput compared to rigid-wall conduits. These results establish lubrication as a powerful mechanism for tuning and simplifying complex fluid transport, with implications for biological systems, soft and jammed materials, and energy-efficient fluids.

cond-mat.soft

Ultra-soft liquid-ferrofluid interfaces

Soft interfaces are ubiquitous in nature, governing quintessential hydrodynamics functions, like lubrication, stability and cargo transport. It is shown here how a magnetic force field at a magnetic-nonmagnetic fluid interface results in an ultra-soft interface with nonlinear elasticity and tunable viscous shear properties. The balance between magnetic pressure, viscous stress and Laplace pressure results in a deformed and stable liquid-in-liquid tube with apparent elasticity in the range 2 kPa -10 kPa, possibly extended by a proper choice of liquid properties. Such highly deformable liquid-liquid interfaces of arbitrary shape with vanishing viscous shear open doors to unique microfluidic phenomena, biomaterial flows and complex biosystems mimicking.

cond-mat.soft

Scaling and flow profiles in magnetically confined liquid-in-liquid channels

Ferrofluids kept in place by permanent magnet quadrupoles can act as liquid walls to surround a second non-magnetic inside, resulting in a liquid fluidic channel with diameter size ranging from mm down to less than 10 micrometer. Micro particle tracking velocimetry (micro PTV) experiments and modeling show that near ideal plug flow is possible in such liquid-in-liquid channels due to the reduced friction at the walls. The measured fluids velocity profiles agree with the predictions of a hydrodynamic model of cylindrical symmetry with a minimal set of hypotheses. By introducing symmetry breaking elements in the system, we show how unique velocity and flow properties can be obtained. Our liquid-in-liquid confinement opens new possibilities for < 10 micrometer-sized microfluidics with low pressures and low shear, with flow characteristics not attainable in comparable solid-wall devices.

physics.flu-dyn

Reconfigurable Multifunctional van der Waals Ferroelectric Devices and Logic Circuits

In this work, we demonstrate the suitability of Reconfigurable Ferroelectric Field-Effect- Transistors (Re-FeFET) for designing non-volatile reconfigurable logic-in-memory circuits with multifunctional capabilities. Modulation of the energy landscape within a homojunction of a 2D tungsten diselenide (WSe$_2$) layer is achieved by independently controlling two split-gate electrodes made of a ferroelectric 2D copper indium thiophosphate (CuInP$_2$S$_6$) layer. Controlling the state encoded in the Program Gate enables switching between p, n and ambipolar FeFET operating modes. The transistors exhibit on-off ratios exceeding 10$^6$ and hysteresis windows of up to 10 V width. The homojunction can change from ohmic-like to diode behavior, with a large rectification ratio of 10$^4$. When programmed in the diode mode, the large built-in p-n junction electric field enables efficient separation of photogenerated carriers, making the device attractive for energy harvesting applications. The implementation of the Re-FeFET for reconfigurable logic functions shows how a circuit can be reconfigured to emulate either polymorphic ferroelectric NAND/AND logic-in-memory or electronic XNOR logic with long retention time exceeding 10$^4$ seconds. We also illustrate how a circuit design made of just two Re-FeFETs exhibits high logic expressivity with reconfigurability at runtime to implement several key non-volatile 2-input logic functions. Moreover, the Re-FeFET circuit demonstrates remarkable compactness, with an up to 80% reduction in transistor count compared to standard CMOS design. The 2D van de Waals Re-FeFET devices therefore exhibit groundbreaking potential for both More-than-Moore and beyond-Moore future of electronics, in particular for an energy-efficient implementation of in-memory computing and machine learning hardware, due to their multifunctionality and design compactness.

cond-mat.mes-hall

Suppressing Rayleigh-Plateau Instability with a Magnetic Force Field for Deformable Interfaces Engineering

The Rayleigh-Plateau instability (RPI) is a classical hydrodynamics phenomenon that prevents a jet of liquid to flow indefinitely within air or another liquid. Here, we show how adding a magnetic force field makes possible its suppression. Enclosing the jet in a ferrofluid held by magnetic forces allows flow focusing without sheath flow, which completely avoids dripping failure at small flow rates and provides conditional stability for a continuous fluid jet. Highly deformable liquid interfaces withstanding spatial and time varying flow conditions within a large parameter space can be realized.

physics.flu-dyn

Deterministic multi-level spin orbit torque switching using He+ microscopy patterning

He$^+$ ion irradiation is used to pattern multiple areas of Pt/Co/W films with different irradiation doses in Hall bars. The resulting perpendicular magnetic anisotropy landscape enables selective multilevel current-induced switching, with full deterministic control of the position and order of the individual switching elements. Key pattern design parameters are specified, opening a way to scalable multilevel switching devices.

cond-mat.mes-hall

Fluid drag reduction by magnetic confinement

The frictional forces of a viscous liquid flow are a major energy loss issue and severely limit microfluidics practical use. Reducing this drag by more than a few tens of percent remain illusive. Here, we show how cylindrical liquid-in-liquid flow leads to drag reduction of 60-99% for sub mm and mm sized channels, irrespective of whether the viscosity of the transported liquid is larger or smaller than that of the encapsulating one. In contrast to lubrication or sheath flow, we do not require the continuous flow of the encapsulating lubricant, here made up of a ferrofluid held in place by magnetic forces. In a laminar flow model with appropriate boundary conditions, we introduce a modified Reynolds number with a scaling that depends on geometrical factors and viscosity ratio of the two liquids. It explains our whole range of data and reveal the key design parameters for optimizing the drag reduction values. Our results therefore open the route to microfluidics designs with pressure gradients possibly reduced by orders of magnitudes.

physics.app-ph

Helium Ion Microscopy for Reduced Spin Orbit Torque Switching Currents

Spin orbit torque driven switching is a favourable way to manipulate nanoscale magnetic objects for both memory and wireless communication devices. The critical current required to switch from one magnetic state to another depends on the geometry and the intrinsic properties of the materials used, which are difficult to control locally. Here we demonstrate how focused helium ion beam irradiation can modulate the local magnetic anisotropy of a Co thin film at the microscopic scale. Real-time in-situ characterisation using the anomalous Hall effect showed up to an order of magnitude reduction of the magnetic anisotropy under irradiation, and using this, multi-level switching is demonstrated. The result is that spin-switching current densities, down to 800 kA cm$^{-2}$, can be achieved on predetermined areas of the film, without the need for lithography. The ability to vary critical currents spatially has implications not only for storage elements, but also neuromorphic and probabilistic computing.

cond-mat.mes-hall

Conductance oscillations in graphene/nanoclusters hybrid material: towards large area single electron devices

Large assemblies of self-organized aluminum nanoclusters embedded in an oxide layer are formed on graphene templates and used to build tunnel-junction devices. Unexpectedly, single-electron-transport behavior with well-defined Coulomb oscillations is observed for a record junction area containing millions of metal islands. Such hybrid materials offer new prospects for single-electron electronics.

cond-mat.mes-hall

Distance Dependence of the Energy Transfer Rate From a Single Semiconductor Nanostructure to Graphene

The near-field Coulomb interaction between a nano-emitter and a graphene monolayer results in strong Förster-type resonant energy transfer and subsequent fluorescence quenching. Here, we investigate the distance dependence of the energy transfer rate from individual, i) zero-dimensional CdSe/CdS nanocrystals and ii) two-dimensional CdSe/CdS/ZnS nanoplatelets to a graphene monolayer. For increasing distances $d$, the energy transfer rate from individual nanocrystals to graphene decays as $1/d^4$. In contrast, the distance dependence of the energy transfer rate from a two-dimensional nanoplatelet to graphene deviates from a simple power law, but is well described by a theoretical model, which considers a thermal distribution of free excitons in a two-dimensional quantum well. Our results show that accurate distance measurements can be performed at the single particle level using graphene-based molecular rulers and that energy transfer allows probing dimensionality effects at the nanoscale.

cond-mat.mes-hall

Random barrier double-well model for resistive switching in tunnel barriers

The resistive switching phenomenon in MgO-based tunnel junctions is attributed to the effect of charged defects inside the barrier. The presence of electron traps in the MgO barrier, that can be filled and emptied, locally modifies the conductance of the barrier and leads to the resistive switching effects. A double-well model for trapped electrons in MgO is introduced to theoretically describe this phenomenon. Including the statistical distribution of potential barrier heights for these traps leads to a power-law dependence of the resistance as a function of time, under a constant bias voltage. This model also predicts a power-law relation of the hysteresis as a function of the voltage sweep frequency. Experimental transport results strongly support this model and in particular confirm the expected power laws dependencies of resistance. They moreover indicate that the exponent of these power laws varies with temperature as theoretically predicted.

cond-mat.mtrl-sci