Searcharxiv⌕ Search

arXiv subjects

Bing Cheng

Publications and source records attributed to Bing Cheng.

At least 37 records · Page 2Linked to original sources

On foundation of generative statistics with G-entropy: a gradient-based approach

This paper explores the interplay between statistics and generative artificial intelligence. Generative statistics, an integral part of the latter, aims to construct models that can generate efficiently and meaningfully new data across the whole of the (usually high dimensional) sample space, e.g. a new photo. Within it, the gradient-based approach is a current favourite that exploits effectively, for the above purpose, the information contained in the observed sample, e.g. an old photo. However, often there are missing data in the observed sample, e.g., missing bits in the old photo. To handle this situation, we have proposed a gradient-based algorithm for generative modelling. More importantly, our paper underpins rigorously this powerful approach by introducing a new G-entropy that is related to the Fisher divergence. (The G-entropy is also of independent interest.) The underpinning has enabled the gradient-based approach to expand its scope. For example, it can now provide a tool for generative model selection. Possible future projects include discrete data and Bayesian variational inference.

stat.ME↗

Decision Focused Causal Learning for Direct Counterfactual Marketing Optimization

Marketing optimization plays an important role to enhance user engagement in online Internet platforms. Existing studies usually formulate this problem as a budget allocation problem and solve it by utilizing two fully decoupled stages, i.e., machine learning (ML) and operation research (OR). However, the learning objective in ML does not take account of the downstream optimization task in OR, which causes that the prediction accuracy in ML may be not positively related to the decision quality. Decision Focused Learning (DFL) integrates ML and OR into an end-to-end framework, which takes the objective of the downstream task as the decision loss function and guarantees the consistency of the optimization direction between ML and OR. However, deploying DFL in marketing is non-trivial due to multiple technological challenges. Firstly, the budget allocation problem in marketing is a 0-1 integer stochastic programming problem and the budget is uncertain and fluctuates a lot in real-world settings, which is beyond the general problem background in DFL. Secondly, the counterfactual in marketing causes that the decision loss cannot be directly computed and the optimal solution can never be obtained, both of which disable the common gradient-estimation approaches in DFL. Thirdly, the OR solver is called frequently to compute the decision loss during model training in DFL, which produces huge computational cost and cannot support large-scale training data. In this paper, we propose a decision focused causal learning framework (DFCL) for direct counterfactual marketing optimization, which overcomes the above technological challenges. Both offline experiments and online A/B testing demonstrate the effectiveness of DFCL over the state-of-the-art methods. Currently, DFCL has been deployed in several marketing scenarios in Meituan, one of the largest online food delivery platform in the world.

cs.LG↗

Evidence for highly damped Higgs mode in infinite-layer nickelates

The dynamics of Higgs mode in superconductors, manifested as coherent oscillations of the superconducting order parameter amplitude, provides vital insights into the nature of the superconducting gap structure and symmetry. Here we utilize two-dimensional terahertz coherent spectroscopy to investigate Higgs dynamics of a newly discovered infinite-layer nickelate superconductor. While we observe distinct nonlinear terahertz responses from the superconducting state, well-defined long-lived Higgs modes, as commonly observed in $s$-wave superconductors, are entirely absent in the nickelate film. Instead, we find the coherent nonlinear terahertz response is dominated by the quasiparticle excitations. These observations strongly indicate that the Higgs mode in infinite-layer nickelates is heavily damped by the quasiparticle excitations at arbitrarily low energies, which is a characteristic of $d$-wave pairing symmetry. Additionally, by examining the temperature dependence of the nonlinear terahertz response, we discover short-range superconducting fluctuations in the vicinity of $T_\mathrm{c}$. Our findings provide proof of a new $d$-wave system and establish a foundation for investigating the unconventional superconductivity in nickelates.

cond-mat.supr-con↗

Low-energy electrodynamics of infinite-layer nickelates: evidence for d-wave superconductivity in the dirty limit

The discovery of superconductivity in infinite-layer nickelates establishes a new category of unconventional superconductors that share structural and electronic similarities with cuprates. Despite exciting advances, such as the establishment of a cuprate-like phase diagram and the observation of charge order and short-range antiferromagnetic fluctuation, the key issues of superconducting pairing symmetry, gap amplitude, and superconducting fluctuation remain elusive. In this work, we utilize static and ultrafast terahertz spectroscopy to address these outstanding problems. We demonstrate that the equilibrium terahertz conductivity and nonequilibrium terahertz responses of an optimally Sr-doped nickelate film ($T_c$ = 17 K) are in line with the electrodynamics of $d$-wave superconductivity in the dirty limit. The gap-to-$T_c$ ratio 2$Δ/k_\mathrm{B}T_\mathrm{c}$ is extracted to be 3.4, indicating the superconductivity falls in the weak-coupling regime. In addition, we observed significant superconducting fluctuation near $T_\mathrm{c}$, while it does not extend into the deep normal state as optimally hole-doped cuprates. Our result highlights a new $d$-wave system which closely resembles the electron-doped cuprates, expanding the family of unconventional superconductivity in oxides.

cond-mat.supr-con↗

Chirality manipulation of ultrafast phase switchings in a correlated CDW-Weyl semimetal

A recently emerging concept for quantum phase discovery is the controlled gapping of linear band crossings in topological semimetals. For example, achieving topological superconducting and charge-density-wave (CDW) gapping could introduce Majorana zero modes and axion electrodynamics, respectively. Light engineering of correlation gaps in topological materials provides a new avenue of achieving exotic topological phases inaccessible by conventional tuning methods such as doping and straining. Here we demonstrate a light control of correlation gaps and ultrafast phase switchings in a model CDW and polaron insulator (TaSe$_4$)$_2$I recently predicted to be an axion insulator. Our ultrafast terahertz photocurrent spectroscopy reveals a two-step, non-thermal melting of polarons and electronic CDW gap via studying the fluence dependence of a {\em longitudinal} circular photogalvanic current. The helicity-dependent photocurrent observed along the propagation of light reveals continuous ultrafast switchings from the polaronic state, to the CDW (axion) phase, and finally to a hidden Weyl phase as the pump fluence increases. Other distinguishing features corroborating with the light-induced switchings include: mode-selective coupling of coherent phonons to polaron and CDW modulation, and the emergence of a {\em non-thermal} chiral photocurrent above pump threshold of CDW-related phonons. The ultrafast chirality control of correlated topological states revealed here is important to realize axion electrodynamics and quantum computing.

cond-mat.str-el↗

Terahertz-driven Local Dipolar Correlation in a Quantum Paraelectric

Light-induced ferroelectricity in quantum paraelectrics is a new avenue of achieving dynamic stabilization of hidden orders in quantum materials. In this work, we explore the possibility of driving transient ferroelectric phase in the quantum paraelectric KTaO$_3$ via intense THz excitation of the soft mode. We observe a long-lived relaxation in the THz-driven second harmonic generation signal (SHG) that lasts up to 20 ps at 10 K which may be attributed to light-induced ferroelectricity. Through analyzing the THz-induced coherent soft-mode oscillation and finding its hardening with fluence well described by a single well potential, we demonstrate intense THz pulses up to 500 kV/cm cannot drive a global ferroelectric phase in KTaO$_3$. Instead, we find the unusual long-lived relaxation of SHG comes from a THz-driven moderate dipolar correlation between the defect-induced local polar structures. We discuss the impact of our findings on current investigations of the THz-induced ferroelectric phase in quantum paraelectrics.

cond-mat.mtrl-sci↗

Probing charge pumping and relaxation of the chiral anomaly in a Dirac semimetal

The linear band crossings of 3D Dirac and Weyl semimetals are characterized by a charge chirality, the parallel or anti-parallel locking of electron spin to its momentum. Such materials are believed to exhibit a ${\bf E} \cdot {\bf B}$ chiral magnetic effect that is associated with the near conservation of chiral charge. Here, we use magneto-terahertz spectroscopy to study epitaxial Cd$_3$As$_2$ films and extract their conductivities $σ(ω)$ as a function of ${\bf E} \cdot {\bf B}$. As field is applied, we observe a remarkably sharp Drude response that rises out of the broader background. Its appearance is a definitive signature of a new transport channel and consistent with the chiral response, with its spectral weight a measure of the net chiral charge and width a measure of the scattering rate between chiral species. The field independence of the chiral relaxation establishes that it is set by the approximate conservation of the isospin that labels the crystalline point-group representations.

cond-mat.mtrl-sci↗

Separated transport relaxation scales and interband scattering in SrRuO$_3$, CaRuO$_3$, and Sr$_2$RuO$_4$ thin films

The anomalous charge transport observed in some strongly correlated metals raises questions as to the universal applicability of Landau Fermi liquid theory. The coherence temperature $T_{FL}$ for normal metals is usually taken to be the temperature below which $T^2$ is observed in the resistivity. Below this temperature, a Fermi liquid with well-defined quasiparticles is expected. However, metallic ruthenates in the Ruddlesden-Popper family, frequently show non-Drude low-energy optical conductivity and unusual $ω/T$ scaling, despite the frequent observation of $T^2$ dc resistivity. Herein we report time-domain THz spectroscopy measurements of several different high-quality metallic ruthenate thin films and show that the optical conductivity can be interpreted in more conventional terms. In all materials, the conductivity has a two-Drude peak lineshape at low temperature and a crossover to a one-Drude peak lineshape at higher temperatures. The two-component low-temperature conductivity is indicative of two well-separated current relaxation rates for different conduction channels. We discuss three particular possibilities for the separation of rates: (a) Strongly energy-dependent inelastic scattering; (b) an almost-conserved pseudomomentum operator that overlaps with the current, giving rise to the narrower Drude peak; (c) the presence of multiple conduction channels that undergoes a crossover to stronger interband scattering at higher temperatures. None of these scenarios require the existence of exotic quasiparticles. The results may give insight into the possible significance of Hund's coupling in determining interband coupling in these materials. Our results also show a route towards understanding the violation of Matthiessen's rule in this class of materials and deviations from the "Gurzhi" scaling relations in Fermi liquids.

cond-mat.str-el↗

THz range Faraday rotation in the Weyl Semimetal Candidate $\mathrm{Co_2TiGe}$

The $\mathrm{Co_2}$ family of ferromagnetic Heusler alloys have attracted interest due to their fully spin-polarized nature, making them ideal for applications in spintronic devices. More recently, the existence of room temperature time-reversal-breaking Weyl nodes near the Fermi level was predicted and confirmed in these systems. As a result of the presence of these Weyl nodes, these systems possess a non-zero momentum space Berry curvature that can dramatically influence transport properties such as the anomalous Hall effect. One of these candidate compounds is $\mathrm{Co_2 Ti Ge}$. Recently, high quality molecular beam epitaxy-grown thin films of $\mathrm{Co_2 Ti Ge}$ have become available. In this work, we present THz-range measurement of MBE-grown $\mathrm{Co_2 Ti Ge}$ films. We measure the THz-range Faraday rotation, which can be understood as a measure of the anomalous Hall effect. We supplement this work with electronic band structure calculations showing that the principal contribution to the anomalous Hall effect in the this material stems from the Berry curvature of the material. Our work shows that this class of Heusler materials shows promise for Weyl semimetal based spintronics.

cond-mat.mes-hall↗

A Large Effective Phonon Magnetic Moment in a Dirac Semimetal

We investigated the magnetoterahertz response of the Dirac semimetal Cd$_3$As$_2$ and observed a particularly low frequency optical phonon, as well as a very prominent and field sensitive cyclotron resonance. As the cyclotron frequency is tuned with field to pass through the phonon, the phonon become circularly polarized as shown by a notable splitting in their response to right- and left-hand polarized light. This splitting can be expressed as an effective phonon magnetic moment that is approximately 2.7 times the Bohr magneton, which is almost four orders of magnitude larger than ab initio calculations predict for phonon magnetic moments in nonmagnetic insulators. This exceedingly large value is due to the coupling of the phonons to the cyclotron motion and is controlled directly by the electron-phonon coupling constant. This field tunable circular-polarization selective coupling provides new functionality for nonlinear optics to create light-induced topological phases in Dirac semimetals.

cond-mat.mes-hall↗

Unconventional free charge in the correlated semimetal Nd2Ir2O7

Nd2Ir2O7 is a correlated semimetal with the pyrochlore structure, in which competing spin-orbit coupling and electron-electron interactions are believed to induce a time-reversal symmetry broken Weyl semimetal phase characterized by pairs of topologically protected Dirac points at the Fermi energy. However, the emergent properties in these materials are far from clear, and exotic new states of matter have been conjectured. Here we demonstrate optically that at low temperatures the free carrier spectral weight is proportional to T^2 where T is the temperature, as expected for massless Dirac electrons. However, we do {\em not} observe the corresponding T^3 term in the specific heat. That the system is not in a Fermi liquid state is further corroborated by the "Planckian" T-linear temperature dependence of the momentum relaxation rate and the progressive opening of a correlation-induced gap at low temperatures. These observations can not be reconciled within the framework of band theory of electron-like quasiparticles and point toward the effective decoupling of the charge transport from the single particle sector.

cond-mat.str-el↗

Efficient Terahertz Harmonic Generation with Coherent Acceleration of Electrons in the Dirac Semimetal Cd3As2

We report strong terahertz (~10^12 Hz) high harmonic generation in thin films of Cd3As2, a three-dimensional Dirac semimetal at room temperature. The third harmonics is detectable with tabletop light source and can be as strong as 100 V/cm by applying the fundamental field of 6.5 kV/cm inside the film, showing an unprecedented efficiency for terahertz frequency conversion. Our time-resolved terahertz spectroscopy and calculations also clarify the microscopic mechanism of the nonlinearity originating in the coherent acceleration of Dirac electrons in momentum space. Our results provide clear insights for nonlinear current of Dirac electrons driven by terahertz field under an influence of scattering, paving the way toward novel devices for high-speed electronics and photonics based on topological semimetals.

cond-mat.mtrl-sci↗

Magnetoterahertz Response and Faraday Rotation from Massive Dirac Fermions in the Topological Crystalline Insulator Pb$_{0.5}$Sn$_{0.5}$Te

Pb$_{1-x}$Sn$_x$Te has been shown to be an interesting tunable topological crystalline insulator system. We present a magneto-terahertz spectroscopic study of thin films of Pb$_{0.5}$Sn$_{0.5}$Te. The complex Faraday rotation angle and optical conductivity in the circular basis are extracted without any additional assumptions. Our quantitative measures of the THz response allow us to show that the sample studied contains two types of bulk carriers. One is $p$-type and originates in 3D Dirac bands. The other is $n$-type and appears to be from more conventional 3D bands. These two types of carriers display different cyclotron resonance dispersions. Through simulating the cyclotron resonance of hole carriers, we can determine the Fermi energy and Fermi velocity. Furthermore, the scattering rates of $p$-type and $n$-type carriers were found to show opposite field dependences, which can be attributed to their different Landau level broadening behaviors under magnetic field. Our work provides a new way to isolate real topological signatures of bulk states in Dirac and Weyl semimetals.

cond-mat.mes-hall↗

Terahertz conductivity of the magnetic Weyl semimetal Mn$_{3}$Sn films

Mn$_{3}$Sn is a non-collinear antiferromagnet which displays a large anomalous Hall effect at room temperature. It is believed that the principal contribution to its anomalous Hall conductivity comes from Berry curvature. Moreover, dc transport and photoemission experiments have confirmed that Mn$_{3}$Sn may be an example of a time-reversal symmetry breaking Weyl semimetal. Due to a small, but finite moment in the room temperature inverse triangular spin structure, which allows control of the Hall current with external field, this material has garnered much interest for next generation memory devices and THz spintronics applications. In this work, we report a THz range study of oriented Mn$_{3}$Sn thin films as a function of temperature. At low frequencies we found the optical conductivity can be well described by a single Drude oscillator. The plasma frequency is strongly suppressed in a temperature dependent fashion as one enters the 260 K helical phase. This may be associated with partial gapping of the Fermi surfaces that comes from breaking translational symmetry along the c-axis. The scattering rate shows quadratic temperature dependence below 200 K, highlighting the possible important role of interactions in this compound.

cond-mat.str-el↗

Electric field modulated topological magnetoelectric effect in Bi$_2$Se$_3$

Topological insulators have been predicted to exhibit a variety of interesting phenomena including a quantized magnetoelectric response and novel spintronics effects due to spin textures on their surfaces. However, experimental observation of these phenomena has proved difficult due to the finite bulk carrier density which may overwhelm the intrinsic topological responses that are expressed at the surface. Here, we demonstrate a novel ionic gel gating technique to tune the chemical potential of Bi$_{2}$Se$_{3}$ thin films while simultaneously performing THz spectroscopy. We can tune the carrier concentration by an order of magnitude and shift the Fermi energy, E$_{F} $ to as low as $\simeq$ 10 meV above the Dirac point. At high bias voltage and magnetic field, we observe a quantized Faraday angle consistent with the topological magnetoelectric effect that can be tuned by ionic gel gating through a number of plateau states

cond-mat.mes-hall↗

Dielectric anomalies and interactions in the 3D quadratic band touching Luttinger semimetal Pr$_2$Ir$_2$O$_7$

Dirac and Weyl semimetals with linearly crossing bands are the focus of much recent interest in condensed matter physics. Although they host fascinating phenomena, their physics can be understood in terms of weakly interacting electrons. In contrast, more than 40 years ago, Abrikosov pointed out that quadratic band touchings are generically strongly interacting. We have performed terahertz spectroscopy on films of the conducting pyrochlore Pr$_2$Ir$_2$O$_7$, which has been shown to host a quadratic band touching. A dielectric constant as large as $\tilde{\varepsilon }/ε_0 \sim 180 $ is observed at low temperatures. In such systems the dielectric constant is a measure of the relative scale of interactions, which are therefore in our material almost two orders of magnitude larger than the kinetic energy. Despite this, the scattering rate exhibits a $T^2$ dependence, which shows that for finite doping a Fermi liquid state survives, however with a scattering rate close to the maximal value allowed.

cond-mat.str-el↗

An optical investigation of the strong spin-orbital coupled magnetic semimetal YbMnBi$_2$

Strong spin-orbit coupling (SOC) can result in ground states with non-trivial topological properties. The situation is even richer in magnetic systems where the magnetic ordering can potentially have strong influence over the electronic band structure. The class of AMnBi$_2$ (A = Sr, Ca) compounds are important in this context as they are known to host massive Dirac fermions with strongly anisotropic dispersion that is believed to be due to the interplay between strong SOC and magnetic degrees of freedom. We report the optical conductivity of YbMnBi$_2$, a newly discovered member of this family and a proposed Weyl semi-metal (WSM) candidate with broken time reversal symmetry. Together with density functional theory (DFT) band structure calculations, we show how the complete conductivity can be interpreted as the sum of a intra-band Drude response and inter-band transitions. We argue that the canting of the magnetic moments that has been proposed to be essential for the realization of the WSM in an otherwise antiferromagnetically ordered system is not necessary to explain the optical conductivity. We believe our data is explained qualitatively by the uncanted magnetic structure with a small offset of the chemical potential from strict stochiometry. There is no definite evidence of bulk Weyl nodes, instead we see signatures of a gapped Dirac dispersion, common in other members of AMnBi$_2$ family or compounds with similar 2D network of Bi atoms.

cond-mat.str-el↗

Measurement of the topological surface state optical conductance in bulk-insulating Sn-doped Bi$_{1.1}$Sb$_{0.9}$Te$_2$S single crystals

Topological surface states have been extensively observed via optics in thin films of topological insulators. However, in typical thick single crystals of these materials, bulk states are dominant and it is difficult for optics to verify the existence of topological surface states definitively. In this work, we studied the charge dynamics of the newly formulated bulk-insulating Sn-doped Bi$_{1.1}$Sb$_{0.9}$Te$_2$S crystal by using time-domain terahertz spectroscopy. This compound shows much better insulating behavior than any other bulk-insulating topological insulators reported previously. The transmission can be enhanced an amount which is 5$\%$ of the zero-field transmission by applying magnetic field to 7 T, an effect which we believe is due to the suppression of topological surface states. This suppression is essentially independent of the thicknesses of the samples, showing the two-dimensional nature of the transport. The suppression of surface states in field allows us to use the crystal slab itself as a reference sample to extract the surface conductance, mobility, charge density and scattering rate. Our measurements set the stage for the investigation of phenomena out of the semi-classical regime, such as the topological magneto-electric effect.

cond-mat.mes-hall↗