arXiv subjects

Biswaroop Mukherjee

Publications and source records attributed to Biswaroop Mukherjee.

At least 19 recordsLinked to original sources

arXiv2026

Osmotically Induced Shape Changes in Membrane Vesicles

We develop a self-consistent free-energy framework in which membrane shape and osmotic pressure are determined simultaneously in a finite reservoir by minimizing bending elasticity and solute entropy. Solute conservation makes osmotic pressure a thermodynamic variable rather than an externally prescribed parameter, producing a nonlinear coupling between membrane mechanics and solvent entropy. This coupling modifies the classical stability condition for spherical vesicles: instability emerges from global free-energy competition rather than the linear Helfrich stability criterion. The resulting critical pressures differ by orders of magnitude from Helfrich predictions and agree with simulations for small and large unilamellar vesicles. The framework is relevant to cellular environments involving biomolecular condensate confinement as well as synthetic vesicles and the development of osmotic-pressure-driven encapsulation platforms.

cond-mat.soft↗

arXiv2024

Hardware-efficient quantum error correction via concatenated bosonic qubits

In order to solve problems of practical importance, quantum computers will likely need to incorporate quantum error correction, where a logical qubit is redundantly encoded in many noisy physical qubits. The large physical-qubit overhead typically associated with error correction motivates the search for more hardware-efficient approaches. Here, using a microfabricated superconducting quantum circuit, we realize a logical qubit memory formed from the concatenation of encoded bosonic cat qubits with an outer repetition code of distance $d=5$. The bosonic cat qubits are passively protected against bit flips using a stabilizing circuit. Cat-qubit phase-flip errors are corrected by the repetition code which uses ancilla transmons for syndrome measurement. We realize a noise-biased CX gate which ensures bit-flip error suppression is maintained during error correction. We study the performance and scaling of the logical qubit memory, finding that the phase-flip correcting repetition code operates below threshold, with logical phase-flip error decreasing with code distance from $d=3$ to $d=5$. Concurrently, the logical bit-flip error is suppressed with increasing cat-qubit mean photon number. The minimum measured logical error per cycle is on average $1.75(2)\%$ for the distance-3 code sections, and $1.65(3)\%$ for the longer distance-5 code, demonstrating the effectiveness of bit-flip error suppression throughout the error correction cycle. These results, where the intrinsic error suppression of the bosonic encodings allows us to use a hardware-efficient outer error correcting code, indicate that concatenated bosonic codes are a compelling paradigm for reaching fault-tolerant quantum computation.

quant-ph↗

arXiv2024

Thermography of the superfluid transition in a strongly interacting Fermi gas

Heat transport is a fundamental property of all physical systems and can serve as a fingerprint identifying different states of matter. In a normal liquid a hot spot diffuses while in a superfluid heat propagates as a wave called second sound. Despite its importance for understanding quantum materials, direct imaging of heat transport is challenging, and one usually resorts to detecting secondary effects, such as changes in density or pressure. Here we establish thermography of a strongly interacting atomic Fermi gas, a paradigmatic system whose properties relate to strongly correlated electrons, nuclear matter and neutron stars. Just as the color of a glowing metal reveals its temperature, the radiofrequency spectrum of the interacting Fermi gas provides spatially resolved thermometry with sub-nanokelvin resolution. The superfluid phase transition is directly observed as the sudden change from thermal diffusion to second sound propagation, and is accompanied by a peak in the second sound diffusivity. The method yields the full heat and density response of the strongly interacting Fermi gas, and therefore all defining properties of Landau's two-fluid hydrodynamics. Our measurements serve as a benchmark for theories of transport in strongly interacting fermionic matter.

cond-mat.quant-gas↗

arXiv2023

Geometric squeezing of rotating quantum gases into the lowest Landau level

The simulation of quantum Hall physics with rotating quantum gases is witnessing a revival due to recent experimental advances that enabled the observation of a Bose-Einstein condensate entirely contained in its lowest kinetic energy state, i.e. the lowest Landau level. We theoretically describe this experimental result, and show that it can be interpreted as a squeezing of the geometric degree of freedom of the problem, the guiding center metric. This "geometric squeezing" offers an unprecedented experimental control over the quantum geometry in Landau-level analogues, and at the same time opens a realistic path towards achieving correlated quantum phases akin to quantum Hall states with neutral atoms.

cond-mat.quant-gas↗

arXiv2023

Observation of chiral edge transport in a rapidly-rotating quantum gas

The frictionless, directional propagation of particles at the boundary of topological materials is one of the most striking phenomena in transport. These chiral edge modes lie at the heart of the integer and fractional quantum Hall effects, and their extraordinary robustness against noise and disorder reflects the quantization of Hall conductivity in these systems. Despite their central importance, controllable injection of edge modes, and direct imaging of their propagation, structure, and dynamics, is challenging. Here, we demonstrate the distillation of individual chiral edge states in a rapidly-rotating bosonic superfluid confined by an optical boundary. Tuning the wall sharpness, we reveal the smooth crossover between soft wall behaviour in which the propagation speed is proportional to wall steepness, and the hard wall regime exhibiting chiral free particles. From the skipping motion of atoms along the boundary, we spectroscopically infer the energy gap between the ground and first excited edge bands, and reveal its evolution from the bulk Landau level splitting for a soft boundary, to the hard wall limit.

cond-mat.quant-gas↗

arXiv2023

Thermodynamics predicts a stable microdroplet phase in polymer-gel mixtures undergoing elastic phase separation

We study the thermodynamics of binary mixtures with the volume fraction of the minority component less than the amount required to form a flat interface and show that the surface tension dominated equilibrium phase of the mixture forms a single macroscopic droplet. Elastic interactions in gel-polymer mixtures stabilize a phase with multiple droplets. Using a mean-field free energy we compute the droplet size as a function of the interfacial tension, Flory parameter, and elastic moduli of the gel. Our results illustrate the role of elastic interactions in dictating the phase behavior of biopolymers undergoing liquid-liquid phase separation.

cond-mat.soft↗

arXiv2021

Canonical Simulation Methodology to Extract Phase Boundaries of Liquid Crystalline Polymer Mixtures

We report a novel multi-scale simulation methodology to quantitatively predict the thermodynamic behaviour of polymer mixtures, that exhibit phases with broken orientational symmetry. Our system consists of a binary mixture of oligomers and rod-like mesogens. Using coarse-grained molecular dynamics (CGMD) simulations we infer the topology of the temperature-dependent free energy landscape from the probability distributions of excess volume fraction of the components. The mixture exhibits nematic and smectic phases as a function of two temperature scales, the nematic-isotropic temperature $T_{NI}$ and the $T_c$, the transition that governs the polymer demixing. Using a mean-field free energy of polymer-dispersed liquid crystals (PDLCs), with suitably chosen parameter values, we construct a mean-field phase diagram that semi-quantitatively match those obtained from CGMD simulations. Our results are applicable to mixtures of synthetic and biological macromolecules that undergo phase separation and are orientable, thereby giving rise to the liquid crystalline phases.

cond-mat.soft↗

arXiv2021

Geometric squeezing into the lowest Landau level

The equivalence between neutral particles under rotation and charged particles in a magnetic field relates phenomena as diverse as spinning atomic nuclei, weather patterns, and the quantum Hall effect. In their quantum descriptions, translations along different directions do not commute, implying a Heisenberg uncertainty relation between spatial coordinates. Here, we exploit the ability to squeeze non-commuting variables to dynamically create a Bose-Einstein condensate occupying a single Landau gauge wavefunction in the lowest Landau level. We directly resolve the extent of the zero-point cyclotron orbits, and demonstrate geometric squeezing of the orbits' guiding centers by more than ${7}~$dB below the standard quantum limit. The condensate attains an angular momentum of more than ${1000}\,{\hbar}$ per particle, and an interatomic distance comparable to the size of the cyclotron orbits. This offers a new route towards strongly correlated fluids and bosonic quantum Hall states.

cond-mat.quant-gas↗

arXiv2021

Crystallization of Bosonic Quantum Hall States

The dominance of interactions over kinetic energy lies at the heart of strongly correlated quantum matter, from fractional quantum Hall liquids, to atoms in optical lattices and twisted bilayer graphene. Crystalline phases often compete with correlated quantum liquids, and transitions between them occur when the energy cost of forming a density wave approaches zero. A prime example occurs for electrons in high magnetic fields, where the instability of quantum Hall liquids towards a Wigner crystal is heralded by a roton-like softening of density modulations at the magnetic length. Remarkably, interacting bosons in a gauge field are also expected to form analogous liquid and crystalline states. However, combining interactions with strong synthetic magnetic fields has been a challenge for experiments on bosonic quantum gases. Here, we study the purely interaction-driven dynamics of a Landau gauge Bose-Einstein condensate in and near the lowest Landau level (LLL). We observe a spontaneous crystallization driven by condensation of magneto-rotons, excitations visible as density modulations at the magnetic length. Increasing the cloud density smoothly connects this behaviour to a quantum version of the Kelvin-Helmholtz hydrodynamic instability, driven by the sheared internal flow profile of the rapidly rotating condensate. At long times the condensate self-organizes into a persistent array of droplets, separated by vortex streets, which are stabilized by a balance of interactions and effective magnetic forces.

cond-mat.quant-gas↗

arXiv2020

Wetting behaviour of a three-phase system in contact with a surface

We extend the Cahn-Landau-de Gennes mean field theory of binary mixtures to understand the wetting thermodynamics of a three phase system, that is in contact with an external surface which prefers one of the phases. We model the system using a phenomenological free energy having three minima corresponding to low, intermediate and high density phases. By systematically varying the \textit{(i)} depth of the central minimum, \textit{(ii)} the surface interaction parameters, we explore the phase behavior, and wetting characteristics of the system across the triple point corresponding to three phase coexistence. We observe a non-monotonic dependence of the surface tension across the triple point that is associated with a complete to partial wetting transition. The methodology is then applied to study the wetting behaviour of a polymer-liquid crystal mixture in contact with a surface using a renormalised free energy. Our work provides a way to interrogate phase behavior and wetting transitions of biopolymers in cellular environments.

cond-mat.soft↗

arXiv2019

Universal Sound Diffusion in a Strongly Interacting Fermi Gas

Transport of strongly interacting fermions governs modern materials -- from the high-$T_c$ cuprates to bilayer graphene --, but also nuclear fission, the merging of neutron stars and the expansion of the early universe. Here we observe a universal quantum limit of diffusivity in a homogeneous, strongly interacting Fermi gas of atoms by studying sound propagation and its attenuation via the coupled transport of momentum and heat. In the normal state, the sound diffusivity ${D}$ monotonically decreases upon lowering the temperature $T$, in contrast to the diverging behavior of weakly interacting Fermi liquids. As the superfluid transition temperature is crossed, ${D}$ attains a universal value set by the ratio of Planck's constant ${h}$ and the particle mass ${m}$. This finding of quantum limited sound diffusivity informs theories of fermion transport, with relevance for hydrodynamic flow of electrons, neutrons and quarks.

cond-mat.quant-gas↗

arXiv2019

Gelation impairs small molecule migration in polymer mixtures

Surface segregation of the low-molecular weight component in a polymeric mixture leads to degradation of industrial formulations. We report a simultaneous phase separation and surface migration phenomena in oligomer-polymer and oligomer-gel systems following a temperature quench. We compute equilibrium and time varying migrant density profiles and wetting layer thickness using coarse grained molecular dynamics and mesoscale hydrodynamics simulations to demonstrate that surface migration in oligomer-gel systems is significantly reduced due to network elasticity. Further, phase separation processes are significantly slowed in gels, modifying the Lifshitz-Slyozov-Wagner (LSW) law $\ell(τ) \sim τ^{1/3}$. Our work allows for rational design of polymer/gel-oligomer mixtures with predictable surface segregation characteristics.

cond-mat.soft↗

arXiv2019

Spectral response and contact of the unitary Fermi gas

We measure radiofrequency (rf) spectra of the homogeneous unitary Fermi gas at temperatures ranging from the Boltzmann regime through quantum degeneracy and across the superfluid transition. For all temperatures, a single spectral peak is observed. Its position smoothly evolves from the bare atomic resonance in the Boltzmann regime to a frequency corresponding to nearly one Fermi energy at the lowest temperatures. At high temperatures, the peak width reflects the scattering rate of the atoms, while at low temperatures, the width is set by the size of fermion pairs. Above the superfluid transition, and approaching the quantum critical regime, the width increases linearly with temperature, indicating non-Fermi-liquid behavior. From the wings of the rf spectra, we obtain the contact, quantifying the strength of short-range pair correlations. We find that the contact rapidly increases as the gas is cooled below the superfluid transition.

cond-mat.quant-gas↗

arXiv2019

Boiling a Unitary Fermi Liquid

We study the thermal evolution of a highly spin-imbalanced, homogeneous Fermi gas with unitarity limited interactions, from a Fermi liquid of polarons at low temperatures to a classical Boltzmann gas at high temperatures. Radio-frequency spectroscopy gives access to the energy, lifetime, and short-range correlations of Fermi polarons at low temperatures $T$. In this regime, we observe a characteristic $T^2$ dependence of the spectral width, corresponding to the quasiparticle decay rate expected for a Fermi liquid. At high $T$, the spectral width decreases again towards the scattering rate of the classical, unitary Boltzmann gas, $\propto T^{-1/2}$. In the transition region between the quantum degenerate and classical regime, the spectral width attains its maximum, on the scale of the Fermi energy, indicating the breakdown of a quasiparticle description. Density measurements in a harmonic trap directly reveal the majority dressing cloud surrounding the minority spins and yield the compressibility along with the effective mass of Fermi polarons.

cond-mat.quant-gas↗

arXiv2016

Homogeneous Atomic Fermi Gases

We report on the creation of homogeneous Fermi gases of ultracold atoms in a uniform potential. In the momentum distribution of a spin-polarized gas, we observe the emergence of the Fermi surface and the saturated occupation of one particle per momentum state. This directly confirms Pauli blocking in momentum space. For the spin-balanced unitary Fermi gas, we observe spatially uniform pair condensates. For thermodynamic measurements, we introduce a hybrid potential that is harmonic in one dimension and uniform in the other two. The spatially resolved compressibility reveals the superfluid transition in a spin-balanced Fermi gas, saturation in a fully polarized Fermi gas, and strong attraction in the polaronic regime of a partially polarized Fermi gas.

cond-mat.quant-gas↗

arXiv2015

From Planar Solitons to Vortex Rings and Lines: Cascade of Solitonic Excitations in a Superfluid Fermi Gas

We follow the time evolution of a superfluid Fermi gas of resonantly interacting $^6$Li atoms after a phase imprint. Via tomographic imaging, we observe the formation of a planar dark soliton, its subsequent snaking, and its decay into a vortex ring, which in turn breaks to finally leave behind a single solitonic vortex. In intermediate stages we find evidence for an exotic structure resembling the $Φ$-soliton, a combination of a vortex ring and a vortex line. Direct imaging of the nodal surface reveals its undulation dynamics and its decay via the puncture of the initial soliton plane. The observed evolution of the nodal surface represents dynamics beyond superfluid hydrodynamics, calling for a microscopic description of unitary fermionic superfluids out of equilibrium.

cond-mat.quant-gas↗

arXiv2014

Sisyphus Cooling of Lithium

Laser cooling to sub-Doppler temperatures by optical molasses is thought to be inhibited in atoms with unresolved, near-degenerate hyperfine structure in the excited state. We demonstrate that such cooling is possible in one to three dimensions, not only near the standard D2 line for laser cooling, but over a range extending to the D1 line. Via a combination of Sisyphus cooling followed by adiabatic expansion, we reach temperatures as low as 40 μK, which corresponds to atomic velocities a factor of 2.6 above the limit imposed by a single photon recoil. Our method requires modest laser power at a frequency within reach of standard frequency locking methods. It is largely insensitive to laser power, polarization and detuning, magnetic fields, and initial hyperfine populations. Our results suggest that optical molasses should be possible with all alkali species.

physics.atom-ph↗

arXiv2014

Motion of a Solitonic Vortex in the BEC-BCS Crossover

We observe a long-lived solitary wave in a superfluid Fermi gas of $^6$Li atoms after phase-imprinting. Tomographic imaging reveals the excitation to be a solitonic vortex, oriented transverse to the long axis of the cigar-shaped atom cloud. The precessional motion of the vortex is directly observed, and its period is measured as a function of the chemical potential in the BEC-BCS crossover. The long period and the correspondingly large ratio of the inertial to the bare mass of the vortex are in good agreement with estimates based on superfluid hydrodynamics that we derive here using the known equation of state in the BEC-BCS crossover.

cond-mat.quant-gas↗