Blair C. Connelly | Searcharxiv

arXiv2026

Geometry-Controlled Polarization Photocurrents in Scalable PtSe2 Infrared Pixels

Polarization-sensitive photodetectors provide multi-dimensional optical information beyond the capabilities of traditional intensity-based detectors. The noble metal dichalcogenide PtSe2 presents unique opportunities for tunable polarization detection due to its strong spin-orbit coupling, material stability, customizable broadband polarization responses, and direct compatibility with a wide range of substrates for back-end-of-line silicon integration. In this work, we demonstrate room-temperature near-infrared to mid-wavelength infrared polarization photoresponses using scalable, as-grown, wide-area PtSe2 films, and we show that the measured polarization response is reshaped by device geometry. Finite-element current-flow simulations reproduce the observed spatial redistribution of the polarization-sensitive response and localize the transverse polarization response near the pixel center. This geometry-enabled separation allows wavelength-dependent laser spot scans to distinguish symmetry-allowed photocurrents from contact-proximate, dichroism-mediated photothermal contributions. At near-infrared wavelengths, we observe spatial response that is consistent with linear-dichroic photothermoelectric currents, whereas mid-wavelength infrared measurements reveal a helicity-dependent photothermal contribution under oblique illumination. These results identify pixel boundary engineering as both a design lever and a diagnostic tool for scalable PtSe2 polarization-sensitive infrared pixels.

physics.optics↗

arXiv2023

Emergence of Three-fold Symmetric Helical Photocurrents in Epitaxial Low Twinned Bi$_2$Se$_3$

We observe enhanced three-fold symmetric helicity-dependent topological photocurrents using time-domain THz spectroscopy in epitaxially-grown Bi2Se3 with reduced crystallographic twinning. It is established how twinned crystal domains introduce competing responses that obscure inherent nonlinear optical responses of the intrinsic crystal structure. Minimizing this defect reveals strong nonlinear optical response currents whose magnitude and direction depend on the alignment of the excitation to the crystal axes and follow the three-fold rotational symmetry of the crystal structure. Notably, the azimuthal dependence of the photoresponse persists for helical excitations -- an unprecedented result we attribute to the photon drag effect, where the photon momentum acts as an applied in-plane field that is stationary in the laboratory frame. Additionally, the sign of the resultant THz signal inverts when the helicity of incident light is switched from right to left circularly polarized, indicating a reversal of the photocurrent. Our results demonstrate that even extended domain defects can obscure intrinsic physical processes, making the study of single domain thin films crucial to the observation of phenomena that couple topological order and crystal symmetries.

cond-mat.mes-hall↗