arXiv subjects

Brant C. Gibson

Publications and source records attributed to Brant C. Gibson.

28 records · Page 2Linked to original sources

arXiv2016

Stimulated emission from NV centres in diamond

Stimulated emission is the process fundamental to laser operation, thereby producing coherent photon output. Despite negatively-charged nitrogen-vacancy (NV$^-$) centres being discussed as a potential laser medium since the 1980's, there have been no definitive observations of stimulated emission from ensembles of NV$^-$ to date. Reasons for this lack of demonstration include the short excited state lifetime and the occurrence of photo-ionisation to the neutral charge state by light around the zero-phonon line. Here we show both theoretical and experimental evidence for stimulated emission from NV$^-$ states using light in the phonon-sidebands. Our system uses a continuous wave pump laser at 532 nm and a pulsed stimulating laser that is swept across the phononic sidebands of the NV$^-$. Optimal stimulated emission is demonstrated in the vicinity of the three-phonon line at 700 nm. Furthermore, we show the transition from stimulated emission to photoionisation as the stimulating laser wavelength is reduced from 700nm to 620 nm. While lasing at the zero-phonon line is suppressed by ionisation, our results open the possibility of diamond lasers based on NV centres, tuneable over the phonon-sideband. This broadens the applications of NV magnetometers from single centre nanoscale sensors to a new generation of ultra-precise ensemble laser sensors, which exploit the contrast and signal amplification of a lasing system.

quant-ph↗

arXiv2016

Remote Nanodiamond Magnetometry

Optical fibres have transformed the way people interact with the world and now permeate many areas of science. Optical fibres are traditionally thought of as insensitive to magnetic fields, however many application areas from mining to biomedicine would benefit from fibre-based remote magnetometry devices. In this work, we realise such a device by embedding nanoscale magnetic sensors into tellurite glass fibres. Remote magnetometry is performed on magnetically active defect centres in nanodiamonds embedded into the glass matrix. Standard optical magnetometry techniques are applied to initialize and detect local magnetic field changes with a measured sensitivity of 26 micron Tesla/square root(Hz). Our approach utilizes straight-forward optical excitation, simple focusing elements, and low power components. We demonstrate remote magnetometry by direct reporting of the magnetic ground states of nitrogen-vacancy defect centres in the optical fibres. In addition, we present and describe theoretically an all-optical technique that is ideally suited to remote fibre-based sensing. The implications of our results broaden the applications of optical fibres, which now have the potential to underpin a new generation of medical magneto-endoscopes and remote mining sensors.

physics.optics↗

arXiv2015

Enhanced photoluminescence from single nitrogen-vacancy defects in nanodiamonds coated with metal-phenolic networks

Fluorescent nanodiamonds are attracting major attention in the field of bio-sensing and biolabeling. In this work we demonstrate a robust approach to surface functionalize individual nanodiamonds with metal-phenolic networks that enhance the photoluminescence from single nitrogen vacancy (NV) centers. We show that single NV centres in the coated nanodiamonds also exhibit shorter lifetimes, opening another channel for high resolution sensing. We propose that the nanodiamond encapsulation suppresses the non-radiative decay pathways of the NV color centers. Our results provide a versatile and assessable way to enhance photoluminescence from nanodiamond defects that can be used in a variety of sensing and imaging applications

physics.optics↗

arXiv2014

Nanodiamond in tellurite glass Part II: practical nanodiamond-doped fibers

Tellurite glass fibers with embedded nanodiamond are attractive materials for quantum photonics applications. Reducing the loss of these fibers in the 600-800 nm wavelength range of nanodiamond fluorescence is essential to exploit the unique properties of nanodiamond in the new hybrid material. The first part of this study reported the origin of loss in nanodiamond-doped glass and impact of glass fabrication conditions. Here, we report the fabrication of nanodiamond-doped tellurite fibers with significantly reduced loss in the visible through further understanding of the impact of glass fabrication conditions on the interaction of the glass melt with the embedded nanodiamond. We fabricated tellurite fibers containing nanodiamond in concentrations up to 0.7 ppm-weight, while reducing the loss by more than an order of magnitude down to 10 dB/m at 600-800 nm.

physics.optics↗

arXiv2014

Nanodiamond in tellurite glass Part I: origin of loss in nanodiamond-doped glass

Tellurite glass fibers with embedded nanodiamond are attractive materials for quantum photonic applications. Reducing the loss of these fibers in the 600-800 nm wavelength range of nanodiamond fluorescence is essential to exploit the unique properties of nanodiamond in the new hybrid material. In the first part of this study, we report the effect of interaction of the tellurite glass melt with the embedded nanodiamond on the loss of the glasses. The glass fabrication conditions such as melting temperature and concentration of NDs added to the melt were found to have critical influence on the interaction. Based on this understanding, we identified promising fabrication conditions for decreasing the loss to levels required for practical applications.

physics.optics↗

arXiv2014

Near orthogonal launch of SPR modes in Au films

We report the excitation of a surface plasmon resonance (SPR) close to the orthogonal axis of a gold (Au) film on borosilicate glass. Direct spectroscopic measurement of SPR shifts using different liquids are made at ~5° incidence within a reflection spectrophotometer. Scattering of light that is able to penetrate across the film at the interfaces is the proposed mechanism by which coupling, and plasmon localization, is established.

physics.optics↗

arXiv2012

Room temperature self-assembly of mixed nanoparticles into complex material systems and devices

The ability to manufacture nanomaterials with complex and structured composition using otherwise incompatible materials increasingly underpins the next generation of technologies. This is translating into growing efforts integrating a wider range of materials onto key technology platforms1 - in photonics, one such platform is silica, a passive, low loss and robust medium crucial for efficient optical transport2. Active functionalisation, either through added gain or nonlinearity, is mostly possible through the integration of active materials3, 4. The high temperatures used in manufacturing of silica waveguides, unfortunately, make it impossible to presently integrate many organic and inorganic species critical to achieving this extended functionality. Here, we demonstrate the fabrication of novel waveguides and devices made up of complex silica based materials using the self-assembly of nanoparticles. In particular, the room temperature fabrication of silica microwires integrated with organic dyes (Rhodamine B) and single photon emitting nanodiamonds is presented.

cond-mat.mtrl-sci↗

arXiv2010

Coupling slot-waveguide cavities for large-scale quantum optical devices

By offering effective modal volumes significantly less than a cubic wavelength, slot-waveguide cavities offer a new in-road into strong atom-photon coupling in the visible regime. Here we explore two-dimensional arrays of coupled slot cavities which underpin designs for novel quantum emulators and polaritonic quantum phase transition devices. Specifically, we investigate the lateral coupling characteristics of diamond-air and GaP-air slot waveguides using numerically-assisted coupled-mode theory, and the longitudinal coupling properties via distributed Bragg reflectors using mode-propagation simulations. We find that slot-waveguide cavities in the Fabry-Perot arrangement can be coupled and effectively treated with a tight-binding description, and are a suitable platform for realizing Jaynes-Cummings-Hubbard physics.

quant-ph↗

arXiv2009

Slot-waveguide cavities for optical quantum information applications

To take existing quantum optical experiments and devices into more practical regimes requires the construction of robust, solid-state implementations. In particular, to observe the strong-coupling regime of atom-photon interactions requires very small cavities and large quality factors. Here we show that the slot-waveguide geometry recently introduced for photonic applications is also promising for quantum optical applications in the visible regime. We study diamond- and GaP-based slot-waveguide cavities (SWCs) compatible with diamond colour centres e.g. nitrogen-vacancy (NV) defect, and show that one can achieve increased single-photon Rabi frequencies of order O(10^11) Hz in ultra-small cavity modal volumes, nearly 2 orders of magnitude smaller than previously studied diamond-based photonic crystal cavities.

quant-ph↗

arXiv2006

Coherent Population Trapping in Diamond N-V Centers at Zero Magnetic Field

Coherent population trapping at zero magnetic field was observed for nitrogen-vacancy centers in diamond under optical excitation. This was measured as a reduction in photoluminescence when the detuning between two excitation lasers matched the 2.88 GHz crystal-field splitting of the color center ground states. This behavior is highly sensitive to strain, which modifies the excited states, and was unexpected following recent experiments demonstrating optical readout of single nitrogen-vacancy electron spins based on cycling transitions. These results demonstrate for the first time that three-level Lambda configurations suitable for proposed quantum information applications can be realized simultaneously for all four orientations of nitrogen-vacancy centers at zero magnetic field.

cond-mat.mes-hall↗