Bingqian Zhang | Searcharxiv

arXiv2026

OmniGUI: Benchmarking GUI Agents in Omni-Modal Smartphone Environments

Current benchmarks for graphical user interface (GUI) agents predominantly rely on static screenshots. However, real-world smartphone interaction routinely requires agents to process transient audio cues and temporal video dynamics that are tightly coupled with the moment of action. To bridge this gap, we introduce OmniGUI, the first step-level benchmark designed to evaluate GUI agents in omni-modal smartphone environments. OmniGUI provides continuous, interleaved multimodal inputs comprising static images, synchronous audio, and video clips at every action step. The dataset encompasses 709 expert-demonstrated episodes (2,579 action steps) across 29 applications, systematically annotated with objective multimodal dependency levels. Because dedicated omni-modal GUI agent frameworks are currently in their nascent stage, we select foundational omni-modal models capable of natively processing interleaved inputs to serve as agent proxies for our initial baselines. Our empirical evaluation reveals that while current models exhibit competency on visually static tasks, their action prediction performance degrades significantly in environments requiring synchronous temporal and auditory signals. Furthermore, ablation studies isolate specific operational bottlenecks, notably cross-modal interference when processing task-irrelevant environmental noise. The complete dataset, evaluation pipeline, and baseline prompts are provided in the supplementary material. Project page: https://omni-gui.github.io.

cs.HC↗

arXiv2025

Universal Catalyst Design Framework for Electrochemical Hydrogen Peroxide Synthesis Facilitated by Local Atomic Environment Descriptors

Developing a universal and precise design framework is crucial to search high-performance catalysts, but it remains a giant challenge due to the diverse structures and sites across various types of catalysts. To address this challenge, herein, we developed a novel framework by the refined local atomic environment descriptors (i.e., weighted Atomic Center Symmetry Function, wACSF) combined with machine learning (ML), microkinetic modeling, and computational high-throughput screening. This framework is successfully integrated into the Digital Catalysis Database (DigCat), enabling efficient screening for 2e- water oxidation reaction (2e- WOR) catalysts across four material categories (i.e., metal alloys, metal oxides and perovskites, and single-atom catalysts) within a ML model. The proposed wACSF descriptors integrating both geometric and chemical features are proven effective in predicting the adsorption free energies with ML. Excitingly, based on the wACSF descriptors, the ML models accurately predict the adsorption free energies of hydroxyl (ΔGOH*) and oxygen (ΔGO*) for such a wide range of catalysts, achieving R2 values of 0.84 and 0.91, respectively. Through density functional theory calculations and microkinetic modeling, a universal 2e- WOR microkinetic volcano model was derived with excellent agreement with experimental observations reported to date, which was further used to rapidly screen high-performance catalysts with the input of ML-predicted ΔGOH*. Most importantly, this universal framework can significantly improve the efficiency of catalyst design by considering multiple types of materials at the same time, which can dramatically accelerate the screening of high-performance catalysts.

cond-mat.mtrl-sci↗