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Björn Kubala

Publications and source records attributed to Björn Kubala.

At least 37 records · Page 2Linked to original sources

Magnetic Impurities on Superconducting Surfaces: Phase Transitions and the Role of Impurity-Substrate Hybridization

Spin-dependent scattering from magnetic impurities inside a superconductor gives rise to Yu-Shiba-Rusinov (YSR) states within the superconducting gap. As such, YSR states have been very successfully modeled with an effective scattering potential (Kondo impurity model). Using a scanning tunneling microscope, we exploit the proximity of the tip to a surface impurity and its influence on the YSR state to make a quantitative connection between the YSR state energy and the impurity-substrate hybridization. We corroborate the coupling between impurity and substrate as a key energy scale for surface derived YSR states using the Anderson impurity model in the mean field approximation, which accurately explains our observations. The model allows to decide on which side of the quantum phase transition the system resides based on additional conductance measurements. We propose that the Anderson impurity model is much more appropriate to describe YSR states from impurities on a superconducting surface than the Kondo impurity model, which is more appropriate for impurities inside a superconductor. We thus provide a first step towards a more quantitative comparison of experimental data with fully correlated calculations based on the Anderson impurity model.

cond-mat.supr-con↗

Dynamical Coulomb Blockade as a Local Probe for Quantum Transport

Quantum fluctuations are imprinted with valuable information about transport processes. Experimental access to this information is possible, but challenging. We introduce the dynamical Coulomb blockade (DCB) as a local probe for fluctuations in a scanning tunneling microscope (STM) and show that it provides information about the conduction channels. In agreement with theoretical predictions, we find that the DCB disappears in a single-channel junction with increasing transmission following the Fano factor, analogous to what happens with shot noise. Furthermore we demonstrate local differences in the DCB expected from changes in the conduction channel configuration. Our experimental results are complemented by ab initio transport calculations that elucidate the microscopic nature of the conduction channels in our atomic-scale contacts. We conclude that probing the DCB by STM provides a technique complementary to shot noise measurements for locally resolving quantum transport characteristics.

cond-mat.mes-hall↗

Josephson junction cavity systems as cousins of the quantum optical micromaser

We explore the similarities and differences between simple theoretical models developed to describe the quantum optical micromaser and Josephson-photonics devices. Whilst the micromaser has long been recognised as an important model for the dynamics of open quantum systems far from equilibrium, so-called Josephson-photonics devices are a recently developed form of superconducting quantum circuit in which the quantum transport of charges through a voltage-biased Josephson junction drives the production of photons in a microwave resonator.

quant-ph↗

Robustness of Yu-Shiba-Rusinov resonances in presence of a complex superconducting order parameter

Robust quantum systems rely on having a protective environment with minimized relaxation channels. Superconducting gaps play an important role in the design of such environments. The interaction of localized single spins with a conventional superconductor generally leads to intrinsically extremely narrow Yu-Shiba-Rusinov (YSR) resonances protected inside the superconducting gap. However, this may not apply to superconductors with nontrivial, energy dependent order parameters. Exploiting the Fe-doped two-band superconductor NbSe$_2$, we show that due to the nontrivial relation between its complex valued and energy dependent order parameters, YSR states are no longer restricted to be inside the gap. They can appear outside the gap (i. e. inside the coherence peaks), where they can also acquire a substantial intrinsic lifetime broadening. T-matrix scattering calculations show excellent agreement with the experimental data and relate the intrinsic YSR state broadening to the imaginary part of the host's order parameters. Our results suggest that non-thermal relaxation mechanisms contribute to the finite lifetime of the YSR states, even within the superconducting gap, making them less protected against residual interactions than previously assumed. YSR states may serve as valuable probes for nontrivial order parameters promoting a judicious selection of protective superconductors.

cond-mat.supr-con↗

Quantum thermodynamics with a Josephson-photonics setup

Josephson-photonics devices have emerged in the last years as versatile platforms to study light-charge interactions far from equilibrium and to create nonclassical radiation. Their potential to operate as nanoscale heat engines has also been discussed. The complementary mode of cooling is investigated here in the regimes of low and large photon occupancy, where nonlinearities are essential.

cond-mat.mes-hall↗

Quantum properties of a strongly driven Josephson junction

A Josephson junction embedded in a dissipative circuit can be externally driven to induce nonlinear dynamics of its phase. Classically, under sufficiently strong driving and weak damping, dynamic multi-stability emerges associated with dynamical bifurcations so that the often used modeling as a Duffing oscillator, which can exhibit bi-stability at the most, is insufficient. The present work analyzes in this regime corresponding quantum properties by mapping the problem onto a highly-nonlinear quasi-energy operator in a rotating frame. This allows us to identify in detail parameter regions where simplifications such as the Duffing approximation are valid, to explore classical-quantum correspondences, and to study how quantum fluctuations impact the effective junction parameters as well as the dynamics around higher amplitude classical fixed points.

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Single Channel Josephson Effect in a High Transmission Atomic Contact

The Josephson effect in scanning tunneling microscopy (STM) is an excellent tool to probe the properties of the superconducting order parameter on a local scale through the Ambegaokar-Baratoff (AB) relation. Using single atomic contacts created by means of atom manipulation, we demonstrate that in the extreme case of a single transport channel through the atomic junction modifications of the current-phase relation lead to significant deviations from the linear AB formula relating the critical current to the involved gap parameters. Using the full current-phase relation for arbitrary channel transmission, we model the Josephson effect in the dynamical Coulomb blockade regime because the charging energy of the junction capacitance cannot be neglected. We find excellent agreement with the experimental data. Projecting the current-phase relation onto the charge transfer operator shows that at high transmission multiple Cooper pair tunneling may occur. These deviations become non-negligible in Josephson-STM, for example, when scanning across single adatoms.

cond-mat.supr-con↗

Thermopower and dynamical Coulomb blockade in non-classical environments

Charge and heat transfer through a nanoscale conductor is not only determined by the transmission properties of the electrons, but can also be strongly impacted by coupling to other degrees of freedom in the environment of the conductor. Here, we analyze the influence of the electromagnetic environment on a simple, yet significant thermoelectric property, the thermopower, in the simple transport scenario of single-charge transfer across a tunnel junction. Considering both thermal and out-of-equilibrium steady-state environments, we find that the thermopower can be strongly affected by the environmental state and can, in turn, act as a sensitive probe of environmental properties.

cond-mat.mes-hall↗

Time-resolved statistics of photon pairs in two-cavity Josephson photonics

We analyze the creation and emission of pairs of highly nonclassical microwave photons in a setup where a voltage-biased Josephson junction is connected in series to two electromagnetic oscillators. Tuning the external voltage such that the Josephson frequency equals the sum of the two mode frequencies, each tunneling Cooper pair creates one additional photon in both of the two oscillators. The time-resolved statistics of photon emission events from the two oscillators is investigated by means of single- and cross-oscillator variants of the second-order correlation function $g^{(2)}(τ)$ and the waiting-time distribution $w(τ)$. They provide insight into the strongly correlated quantum dynamics of the two oscillator subsystems and reveal a rich variety of quantum features of light including strong antibunching and the presence of negative values in the Wigner function.

cond-mat.mes-hall↗

Generating entangled quantum microwaves in a Josephson-photonics device

When connecting a voltage-biased Josephson junction in series to several microwave cavities, a Cooper-pair current across the junction gives rise to a continuous emission of strongly correlated photons into the cavity modes. Tuning the bias voltage to the resonance where a single Cooper pair provides the energy to create an additional photon in each of the cavities, we demonstrate the entangling nature of these creation processes by simple witnesses in terms of experimentally accessible observables. To characterize the entanglement properties of the such created quantum states of light to the fullest possible extent, we then proceed to more elaborate entanglement criteria based on the knowledge of the full density matrix and provide a detailed study of bi- and multipartite entanglement. In particular, we illustrate how due to the relatively simple design of these circuits changes of experimental parameters allow one to access a wide variety of entangled states differing, e.g., in the number of entangled parties or the dimension of state space. Such devices, besides their promising potential to act as a highly versatile source of entangled quantum microwaves, may thus represent an excellent natural testbed for classification and quantification schemes developed in quantum information theory.

cond-mat.mes-hall↗

Electronic and photonic counting statistics as probes of non-equilibrium quantum dynamics

When a mesoscopic conductor is coupled to a high-quality electromagnetic cavity the flow of charges and the flux of photons leaking out of the cavity can both depend strongly on the coupled quantum dynamics of the system. Using a voltage-biased Josephson junction as a model system, we demonstrate that there is a simple connection between the full counting statistics of the charges and the photons in the long time limit. We then reveal the intimate relation between the counting statistics and the nonlinear dynamics of the system, uncovering novel regimes of coherent charge and photon transport associated with bifurcations in the classical dynamics of the system.

cond-mat.mes-hall↗

Time-resolved statistics of nonclassical light in Josephson photonics

The interplay of the tunneling transfer of charges and the emission and absorption of light can be investigated in a setup, where a voltage-biased Josephson junction is connected in series with a microwave cavity. We focus here on the emission processes of photons and analyze the underlying time-dependent statistics using the second-order correlation function $g^{(2)}(τ)$ and the waiting-time distribution $w(τ)$. Both observables highlight the crossover from a coherent light source to a single-photon source. Due to the nonlinearity of the Josephson junction, tunneling Cooper pairs can create a great variety of non-classical states of light even at weak driving. Analytical results for the weak driving as well as the classical regime are complemented by a numerical treatment for the full nonlinear case. We also address the question of possible relations between $g^{(2)}(τ)$ and $w(τ)$ as well as the specific information which is provided by each of them.

cond-mat.mes-hall↗

Josephson photonics with a two-mode superconducting circuit

We analyze the quantum dynamics of two electromagnetic oscillators coupled in series to a voltage biased Josephson junction. When the applied voltage leads to a Josephson frequency across the junction which matches the sum of the two mode frequencies, tunneling Cooper pairs excite photons in both modes simultaneously leading to far-from-equilibrium states. These states display highly non-classical features including strong anti-bunching, violation of Cauchy-Schwartz inequalities, and number squeezing. The regimes of low and high photon occupancies allow for analytical results which are supported by a full numerical treatment. The impact of asymmetries between the two modes is explored, revealing a pronounced enhancement of number squeezing when the modes are damped at different rates.

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Non-equilibrium dynamics of the Dicke model for mesoscopic aggregates: signatures of superradiance

In the dissipative quantum dynamics of a mesoscopic aggregate of excited two level systems (atoms) coupled to a single resonance mode of a cavity, two physical phenomena associated with superradiance appear. A pronounced emission peak on short time scales is related to the known superradiant burst of excited atoms cooperatively radiating into free space. It is followed by relaxation to a stationary state of the composite system such that for sufficiently large atom-field coupling a strongly correlated state emerges. The crossover to this state can be interpreted as the precursor of the transition from normal to superradiant phase in the thermodynamic limit of the Dicke Hamiltonian. Motivated by recent experimental activities, these features are investigated in detail for a mesoscopic number of atoms and a cavity embedded in a dissipative medium described by a damped Dicke model. We identify observables and characteristics of the quantum dynamics on shorter time scales which allow to clearly distinguish weakly correlated from strongly correlated Dicke physics.

quant-ph↗

Non-classical light from superconducting resonators coupled to voltage-biased Josephson junctions

The interplay of the tunneling transfer of charges and the emission and absorption of light can be investigated in a set-up, where a voltage-biased Josephson junction is placed in series to a microwave cavity. Here, we concentrate on the emission process and show that due to the inherent nonlinearity of the Josephson junction tunneling Cooper-pairs can create a variety of non-classical states of light. Depending on experimental parameters and tuning the device can be described by effective Hamiltonians, indicating specific photon creation mechanisms which lead to strongly bunched or anti-bunched light emission. We derive explicit analytical expressions for the photon correlation function $g^{(2)}(τ=0)$ for these different processes and investigate their full crossover numerically. Photon distribution functions show squeezing and other interesting non-Poissonian behavior.

cond-mat.mes-hall↗

From Coulomb blockade to nonlinear quantum dynamics in a superconducting circuit with a resonator

Motivated by recent experiments on superconducting circuits consisting of a dc-voltage biased Josephson junction in series with a resonator, quantum properties of these devices far from equilibrium are studied. This includes a crossover from a domain of incoherent to a domain of coherent Cooper pair tunneling, where the circuit realizes a driven nonlinear oscillator. Equivalently, weak photon-charge coupling turns into strong correlations captured by a single degree of freedom. Radiated photons offer a new tool to monitor charge flow and current noise gives access to nonlinear dynamics, which allows to analyze quantum-classical boundaries.

cond-mat.mes-hall↗

Decoherence in a Double-Dot Aharonov-Bohm Interferometer

Coherence in electronic interferometers is typically believed to be restored fully in the limit of small voltages, frequencies and temperatures. However, it is crucial to check this essentially perturbative argument by nonperturbative methods. Here, we use the numerical renormalization group to study ac transport and decoherence in an experimentally realizable model interferometer, a parallel double quantum dot coupled to a phonon mode. The model allows to clearly distinguish renormalization effects from decoherence. We discuss finite frequency transport and confirm the restoration of coherence in the dc limit.

cond-mat.mes-hall↗

Collective dynamics in optomechanical arrays

The emerging field of optomechanics seeks to explore the interaction between nanomechanics and light. Recently, the exciting concept of optomechanical crystals has been introduced, where defects in photonic crystal structures are used to generate both localized optical and mechanical modes that interact with each other. Here we start exploring the collective dynamics of arrays consisting of many coupled optomechanical cells. We show that such "optomechanical arrays" can display synchronization and that they can be described by a modified Kuramoto model that allows to explain and predict most of the features that will be observable in future experiments.

cond-mat.mes-hall↗