arXiv subjects

Brian B. Maranville

Publications and source records attributed to Brian B. Maranville.

15 recordsLinked to original sources

arXiv2025

Net Magnetization and Inhomogeneous Magnetic Order in a High-Tc Nickelate Superconductor

High-temperature and high-magnetic-field-induced re-entrant superconductivity has been discovered in the infinite-layer nickelate $\mathrm{Sm_{1-x-y} Eu_x Ca_y Ni O_2}$ (SECNO). Infinite-layer nickelates are the closest known analogues of high-$\mathrm{T}_c$ cuprate superconductors, yet they host distinct magnetic ground states. Using low-energy muon spin relaxation and polarized neutron reflectometry, we reveal the magnetic order in SECNO. We find that magnetic freezing occurs at a higher-temperature than in other nickelate compounds, and that a substantial net magnetization of 55 $\,\mathrm{kA}\,\mathrm{m}^{-1}$ $\pm10 \,\mathrm{kA}\,\mathrm{m}^{-1}$ emerges and remains largely unchanged across the superconducting transition. The magnetism in SECNO is disordered and nonuniform.

cond-mat.supr-con↗

arXiv2025

Complex Magnetic Ordering in Candidate Topological Superconductors

The search for chiral topological superconductivity in magnetic topological insulator (TI)-FeTe heterostructures is a key frontier in condensed matter physics, with potential applications in topological quantum computing. The combination of ferromagnetism, superconductivity, and topologically nontrivial surface states brings together the key elements required for chiral Majorana physics. In this work, we examine the interplay between magnetism and superconductivity at the interfaces between FeTe and a series of TI overlayers. In superconducting MnBi$_2$Te$_4$/FeTe, any interfacial suppression of antiferromagnetism must affect at most a few nanometers. On the other hand, (Bi,Sb)$_2$Te$_3$/FeTe layers exhibit near-total suppression of antiferromagnetic ordering. Ferromagnetic Cr$_x$(Bi,Sb)$_{2-x}$Te$_3$ (CBST)/FeTe bilayers exhibit net magnetization in both CBST and FeTe layers, with evidence of interactions between superconductivity and ferromagnetism. These observations identify magnetic TI/FeTe interfaces as an exceptionally robust platform to realize chiral topological superconductivity.

cond-mat.supr-con↗

arXiv2023

Three-Dimensional Structure of Hybrid Magnetic Skyrmions Determined by Neutron Scattering

Magnetic skyrmions are topologically protected chiral spin textures which present opportunities for next-generation magnetic data storage and logic information technologies. The topology of these structures originates in the geometric configuration of the magnetic spins - more generally described as the structure. While the skyrmion structure is most often depicted using a 2D projection of the three-dimensional structure, recent works have emphasized the role of all three dimensions in determining the topology and their response to external stimuli. In this work, grazing-incidence small-angle neutron scattering and polarized neutron reflectometry are used to determine the three-dimensional structure of hybrid skyrmions. The structure of the hybrid skyrmions, which includes a combination of Néel-like and Bloch-like components along their length, is expected to significantly contribute to their notable stability, which includes ambient conditions. To interpret the neutron scattering data, micromagnetic simulations of the hybrid skyrmions were performed, and the corresponding diffraction patterns were determined using a Born approximation transformation. The converged magnetic profile reveals the magnetic structure along with the skyrmion depth profile, including the thickness of the Bloch and Néel segments and the diameter of the core.

cond-mat.mes-hall↗

arXiv2022

Exchange-biased quantum anomalous Hall effect

The quantum anomalous Hall (QAH) effect is characterized by a dissipationless chiral edge state with a quantized Hall resistance at zero magnetic field. Manipulating the QAH state is of great importance in both the understanding of topological quantum physics and the implementation of dissipationless electronics. Here, we realized the QAH effect in the magnetic topological insulator Cr-doped (Bi,Sb)2Te3 (CBST) grown on an uncompensated antiferromagnetic insulator Al-doped Cr2O3. Through polarized neutron reflectometry (PNR), we find a strong exchange coupling between CBST and Al-Cr2O3 surface spins fixing interfacial magnetic moments perpendicular to the film plane. The interfacial coupling results in an exchange-biased QAH effect. We further demonstrate that the magnitude and sign of the exchange bias can be effectively controlled using a field training process to set the magnetization of the Al-Cr2O3 layer. Our work demonstrates the use of the exchange bias effect to effectively manipulate the QAH state, opening new possibilities in QAH-based spintronics.

cond-mat.mes-hall↗

arXiv2022

Chiral Spin Bobbers in Exchange-Coupled Hard-Soft Magnetic Bilayers

The spin structure of exchange-coupled MnBi:Co-Fe bilayers is investigated by X-ray magnetic circular dichroism (XMCD), polarized neutron reflectometry (PNR), and micromagnetic simu-lations. The purpose of the present research is two-fold. First, the current search for new permanent-magnet materials includes hard-soft nanocomposites, and the analysis of coercivity mechanisms in these structures is an important aspect of this quest. Second, topological micro-magnetic structures such as skyrmions have recently become of intense fundamental and applied research, for example in the context of spin-based electronics. We find that the magnetization reversal of the MnBi:Co-Fe bilayer structure involves a curling-type twisting of the magnetization in the film plane. This curling in the exchange-coupled hard-soft magnetic bilayers is reminiscent of chiral spin structures known as bobbers and, in fact, establishes a new type of skyrmionic spin structure.

cond-mat.mtrl-sci↗

arXiv2021

An implementation of an efficient direct Fourier transform of polygonal areas and volumes

Calculations of the Fourier transform of a constant quantity over an area or volume defined by polygons (connected vertices) are often useful in modeling wave scattering, or in fourier-space filtering of real-space vector-based volumes and area projections. If the system is discretized onto a regular array, Fast Fourier techniques can speed up the resulting calculations but if high spatial resolution is required the initial step of discretization can limit performance; at other times the discretized methods result in unacceptable artifacts in the resulting transform. An alternative approach is to calculate the full Fourier integral transform of a polygonal area as a sum over the vertices, which has previously been derived in the literature using the divergence theorem to reduce the problem from a 3-dimensional to line integrals over the perimeter of the polygon surface elements, and converted to a sum over the straight segments of that contour. We demonstrate a software implementation of this algorithm and show that it can provide accurate approximations of the Fourier transform of real shapes with faster convergence than a block-based (voxel) discretization.

math.NA↗

arXiv2020

Layering of magnetic nanoparticles at amorphous magnetic templates with perpendicular anisotropy

We reveal the assembly of monodisperse magnetite nanoparticles of sizes 5 nm, 15 nm and 25 nm from dilute water-based ferrofluids onto an amorphous magnetic template with out-of-plane anisotropy. From neutron reflectometry experiments we extract density profiles and show that the particles self-assemble into layers at the magnetic surface. The layers are extremely stable against cleaning and rinsing of the substrate. The density of the layers is determined by and increases with the remanent magnetic moment of the particles.

cond-mat.soft↗

arXiv2018

Precipitating Ordered Skyrmion Lattices from Helical Spaghetti

Magnetic skyrmions have been the focus of intense research due to their potential applications in ultra-high density data and logic technologies, as well as for the unique physics arising from their antisymmetric exchange term and topological protections. In this work we prepare a chiral jammed state in chemically disordered (Fe, Co)Si consisting of a combination of randomly-oriented magnetic helices, labyrinth domains, rotationally disordered skyrmion lattices and/or isolated skyrmions. Using small angle neutron scattering, (SANS) we demonstrate a symmetry-breaking magnetic field sequence which disentangles the jammed state, resulting in an ordered, oriented skyrmion lattice. The same field sequence was performed on a sample of powdered Cu2OSeO3 and again yields an ordered, oriented skyrmion lattice, despite relatively non-interacting nature of the grains. Micromagnetic simulations confirm the promotion of a preferred skyrmion lattice orientation after field treatment, independent of the initial configuration, suggesting this effect may be universally applicable. Energetics extracted from the simulations suggest that approaching a magnetic hard axis causes the moments to diverge away from the magnetic field, increasing the Dzyaloshinskii-Moriya energy, followed subsequently by a lattice re-orientation. The ability to facilitate an emergent ordered magnetic lattice with long-range orientation in a variety of materials despite overwhelming internal disorder enables the study of skyrmions even in imperfect powdered or polycrystalline systems and greatly improves the ability to rapidly screen candidate skyrmion materials.

cond-mat.mes-hall↗

arXiv2018

Ionic Tuning of Cobaltites at the Nanoscale

Control of materials through custom design of ionic distributions represents a powerful new approach to develop future technologies ranging from spintronic logic and memory devices to energy storage. Perovskites have shown particular promise for ionic devices due to their high ion mobility and sensitivity to chemical stoichiometry. In this work, we demonstrate a solid-state approach to control of ionic distributions in (La,Sr)CoO$_{3}$ thin films. Depositing a Gd capping layer on the perovskite film, oxygen is controllably extracted from the structure, up-to 0.5 O/u.c. throughout the entire 36 nm thickness. Commensurate with the oxygen extraction, the Co valence state and saturation magnetization show a smooth continuous variation. In contrast, magnetoresistance measurements show no-change in the magnetic anisotropy and a rapid increase in the resistivity over the same range of oxygen stoichiometry. These results suggest significant phase separation, with metallic ferromagnetic regions and oxygen-deficient, insulating, non-ferromagnetic regions, forming percolated networks. Indeed, X-ray diffraction identifies oxygen-vacancy ordering, including transformation to a brownmillerite crystal structure. The unexpected transformation to the brownmillerite phase at ambient temperature is further confirmed by high-resolution scanning transmission electron microscopy which shows significant structural - and correspondingly chemical - phase separation. This work demonstrates room-temperature ionic control of magnetism, electrical resistivity, and crystalline structure in a 36 nm thick film, presenting new opportunities for ionic devices that leverage multiple material functionalities.

cond-mat.mtrl-sci↗

arXiv2018

Distributed Error-Function Roughness in Refl1d Reflectometry Fitting Program

The Refl1d program is used for modeling and fitting data from neutron and X-ray reflectometry experiments. The model of the (thin-film) samples is typically constructed of discrete layers of different scattering-length densities (SLD). Interlayer roughness is represented as an error-function transition from one layer to the next. Previous versions of the software truncated this error-function at the next interface. This strategy has the advantage of preventing layers with unbounded effective extent, but it can also result in SLD depth profiles that do not conform to the physical expectations of the users (such as introducing sharp transitions) whenever the layer roughness approaches the thickness of the layer. In this article we introduce a new version of the software in which the option is provided to extend the roughness of each layer over the entire structure; the resulting SLD profiles often more closely resemble the physical models intended by the user. Most importantly no sharp transitions are introduced by truncating the roughness, when a smooth transition is often desired when adding rough layers together.

physics.comp-ph↗

arXiv2016

Beyond the Interface Limit: Structural and Magnetic Depth Profiles of Voltage-Controlled Magneto-Ionic Heterostructures

Electric-field control of magnetism provides a promising route towards ultralow power information storage and sensor technologies. The effects of magneto-ionic motion have so far been prominently featured in the direct modification of interface chemical and physical characteristics. Here we demonstrate magnetoelectric coupling moderated by voltage-driven oxygen migration beyond the interface limit in relatively thick AlOx/GdOx/Co (15 nm) films. Oxygen migration and its ramifications on the Co magnetization are quantitatively mapped with polarized neutron reflectometry under thermal and electro-thermal conditionings. The depth-resolved profiles uniquely identify interfacial and bulk behaviors and a semi-reversible suppression and recovery of the magnetization. Magnetometry measurements show that the conditioning changes the microstructure so as to disrupt long-range ferromagnetic ordering, resulting in an additional magnetically soft phase. X-ray spectroscopy confirms electric field induced changes in the Co oxidation state but not in the Gd, suggesting that the GdOx transmits oxygen but does not source or sink it. These results together provide crucial insight into controlling magnetic heterostructures via magneto-ionic motion, not only at the interface, but also throughout the bulk of the films.

cond-mat.mes-hall↗

arXiv2016

Measurement and modeling of polarized specular neutron reflectivity in large magnetic fields

The presence of a large applied magnetic field removes the degeneracy of the vacuum energy states for spin-up and spin-down neutrons. For polarized neutron reflectometry, this must be included in the reference potential energy of the Schrödinger equation that is used to calculate the expected scattering from a magnetic layered structure. For samples with magnetization that is purely parallel or antiparallel to the applied field which defines the quantization axis, there is no mixing of the spin states (no spin-flip scattering) and so this additional potential is constant throughout the scattering region. When there is non-collinear magnetization in the sample however, there will be significant scattering from one spin state into the other and the reference potentials will differ between the incoming and outgoing wavefunctions, changing the angle and intensities of the scattering. The theory of the scattering and recommended experimental practices for this type of measurement are presented, as well as an example measurement.

cond-mat.mtrl-sci↗

arXiv2014

Determination of the effective transverse coherence of the neutron wave packet as employed in reflectivity investigations of condensed matter structures Part I: Measurements

The primary purpose of this investigation is to determine the effective coherent extent of the neutron wave packet transverse to its mean propagation vector k, when it is prepared in a typical instrument used to study the structure of materials in thin film form via specular reflection. There are two principal reasons for doing so. One has to do with the fundamental physical interest in the characteristics of a free neutron as a quantum object while the other is of a more practical nature, relating to the understanding of how to interpret elastic scattering data when the neutron is employed as a probe of condensed matter structure on an atomic or nanometer scale. Knowing such a basic physical characteristic as the neutron's effective transverse coherence can dictate how to properly analyze specular reflectivity data obtained for material film structures possessing some amount of in-plane inhomogeneity. In this study we describe a means of measuring the effective transverse coherence length of the neutron wave packet by specular reflection from a series of diffraction gratings of different spacings. Complementary non-specular measurements of the widths of grating reflections were also performed which corroborate the specular results. (Part I principally describes measurements interpreted according to the theoretical picture presented in Part II.) Each grating was fabricated by lift-off photo-lithography patterning of a nickel film (approximately 1000 Angstroms thick) formed by physical vapor deposition on a flat silicon crystal surface. The grating periods ranged from 10 microns (5 microns Ni stripe, 5 microns intervening space) to several hundred microns. The transverse coherence length, modeled as the width of the wave packet, was determined from an analysis of the specular reflectivity curves of the set of gratings.

cond-mat.mtrl-sci↗

arXiv2011

3D Spatially Resolved Neutron Diffraction from a Disordered Vortex Lattice

The vortex matter in bulk type-II superconductors serves as a prototype system for studying the random pinning problem in condensed matter physics. Since the vortex lattice is embedded in an atomic lattice, small angle neutron scattering (SANS) is the only technique that allows for direct structural studies. In traditional SANS methods, the scattering intensity is a measure of the structure factor averaged over the entire sample. Recent studies in vortex physics have shown that it is highly desirable to develop a SANS technique which is capable of resolving the spatial inhomogeneities in the bulk vortex state. Here we report a novel slicing neutron diffraction technique using atypical collimation and an areal detector which allows for observing the three dimensional (3D) disorder of the vortex matter inside an as-grown Nb single crystal.

cond-mat.mtrl-sci↗

arXiv2011

Direct Evidence for Edge-Contaminated Vortex Phase in a Nb Single Crystal using Neutron Diffraction

We report the first direct observation of a disordered vortex matter phase existing near the edge of a bulk type-II superconductor Nb using a novel position-sensitive neutron diffraction technique. This "edge-contaminated" vortex state was implicated in previous studies using transport techniques and was postulated to have played a significant role in the behavior of vortex dynamics in a wide range of type-II superconductors. It is found that upon thermal annealing, the vortex matter in the bulk undergoes re-ordering, suggesting that the edge-contaminated bulk vortex state is metastable. The edge vortex state remains disordered after repeated thermal annealing, indicating spatial coexistence of a vortex glass with a Bragg glass. This observation resolves many outstanding issues concerning the peak effect in type-II superconductors.

cond-mat.supr-con↗