arXiv subjects

Bin Zeng

Publications and source records attributed to Bin Zeng.

52 records · Page 3Linked to original sources

arXiv2011

Comparative investigation of third and fifth harmonic generation in atomic and molecular gases driven by mid-infrared ultrafast laser pulses

We report on the comparative experimental investigation on third and fifth harmonic generation (THG and FHG) in atomic and molecular gases driven by mid-infrared ultrafast laser pulses at a wavelength of ~1500 nm. We observe that the conversion efficiencies of both the THG and FHG processes saturate at similar peak intensities close to ~1.5\times1014 W/cm2 for argon, nitrogen, and air, whose ionization potentials are close to each other. Near the saturation intensity, the ratio of yields of the FHG and THG reaches ~10-1 for all the gases. Our results show that high-order Kerr effects do exist, whereas they are insufficient to balance the Kerr self-focusing without the assistance of plasma generation.

physics.optics↗

arXiv2011

Anomalous Properties in the Normal and Superconducting States of LaRu$_3$Si$_2$

Superconductivity in LaRu$_3$Si$_2$ with the honeycomb structure of Ru atoms has been investigated. It is found that the normal state specific heat C/T exhibits a deviation from the Debye model down to the lowest temperature. A relation $C/T = γ_n+βT^2-ATlnT$ which concerns the electron correlations can fit the data very well. The suppression to the superconductivity by the magnetic field is not the mean-field like, which is associated well with the observation of strong superconducting fluctuations. The field dependence of the induced quasiparticle density of states measured by the low temperature specific heat shows a non-linear feature, indicating the significant contributions given by the delocalized quasiparticles.

cond-mat.supr-con↗

arXiv2011

High-brightness switchable multi-wavelength remote laser in air

Remote laser in air based on amplified spontaneous emission (ASE) has produced rather well-collimated coherent beams in both backward and forward propagation directions, opening up possibilities for new remote sensing approaches. The remote ASE-based lasers were shown to enable operation either at ~391 and 337 nm using molecular nitrogen or at ~845 nm using molecular oxygen as gain medium, depending on the employed pump lasers. To date, a multi-wavelength laser in air that allows for dynamically switching the operating wavelength has not yet been achieved, although this type of laser is certainly of high importance for detecting multiple hazard gases. In this Letter, we demonstrate, for the first time to our knowledge, a harmonic-seeded switchable multi-wavelength laser in air driven by intense mid-infrared femtosecond laser pulses. Furthermore, population inversion in the multi-wavelength remote laser occurs at an ultrafast time-scale (i.e., less than ~200 fs) owing to direct formation of excited molecular nitrogen ions by strong-field ionization of inner-valence electrons, which is fundamentally different from the previously reported pumping mechanisms based either on electron recombination of ionized molecular nitrogen or on resonant two-photon excitation of atomic oxygen fragments resulting from resonant two-photon dissociation of molecular oxygen. The bright multi-wavelength laser in air opens the perspective for remote detection of multiple pollutants based on nonlinear spectroscopy.

physics.atom-ph↗

arXiv2011

Nodeless superconductivity in K$_x$Fe$_{2-y}$Se$_2$ single crystals revealed by low temperature specific heat

Low temperature specific heat (SH) has been measured in K$_x$Fe$_{2-y}$Se$_2$ single crystals with T$_c$ = 32 K. The SH anomaly associated with the superconducting transition is moderate and sharp yielding a value of $ΔC/T \mid_{T_c}$ = 11.6 $\pm$ 1.0 $mJ/mol K^2$. The residual SH coefficient $γ(0)$ in the superconducting state at T$\rightarrow$ 0 is very small with a value of about 0.39 $mJ/mol K^2$. The magnetic field induced enhancement of the low-T SH exhibits a rough linear feature indicating a nodeless gap. This is further supported by the scaling based on the s-wave approach of the low-T data at different magnetic fields. A rough estimate tells that the normal state SH coefficient $γ_n$ is about 6 $\pm$ 0.5 $mJ/mol K^2$ leading to $ΔC/γ_nT\mid_{T_c}$ = 1.93 and placing this new superconductor in the strong coupling region.

cond-mat.supr-con↗

arXiv2010

Low Temperature Specific Heat of Optimally Doped BaFe$_{2-x}$$TM_x$As$_{2}$ ($TM$ = Co and Ni) Single Crystals: Constraint on the Pairing Gap

Low temperature specific heat has been measured in optimally doped and highly overdoped non-superconducting BaFe$_{2-x}$TM$_x$As$_{2}$ ($TM$ = Co and Ni) single crystals. By using the data of the overdoped samples, we successfully removed the phonon contribution of the optimally doped ones, and derived the electronic specific heat coefficient $γ_e$. Remarkably, we found a continuing temperature dependent $γ_e(T)$ which follows the quadratic relation $γ_e=γ_0+αT^2$ in the low temperature limit. Together with the very small residual term $γ_0$, linear magnetic field dependence of $γ_e$, it is concluded that there are either small segments of nodal lines, or point-like nodes in these samples.

cond-mat.supr-con↗

arXiv2010

Observation of Lattice and Andreev Bound States of Vortices in Ba0.6K0.4Fe2As2 Single Crystals with Scanning Tunneling Microscopy/Spectroscopy

For a type-II superconductor, when the applied magnetic field is higher than the lower critical value Hc1, the magnetic flux will penetrate into the superconductor and form quantized vortices, which usually are arranged in an Abrikosov lattice. For the newly discovered iron pnictide superconductors, previous measurements have shown that, in electron-doped BaFe2As2, the vortices form a highly disordered structure. In addition, the density of states (DOS) within the vortex cores1 do not exhibit the Andreev bound states in conventional superconductors. In this Letter, we report the observation of a triangular vortex lattice and the Andreev bound states in hole-doped BaFe2As2 by using a low temperature scanning tunneling microscope (STM). Detailed study of the vortex cores reveals that the spectrum of the Andreev bound states inside the vortex core exhibits a distinct spatial evolution: at the center of the vortex core, it appears as a single peak at 0.5 mV below the Fermi-energy; away from the core center, it gradually evolves into two sub-peaks and they eventually fade out. The drastic differences between the vortex cores of the electron-doped and hole-doped counterparts are illusive to the pairing mechanism of the iron pnictide superconductors.

cond-mat.supr-con↗

arXiv2010

Low temperature specific heat in BaFe1.9Ni0.1As2 single crystals

Low-temperature specific heat was measured on the BaFe1.9Ni0.1As2 single crystals with critical transi-tion temperature Tc = 20.1 K. A clear specific heat jump with the value \DeltaC/T|Tc \approx 23 mJ/mol K^2 has been observed. In addition, a roughly linear magnetic field dependence of the electronic specific heat coefficient Δγ(H) is found in the zero-temperature limit, suggesting that at least one Fermi pocket, probably the hole derivative one, is fully gapped with a small anisotropy in the present sample. A slight curvature of the curve Δγ(H) may suggest a complex gap structure (anisotropic gap or nodes) at other Fermi surfaces.

cond-mat.supr-con↗

arXiv2009

Structural and transport properties of Sr2VO{3-delta}FeAs superconductors with different oxygen deficiencies

Sr2VO{3-delta}FeAs superconductors with different oxygen deficiencies have been successfully fabricated. It is found that the superconducting transition temperature drops down monotonically with the increase of oxygen deficiency. The diminishing of superconductivity is accompanied by the enhancement of residual resistivity, indicating an unraveled scattering effect induced by the oxygen deficiency. The highest superconducting transition temperature at about 40 K is achieved near the stoichiometrical sample Sr$_2$VO$_{3}$FeAs. Surprisingly, the X-ray photoelectron spectroscopy (XPS) shows that the vanadium has a "5+" valence state in the samples. The Hall effect measurements reveal that the density of charge carriers (electron-like here) varies qualitatively with the increase of oxygen deficiency. Magnetotransport measurements show that the superconducting transition changes from one-step-like shape at low fields to two-step-like one at high fields, indicating a high anisotropy.

cond-mat.supr-con↗

arXiv2009

Superconductivity at 15.6 K in Calcium-doped Tb_{1-x}Ca_xFeAsO: the structure requirement for achieving superconductivity in the hole-doped 1111 phase

Superconductivity at about 15.6 K was achieved in Tb_{1-x}Ca_xFeAsO by partially substituting Tb^{3+} with Ca^{2+} in the nominal doping region x = 0.40 \sim 0.50. A detailed investigation was carried out in a typical sample with doping level of x = 0.44. The upper critical field of this sample was estimated to be 77 Tesla from the magnetic field dependent resistivity data. The domination of hole-like charge carriers in the low-temperature region was confirmed by Hall effect measurements. The comparison between the calcium-doped sample Pr_{1-x}Ca_xFeAsO (non-superconductive) and the Strontium-doped sample Pr_{1-x}Sr_xFeAsO (superconductive) suggests that a lager ion radius of the doped alkaline-earth element compared with that of the rare-earth element may be a necessary requirement for achieving superconductivity in the hole-doped 1111 phase.

cond-mat.supr-con↗

arXiv2009

Transition of stoichiometricSr2VO3FeAs to a superconducting state at 37.2 K

The superconductor Sr4V2O6Fe2As2 with transition temperature at 37.2 K has been fabricated. It has a layered structure with the space group of p4/nmm, and with the lattice constants a = 3.9296Aand c = 15.6732A. The observed large diamagnetization signal and zero-resistance demonstrated the bulk superconductivity. The broadening of resistive transition was measured under different magnetic fields leading to the discovery of a rather high upper critical field. The results also suggest a large vortex liquid region which reflects high anisotropy of the system. The Hall effect measurements revealed dominantly electron-like charge carriers in this material. The superconductivity in the present system may be induced by oxygen deficiency or the multiple valence states of vanadium.

cond-mat.supr-con↗

arXiv2009

Impurity Scattering Effect on Superconductivity and the Violation of Anderson Theorem in Ba(Fe_{1-x}Co_x)_2As_2 Single Crystals

Low-temperature specific heat (SH) and resistivity were measured on Ba(Fe_{1-x}Co_x)_2As_2 single crystals in wide doping region. A sizeable residual specific heat coefficient γ_0 was observed in the low temperature limit of all samples. The specific heat jump near T_c, i.e. ΔC/T|_{T_c} and the upper critical field H_{c2}^c (H||c) were also determined. It is found that -γ_0, ΔC/T|_{T_c}, \sqrt{H_{c2}^c} and T_c all shared a similar evolution with doping. All these can be well understood within the model of S$^\pm$ pairing symmetry when accounting the Co-dopants as unitary scattering centers in the FeAs planes. Our results give a direct evidence for the violation of the Anderson theorem in FeAs-based superconductors.

cond-mat.supr-con↗

arXiv2009

Superconductivity in Ti-doped Iron-Arsenide Compound Sr4Cr0.8Ti1.2O6Fe2As2

Superconductivity was achieved in Ti-doped iron-arsenide compound Sr4Cr0.8Ti1.2O6Fe2As2 (abbreviated as Cr-FeAs-42622). The x-ray diffraction measurement shows that this material has a layered structure with the space group of \emph{P4/nmm}, and with the lattice constants a = b = 3.9003 A and c = 15.8376 A. Clear diamagnetic signals in ac susceptibility data and zero-resistance in resistivity data were detected at about 6 K, confirming the occurrence of bulk superconductivity. Meanwhile we observed a superconducting transition in the resistive data with the onset transition temperature at 29.2 K, which may be induced by the nonuniform distribution of the Cr/Ti content in the FeAs-42622 phase, or due to some other minority phase.

cond-mat.supr-con↗

arXiv2009

Superconductivity at 22.3 K in SrFe2-xIrxAs2

By substituting the Fe with the 5d-transition metal Ir in SrFe2As2, we have successfully synthesized the superconductor SrFe2-xIrxAs2 with Tc = 22.3 K at x = 0.5. X-ray diffraction indicates that the material has formed the ThCr2Si2-type structure with a space group I4/mmm. The temperature dependence of resistivity and dc magnetization both reveal sharp superconducting transitions at around 22 K. An estimate on the diamagnetization signal reveals a high Meissner shielding volume. Interestingly, the normal state resistivity exhibits a roughly linear behavior up to 300 K. The superconducting transitions at different magnetic fields were also measured yielding a slope of -dHc2/dT = 3.8 T/K near Tc. Using the Werthamer-Helfand-Hohenberg (WHH) formula, the upper critical field at zero K is found to be about 58 T. Counting the possible number of electrons doped into the system in SrFe2-xIrxAs2, we argue that the superconductivity in the Ir-doped system is different from the Co-doped case, which should add more ingredients to the underlying physics of the iron pnictide superconductors.

cond-mat.supr-con↗

arXiv2009

Synthesis, structural and transport properties of the hole-doped Superconductor Pr_{1-x}Sr_xFeAsO

Superconductivity was achieved in PrFeAsO by partially substituting Pr^{3+} with Sr^{2+}. The electrical transport properties and structure of this new superconductor Pr_{1-x}Sr_xFeAsO at different doping levels (x = 0.05$\sim$ 0.25) were investigated systematically. It was found that the lattice constants (a-axis and c-axis) increase monotonously with Sr or hole concentration. The superconducting transition temperature at about 16.3 K (95% $ρ_n$) was observed around the doping level of 0.20$\sim$ 0.25. A detailed investigation was carried out in the sample with doping level of x = 0.25. The domination of hole-like charge carriers in this material was confirmed by Hall effect measurements. The magnetoresistance (MR) behavior can be well described by a simple two-band model. The upper critical field of the sample with T_c = 16.3 K (x = 0.25) was estimated to be beyond 45 Tesla. Our results suggest that the hole-doped samples may have higher upper critical fields comparing to the electron-doped ones, due to the higher quasi-particle density of states at the Fermi level.

cond-mat.supr-con↗

arXiv2008

(Sr_3Sc_2O_5)Fe_2As_2 as a possible parent compound for FeAs-based superconductors

A new compound with the FeAs-layers, namely (Sr_3Sc_2O_5)Fe_2As_2 (abbreviated as FeAs-32522), was successfully fabricated. It has a layered structure with the space group of I4/mmm, and with the lattice constants a = 4.069 $Å$ and c = 26.876 $Å$. The in-plane Fe ions construct a square lattice which is close to that of other FeAs-based superconductors, such as REFeAsO (RE = rare earth elements) and (Ba,Sr)Fe_2As_2. However the inter FeAs-layer spacing in the new compound is greatly enlarged. The temperature dependence of resistivity exhibits a weak upturn in the low temperature region, but a metallic behavior was observed above about 60 K. The magnetic susceptibility shows also a non-monotonic behavior. Interestingly, the well-known resistivity anomaly which was discovered in all other parent compounds, such as REFeAsO, (Ba,Sr)Fe_2As_2 and (Sr,Ca,Eu)FeAsF and associated with the Spin-Density-Wave (SDW)/structural transition has not been found in the new system either on the resistivity data or the magnetization data. This could be induced by the large spacing distance between the FeAs-planes, therefore the antiferromagnetic correlation between the moments of Fe ions in neighboring FeAs-layers cannot be established. Alternatively it can also be attributed to the self-doping effect between Fe and Sc ions. The Hall coefficient R_H is negative but strongly temperature dependent in wide temperature region, which indicates the dominance of electrical conduction by electron-like charge carriers and probably a multi-band effect or a spin related scattering effect. It is found that the magnetoresistance cannot be described by the Kohler's rule, which gives further support to above arguments.

cond-mat.supr-con↗

arXiv2008

High-T_c superconductivity induced by doping rare earth elements into CaFeAsF

We have successfully synthesized the fluoride-arsenide compounds Ca$_{1-x}$RE$_x$FeAsF (RE=Nd, Pr; x=0, 0.6). The x-ray powder diffraction confirmed that the main phases of our samples are Ca$_{1-x}$RE$_x$FeAsF with the ZrCuSiAs structure. By measuring resistivity, superconductivity was observed at 57.4 K in Nd-doped and 52.8 K in Pr-doped samples with x=0.6. Bulk superconductivity was also proved by the DC magnetization measurements in both samples. Hall effect measurements revealed hole-like charge carriers in the parent compound CaFeAsF with a clear resistivity anomaly below 118 K, while the Hall coefficient $R_H$ in the normal state is negative for the superconducting samples Ca$_{0.4}$Nd$_{0.6}$FeAsF and Ca$_{0.4}$Pr$_{0.6}$FeAsF. This indicates that the rare earth element doping introduces electrons into CaFeAsF which induces the high temperature superconductivity.

cond-mat.supr-con↗