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Brian J. Smith

Publications and source records attributed to Brian J. Smith.

At least 19 recordsLinked to original sources

High-fidelity, quasi-deterministic entanglement generation using phase-matched spectral islands in a zero-added-loss multiplexing architecture

Spontaneous parametric down-converters (SPDCs) are the best available entanglement sources for distributing entanglement in a quantum internet. However, their intrinsically probabilistic nature, and their need to operate at low brightness to suppress multipair events, dictate that multiplexed SPDC arrays are required for high-rate distribution in that application. Early SPDC multiplexing proposals involved path switching, whose switching losses significantly degrade performance. The present paper proposes and analyzes a scheme for spectral multiplexing that provides entanglement-distribution rates well in excess of the state of the art. It builds on zero-added-loss multiplexing (ZALM)~[Phys. Rev. Appl. {\bf 19}, 054029 (2023)] for high-rate heralded entanglement generation, which does not require a switched array of SPDCs. Our ZALM's SPDCs rely on nonlinear crystals with $N_I$ phase-matched spectral islands, each generating two-mode squeezed-vacuum states. Also, our ZALM's multiplexing protocol uses both same-island and cross-island heralding, which allows the entanglement-delivery rate to approximately scale as $N_I^2$ in the realistic weak-squeezing regime. As a result, our scheme uses an order of magnitude fewer spectral channels than the original ZALM proposal, which may enable near-term implementations of satellite-to-ground or fiber-optic based ZALM architectures.

quant-ph

Entanglement source and quantum memory analysis for zero added-loss multiplexing

High-rate, high-fidelity entanglement distribution is essential to the creation of a quantum internet, but recent achievements in fiber and satellite-based entanglement distribution fall far short of what is needed. Chen et al. [Phys. Rev. Appl. 19, 054209 (2023)] proposed a means for dramatically increasing entanglement-distribution rates via zero added-loss multiplexing (ZALM). ZALM's quantum transmitter employs a pair of Sagnac-configured spontaneous parametric downconverters (SPDCs), channelization via dense wavelength-division multiplexing (DWDM) filtering, and partial Bell-state measurements (BSMs) to realize a heralded source of frequency-multiplexed polarization-entangled biphotons. Each biphoton is transmitted to Alice and Bob with a classical message identifying its frequency channel and the heralded entangled state. Their quantum receivers use DWDM filtering and mode conversion to interface their received biphotons to intra-cavity color-center quantum memories. This paper delves deeply into ZALM's SPDCs, partial-BSMs, and loading of Alice and Bob's quantum memories. It derives the density operators for the SPDC sources and the quantum memories, allowing heralding probability, heralding efficiency, and fidelity to be evaluated for both the polarization-entangled biphotons and the loaded quantum memories, thus enabling exploration of the parameter space for optimizing ZALM performance. Even without optimization analysis, the paper already demonstrates two critical features of the ZALM architecture: the necessity of achieving a near-separable channelized biphoton wave function to ensure the biphoton sent to Alice and Bob is of high purity; and the premium placed on Alice and Bob's temporal-mode converters' enabling narrowband push-pull memory loading to ensure the arriving biphoton's state is faithfully transferred to the intra-cavity color centers.

quant-ph

Limitations in Fluorescence-Detected Entangled Two-Photon-Absorption Experiments: Exploring the Low- to High-Gain Squeezing Regimes

We closely replicated and extended a recent experiment ("Spatial properties of entangled two-photon absorption," Phys. Rev. Lett. 129, 183601, 2022) that reportedly observed enhancement of two-photon absorption rates in molecular samples by using time-frequency-entangled photon pairs, and we found that in the low-flux regime, where such enhancement is theoretically predicted in-principle, the two-photon fluorescence signal is below detection threshold using current state-of-the-art methods. The results are important in the context of efforts to enable quantum-enhanced molecular spectroscopy and imaging at ultra-low optical flux. Using an optical parametric down-conversion photon-pair source that can be varied from the low-gain spontaneous regime to the high-gain squeezing regime, we observed two-photon-induced fluorescence in the high-gain regime but in the low-gain regime any fluorescence was below detection threshold. We supplemented the molecular fluorescence experiments with a study of nonlinear-optical sum-frequency generation, for which we are able to observe the low-to-high-gain crossover, thereby verifying our theoretical models and experimental techniques. The observed rates (or lack thereof) in both experiments are consistent with theoretical predictions and with our previous experiments, and indicate that time-frequency photon entanglement does not provide a practical means to enhance in-solution molecular two-photon fluorescence spectroscopy or imaging with current techniques.

quant-ph

Interferometric imaging using shared quantum entanglement

Quantum entanglement-based imaging promises significantly increased resolution by extending the spatial separation of optical collection apertures used in very-long-baseline interferometry for astronomy and geodesy. We report a table-top entanglement-based interferometric imaging technique that utilizes two entangled field modes serving as a phase reference between two apertures. The spatial distribution of a simulated thermal light source is determined by interfering light collected at each aperture with one of the entangled fields and performing joint measurements. This experiment demonstrates the ability of entanglement to implement interferometric imaging.

quant-ph

Smartphone-based measurements of the optical properties of snow

Snow is a highly complex medium composed of ice crystals of various shapes and sizes. Knowledge of its intrinsic optical properties such as the scattering and absorption coefficient is tantamount to radiative transfer models in climate research. The absorption coefficient, in particular, allows us to access information about light-absorbing particles contained in the snow. In contrast to snow's apparent properties like the albedo, measuring the intrinsic properties is challenging. Here, we present a simple apparatus that can measure bulk optical properties of snow using readily available components and a smartphone camera, and a robust diffuse-optical framework for data analysis. We demonstrate the instrument both on scattering phantoms with known scattering and absorption coefficient as well as in the field. Its low cost, simplicity and portability uniquely qualify this setup for large-scale field work, undergraduate education and citizen science.

physics.ins-det

Direct measurement of optical properties of glacier ice using a photon-counting diffuse LiDAR

The production of meltwater from glacier ice, which is exposed at the margins of land ice during the summer, is responsible for a large proportion of glacier mass loss. The rate of meltwater production from glacier ice is especially sensitive to its physical structure and chemical composition which combine to determine the albedo of glacier ice. However, the optical properties of near-surface glacier ice are not well known since most prior work has focused on ice made in the laboratory or from deep cores. Here, we demonstrate a measurement technique based on diffuse propagation of nanosecond-duration laser pulses in near-surface glacier ice that enables the independent measurement of the scattering and absorption coefficients, allowing for a complete description of the processes governing radiative transfer. We employ a photon-counting detector to overcome the high losses associated with diffuse optics. The instrument is highly portable and rugged, making it optimally suited for deployment in remote regions. A set of measurements taken on Collier Glacier, Oregon, serves as a demonstration of the technique. These measurements provide insight into both physical structure and composition of near-surface glacier ice and open new avenues for the analysis of light-absorbing impurities and remote sensing of the cryosphere.

physics.optics

Quantum-enhanced interferometry by entanglement-assisted rejection of environmental noise

Sensing and measurement tasks in severely adverse conditions such as loss, noise and dephasing can be improved by illumination with quantum states of light. Previous results have shown a modest reduction in the number of measurements necessary to achieve a given precision. Here, we compare three illumination strategies for estimating the relative phase in a noisy, lossy interferometer. When including a common phase fluctuation in the noise processes, we show that using an entangled probe achieves an advantage in parameter estimation precision that scales with the number of entangled modes. This work provides a theoretical foundation for the use of highly multimode entangled states of light for practical measurement tasks in experimentally challenging conditions.

quant-ph

Diffuse optics for glaciology

Optical probing of glaciers has the potential for tremendous impact on environmental science. However, glacier ice is turbid, which prohibits the use of most established optical measurements for determining a glacier's interior structure. Here, we propose a method for determining the depth, scattering and absorption length based upon diffuse propagation of short optical pulses. Our model allows us to extract several characteristics of the glacier. Performing Monte Carlo simulations implementing Mie scattering and mixed boundary conditions, we show that the proposed approach should be feasible with current technology. The results suggest that optical properties and geometry of the glacier can be extracted from realistic measurements, which could be implemented with low cost and small footprint.

physics.optics

Gaussian versus non-Gaussian filtering of phase-insensitive nonclassicality

Measures of quantum properties are essential to understanding the fundamental differences between quantum and classical systems as well as quantifying resources for quantum technologies. Here two broad classes of bosonic phase-space functions, which are filtered versions of the Glauber-Sudarshan $P$ function, are compared with regard to their ability to uncover nonclassical effects of light through their negativities. Gaussian filtering of the $P$ function yields the family of $s$-parametrized quasiprobabilities, while more powerful regularized nonclassicality quasiprobabilities are obtained by non-Gaussian filtering. A method is proposed to directly sample such phase-space functions for the restricted case of phase-independent quantum states from balanced homodyne measurements. This overcomes difficulties of previous approaches that manually append uniformly distributed optical phases to the measured quadrature data. We experimentally demonstrate this technique for heralded single- and two-photon states using balanced homodyne detection with varying efficiency. The $s$-parametrized quasiprobabilities, which can be directly sampled, are non-negative for detection efficiencies below 0.5. By contrast, we show that significant negativities of non-Gaussian filtered quasiprobabilities uncover nonclassical effects even for low efficiencies.

quant-ph

Spectrally-resolved four-photon interference of time-frequency entangled photons

Pairs of photons entangled in their time-frequency degree of freedom are of great interest in quantum optics research and applications, due to their relative ease of generation and their high capacity for encoding information. Here we analyze, both theoretically and experimentally, the behavior of phase-insensitive spectrally-resolved interferences arising from two pairs of time-frequency entangled photons. At its core, this is a multimode entanglement swapping experiment, whereby a spectrally resolved joint measurement on the idler photons from both pairs results in projecting the signal photons onto a Bell state whose form depends on the measurement outcome. Our analysis is a thorough exploration of what can be achieved using time-frequency entanglement and spectrally-resolved Bell-state measurements.

quant-ph

A positive operator-valued measure for two-photon detection via sum-frequency generation

Spontaneous parametric down conversion (PDC), in the perturbative limit, can be considered as a probabilistic splitting of one input photon into two output photons. Conversely, sum-frequency generation (SFG) implements the reverse process of combining two input photons into one. Here we show that a single-photon projective measurement in the temporal-mode basis of the output photon of a two-photon SFG process effects a generalized measurement on the input two-photon state. We describe the positive-operator-valued measure (POVM) associated with such a measurement, and show that its elements are proportional to the two-photon states produced by the time-reversed PDC process. Such a detection acts as a joint measurement on two photons, and is thus an important component of many quantum information processing protocols relying on photonic entanglement. Using the retrodictive approach, we analyze the properties of the two-photon POVM that are relevant for quantum protocols exploiting two-photon states and measurements.

quant-ph

Quantifying the enhancement of two-photon absorption due to spectral-temporal entanglement

When a low flux of time-frequency-entangled photon pairs (EPP) illuminates a two-photon transition, the rate of two-photon absorption (TPA) can be enhanced considerably by the quantum nature of photon number correlations and frequency correlations. We present a quantum-theoretic derivation of entangled TPA (ETPA) and calculate an upper bound on the amount of quantum enhancement that is possible in such systems. The derived bounds indicate that in order to observe ETPA the experiments would need to operate at a combination of significantly higher rates of EPP illumination, molecular concentrations, and conventional TPA cross sections than are achieved in typical experiments.

quant-ph

Heralding multiple photonic pulsed Bell-pairs via frequency-resolved entanglement swapping

Entanglement is a unique property of quantum systems and an essential resource for many quantum technologies. The ability to transfer or swap entanglement between systems is an important protocol in quantum information science. Entanglement between photons forms the basis of distributed quantum networks and the demonstration of photonic entanglement swapping is essential for their realization. Here an experiment demonstrating entanglement swapping from two independent multimode time-frequency entangled sources is presented, resulting in multiple heralded temporal-mode Bell states. Entanglement in the heralded states is verified by measuring conditional anti-correlated joint spectra as well as quantum beating in two-photon interference. Our proof-of-concept experiment is able to distinguish up to five orthogonal Bell pairs within the same setup, limited in principle only by the entanglement of the sources.

quant-ph

Experimental feasibility of molecular two-photon absorption with isolated time-frequency-entangled photon pairs

Entangled photon pairs have been promised to deliver a substantial quantum advantage for two-photon absorption spectroscopy. However, recent work has challenged the previously reported magnitude of quantum enhancement in two-photon absorption. Here, we present an experimental comparison of sum-frequency generation and molecular absorption, each driven by isolated photon pairs. We establish an upper bound on the enhancement for entangled-two-photon absorption in Rhodamine-6G, which lies well below previously reported values.

quant-ph

Two-photon absorption of time-frequency-entangled photon pairs by molecules: the roles of photon-number correlations and spectral correlations

While two-photon absorption (TPA) and other forms of nonlinear interactions of molecules with isolated time-frequency-entangled photon pairs (EPP) have been predicted to display a variety of fascinating effects, their potential use in practical quantum-enhanced molecular spectroscopy requires close examination. This paper presents a detailed theoretical study of quantum-enhanced TPA by both photon-number correlations and spectral correlations, including an account of the deleterious effects of dispersion. While such correlations in EPP created by spontaneous parametric down conversion can increase the TPA rate significantly in the regime of extremely low optical flux, we find that for typical molecules in solution this regime corresponds to such low TPA event rates as to be unobservable in practice. Our results support the usefulness of EPP spectroscopy in atomic or other narrow-linewidth systems, while questioning the efficacy of such approaches for broadband systems including molecules in solution.

quant-ph

Temporal mode transformations by sequential time and frequency phase modulation for applications in quantum information science

Controlling the temporal mode shape of quantum light pulses has wide ranging application to quantum information science and technology. Techniques have been developed to control the bandwidth, allow shifting in the time and frequency domains, and perform mode-selective beam-splitter-like transformations. However, there is no present scheme to perform targeted multimode unitary transformations on temporal modes. Here we present a practical approach to realize general transformations for temporal modes. We show theoretically that any unitary transformation on temporal modes can be performed using a series of phase operations in the time and frequency domains. Numerical simulations show that several key transformations on temporal modes can be performed with greater than 95% fidelity using experimentally feasible specifications.

physics.optics

Deep segmentation networks predict survival of non-small cell lung cancer

Non-small-cell lung cancer (NSCLC) represents approximately 80-85% of lung cancer diagnoses and is the leading cause of cancer-related death worldwide. Recent studies indicate that image-based radiomics features from positron emission tomography-computed tomography (PET/CT) images have predictive power on NSCLC outcomes. To this end, easily calculated functional features such as the maximum and the mean of standard uptake value (SUV) and total lesion glycolysis (TLG) are most commonly used for NSCLC prognostication, but their prognostic value remains controversial. Meanwhile, convolutional neural networks (CNN) are rapidly emerging as a new premise for cancer image analysis, with significantly enhanced predictive power compared to other hand-crafted radiomics features. Here we show that CNN trained to perform the tumor segmentation task, with no other information than physician contours, identify a rich set of survival-related image features with remarkable prognostic value. In a retrospective study on 96 NSCLC patients before stereotactic-body radiotherapy (SBRT), we found that the CNN segmentation algorithm (U-Net) trained for tumor segmentation in PET/CT images, contained features having strong correlation with 2- and 5-year overall and disease-specific survivals. The U-net algorithm has not seen any other clinical information (e.g. survival, age, smoking history) than the images and the corresponding tumor contours provided by physicians. Furthermore, through visualization of the U-Net, we also found convincing evidence that the regions of progression appear to match with the regions where the U-Net features identified patterns that predicted higher likelihood of death. We anticipate our findings will be a starting point for more sophisticated non-intrusive patient specific cancer prognosis determination.

eess.IV

Single-photon characterization by two-photon spectral interferometry

Single-photon sources are a fundamental resource in quantum optics. The indistinguishability and purity of photons emitted from different sources are crucial (necessary, essential) properties for many quantum applications to ensure high-visibility interference between different sources. The state of a single-photon source is described by the modes occupied by the single light quanta. Thus the ability to determine the mode structure of a single-photon source provides a means to assess its quality, compare different sources, and provide feedback for source engineering. Here, we propose and demonstrate an experimental scheme that allows for complete characterization of the spectral-temporal state of a pulsed single-photon source. The density matrix elements of the single-photon source are determined by spectral interferometry with a known single-photon reference. Frequency-resolved coincidence measurements are performed after the unknown single-photon source is interfered with a single-photon reference pulse. Fourier analysis of the frequency-resolved two-photon interference pattern reveals the spectral-temporal density matrix of the broadband single-photon source. We present an experimental realization of this method for pure and mixed state pulsed, single-photon sources.

quant-ph