arXiv subjects

Bettina Frank

Publications and source records attributed to Bettina Frank.

10 recordsLinked to original sources

arXiv2026

Analysis of the Topology of a Plasmonic Target-Skyrmion Texture

Topological concepts are frequently used to describe structured optical fields, including plasmonic near fields. Topological descriptions in terms of skyrmion numbers implicitly assume the compactness of the underlying manifold. Even when skyrmion-like textures appear locally, the compactness is usually not fulfilled in extended optical fields. Here, we use photoemission electron microscopy to investigate a plasmonic nano-focus that exhibits a sequence of radially extending alternating skyrmion and antiskyrmion textures. The full spatio-temporal reconstruction of the electric field vectors and their topology is accessible by vector polarimetry. The experiments confirm the expected oscillatory behavior of the skyrmion number and demonstrate that a global skyrmion number cannot be assigned in such non-compact fields.

physics.optics↗

arXiv2026

Intrinsic plasmon canalization in the biaxial van der Waals crystal MoOCl$_2$

Anisotropic polaritons in low-symmetry crystals allow for subwavelength confinement and directional routing of light. The most extreme form of such anisotropy arises at the topological transition between elliptical and hyperbolic dispersion, where the isofrequency contours collapse into parallel lines and polaritons propagate in a diffractionless, beam-like fashion. This canalization regime has previously been accessed through twisted heterostructures or engineered metasurfaces. Here we show that natural canalization can be achieved without any fabrication or structuring by exploiting the intrinsic elliptical-to-hyperbolic transition in the van der Waals crystal MoOCl$_2$ at room temperature. Using near-field imaging, we directly visualize plasmon-polariton canalization emerging at the low-loss Drude crossing point along the [010] crystal axis. Owing to the moderate slope of the Drude permittivity, the resulting polaritons remain highly directional across a broad spectral window. This weak dispersion also enables robust thickness-dependent tuning, and we demonstrate, both experimentally and theoretically, that the canalization wavelength can be adjusted by more than 1 μm simply by varying the flake thickness. This work brings canalized polariton propagation into the 4.5 - 6 μm range, beyond the frequency limits of phonon-polariton platforms and overlapping with important molecular vibrations, opening new opportunities for mid-IR nanophotonics and sensing.

physics.optics↗

arXiv2026

Phonon-polaritonic skyrmions: Transition from bubble- to Néel-type

Optical skyrmions are members of the emerging topological branch of solid-state physics and photonics, allowing for control over topological light textures through light-matter interactions. However, in nanophotonics their practical application has been severely limited by high inherent losses in plasmonic materials, resulting in the lack of tunability between different topological properties. Here, we utilize the strong dispersion of silicon carbide thin films to realize highly confined surface phonon-polariton skyrmion lattices, which we image via near-field microscopy. We experimentally demonstrate topological tuning between bubble- and Néel-type skyrmions, a unique advantage that polar dielectrics offer over most existing approaches. Changing the excitation wavelength by only 10% switches the skyrmion type, revealed by examination of the skyrmion number density contrast. Analysis of domain wall size and steepness in analogy to magnetic materials also confirms this transition. Our results are a starting point to investigate other topological features in phononic systems such as merons, skyrmion bags, and other complex structured light fields. Furthermore, strong light-matter hybridization and nonlinear effects owing to anharmonicity of the phonons may be observed in the future, possibly leading towards the discovery of polaritonic skyrmion-skyrmion interactions and hence applications in topology-based information processing.

physics.optics↗

arXiv2024

Spatio-temporal topology of plasmonic spin meron pairs revealed by polarimetric photo-emission microscopy

Topology is the study of geometrical properties and spatial relations unaffected by continuous changes, and has become an important tool for understanding complex physical systems. Although recent optical experiments have inferred the existence of vector fields with the topologies of merons, the inability to extract the full three dimensional vectors misses a richer set of topologies that have not yet been fully explored. In our work, we extend the study of the topology of electromagnetic fields on surfaces to a spin quasi-particle with the topology of a meron pair, formed by interfering surface plasmon polaritons, and show that the in-plane vectors are constrained by the embedding topology of the space as dictated by the Poincare-Hopf theorem. In addition we explore the time evolution of the three dimensional topology of the spin field formed by femtosecond laser pulses. These experiments are possible using our here developed method called polarimetric photoemission electron microscopy (polarimetric PEEM) that combines an optical pump-probe technique and polarimetry with photo-emission electron microscopy. This method allows for the accurate generation of surface plasmon polariton fields and their subsequent measurement, revealing both the spatial distribution of the full three-dimensional electromagnetic fields at deep sub-wavelength resolution and their time evolution.

physics.optics↗

arXiv2024

Plasmonic Twistronics: Discovery of Plasmonic Skyrmion Bags

The study of van der Waals heterostructures with an interlayer twist, known as "twistronics", has been instrumental in advancing contemporary condensed matter research. Most importantly, it has underpinned the emergence of a multitude of strongly-correlated phases, many of which derive from the topology of the physical system. Here, we explore the application of the twistronics paradigm in plasmonic systems with nontrivial topology, by creating a moiré skyrmion superlattice using two superimposed plasmonic skyrmion lattices, twisted at a "magic" angle. The complex electric field distribution of the moiré skyrmion superlattice is measured using time-resolved vector microscopy, revealing that each super-cell possesses very large topological invariants and harbors a "skyrmion bag", the size of which is controllable by the twist angle and center of rotation. Our work shows how twistronics leads to a diversity of topological features in optical fields, providing a new route to locally manipulate electromagnetic field distributions, which is crucial for future structured light-matter interaction.

physics.optics↗

arXiv2024

Skyrmion Bag Robustness in Plasmonic Bilayer and Trilayer Moiré Superlattices

Twistronics is studied intensively in twisted 2D heterostructures and its extension to trilayer moiré structures has proven beneficial for the tunability of unconventional correlated states and superconductivity in twisted trilayer graphene. Just recently, the concept of twistronics has been applied to plasmonic lattices with nontrivial topology, demonstrating that bilayer moiré skyrmion lattices harbor multi-skyrmion textures called skyrmion bags. Here, we explore the properties of plasmonic trilayer moiré superlattices that are created by the interference of three twisted skyrmion lattices. More specifically, we explore the properties of periodic superlattices and their topological invariants. We also demonstrate that twisted trilayer skyrmion lattices harbor the same skyrmion bags as twisted bilayer skyrmion lattices. We quantify the robustness of these skyrmion bags by the stability of their topological numbers against certain disturbance fields that leads to experimental designs for topological textures with maximum robustness.

physics.optics↗

arXiv2021

Phyllotaxis-inspired Nanosieves with Multiplexed Orbital Angular Momentum

Nanophotonic platforms such as metasurfaces, achieving arbitrary phase profiles within ultrathin thickness, emerge as miniaturized, ultracompact and kaleidoscopic optical vortex generators. However, it is often required to segment or interleave independent subarray metasurfaces to multiplex optical vortices in a single nano device, which in turn affects the compactness and channel capacity of the device. Here, inspired by phyllotaxis patterns in pine cones and sunflowers, we theoretically prove and experimentally report that multiple optical vortices can be produced in a single compact phyllotaxis nanosieve, both in free space and on a chip, where one metaatom may contribute to many vortices simultaneously. The time resolved dynamics of on chip interference wavefronts between multiple plasmonic vortices was revealed by ultrafast time-resolved photoemission electron microscopy. Our nature inspired optical vortex generator would facilitate various vortex related optical applications, including structured wavefront shaping, free space and plasmonic vortices, and high capacity information metaphotonics.

physics.optics↗

arXiv2021

Femtosecond field-driven on-chip unidirectional electronic currents in nonadiabatic tunnelling regime

Recently, asymmetric plasmonic nanojunctions [Karnetzky et. al., Nature Comm. 2471, 9 (2018)] have shown promise as on-chip electronic devices to convert femtosecond optical pulses to current bursts, with a bandwidth of multi-terahertz scale, although yet at low temperatures and pressures. Such nanoscale devices are of great interest for novel ultrafast electronics and opto-electronic applications. Here, we operate the device in air and at room temperature, revealing the mechanisms of photoemission from plasmonic nanojunctions, and the fundamental limitations on the speed of optical-to-electronic conversion. Inter-cycle interference of coherent electronic wavepackets results in a complex energy electron distribution and birth of multiphoton effects. This energy structure, as well as reshaping of the wavepackets during their propagation from one tip to the other, determine the ultrafast dynamics of the current. We show that, up to some level of approximation, the electron flight time is well-determined by the mean ponderomotive velocity in the driving field.

cond-mat.mes-hall↗

arXiv2020

Highly Confined In-plane Exciton-Polaritons in Monolayer Semiconductors

2D materials support unique excitations of quasi-particles that consist of a material excitation and photons called polaritons. Especially interesting are in-plane propagating polaritons which can be confined to a single monolayer and carry large momentum. In this work, we report the existence of a new type of in-plane propagating polariton, supported on monolayer transition-metal-dicalcogonide (TMD) in the visible spectrum, which has not yet been observed. This 2D in-plane exciton-polariton (2DEP) is described by the coupling of an electromagnetic light field with the collective oscillations of the excitons supported by monolayer TMDs. We expose the specific experimental conditions required for the excitation of the 2DEP and show that these can be created if the TMD is encapsulated with hexagonal-boron-nitride (hBN) and cooled to cryogenic temperatures. In addition, we compare the properties of the 2DEPs with those of surface-plasmons-polaritons (SPPs) at the same spectral range, and find that the 2DEP exhibit over two orders-of-magnitude larger wavelength confinement. Finally, we propose two configurations for the possible experimental observation of 2DEPs.

physics.optics↗

arXiv2019

Near-unity light absorption in a monolayer WS2 van der Waals heterostructure cavity

Excitons in monolayer transition-metal-dichalcogenides (TMDs) dominate their optical response and exhibit strong light-matter interactions with lifetime-limited emission. While various approaches have been applied to enhance light-exciton interactions in TMDs, the achieved strength have been far below unity, and a complete picture of its underlying physical mechanisms and fundamental limits has not been provided. Here, we introduce a TMD-based van der Waals heterostructure cavity that provides near-unity excitonic absorption, and emission of excitonic complexes that are observed at ultra-low excitation powers. Our results are in full agreement with a quantum theoretical framework introduced to describe the light-exciton-cavity interaction. We find that the subtle interplay between the radiative, non-radiative and dephasing decay rates plays a crucial role, and unveil a universal absorption law for excitons in 2D systems. This enhanced light-exciton interaction provides a platform for studying excitonic phase-transitions and quantum nonlinearities and enables new possibilities for 2D semiconductor-based optoelectronic devices.

physics.optics↗