arXiv subjects

Boris Maiorov

Publications and source records attributed to Boris Maiorov.

16 recordsLinked to original sources

arXiv2026

Leveraging mechanical resonances for the selection of promising materials in complex phase spaces

The "high-entropy" paradigm has been applied to a central challenge in materials science, the design of new functional materials with enhanced performance for targeted applications, with some notable successes over the last twenty years. However, the immensity of the high-entropy design space remains a major impediment to discovering optimal compositions with tailored microstructures. Suites of high-throughput computational tools have been developed to address this problem, but there is a compelling need to inform these models with fast, economical, non-destructive, and versatile experimental guidance. In this work, we demonstrate mechanical resonance measurements can fulfill this need. Mechanical resonance measurements enable the rapid, non-destructive assessment of materials created by novel syntheses and/or processes and provide high-accuracy determinations of elastic constants to directly benchmark models. We exemplify these capabilities on W-Ta-Cr-V-Hf and Mo-Nb-Ti-V-Zr refractory high-entropy alloys and suggest methodologies for the wider adoption and application of mechanical resonance measurements.

cond-mat.mtrl-sci↗

arXiv2025

Re-entrant unconventional superconductivity induced by rare-earth substitution in Nd1-xEuxNiO2 thin films

High temperature superconductivity is typically associated with strong coupling and a large superconducting gap, yet these characteristics have not been demonstrated in the nickelates. Here, we provide experimental evidence that Eu substitution in the spacer layer of Nd1-xEuxNiO2 (NENO) thin films enhances the superconducting gap, driving the system toward a strong-coupling regime. This is accompanied by a magnetic-exchange-driven magnetic-field-enhanced superconductivity. We investigate the upper critical magnetic field, Hc2, and superconducting gap of superconducting NENO thin films with x=0.2 to 0.35. Magnetoresistance measurements reveal magnetic-field-enhanced superconductivity in NENO films. We interpret this phenomenon as a result of interaction between magnetic Eu ions and superconducting states in the Ni dx2-y2 orbital. The upper critical magnetic field strongly violates the weak-coupling Pauli limit. Infrared spectroscopy confirms a large gap-to-Tc ratio $2 \Delta k_B T_c \approx 5 - 6$, indicating a stronger coupling pairing mechanism in NENO relative to the Sr-doped NdNiO2. The substitution of Eu in the rare-earth layer provides a method to modify the superconducting gap in Nd-based nickelates, an essential factor in engineering high-Tc superconductivity in infinite-layer nickelates.

cond-mat.supr-con↗

arXiv2025

High Entropy Engineering of Magnetic Kagome Lattice (Gd,Tb,Dy,Ho,Er)Mn6Sn6

The magnetic kagome lattice compound RMn6Sn6 (R=rare earth) is an emerging platform to exploit the interplay between magnetism and topological electronic states where a variety of exciting findings such as flat bands, Dirac points as well as the dramatic dependence of magnetic order on the rare-earth element have been reported. High entropy through rare earth alloying, on the other hand, provides another knob to control over the physical properties in this system. Here, by the marriage of high entropy and the magnetic kagome lattice, we obtain (Gd,Tb,Dy,Ho,Er)Mn6Sn6 single crystals and systematically investigate their magnetic and transport properties. Different from the parent phases, the high entropy 166 material displays multiple novel magnetic transitions induced by temperature and external magnetic fields. Furthermore, linear magnetoresistance persisting up to 20 T has been revealed at 4 K. The intrinsic nontrivial band topology also survives in the high entropy form, as evidenced by the intrinsic anomalous Hall effect. Our results highlight high entropy as a powerful approach for tuning the interplay of charge, spin and lattice degree of freedom in magnetic topological materials.

cond-mat.mtrl-sci↗

arXiv2025

Determining the Nature of Magnetism in Altermagnetic Candidate RuO$_2$

The terminology "altermagnetism" has recently been adopted to describe collinear magnetic order with no net magnetization and non-relativisitic, momentum-dependent spin-splitting. The archetypal material used to theoretically explore altermagnetism is RuO$_2$, but there has been significant debate as to whether RuO$_2$ possesses magnetic, let alone altermagnetic, order. To address questions surrounding the nature of magnetism in RuO$_2$, we combine symmetry-sensitive torque magnetometry and magnetization measurements in single crystals. The data are inconsistent with collinear magnetic order possessing a Néel vector along the $c-$axis. Torque magnetometry further demonstrates an isotropic magnetic susceptibility within the $ab-$plane, indicative of neither a Néel vector within the $ab-$plane nor a field-induced Néel vector reorientation. Magnetic quantum oscillations from both techniques reveal a nearly spherical Fermi surface pocket at the Brillouin zone center, in agreement with paramagnetic electronic structure calculations. Taken together, these data indicate no detectable long-range magnetic order and, by extension, suggest no altermagnetism in high-quality RuO$_2$ single crystals.

cond-mat.mtrl-sci↗

arXiv2025

Adaptation of Wallace's Approach to the Specific Heat of Elemental Solids with Significant Intrinsic Anharmonicity, Particularly the Light Actinide Metals

The quasiharmonic approximation is the most common method for modeling the specific heat of solids; however, it fails to capture the effects of intrinsic anharmonicity. In this study, we introduce the "elastic softening approximation," an alternative approach to modeling intrinsic anharmonic effects on thermodynamic quantities, which is grounded in Wallace's thermodynamic framework that tracks entropy changes resulting from the continuous change (e.g., softening) of phonons as a function of temperature. A key finding of our study is a direct correlation between Poisson's ratio and the differential rate of phonon softening at finite frequencies, compared to lower frequencies relevant to elastic moduli measurements. We observe that elemental solids such as $α$-Be, diamond, Al, Cu, In, W, Au, and Pb, which span a wide range of Poisson's ratios and exhibit varying degrees of intrinsic anharmonicity, consistently follow this trend. When applied to $α$-U, $α$-Pu, and $δ$-Pu, our method reveals unusually large anharmonic phonon contributions at elevated temperatures across all three light actinide metals. These findings are attributed to the unique combination of enhanced covalency and softer elastic moduli inherent in the actinides, potentially influenced by their 5f-electron bonding.

cond-mat.mtrl-sci↗

arXiv2023

Superconductivity above 180 K in Ca-Mg Ternary Superhydrides at Megabar Pressures

The discovery of high-temperature superconductivity above 240 K in binary La-H and Y-H systems inspired further predictions of even higher transition temperatures in compounds such as YH10 and MgH6, which are likely to be dynamically unstable. Ternary superhydrides provide alternative pathways to stabilize desired near-room temperature superconducting phases. However, the synthesis of new ternary hydrides remains challenging because most of the precursor reactants do not exist in desired stoichiometry at ambient conditions. Here we report that using the existing binary intermetallic CaMg2 and 1:1 Ca-Mg mixture as starting reactants, we have successfully synthesized novel Ca-Mg-based ternary superhydrides at megabar pressures. Electrical resistivity measurements show Tc approaching 168 K at 310 GPa in the CaMg2-based superhydride and 182 K in 1:1 the Ca-Mg superhydride at 324 GPa.

cond-mat.supr-con↗

arXiv2023

Sudden adiabaticity entering field-induced state in UTe2

There has been a recent surge of interest in UTe$_2$ due to its unconventional magnetic field (H) reinforced spin-triplet superconducting phases persisting at fields far above the simple Pauli limit for H $\parallel$ [010]. Magnetic fields in excess of 35 T then induce a field-polarized magnetic state via a first-order-like phase transition. More controversially, for field orientations close to H $\parallel$ [011] and above 40 T, electrical resistivity measurements suggest that a further superconducting state may exist. However, no Meissner effect or thermodynamic evidence exists to date for this phase making it difficult to exclude a simple low-resistance metallic state. In this paper, we describe a study using thermal, electrical, and magnetic probes in magnetic fields of up to 55 T applied between the [010] ($b$) and [001] ($c$) directions. Our MHz conductivity data reveal the field-induced state of low or vanishing electrical resistance; simultaneous magnetocaloric effect measurements (i.e. changes in sample temperature due to changing magnetic field), show the first definitive evidence for adiabaticity and thermal behavior characteristic of bulk field-induced superconductivity.

cond-mat.supr-con↗

arXiv2022

Thermodynamic approach for enhancing superconducting critical current performance

The addition of artificial pinning centers has led to an impressive increase in critical current density ($J_{\rm c}$) in a superconductor, enabling record-breaking all-superconducting magnets and other applications. $J_{\rm c}$ has reached $\sim 0.2$-$0.3$ $J_{\rm d}$, where $J_{\rm d}$ is the depairing current density, and the numerical factor depends on the pinning optimization. By modifying $λ$ and/or $ξ$, the penetration depth and coherence length, respectively, we can increase $J_{\rm d}$. For (Y$_{0.77}$Gd$_{0.23}$)Ba$_2$Cu$_3$O$_y$ ((Y,Gd)123) we achieve this by controlling the carrier density, which is related to $λ$ and $ξ$. We also tune $λ$ and $ξ$ by controlling the chemical pressure in the Fe-based superconductors, BaFe$_2$(As$_{1-x}$P$_x$)$_2$ films. The variation of $λ$ and $ξ$ leads to an intrinsic improvement of $J_{\rm c}$, via $J_{\rm d}$, obtaining extremely high values of $J_{\rm c}$ of $130$ MA/cm$^2$ and $8.0$ MA/cm$^2$ at $4.2$ K, consistent with an enhancement of $J_{\rm d}$ of a factor of $2$ for both incoherent nanoparticle-doped (Y,Gd)123 coated conductors (CCs) and BaFe$_2$(As$_{1-x}$P$_x$)$_2$ films, showing that this new material design is useful to achieving high critical current densities for a wide array of superconductors. The remarkably high vortex-pinning force in combination with this thermodynamic and pinning optimization route for the (Y,Gd)123 CCs reached $\sim 3.17$ TN/m$^3$ at $4.2$ K and 18 T (${\bf H}\parallel c$), the highest values ever reported in any superconductor.

cond-mat.supr-con↗

arXiv2021

Magnetoelastic standing waves induced in UO$_{2}$ by microsecond magnetic field pulses

Magnetoelastic measurements in the piezomagnetic antiferromagnet UO$_{2}$ were performed via the fiber Bragg grating method in magnetic fields up to $150\,\mathrm{T}$ generated by a single-turn coil setup. We show that in short timescales, order of a few micro seconds, pulsed-magnetic fields excite mechanical resonances at temperatures ranging from $10\,\mathrm{K}$ to $300\,\mathrm{K}$, in the paramagnetic as well as within the robust antiferromagnetic state of the material. These resonances, which are barely attenuated within the 100 ms observations, are attributed to the strong magnetoelastic coupling in UO$_{2}$ combined with the high crystallographic quality of the single crystal samples. They compare well with mechanical resonances obtained by a resonant ultrasound technique and superimpose on the known non-monotonic magnetostriction background. A clear phase-shift of $π$ in the lattice oscillations is, unexpectedly, observed in the antiferromagnetic state when the magnetic field overcomes the piezomagnetic switch-field $H_c \simeq -18\,\mathrm{T}$. We further present simulations and a theoretical argument to explain the observed phenomena.

cond-mat.mtrl-sci↗

arXiv2020

Skyrmion lattice creep at ultra-low current densities

Magnetic skyrmions are well-suited for encoding information because they are nano-sized, topologically stable, and only require ultra-low critical current densities $j_c$ to depin from the underlying atomic lattice. Above $j_c$ skyrmions exhibit well-controlled motion, making them prime candidates for race-track memories. In thin films thermally-activated creep motion of isolated skyrmions was observed below $j_c$ as predicted by theory. Uncontrolled skyrmion motion is detrimental for race-track memories and is not fully understood. Notably, the creep of skyrmion lattices in bulk materials remains to be explored. Here we show using resonant ultrasound spectroscopy--a probe highly sensitive to the coupling between skyrmion and atomic lattices--that in the prototypical skyrmion lattice material MnSi depinning occurs at $j_c^*$ that is only 4 percent of $j_c$. Our experiments are in excellent agreement with Anderson-Kim theory for creep and allow us to reveal a new dynamic regime at ultra-low current densities characterized by thermally-activated skyrmion-lattice-creep with important consequences for applications.

cond-mat.str-el↗

arXiv2019

Novel dynamics and critical currents in fast superconducting vortices at high pulsed magnetic fields

Non-linear electrical transport studies at high-pulsed magnetic fields, above the range accessible by DC magnets, are of direct fundamental relevance to the physics of superconductors, domain-wall, charge-density waves, and topological semi-metal. All-superconducting very-high field magnets also make it technologically relevant to study vortex matter in this regime. However, pulsed magnetic fields reaching 100 T in milliseconds impose technical and fundamental challenges that have prevented the realization of these studies. Here, we present a technique for sub-microsecond, smart, current-voltage measurements, which enables determining the superconducting critical current in pulsed magnetic fields, beyond the reach of any DC magnet. We demonstrate the excellent agreement of this technique with low DC field measurements on Y$_{0.77}$Gd$_{0.23}$Ba$_2$Cu$_3$O$_7$ coated conductors with and without BaHfO$_3$ nanoparticles. Exploring the uncharted high magnetic field region, we discover a characteristic influence of the magnetic field rate of change ($dH/dt$) on the current-voltage curves in a superconductor. We fully capture this unexplored vortex physics through a theoretical model based on the asymmetry of the vortex velocity profile produced by the applied current.

cond-mat.supr-con↗

arXiv2018

Skyrmion Topological Hall Effect near Room Temperature

Magnetic skyrmions are stable nanosized spin structures that can be displaced at low electrical current densities. Because of these properties, they have been proposed as building blocks of future electronic devices with unprecedentedly high information density and low energy consumption. The electrical detection of skyrmions via the Topological Hall Effect (THE), has so far been demonstrated only at cryogenic temperatures. Here, we report the observation of a skyrmion Topological Hall Effect near room temperature (276 K) in a mesoscopic lamella of FeGe. This region unambiguously coincides with the skyrmion lattice location revealed by neutron scattering. We provide clear evidence of a reentrant helicoid magnetic phase adjacent to the skyrmion phase, and discuss the large THE amplitude (5 n$Ω$.cm) in view of the ordinary Hall Effect.

cond-mat.mes-hall↗

arXiv2017

Elasticity in the skyrmion phase unveils depinning at ultra-low current densities

Controlled movement of nano-scale stable magnetic objects has been proposed as the foundation for a new generation of magnetic storage devices. Magnetic skyrmions, vortex-like spin textures stabilized by their topology are particularly promising candidates for this technology. Their nanometric size and ability to be displaced in response to an electrical current density several orders of magnitude lower than required to induce motion of magnetic domain walls suggest their potential for high-density memory devices that can be operated at low power. However, to achieve this, skyrmion movement needs to be controlled, where a key question concerns the coupling of skyrmions with the underlying atomic lattice and disorder (pinning). Here, we use Resonant Ultrasound Spectroscopy (RUS), a probe highly sensitive to changes in the elastic properties, to shed new light on skyrmion elasticity and depinning in the archetypal skyrmion material MnSi. In MnSi, skyrmions form a lattice that leads to pronounced changes in the elastic properties of the atomic lattice as a result of magneto-crystalline coupling. Without an applied current, the shear and compressional moduli of the underlying crystal lattice exhibit an abrupt change in the field-temperature range where skyrmions form. For current densities exceeding $j_c^*$ the changes of elastic properties vanish, signaling the decoupling of skyrmion and atomic lattices. Interestingly, $j_c^*$, which we identify as the onset of skyrmion depinning, is about 20 times smaller than $j_c$ previously measured via non-linear Hall effect. Our results suggest the presence of a previously-undetected intermediate dynamic regime possibly dominated by skyrmion-creep motion with important consequences for potential applications.

cond-mat.str-el↗

arXiv2016

Universal Lower Limit on Vortex Creep in Superconductors

Superconductors are excellent testbeds for studying vortices, topological excitations that also appear in superfluids, liquid crystals, and Bose-Einstein condensates. Vortex motion can be disruptive; it can cause phase transitions, glitches in pulsars, and losses in superconducting microwave circuits, and it limits the current carrying capacity of superconductors. Understanding vortex dynamics is therefore of fundamental and technological importance, and the competition between the effects of thermal energy and energy barriers defined by material disorder is not completely understood. In particular, early measurements of thermally-activated vortex motion (creep) in iron-based superconductors unveiled fast rates (S) comparable to measurements of YBa2Cu3O7 (YBCO). This was puzzling because S is thought to somehow positively correlate with the Ginzburg number (Gi), and Gi is orders of magnitude lower in most iron-based superconductors than in YBCO. Here, we report very slow creep in BaFe2(As0.67P0.33)2 films, and propose that there is a universal minimum realizable (where Tc is the superconducting transition temperature) that has been achieved in our films, few other materials, and violated by none. This limitation provides new clues on how to design materials with slow creep and helps elucidate open questions regarding the interplay between system-specific length scales and vortex dynamics.

cond-mat.supr-con↗

arXiv2002

Hole-doping dependence of percolative phase separation in Pr_(0.5-delta)Ca_(0.2+delta)Sr_(0.3)MnO_(3) around half doping

We address the problem of the percolative phase separation in polycrystalline samples of Pr$_{0.5-δ}$Ca$_{0.2+δ}$Sr$_{0.3}$MnO$_3$ for $-0.04\leq δ\leq 0.04$ (hole doping $n$ between 0.46 and 0.54). We perform measurements of X-ray diffraction, dc magnetization, ESR, and electrical resistivity. These samples show at $T_C$ a paramagnetic (PM) to ferromagnetic (FM) transition, however, we found that for $n>0.50$ there is a coexistence of both of these phases below $T_C$. On lowering $T$ below the charge-ordering (CO) temperature $T_{CO}$ all the samples exhibit a coexistence between the FM metallic and CO (antiferromagnetic) phases. In the whole $T$ range the FM phase fraction ($X$) decreases with increasing $n$. Furthermore, we show that only for $n\leq 0.50$ the metallic fraction is above the critical percolation threshold $X_C\simeq 15.5%$. As a consequence, these samples show very different magnetoresistance properties. In addition, for $n\leq 0.50$ we observe a percolative metal-insulator transition at $T_{MI}$, and for $T_{MI}<T<T_{CO}$ the insulating-like behavior generated by the enlargement of $X$ with increasing $T$ is well described by the percolation law $ρ^{-1}=σ\sim (X-X_C)^t$, where $t$ is a critical exponent. On the basis of the values obtained for this exponent we discuss different possible percolation mechanisms, and suggest that a more deep understanding of geometric and dimensionality effects is needed in phase separated manganites. We present a complete $T$ vs $n$ phase diagram showing the magnetic and electric properties of the studied compound around half doping.

cond-mat.str-el↗

arXiv2002

Elastic-to-plastic crossover below the peak effect in the vortex solid of YBa2Cu3O7 single crystals

We report on transport and ac susceptibility studies below the peak effect in twinned YBa2Cu3O7 single crystals. We find that disorder generated at the peak effect can be partially inhibited by forcing vortices to move with an ac driving current. The vortex system can be additionally ordered below a well-defined temperature where elastic interactions between vortices overcome pinning-generated stress and a plastic to elastic crossover seems to occur. The combined effect of these two processes results in vortex structures with different mobilities that give place to history effects.

cond-mat.supr-con↗