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Bernd Aichner

Publications and source records attributed to Bernd Aichner.

13 recordsLinked to original sources

Tailoring the properties of YBa$_{2}$Cu$_{3}$O$_{7-\delta}$ thin films by 30 keV He$^+$ irradiation: An enabling route to superconducting device nanopatterning

Focused helium ion beam (He-FIB) irradiation with 30 keV ions is a key tool for nanoscale patterning and defect engineering in high transition temperature (Tc) cuprate superconducting devices, yet its usable fluence window is constrained by the competing requirements of reliable superconductivity suppression and minimal structural degradation. In this work, we provide a comprehensive dataset on the effects of large-area 30 keV He+ ion exposure on the electric transport and superconducting properties of epitaxial YBa2Cu3O7 (YBCO) thin films. X-ray diffraction shows a fluence-driven loss of crystalline order accompanied by an out-of-plane lattice expansion and an orthorhombic-to-tetragonal transition, culminating at predominant amorphization at the highest fluence of 1 x 10^16 cm^-2. Raman spectra exhibit increasing disorder while lacking signatures of oxygen depletion, indicating that irradiation mainly generates oxygen-related Frenkel defects rather than changing the carrier concentration. Consistently, with increasing fluence, the normal-state resistivity \rho_N(T) at temperature T above Tc increases strongly, while d \rho_N/d T remains nearly unchanged at moderate fluence. The suppression of Tc is accurately described by Abrikosov-Gor'kov pair breaking and reaches complete quenching of superconductivity at 4.5 x 10^15 cm^-2. The anisotropic upper critical fields decrease approximately exponentially with increasing fluence, the vortex activation energy is reduced, and the anisotropy drops, in contrast to oxygen-depleted YBCO. Hall-angle analysis confirms a nearly constant carrier density but a systematic increase in defect scattering and reduced mobility, consistent with a crossover toward the dirty limit at high fluence. These results establish quantitative fluence thresholds and a practical operational window for He-FIB nanopatterning of YBCO quantum circuits.

cond-mat.supr-con

Effect of pulse duration on current-induced selective oxygen migration in high-Tc superconductors

High current densities can induce the directional diffusion of atoms in metallic films. In YBa$_2$Cu$_3$O$_{7-\delta}$ (YBCO), this electromigration process selectively acts on oxygen atoms lying in the Cu-O chains, permitting to vary the oxygen concentration in a targeted spot of high current density. This approach has proven successful in mapping the phase diagram of the material as a function of carrier concentration or as a way to manufacture memristive devices owing to its reversibility under small bipolar excitations. Thus far, most of the investigations have been limited to pulsed excitation with current/voltage pulses on a millisecond or longer scale, for which thermal effects undeniably influence the process. In the present work, we explore the impact of pulse length $\delta t$ on the onset current of electromigration, $I_{\text{EM}}$, of YBCO bridges, covering the range from 200 ns to 1 ms. As $\delta t$ decreases below $\sim 10~\mu$s, $I_{\text{EM}}$ exhibits a rapid increase. Analytical and numerical estimates of the local temperature show that as pulses shorten, the temperature decreases, making the electromigration process more athermal. These findings are relevant for the operation of memristors and should be taken into account when describing the effects of thermomagnetic instabilities in thin films.

cond-mat.supr-con

YSGAG: The Ideal Substrate for YIG in Quantum Magnonics

Quantum magnonics leverages the quantum properties of magnons to advance nanoscale quantum information technologies. Ferrimagnetic yttrium iron garnet (YIG), known for exceptionally long magnon lifetimes, is a cornerstone material typically grown as thin films on gadolinium gallium garnet (GGG) for lattice matching. However, paramagnetic GGG introduces detrimental damping at low temperatures due to substrate magnetization, undermining quantum applications. Here, we study magnetic damping in a 150$\,$nm-thick YIG film on a yttrium scandium gallium aluminum garnet (YSGAG) substrate, a newly developed diamagnetic alternative to GGG. Using ferromagnetic resonance spectroscopy down to 30$\,$mK, we compare YIG/YSGAG with a conventional YIG/GGG reference system. We demonstrate that the YIG/YSGAG system maintains low damping from 300$\,$K to 30$\,$mK, with $\alpha = 4.29\times10^{-5}$ at room temperature, comparable to the best YIG/GGG films and bulk YIG, with no low-temperature upturn. The diamagnetic substrate eliminates the dissipation mechanisms that dominate on magnetized GGG, preserving low magnetic damping across the full temperature range. Consequently, YSGAG serves as an ideal substrate for YIG films in quantum magnonics and is paving the way for the development of spin-wave-based quantum technologies.

cond-mat.mes-hall

SOT Enabled 3D Magnetic Field Sensor with Low Offset and High Sensitivity

In this work we demonstrate a spin-orbit torque (SOT) magnetic field sensor, designed as a Ta/CoFeB/MgO structure, with high sensitivity and capable of active offset compensation in all three spatial directions. This is described and verified in both experiment and simulation. The measurements of magnetic fields showed an offset of 36, 50, and 37$\mathrm{\mu T}$ for x-, y-, and z-fields. Furthermore, the sensitivities of these measurements had values of 590, 580, and 490$\mathrm{V\,A^{-1}\,T^{-1}}$ in the x-, y-, and z-direction. In addition, the robustness to bias fields is demonstrated via experiments and single spin simulations by applying bias fields in y-direction. Cross sensitivities were further analyzed via single spin simulations performing a parameter sweep of different bias fields in the y- and z-direction up to $\pm$1mT. Finally, the extraction of the SOT parameters $\eta_\mathrm{DL}$ and $\eta_\mathrm{FL}$ is shown via optimization of a single-spin curve to the experimental measurements.

cond-mat.mes-hall

Enhanced superconducting properties of Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$ films with sub-50-nm thickness

Few-unit cell thick Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$ (Bi-2212) layers have recently attracted much interest due to their extreme anisotropy and two-dimensional superconductivity, although they are typically susceptible to ambient conditions. In this study, we report on thin films approximately 13 unit cells thick that are stable in air, exhibit high anisotropy, and demonstrate extraordinarily high critical currents. By examining the superconducting transition under magnetic fields applied in both out-of-plane and in-plane orientations, we estimate key parameters such as pinning potentials, coherence lengths, London penetration depth, anisotropy factor, and the Ginzburg-Landau parameter. The volume pinning force is better described by a model incorporating an exponential decay term attributed to pronounced thermally-assisted flux flow. The Hall effect in the Bi-2212 films exhibits an extensive anomaly with a double sign change that may challenge existing theoretical explanations for this poorly understood phenomenon in copper-oxide superconductors.

cond-mat.supr-con

Temporal Evolution of Defects and Related Electric Properties in He-Irradiated YBa$_{2}$Cu$_{3}$O$_{7-\delta}$ Thin Films

Thin films of the superconductor YBa$_2$Cu$_3$O$_{7-\delta}$ (YBCO) were modified by low-energy light-ion irradiation employing collimated or focused He$^+$ beams, and the long-term stability of irradiation-induced defects was investigated. For films irradiated with collimated beams, the resistance was measured in situ during and after irradiation and analyzed using a phenomenological model. The formation and stability of irradiation-induced defects are highly influenced by temperature. Thermal annealing experiments conducted in an Ar atmosphere at various temperatures demonstrated a decrease in resistivity and allowed us to determine diffusion coefficients and the activation energy $\Delta E = (0.31 \pm 0.03)$ eV for diffusive oxygen rearrangement within the YBCO unit cell basal plane. Additionally, thin YBCO films, nanostructured by focused He$^+$-beam irradiation into vortex pinning arrays, displayed significant commensurability effects in magnetic fields. Despite the strong modulation of defect densities in these pinning arrays, oxygen diffusion during room-temperature annealing over almost six years did not compromise the signatures of vortex matching, which remained precisely at their magnetic fields predicted by the pattern geometry. Moreover, the critical current increased substantially within the entire magnetic field range after long-term storage in dry air. These findings underscore the potential of ion irradiation in tailoring the superconducting properties of thin YBCO films.

cond-mat.supr-con

Vortex matching at 6 T in YBa$_2$Cu$_3$O$_{7-\delta}$ thin films by imprinting a 20 nm-periodic pinning array with a focused helium ion beam

Controlled engineering of vortex pinning sites in copper-oxide superconductors is a critical issue in manufacturing devices based on magnetic flux quanta. To address this, we employed a focused He-ion beam (He-FIB) to irradiate thin YBa$_2$Cu$_3$O$_{7-\delta}$ films and create ultradense hexagonal arrays of defects with lattice spacings as small as 20 nm. Critical current and magnetoresistance measurements demonstrate efficient pinning by an unprecedentedly high matching field of 6 T visible in a huge temperature range from the critical temperature $T_c$ down to 2 K. These results show that He-FIB irradiation provides excellent opportunities for the development and application of superconducting fluxonic devices based on Abrikosov vortices. In particular, our findings suggest that such devices can operate at temperatures far below $T_c$, where superconductivity is robust.

cond-mat.supr-con

Skyrmionic device for three dimensional magnetic field sensing enabled by spin-orbit torques

Magnetic skyrmions are topologically protected local magnetic solitons that are promising for storage, logic or general computing applications. In this work, we demonstrate that we can use a skyrmion device based on [W/CoFeB/MgO] 1 0 multilayers for three-dimensional magnetic field sensing enabled by spin-orbit torques (SOT). We stabilize isolated chiral skyrmions and stripe domains in the multilayers, as shown by magnetic force microscopy images and micromagnetic simulations. We perform magnetic transport measurements to show that we can sense both in-plane and out-of-plane magnetic fields by means of a differential measurement scheme in which the symmetry of the SOT leads to cancelation of the DC offset. With the magnetic parameters obtained by vibrating sample magnetometry and ferromagnetic resonance measurements, we perform finite-temperature micromagnetic simulations, where we investigate the fundamental origin of the sensing signal. We identify the topological transformation between skyrmions, stripes and type-II bubbles that leads to a change in the resistance that is read-out by the anomalous Hall effect. Our study presents a novel application for skyrmions, where a differential measurement sensing concept is applied to quantify external magnetic fields paving the way towards more energy efficient applications in skyrmionics based spintronics.

cond-mat.mes-hall

Phase purity and surface morphology of high-Jc superconducting Bi2Sr2Ca1Cu2O8+δ thin films

Bi2Sr2Ca1Cu2O8+d (Bi-2212) thin films with thicknesses less than 50 nm (<20 unit cells) are grown by pulsed laser deposition (PLD) onto (001) LaAlO3 (LAO) single crystal substrates. Phase-pure and smooth c-axis oriented Bi-2212 films with optimal oxygen doping, critical temperature Tc0 up to 86 K, and critical current density Jc(60 K) above 1 MA/cm2 are obtained for samples that are annealed in situ at temperatures below 700 °C. At higher temperature Bi-2212 films on LAO substrates partially decompose to non-superconducting impurity phases, while films on MgO and SrTiO3 substrates are stable. The broadening of Tc of the metal-to-superconductor resistive phase transition in magnetic fields is much larger for thin films of Bi-2212 as compared to YBa2Cu3O7. The magnetic field-induced suppression of Tc0 is stronger for Bi-2212 films containing impurity phases as compared to the phase-pure Bi-2212 films. The degradation of LAO substrate crystals after several steps of deposition and chemical removal of the Bi-2212 layer is investigated. New, commercially prepared substrates provide Bi-2212 films with smallest surface roughness (3 nm) and strong out-of-plane texture. However, thin films of almost the same quality are obtained on re-used LAO substrates that are mechanically polished after the chemical etching.

cond-mat.supr-con

Angle-dependent Magnetoresistance of an Ordered Bose Glass of Vortices in YBa$_{2}$Cu$_{3}$O$_{7-δ}$ Thin Films with a Periodic Pinning~Lattice

The competition between intrinsic disorder in superconducting YBa$_{2}$Cu$_{3}$O$_{7-δ}$ (YBCO) thin films and an ultradense triangular lattice of cylindrical pinning centers spaced at 30 nm intervals results in an ordered Bose glass phase of vortices. The samples were created by scanning the focused beam of a helium-ion microscope over the surface of the YBCO thin film to form columns of point defects where superconductivity was locally suppressed. The voltage-current isotherms reveal critical behavior and scale in the vicinity of the second-order glass transition. The latter exhibits a distinct peak in melting temperature ($T_g$) vs. applied magnetic field ($B_a$) at the magnetic commensurability field, along with a sharp rise in the lifetimes of glassy fluctuations. Angle-dependent magnetoresistance measurements in constant-Lorentz-force geometry unveil a strong increase in anisotropy compared to a pristine reference film where the density of vortices matches that of the columnar defects. The pinning is therefore, dominated by the magnetic-field component parallel to the columnar defects, exposing its one-dimensional character. These results support the idea of an ordered Bose glass phase.

cond-mat.supr-con

Ordered Bose Glass of Vortices in Superconducting YBa$_{2}$Cu$_{3}$O$_{7-δ}$ Thin Films with a Periodic Pin Lattice Created by Focused Helium Ion Irradiation

The defect-rich morphology of YBa$_{2}$Cu$_{3}$O$_{7-δ}$ (YBCO) thin films leads to a glass-like arrangement of Abrikosov vortices which causes the resistance to disappear in vanishing current densities. This vortex glass consists of entangled vortex lines and is identified by a characteristic scaling of the voltage-current isotherms. Randomly distributed columnar defects stratify the vortex lines and lead to a Bose glass. Here, we report on the observation of an ordered Bose glass in a YBCO thin film with a hexagonal array of columnar defects with 30 nm spacings. The periodic pinning landscape was engineered by a focused beam of 30 keV He$^+$ ions in a helium-ion microscope.

cond-mat.supr-con

Angular magnetic-field dependence of vortex matching in pinning lattices fabricated by focused or masked helium ion beam irradiation of superconducting YBa$_2$Cu$_3$O$_{7-δ}$ thin films

The angular dependence of magnetic-field commensurability effects in thin films of the cuprate high-critical-temperature superconductor YBa$_{2}$Cu$_{3}$O$_{7-δ}$ (YBCO) with an artificial pinning landscape is investigated. Columns of point defects are fabricated by two different methods of ion irradiation -- scanning the focused 30 keV ion beam in a helium ion microscope or employing the wide-field 75 keV He$^+$ beam of an ion implanter through a stencil mask. Simulations of the ion-target interactions and the resulting collision cascades reveal that with both methods square arrays of defect columns with sub-$μ$m spacings can be created. They consist of dense point-defect clusters, which act as pinning centers for Abrikosov vortices. This is verified by the measurement of commensurable peaks of the critical current and related minima of the flux-flow resistance vs magnetic field at the matching fields. In oblique magnetic fields the matching features are exclusively governed by the component of the magnetic field parallel to the axes of the columnar defects, which confirms that the magnetic flux is penetrated along the defect columns. We demonstrate that the latter dominate the pinning landscape despite of the strong intrinsic pinning in thin YBCO films.

cond-mat.supr-con

Ultradense Tailored Vortex Pinning Arrays in Superconducting YBa$_2$Cu$_3$O$_{7-δ}$ Thin Films Created by Focused He Ion Beam Irradiation for Fluxonics Applications

Magnetic fields penetrate a type-II superconductor as magnetic flux quanta, called vortices. In a clean superconductor they arrange in a hexagonal lattice, while by adding periodic artificial pinning centers many other arrangements can be realized. Using the focused beam of a helium ion microscope we have fabricated periodic patterns of dense pinning centers with spacings as small as 70 nm in thin films of the cuprate superconductor YBa$_{2}$Cu$_{3}$O$_{7-δ}$. In these ultradense kagomé-like patterns, the voids lead to magnetic caging of vortices, resulting in unconventional commensurability effects that manifest themselves as peaks in the critical current and minima in the resistance versus applied magnetic field up to $\sim 0.4\,$T. The various vortex patterns at different magnetic fields are analyzed by molecular dynamics simulations of vortex motion, and the magnetic field dependence of the critical current is confirmed. These findings open the way for a controlled manipulation of vortices in cuprate superconductors by artificial sub-100 nm pinning landscapes.

cond-mat.supr-con