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Bradley A. Foreman

Publications and source records attributed to Bradley A. Foreman.

12 recordsLinked to original sources
arXiv2019

Complementarity has empirically relevant consequences for the definition of quantum states

The Copenhagen interpretation of quantum mechanics, which first took shape in Bohr's landmark 1928 paper on complementarity, remains an enigma. Although many physicists are skeptical about the necessity of Bohr's philosophical conclusions, his pragmatic message about the importance of the whole experimental arrangement is widely accepted. It is, however, generally also agreed that the Copenhagen interpretation has no direct consequences for the mathematical structure of quantum mechanics. Here I show that the application of Bohr's main concepts of complementarity to the subsystems of a closed system requires a change in the definition of the quantum state. The appropriate definition is as an equivalence class similar to that used by von Neumann to describe macroscopic subsystems. He showed that such equivalence classes are necessary in order to maximize information entropy and achieve agreement with experimental entropy. However, the significance of these results for the quantum theory of measurement has been overlooked. Current formulations of measurement theory are therefore manifestly in conflict with experiment. This conflict is resolved by the definition of the quantum state proposed here.

quant-ph↗
arXiv2019

Emergence of outcomes in quantum mechanics

A persistent focus on the concept of emergence as a core element of the scientific method allows a clean separation, insofar as this is possible, of the physical and philosophical aspects of the problem of outcomes in quantum mechanics. The philosophical part of the problem is to explain why a closed system has definite experimental outcomes. The physical part is to show mathematically that there exists a limit in which the contradiction between unitary Schroedinger dynamics and a reduction process leading to distinct outcomes becomes negligible according to an explicitly stated criterion, and to make this criterion as objective as possible. The physical problem is solved here by redefining the notion of a quantum state and finding a suitable measure for the change of state upon reduction. The appropriate definition of the quantum state is not as a ray or density operator in Hilbert space, but rather as an equivalence class consisting of all density operators in a given subspace, the members of which all describe the same experimental outcome. For systems containing only subsystems that are integrated with their environments, these equivalence classes can be represented mathematically by projection operators, and the resulting formalism is closely related to that used by von Neumann to study the increase of entropy predicted by the second law of thermodynamics. However, nearly isolated subsystems are reduced only indirectly, as a consequence of their interaction with integrated subsystems. The reduced states of isolated subsystems are the same conditional states used in the definition of quantum discord. The key concepts of decoherence theory can all be adapted to fit this definition of a quantum state, resulting in a unified theory capable of resolving, in principle, all aspects of the quantum measurement problem. The theory thus obtained is weakly objective but not strongly objective.

quant-ph↗
arXiv2016

Subsystems and time in quantum mechanics

This paper investigates the relationship between subsystems and time in a closed nonrelativistic system of interacting bosons and fermions. It is possible to write any state vector in such a system as an unentangled tensor product of subsystem vectors, and to do so in infinitely many ways. This requires the superposition of different numbers of particles, but the theory can describe in full the equivalence relation that leads to a particle-number superselection rule in conventionally defined subsystems. Time is defined as a functional of subsystem changes, thus eliminating the need for any reference to an external time variable. The dynamics of the unentangled subsystem decomposition is derived from a variational principle of dynamical stability, which requires the decomposition to change as little as possible in any given infinitesimal time interval, subject to the constraint that the state of the total system satisfy the Schroedinger equation. The resulting subsystem dynamics is deterministic. This determinism is regarded as a conceptual tool that observers can use to make inferences about the outside world, not as a law of nature. The experiences of each observer define some properties of that observer's subsystem during an infinitesimal interval of time (i.e., the present moment); everything else must be inferred from this information. The overall structure of the theory has some features in common with quantum Bayesianism, the Everett interpretation, and dynamical reduction models, but it differs significantly from all of these. The theory of information described here is largely qualitative, as the most important equations have not yet been solved. The quantitative level of agreement between theory and experiment thus remains an open question.

quant-ph↗
arXiv2007

Accurate quadratic-response approximation for the self-consistent pseudopotential of semiconductor nanostructures

Quadratic-response theory is shown to provide a conceptually simple but accurate approximation for the self-consistent one-electron potential of semiconductor nanostructures. Numerical examples are presented for GaAs/AlAs and InGaAs/InP (001) superlattices using the local-density approximation to density-functional theory and norm-conserving pseudopotentials without spin-orbit coupling. When the reference crystal is chosen to be the virtual-crystal average of the two bulk constituents, the absolute error in the quadratic-response potential for Gamma(15) valence electrons is about 2 meV for GaAs/AlAs and 5 meV for InGaAs/InP. Low-order multipole expansions of the electron density and potential response are shown to be accurate throughout a small neighborhood of each reciprocal lattice vector, thus providing a further simplification that is confirmed to be valid for slowly varying envelope functions. Although the linear response is about an order of magnitude larger than the quadratic response, the quadratic terms are important both quantitatively (if an accuracy of better than a few tens of meV is desired) and qualitatively (due to their different symmetry and long-range dipole effects).

cond-mat.mtrl-sci↗
arXiv2007

Unambiguous symmetry assignment for the top valence band of ZnO by magneto-optical studies of the free A-exciton state

We studied the circular polarization and angular dependences of the magneto-photoluminescence spectra of the free A-exciton 1S state in wurtzite ZnO at T = 5 K. The circular polarization properties of the spectra clearly indicate that the top valence band has Gamma_7 symmetry. The out-of-plane component of the magnetic field, which is parallel to the sample's c axis, leads to linear Zeeman splitting of both the dipole-allowed Gamma_5 exciton state and the weakly allowed Gamma_1/Gamma_2 exciton states. The in-plane field, which is perpendicular to the c axis, increases the oscillator strength of the weak Gamma_1/Gamma_2 states by forming a mixed exciton state.

cond-mat.mtrl-sci↗
arXiv2007

Choosing a basis that eliminates spurious solutions in k.p theory

A small change of basis in k.p theory yields a Kane-like Hamiltonian for the conduction and valence bands of narrow-gap semiconductors that has no spurious solutions, yet provides an accurate fit to all effective masses. The theory is shown to work in superlattices by direct comparison with first-principles density-functional calculations of the valence subband structure. A reinterpretation of the standard data-fitting procedures used in k.p theory is also proposed.

cond-mat.mtrl-sci↗
arXiv2007

Valence-band mixing in first-principles envelope-function theory

This paper presents a numerical implementation of a first-principles envelope-function theory derived recently by the author [B. A. Foreman, Phys. Rev. B 72, 165345 (2005)]. The examples studied deal with the valence subband structure of GaAs/AlAs, GaAs/Al(0.2)Ga(0.8)As, and In(0.53)Ga(0.47)As/InP (001) superlattices calculated using the local density approximation to density-functional theory and norm-conserving pseudopotentials without spin-orbit coupling. The heterostructure Hamiltonian is approximated using quadratic response theory, with the heterostructure treated as a perturbation of a bulk reference crystal. The valence subband structure is reproduced accurately over a wide energy range by a multiband envelope-function Hamiltonian with linear renormalization of the momentum and mass parameters. Good results are also obtained over a more limited energy range from a single-band model with quadratic renormalization. The effective kinetic-energy operator ordering derived here is more complicated than in many previous studies, consisting in general of a linear combination of all possible operator orderings. In some cases the valence-band Rashba coupling differs significantly from the bulk magnetic Luttinger parameter. The splitting of the quasidegenerate ground state of no-common-atom superlattices has non-negligible contributions from both short-range interface mixing and long-range dipole terms in the quadratic density response.

cond-mat.mtrl-sci↗
arXiv2005

Quadratic response theory for spin-orbit coupling in semiconductor heterostructures

This paper examines the properties of the self-energy operator in lattice-matched semiconductor heterostructures, focusing on nonanalytic behavior at small values of the crystal momentum, which gives rise to long-range Coulomb potentials. A nonlinear response theory is developed for nonlocal spin-dependent perturbing potentials. The ionic pseudopotential of the heterostructure is treated as a perturbation of a bulk reference crystal, and the self-energy is derived to second order in the perturbation. If spin-orbit coupling is neglected outside the atomic cores, the problem can be analyzed as if the perturbation were a local spin scalar, since the nonlocal spin-dependent part of the pseudopotential merely renormalizes the results obtained from a local perturbation. The spin-dependent terms in the self-energy therefore fall into two classes: short-range potentials that are analytic in momentum space, and long-range nonanalytic terms that arise from the screened Coulomb potential multiplied by a spin-dependent vertex function. For an insulator at zero temperature, it is shown that the electronic charge induced by a given perturbation is exactly linearly proportional to the charge of the perturbing potential. These results are used in a subsequent paper to develop a first-principles effective-mass theory with generalized Rashba spin-orbit coupling.

cond-mat.mtrl-sci↗
arXiv2005

First-principles envelope-function theory for lattice-matched semiconductor heterostructures

In this paper a multi-band envelope-function Hamiltonian for lattice-matched semiconductor heterostructures is derived from first-principles norm-conserving pseudopotentials. The theory is applicable to isovalent or heterovalent heterostructures with macroscopically neutral interfaces and no spontaneous bulk polarization. The key assumption -- proved in earlier numerical studies -- is that the heterostructure can be treated as a weak perturbation with respect to some periodic reference crystal, with the nonlinear response small in comparison to the linear response. Quadratic response theory is then used in conjunction with k.p perturbation theory to develop a multi-band effective-mass Hamiltonian (for slowly varying envelope functions) in which all interface band-mixing effects are determined by the linear response. To within terms of the same order as the position dependence of the effective mass, the quadratic response contributes only a bulk band offset term and an interface dipole term, both of which are diagonal in the effective-mass Hamiltonian. Long-range multipole Coulomb fields arise in quantum wires or dots, but have no qualitative effect in two-dimensional systems beyond a dipole contribution to the band offsets.

cond-mat.mtrl-sci↗
arXiv2005

First-principles effective-mass Hamiltonian for semiconductor nanostructures in a magnetic field

A multi-band effective-mass Hamiltonian is derived for lattice-matched semiconductor nanostructures in a slowly varying external magnetic field. The theory is derived from the first-principles magnetic-field coupling Hamiltonian of Pickard and Mauri, which is applicable to nonlocal norm-conserving pseudopotentials in the local density approximation to density functional theory. The pseudopotential of the nanostructure is treated as a perturbation of a bulk reference crystal, with linear and quadratic response terms included in k.p perturbation theory. The resulting Hamiltonian contains several interface terms that have not been included in previous work on nanostructures in a magnetic field. The derivation provides the first direct analytical expressions showing how the coupling of the nonlocal potential to the magnetic field influences the effective magnetic dipole moment of the electron.

cond-mat.mtrl-sci↗
arXiv2002

Consequences of local gauge symmetry in empirical tight-binding theory

A method for incorporating electromagnetic fields into empirical tight-binding theory is derived from the principle of local gauge symmetry. Gauge invariance is shown to be incompatible with empirical tight-binding theory unless a representation exists in which the coordinate operator is diagonal. The present approach takes this basis as fundamental and uses group theory to construct symmetrized linear combinations of discrete coordinate eigenkets. This produces orthogonal atomic-like "orbitals" that may be used as a tight-binding basis. The coordinate matrix in the latter basis includes intra-atomic matrix elements between different orbitals on the same atom. Lattice gauge theory is then used to define discrete electromagnetic fields and their interaction with electrons. Local gauge symmetry is shown to impose strong restrictions limiting the range of the Hamiltonian in the coordinate basis. The theory is applied to the semiconductors Ge and Si, for which it is shown that a basis of 15 orbitals per atom provides a satisfactory description of the valence bands and the lowest conduction bands. Calculations of the dielectric function demonstrate that this model yields an accurate joint density of states, but underestimates the oscillator strength by about 20% in comparison to a nonlocal empirical pseudopotential calculation.

cond-mat.mtrl-sci↗