arXiv subjects

Bo-Han Chen

Publications and source records attributed to Bo-Han Chen.

6 recordsLinked to original sources

arXiv2026

Attosecond-Stable Two-Dimensional Spectroscopy by a Sagnac-Based Modulating System and a sub-4-fs Continuum Source

We present a two-dimensional electronic spectroscopy (2DES) platform driven by a novel Coherent Loop-based Integrated Modulating and Beamsplitting System (CLIMBS). Coupled with an octave-spanning multiple-plate continuum (MPC) source, CLIMBS enables broadband, phase-coherent measurements with attosecond-level time delay precision. Its Sagnac-inspired, nearly common-path geometry provides exceptional long-term phase stability without active feedback, eliminating beam walk-off and preserving beam pointing during delay scans. Delay calibration using spectrally resolved interferometric fringes yielded a wedge angle in excellent agreement with the designed geometry, confirming precise, linear coherence time control. The MPC technique generates broadband excitation pulses spanning 550--980 nm and temporally compressed to 3.7 fs. This bright, few-cycle source enables simultaneous interrogation of widely separated electronic and vibronic transitions, with high temporal and spectral resolution, allowing 2DES to capture vibronic cross peaks, energy-transfer pathways, and undistorted ground-state bleaching (GB), stimulated emission (SE), and excited-state absorption (ESA) features across a broad spectral window. System performance was benchmarked on chlorophyll-a in methanol, where the excitation bandwidth fully covers the $Q_x$ and $Q_y$ bands, ensuring distortion-free spectra. The nearly collinear configuration of CLIMBS eliminates beam walk-off during delay scanning, supports ultrabroadband few-cycle 2DES enabled by the high-brightness MPC source, and maintains attosecond-level phase stability, providing a simple and robust platform for high-fidelity multidimensional spectroscopy.

physics.optics↗

arXiv2024

Revisiting the Mysterious Origin of FRB 20121102A with Machine-learning Classification

Fast radio bursts (FRBs) are millisecond-duration radio waves from the Universe. Even though more than 50 physical models have been proposed, the origin and physical mechanism of FRB emissions are still unknown. The classification of FRBs is one of the primary approaches to understanding their mechanisms, but previous studies classified conventionally using only a few observational parameters, such as fluence and duration, which might be incomplete. To overcome this problem, we use an unsupervised machine-learning model, the Uniform Manifold Approximation and Projection (UMAP) to handle seven parameters simultaneously, including amplitude, linear temporal drift, time duration, central frequency, bandwidth, scaled energy, and fluence. We test the method for homogeneous 977 sub-bursts of FRB 20121102A detected by the Arecibo telescope. Our machine-learning analysis identified five distinct clusters, suggesting the possible existence of multiple different physical mechanisms responsible for the observed FRBs from the FRB 20121102A source. The geometry of the emission region and the propagation effect of FRB signals could also make such distinct clusters. This research will be a benchmark for future FRB classifications when dedicated radio telescopes such as the Square Kilometer Array (SKA) or Bustling Universe Radio Survey Telescope in Taiwan (BURSTT) discover more FRBs than before.

astro-ph.HE↗

arXiv2022

Constraining the Hubble constant and its lower limit from the proper motion of extragalactic radio jets

The Hubble constant ($H_{0}$) is a measurement to describe the expansion rate of the Universe in the current era. However, there is a $4.4σ$ discrepancy between the measurements from the early Universe and the late Universe. In this research, we propose a model-free and distance-free method to constrain $H_{0}$. Combining Friedman-Lemaître-Robertson-Walker cosmology with geometrical relation of the proper motion of extragalactic jets, the lower limit ($H_{\rm 0,min}$) of $H_{0}$ can be determined using only three cosmology-free observables: the redshifts of the host galaxies, as well as the approaching and receding angular velocities of radio jets. Using these, we propose to use the Kolmogorov-Smirnov test (K-S test) between cumulative distribution functions of $H_{\rm 0,min}$ to differentiate cosmology. We simulate 100, 200, and 500 extragalactic jets with 3 levels of accuracy of the proper motion ($μ_{a}$ and $μ_{r}$), at $10\%$, $5\%$, and $1\%$, corresponding to the accuracies of the current and future radio interferometers. We perform K-S tests between the simulated samples as theoretical distributions with different $H_{0}$ and power-law index of velocity distribution of jets and mock observational data. Our result suggests increasing sample sizes leads to tighter constraints on both power-law index and the Hubble constant at moderate accuracy (i.e., $10\%$ and $5\%$) while at $1\%$ accuracy, increasing sample sizes leads to tighter constraints on power-law index more. Improving accuracy results in better constraints in the Hubble constant compared with the power-law index in all cases but it alleviates the degeneracy.

astro-ph.CO↗

arXiv2022

Double-pass multiple-plate continuum for high temporal contrast nonlinear pulse compression

We propose a new architecture, double-pass multiple-plate continuum (DPMPC), for nonlinear pulse compression. In addition to smaller footprint, a double-pass configuration is designed to achieve substantial bandwidth broadening without incurring noticeable higher-order dispersion, thus improving the temporal contrast over those of traditional single-pass geometry when only quadratic spectral phase can be compensated. In our proof-of-concept experiment, 187~$μ$J, 190-fs Yb-based laser pulse is compressed to 20~fs with high throughput (75%), high Strehl ratio (0.76) and excellent beam homogeneity by using DPMPC. Subsequently generated octave-spanning spectrum exhibits a significantly raised blue tail compared with that driven by pulses from a single-pass counterpart.

physics.optics↗

arXiv2021

Free-electron tomography of few-cycle optical waveforms

Ultrashort light pulses are ubiquitous in modern research, but the electromagnetic field of the optical cycles is usually not easy to obtain as a function of time. Field-resolved pulse characterization requires either a nonlinear-optical process or auxiliary sampling pulses that are shorter than the waveform under investigation, and pulse metrology without at least one of these two prerequisites is often thought to be impossible. Here we report how the optical field cycles of laser pulses can be characterized with a field-linear sensitivity and no short probe events. We let a free-space electron beam cross with the waveform of interest. The randomly arriving electrons interact by means of their elementary charge with the optical waveform in a linear-optical way and reveal the optical cycles as the turning points in a time-integrated deflection histogram on a screen. The sensitivity of the method is only limited by the emittance of the electron beam and can reach the level of thermal radiation and vacuum fluctuations. Besides overturning a common belief in optical pulse metrology, the idea also provides practical perspectives for in-situ characterization and optimization of optical waveforms in higher-harmonics experiments, ultrafast transmission electron microscopes, laser-driven particle accelerators, free-electron lasers or generally any experiments with waveform-controlled pulses in a vacuum environment.

physics.optics↗

arXiv2019

Asymmetric nonlinear optics of a polar chemical bond

A dielectric material's response to light is macroscopically described by electric displacement fields due to polarization and susceptibility, but the atomistic origin is light-cycle-driven motion of electron densities in the restoring forces of the atomic environment. Here we report how the macroscopic nonlinear-optical response of a heteronuclear crystal relates to the alignment and orientation of its chemical bonds. Substantial nonlinear emission is only observed if the electric field of an optical single-cycle pulse points from the less electronegative to the more electronegative element and not vice versa. This asymmetry is a consequence of the unbalanced real-space motion of valence charges along the direction of the bonds. These results connect a material's chemical structure to the optical response and may facilitate the comprehension and design of novel materials for applications in optics and lasers on basis of the atoms and how they connect.

physics.optics↗