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Bertrand Lefloch

Publications and source records attributed to Bertrand Lefloch.

51 records · Page 3Linked to original sources

Abundance of HOCO+ and CO2 in the outer layers of the L1544 prestellar core

The L1544 prestellar core has been observed as part of the ASAI IRAM Large Program at 3 mm. These observations led to the detection of many complex molecules. In this Letter, we report the detection of two lines, at 85.5 GHz (4,0,4-3,0,3) and 106.9 GHz (5,0,5-4,0,4), respectively, of the protonated carbon dioxide ion, HOCO+. We also report the tentative detection of the line at 100.4 GHz (5,0,5-4,0,4) of DOCO+. The non-LTE analysis of the detected lines shows that the HOCO+ emission originates in the external layer where non-thermal desorption of other species has previously been observed. Its abundance is (5 +/- 2) e-11. Modelling of the chemistry involved in the formation and destruction of HOCO+ provides a gaseous CO2 abundance of 2e-7 (with respect to H2) with an upper limit of 2e-6.

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Infalling-Rotating Motion and Associated Chemical Change in the Envelope of IRAS 16293-2422 Source A Studied with ALMA

We have analyzed rotational spectral line emission of OCS, CH3OH, HCOOCH3, and H2CS observed toward the low-mass Class 0 protostellar source IRAS 16293-2422 Source A at a sub-arcsecond resolution (~0".6 x 0".5) with ALMA. Significant chemical differentiation is found at a 50 AU scale. The OCS line is found to well trace the infalling-rotating envelope in this source. On the other hand, the CH3OH and HCOOCH3 distributions are found to be concentrated around the inner part of the infalling-rotating envelope. With a simple ballistic model of the infalling-rotating envelope, the radius of the centrifugal barrier (a half of the centrifugal radius) and the protostellar mass are evaluated from the OCS data to be from 40 to 60 AU and from 0.5 to 1.0 Msun, respectively, assuming the inclination angle of the envelope/disk structure to be 60 degrees (90 degrees for the edge-on configuration). Although the protostellar mass is correlated with the inclination angle, the radius of the centrifugal barrier is not. This is the first indication of the centrifugal barrier of the infalling-rotating envelope in a hot corino source. CH3OH and HCOOCH3 may be liberated from ice mantles due to weak accretion shocks around the centrifugal barrier, and/or due to protostellar heating. The H2CS emission seems to come from the disk component inside the centrifugal barrier in addition to the envelope component. The centrifugal barrier plays a central role not only in the formation of a rotationally-supported disk but also in the chemical evolution from the envelope to the protoplanetary disk.

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Geometric and Kinematic Structure of the Outflow/Envelope System of L1527 Revealed by Subarcsecond-resolution Observation of CS

Subarcsecond-resolution images of the rotational line emissions of CS and c-C$_3$H$_2$ obtained toward the low-mass protostar IRAS 04368$+$2557 in L1527 with the Atacama Large Millimeter/submillimeter Array are investigated to constrain the orientation of the outflow/envelope system. The distribution of CS consists of an envelope component extending from north to south and a faint butterfly-shaped outflow component. The kinematic structure of the envelope is well reproduced by a simple ballistic model of an infalling rotating envelope. Although the envelope has a nearly edge-on configuration, the inclination angle of the rotation axis from the plane of the sky is found to be 5$^\circ$, where we find that the western side of the envelope faces the observer. This configuration is opposite to the direction of the large-scale ($\sim$ 10$^4$ AU) outflow suggested previously from the $^{12}$CO ($J$=3$-$2) observation, and to the morphology of infrared reflection near the protostar ($\sim$ 200 AU). The latter discrepancy could originate from high extinction by the outflow cavity of the western side, these discrepancies or may indicate that the outflow axis is not parallel to the rotation axis of the envelope. Position-velocity diagrams show the accelerated outflow cavity wall, and its kinematic structure in the 2000 AU scale is explained by a standard parabolic model with the inclination angle derived from the analysis of the envelope. The different orientation of the outflow between the small and large scale implies a possibility of precession of the outflow axis. The shape and the velocity of the outflow in the vicinity of the protostar are compared with those of other protostars.

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Subarcsecond Analysis of Infalling-Rotating Envelope around the Class I Protostar IRAS 04365+2535

Sub-arcsecond images of the rotational line emission of CS and SO have been obtained toward the Class I protostar IRAS 04365$+$2535 in TMC-1A with ALMA. A compact component around the protostar is clearly detected in the CS and SO emission. The velocity structure of the compact component of CS reveals infalling-rotating motion conserving the angular momentum. It is well explained by a ballistic model of an infalling-rotating envelope with the radius of the centrifugal barrier (a half of the centrifugal radius) of 50 AU, although the distribution of the infalling gas is asymmetric around the protostar. The distribution of SO is mostly concentrated around the radius of the centrifugal barrier of the simple model. Thus a drastic change in chemical composition of the gas infalling onto the protostar is found to occur at a 50 AU scale probably due to accretion shocks, demonstrating that the infalling material is significantly processed before being delivered into the disk.

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Abundance Anomaly of the $^{13}$C Isotopic Species of c-C$_3$H$_2$ in the Low-Mass Star Formation Region L1527

The rotational spectral lines of c-C$_3$H$_2$ and two kinds of the $^{13}$C isotopic species, c-$^{13}$CCCH$_2$ ($C_{2v}$ symmetry) and c-CC$^{13}$CH$_2$ ($C_s$ symmetry) have been observed in the 1-3 mm band toward the low-mass star-forming region L1527. We have detected 7, 3, and 6 lines of c-C$_3$H$_2$, c-$^{13}$CCCH$_2$ , and c-CC$^{13}$CH$_2$, respectively, with the Nobeyama 45 m telescope, and 34, 6, and 13 lines, respectively, with the IRAM 30 m telescope, where 7, 2, and 2 transitions, respectively, are observed with the both telescopes. With these data, we have evaluated the column densities of the normal and $^{13}$C isotopic species. The [c-C$_3$H$_2$]/[c-$^{13}$CCCH$_2$] ratio is determined to be $310\pm80$, while the [c-C$_3$H$_2$]/[c-CC$^{13}$CH$_2$] ratio is determined to be $61\pm11$. The [c-C$_3$H$_2$]/[c-$^{13}$CCCH$_2$] and [c-C$_3$H$_2$]/[c-CC$^{13}$CH$_2$] ratios expected from the elemental $^{12}$C/$^{13}$C ratio are 60-70 and 30-35, respectively, where the latter takes into account the statistical factor of 2 for the two equivalent carbon atoms in c-C$_3$H$_2$. Hence, this observation further confirms the dilution of the $^{13}$C species in carbon-chain molecules and their related molecules, which are thought to originate from the dilution of $^{13}$C$^+$ in the gas-phase C$^+$ due to the isotope exchange reaction: $\mathrm{^{13}C^++CO\rightarrow{}^{13}CO+C^+}$. Moreover, the abundances of the two $^{13}$C isotopic species are different from each other. The ratio of c-$\mathrm{^{13}CCCH_2}$ species relative to c-$\mathrm{CC^{13}CH_2}$ is determined to be $0.20\pm0.05$. If $^{13}$C were randomly substituted for the three carbon atoms, the [c-$\mathrm{^{13}CCCH_2}$]/[c-$\mathrm{CC^{13}CH_2}$] ratio would be 0.5. Hence, the observed ratio indicates that c-$\mathrm{CC^{13}CH_2}$ exists more favorably. Possible origins of the different abundances are discussed.

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The origin of complex organic molecules in prestellar cores

Complex organic molecules (COMs) have been detected in a variety of environments, including cold prestellar cores. Given the low temperature of these objects, these last detections challenge existing models. We report here new observations towards the prestellar core L1544. They are based on an unbiased spectral survey of the 3mm band at the IRAM-30m telescope, as part of the Large Program ASAI. The observations allow us to provide the full census of the oxygen bearing COMs in this source. We detected tricarbon monoxide, methanol, acetaldehyde, formic acid, ketene, and propyne with abundances varying from 5e-11 to 6e-9. The non-LTE analysis of the methanol lines shows that they are likely emitted at the border of the core, at a radius of ~8000 AU where T~10 K and nH2~2e4 cm-3. Previous works have shown that water vapour is enhanced in the same region because of the photodesorption of water ices. We propose that a non-thermal desorption mechanism is also responsible for the observed emission of methanol and COMs from the same layer. The desorbed oxygen and a tiny amount of desorbed methanol and ethene are enough to reproduce the abundances of tricarbon monoxide, methanol, acetaldehyde and ketene measured in L1544. These new findings open the possibility that COMs in prestellar cores originate in a similar outer layer rather than in the dense inner cores, as previously assumed, and that their formation is driven by the non-thermally desorbed species.

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The CHESS survey of the L1157-B1 shock: the dissociative jet shock as revealed by Herschel--PACS

Outflows generated by protostars heavily affect the kinematics and chemistry of the hosting molecular cloud through strong shocks that enhance the abundance of some molecules. L1157 is the prototype of chemically active outflows, and a strong shock, called B1, is taking place in its blue lobe between the precessing jet and the hosting cloud. We present the Herschel-PACS 55--210 micron spectra of the L1157-B1 shock, showing emission lines from CO, H2O, OH, and [OI]. The spatial resolution of the PACS spectrometer allows us to map the warm gas traced by far-infrared (FIR) lines with unprecedented detail. The rotational diagram of the high-Jup CO lines indicates high-excitation conditions (Tex ~ 210 +/- 10 K). We used a radiative transfer code to model the hot CO gas emission observed with PACS and in the CO (13-12) and (10-9) lines measured by Herschel-HIFI. We derive 200 10^5 cm-3. The CO emission comes from a region of about 7 arcsec located at the rear of the bow shock where the [OI] and OH emission also originate. Comparison with shock models shows that the bright [OI] and OH emissions trace a dissociative J-type shock, which is also supported by a previous detection of [FeII] at the same position. The inferred mass-flux is consistent with the "reverse" shock where the jet is impacting on the L1157-B1 bow shock. The same shock may contribute significantly to the high-Jup CO emission.

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Hot corinos in NGC1333-IRAS4B and IRAS2A

(Abridged) We aim to enlarge the number of known hot corinos and carry out a first comparative study with hot cores. The ultimate goal is to understand whether complex organic molecules form in the gas phase or on grain surfaces, and what the possible key parameters are. We observed millimeter rotational transitions of HCOOH, HCOOCH3, CH3OCH3, CH3CN, and C2H5CN in a sample of low-mass protostars with the IRAM-30m. Using the rotational diagram method coupled with the information about the sources' structure, we calculate the abundances of the observed molecules. To interpret these abundances, we review the proposed formation processes of the above molecules. We report the detection of HCOOCH3 and/or CH3CN towards NGC1333-IRAS4B and NGC1333-IRAS2A. We find that abundance ratios of O-bearing molecules to methanol or formaldehyde in hot corinos are comparable and about unity, and are relatively (depending on how the ratios are determined) higher than those in hot cores and in Galactic center clouds. So far, complex organic molecules were detected in all the hot corinos where they were searched for, suggesting that it is a common phase for low-mass protostars. While some evidence points to grain-surface synthesis (either in the cold or warm-up phase) of these molecules (in particular for HCOOH and HCOOCH3), the present data do not allow us to disregard gas-phase formation. More observational, laboratory, and theoretical studies are required to improve our understanding of hot corinos.

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Sulphur chemistry and molecular shocks: the case of NGC1333-IRAS2

We present SO and SO2 observations in the region of the low mass protostar IRAS2/NGC1333. The East-West outflow originating from this source has been mapped in four transitions of both SO and SO2. In addition, CS observations published in the literature have been used. We compute the SO, SO2 and CS column densities and the physical conditions at several positions of the outflow using LTE and a non-LTE LVG approximations. The SO2/SO and CS/SO abundance ratios are compared with the theoretical predictions of a chemical model adapted to the physical conditions in the IRAS2 outflow. The SO2/SO abundance ratios are constant in the two lobes of the outflow whereas CS/SO is up to 6 times lower in the shocked gas of the East lobe than in the West one. The comparison with the chemical model allows us to constrain the age of the outflow produced by IRAS2 to >5e3yr. We find low densities and temperatures for the outflow of IRAS2 (< 1e6 cm-3 and >70 K) from SO and SO2 emission probably because the two molecules trace the cooled entrained material. The East lobe of the outflow shows denser gas compared to the West lobe. We also discuss some constraints on the depleted form of sulphur.

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Near-arcsecond resolution observations of the hot corino of the solar type protostar IRAS 16293-2422

Complex organic molecules have previously been discovered in solar type protostars, raising the questions of where and how they form in the envelope. Possible formation mechanisms include grain mantle evaporation, interaction of the outflow with its surroundings or the impact of UV/X-rays inside the cavities. In this Letter we present the first interferometric observations of two complex molecules, CH3CN and HCOOCH3, towards the solar type protostar IRAS16293-2422. The images show that the emission originates from two compact regions centered on the two components of the binary system. We discuss how these results favor the grain mantle evaporation scenario and we investigate the implications of these observations for the chemical composition and physical and dynamical state of the two components.

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Complex molecules in the hot core of the low mass protostar NGC1333-IRAS4A

We report the detection of complex molecules (HCOOCH_3, HCOOH and CH_3CN), signposts of a "hot core" like region, toward the low mass, Class 0 source NGC1333-IRAS4A. This is the second low mass protostar where such complex molecules have been searched for and reported, the other source being IRAS16293-2422. It is therefore likely that compact (few tens of AUs) regions of dense and warm gas, where the chemistry is dominated by the evaporation of grain mantles, and where complex molecules are found, are common in low mass Class 0 sources.Given that the chemical formation timescale is much shorter than the gas hot core crossing time, it is not clear whether the reported complex molecules are formed on the grain surfaces (first generation molecules) or in the warm gas by reactions involving the evaporated mantle constituents (second generation molecules). We do not find evidence for large differences in the molecular abundances, normalized to the formaldehyde abundance, between the two solar type protostars, suggesting perhaps a common origin.

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The H2CO abundance in the inner warm regions of low mass protostellar envelopes

We present a survey of the formaldehyde emission in a sample of eight Class 0 protostars obtained with the IRAM and JCMT telescopes. The data have been analyzed with three different methods with increasing level of sophistication. We first analyze the observed emission in the LTE approximation, and derive rotational temperatures between 11 and 40 K, and column densities between 1 and 20 x 10^13 cm^-2. Second, we use a LVG code and derive larger kinetic temperatures, between 30 and 90 K, consistent with subthermally populated levels and densities from 1 to 6 x 10^5 cm^-3. The column densities from the LVG modeling are within a factor of 10 with respect to those derived in the LTE approximation. Finally, we analyze the observations based upon detailed models for the envelopes surrounding the protostars, using temperature and density profiles previously derived from continuum observations. We approximate the formaldehyde abundance across the envelope with a jump function, the jump occurring when the dust temperature reaches 100 K, the evaporation temperature of the grain mantles. The observed formaldehyde emission is well reproduced only if there is a jump, more than two orders of magnitude, in four sources. In the remaining four sources the data are consistent with a formaldehyde abundance jump, but the evidence is more marginal (~2 sigma). The inferred inner H2CO abundance varies between 1 x 10^-8 and 6 x 10^-6. We discuss the implications of these jumps for our understanding of the origin and evolution of ices in low mass star forming regions. Finally, we give predictions for the submillimeter H2CO lines, which are particularly sensitive to the abundance jumps.

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CO Depletion and Deuterium Fractionation in Prestellar Cores

We report the detection of D2CO in a sample of starless dense cores, in which we previously measured the degree of CO depletion. The deuterium fractionation is found extremely high, [D2CO]/[H2CO] ~ 1-10 %, similar to that reported in low-mass protostars. This provides convincing evidence that D2CO is formed in the cold pre-stellar cores, and later desorbed when the gas warms up in protostars. We find that the cores with the highest CO depletions have also the largest [D2CO]/[H2CO] ratios, supporting the theoretical prediction that deuteration increases with increasing CO depletion.

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The Degree of CO Depletion in Pre-stellar Cores

We present new results on CO depletion in a sample of nearby pre-stellar cores, based on observations of the millimeter C17O and C18O lines and the 1.3 mm dust emission with the IRAM 30m telescope. In most cases, the distribution of CO is much flatter than that of the dust, whereas other tracers, like N2H+, still probe the latter. In the centre of these objects, we estimate CO to be underabundant by a factor 4-15 depending on the cores. The CO underabundance is more pronounced in the central regions and appears to decrease with increasing distance from the core centre. This underabundance is most likely due to the freezing out of CO onto the dust grains in the cold, dense parts of the cores. We find evidence for an increase of the CO depletion degree with the core density.

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Extended Far-Infrared CO Emission in the Orion OMC-1 Core

We report on sensitive far-infrared observations of $^{12}$CO pure rotational transitions in the OMC-1 core of Orion. The lines were observed with the Long Wavelength Spectrometer (LWS) in the grating mode on board the Infrared Space Observatory (ISO), covering the 43-197 $μ$m wavelength range. The transitions from $J_{up}=14$ up to $J_{up}=19$ have been identified across the whole OMC-1 core and lines up to $J_{up}= 43$ have been detected towards the central region, KL/IRc2. In addition, we have taken high-quality spectra in the Fabry-Perot mode of some of the CO lines. In KL/IRc2 the lines are satisfactorily accounted for by a three-temperature model describing the plateau and ridge emission. The fluxes detected in the high-$J$ transitions ($J_{up} > 34$) reveal the presence of a very hot and dense gas component ($T=1500-2500$ K; $\rm N(CO)$=2\times 10^{17}\cmmd$), probably originating from some of the embedded sources previously observed in the $\rm H_2$ near-infrared lines. At all other positions in the OMC-1 core, we estimate kinetic temperatures $\geq 80$ K and as high as 150 K at some positions around IRc2, from a simple Large-Velocity Gradient model.

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