SearcharxivSearch

arXiv subjects

Bibekananda Datta

Publications and source records attributed to Bibekananda Datta.

3 recordsLinked to original sources

A transient nonlinear finite element framework and implementation of coupled electro-chemo-mechanics of polyelectrolyte hydrogels

Polyelectrolyte (PE) hydrogels exhibit complex behavior characterized by large mechanical deformations, nonlinear stress response, solvent transport, and ion diffusion. The interplay between these mechanisms can lead to unexpected swelling dynamics, deformation patterns, and stress response. As such, advanced computational tools are needed for the efficient design of PE hydrogel-based devices, such as actuators and sensors for soft robotics, microfluidic valves, and drug delivery systems. In this work, we develop a numerical framework to simulate the coupled electro-chemo-mechanical behavior of PE hydrogels using finite element analysis. Applying this framework, an electro-chemo-mechanical model for PE hydrogels in a dilute ionic solution is implemented as a user element (UEL) subroutine in Abaqus/Standard. The model and UEL implementation are validated by comparing to experiments in the literature for transient free-swelling of a DMAEA gel in a solution of varying ionic strengths, then applied to study the consolidation behavior under confined compression and the transient bending behavior of a hydrogel bilayer. The simulations show that the ionic strength of the external solution, fixed charge density, and Flory-Huggins parameter play significant roles in the magnitude of the transient swelling and consolidation behavior.

cond-mat.soft

A finite viscoelastic constitutive model for low to high strain rate response of elastomers with application of strain rate-induced glass transition

Amorphous elastomers exhibit significant rate-stiffening and unique viscous flow characteristics across a wide range of strain rates, often undergoing glass transition above a strain rate threshold. We have developed a thermodynamically-consistent and micromechanically-inspired constitutive model for soft elastomers to capture the rate-dependent stress-strain behavior and hysteresis when subjected to low to high strain rates. Our proposed constitutive model encapsulates the viscous flow of materials through molecular motion at low strain rates and intermolecular rearrangement and alignment of the molecules at high strain rates, essentially covering the glass transition. We applied our constitutive model to uniaxial compression experiments performed at low and high strain rates for polyborosiloxane (PBS) to identify the material parameters, and subsequently, performed numerical simulations of single and multi-cycle compression, stress relaxation, and small amplitude oscillatory tension-compression. Our analyses indicate that the model predicts higher total energy dissipation with increasing strain rate; however, dissipation associated with molecular relaxation decreases because, beyond a crossover strain rate, intermolecular rearrangement and alignment become dominant, which is consistent with the onset of the glass transition. For cyclic loading-unloading, we observed that dissipation over a cycle remains constant at low strain rates but decreases non-monotonically at high strain rates before becoming constant, with the peak stress over the cycle becoming higher, which can be interpreted as more loading being carried elastically by the polymer network as the intermolecular rearrangement process occurs. Additionally, our model was able to qualitatively predict the storage modulus and loss modulus in the limit of small strain over a wide range of frequency sweeps.

cond-mat.soft

A Data-Driven Approach to Geometric Modeling of Systems with Low-Bandwidth Actuator Dynamics

It is challenging to perform system identification on soft robots due to their underactuated, high-dimensional dynamics. In this work, we present a data-driven modeling framework, based on geometric mechanics (also known as gauge theory) that can be applied to systems with low-bandwidth control of the system's internal configuration. This method constructs a series of connected models comprising actuator and locomotor dynamics based on data points from stochastically perturbed, repeated behaviors. By deriving these connected models from general formulations of dissipative Lagrangian systems with symmetry, we offer a method that can be applied broadly to robots with first-order, low-pass actuator dynamics, including swelling-driven actuators used in hydrogel crawlers. These models accurately capture the dynamics of the system shape and body movements of a simplified swimming robot model. We further apply our approach to a stimulus-responsive hydrogel simulator that captures the complexity of chemo-mechanical interactions that drive shape changes in biomedically relevant micromachines. Finally, we propose an approach of numerically optimizing control signals by iteratively refining models, which is applied to optimize the input waveform for the hydrogel crawler. This transfer to realistic environments provides promise for applications in locomotor design and biomedical engineering.

cs.RO