Searcharxiv⌕ Search

arXiv subjects

Brian M. Andersen

Publications and source records attributed to Brian M. Andersen.

At least 37 records · Page 2Linked to original sources

Gapless superconductivity from extremely dilute magnetic disorder in 2H-NbSe2-xSx

Most superconducting materials exhibit a vanishing density of states at the Fermi level and Anderson's theorem posits that the superconducting gap is robust against nonmagnetic disorder. Although dilute magnetic impurities lead to localized in-gap states, these states typically have no bearing on the material's bulk superconducting properties. However, numerous experiments reveal a finite density of states at the Fermi level in systems with an apparently negligible number of magnetic impurities. Here, using scanning tunneling microscopy and self-consistent Bogoliubov-de Gennes calculations, we find that gapless superconductivity emerges in 2H-NbSe2-xSx at remarkably low magnetic impurity concentrations. Furthermore, our density functional theory calculations and in-gap quasiparticle interference measurements demonstrate that the Se-S substitution significantly modifies the band structure. This modification favours nesting and dictates the in-gap scattering for x>0, in stark contrast to the dominant charge density wave interactions in pure 2H-NbSe2. Our findings reveal an unusual superconducting response to disorder and highlight the importance of incorporating material-specific band structures in the understanding of a superconductor's response to even very low concentrations of magnetic impurities.

cond-mat.supr-con↗

Local signatures of altermagnetism

Altermagnets constitute a class of collinear compensated Néel ordered magnets that break time-reversal symmetry and feature spin-split band structures. Based on versatile microscopic models able to capture the altermagnetic sublattice degrees of freedom, we study characteristic local signatures of altermagnetism near disorder sites. We give a complete list of two-dimensional models that exhibit altermagnetism classified by their corresponding layer groups. Specifically, we calculate the local density of states in the vicinity of pointlike nonmagnetic impurities and expose its spatial dependence for two minimal models showcasing $d$-wave and $g$-wave altermagnetism. The momentum structure of the nodes ($d$-wave, $g$-wave, etc.) is directly imprinted on the total local density of states, thus measurable by scanning tunneling conductance experiments. This signature is present both in the spin-resolved as well as the spin-summed local density of states. We find a weaker response in the nonmagnetic state from the anisotropic crystal environment and uncover the importance of the sublattice degree of freedom to model altermagnets. We also study coexistence phases of altermagnetism and superconductivity and provide predictions for the local impurity response of in-gap bound states. The response of impurity bound states strongly enhances the distinct altermagnetic signature.

cond-mat.str-el↗

Quasi-symmetry Constrained Spin Ferromagnetism in Altermagnets

Altermagnets break time-reversal symmetry and their spin-orbit coupling (SOC) allow for an anomalous Hall effect (AHE) that depends on the direction of the Néel ordering vector. The AHE and the ferromagnetic spin moment share the same symmetry and hence are usually proportional. However, density functional theory (DFT) calculations find that the AHE exists with negligible ferromagnetic spin moment for some compounds, whereas it reaches sizable values for other altermagnets. By examining realistic minimal models for altermagnetism in which the DFT phenomenology is captured, we uncover a general SOC-enabled quasi-symmetry, the uniaxial spin space-group, that provides a natural explanation for the amplitude of the ferromagnetic spin moment across the vast range of different altermagnetic materials. Additionally, we derive analytic expressions for the magnetic anisotropy energy, providing a simple means to identify the preferred Néel vector orientation for altermagnets.

cond-mat.str-el↗

Existence of Hebel-Slichter peak in unconventional kagome superconductors

We perform a theoretical investigation of the spin susceptibility of unconventional superconductivity on the kagome lattice. Despite the existence of a sign-changing gap structure, which sums to zero over the Fermi surface, we show that such unconventional pairing states may exhibit a Hebel-Slichter peak in the temperature-dependent spin-lattice relaxation rate. It originates from destructive sublattice interference effects. For the same reason, unconventional pairing states on the kagome lattice tend not to exhibit a neutron resonance peak. These results supplement previous theoretical studies of the surprising robustness of sign-changing gap structures to disorder on the kagome lattice. Taken together these findings imply that unconventional superconductivity on the kagome lattice is deceptive in the sense that its properties may appear similar to conventional non-sign-changing superconductivity. These results may be of relevance to the superconducting state of the kagome superconductors $A$V$_3$Sb$_5$ ($A$: K, Rb, Cs) and CsTi$_3$Bi$_5$.

cond-mat.supr-con↗

Unconventional pairing in Ising superconductors: Application to monolayer NbSe$_2$

The presence of a non-centrosymmetric crystal structure and in-plane mirror symmetry allows an Ising spin-orbit coupling to form in some two-dimensional materials. Examples include transition metal dichalcogenide superconductors like monolayer NbSe$_2$, MoS$_2$, TaS$_2$, and PbTe$_2$, where a nontrivial nature of the superconducting state is currently being explored. In this study, we develop a microscopic formalism for Ising superconductors that captures the superconducting instability arising from a momentum-dependent spin- and charge-fluctuation-mediated pairing interaction. We apply our pairing model to the electronic structure of monolayer NbSe$_2$, where first-principles calculations reveal the presence of strong paramagnetic fluctuations. Our calculations provide a quantitative measure of the mixing between the even- and odd-parity superconducting states and its variation with Coulomb interaction. Further, numerical analysis in the presence of an external Zeeman field reveals the role of Ising spin-orbit coupling and mixing of odd-parity superconducting state in influencing the low-temperature enhancement of the critical magnetic field.

cond-mat.supr-con↗

Minimal Models for Altermagnetism

Altermagnets feature vanishing net magnetization, like antiferromagnets, but exhibit time-reversal symmetry breaking and momentum-dependent spin-split band structures. Motivated by the prevalence of altermagnetic materials with non-symmorphic symmetry-dictated band degeneracies, we provide realistic minimal models for altermagnetism by constructing tight-binding models for nonsymmorphic space groups with a sublattice defined by two magnetic atoms. These models can be applied to monoclinic, orthorhombic, tetragonal, rhombohedral, hexagonal, and cubic materials and can describe d-wave, g-wave, and i-wave altermagnetism. By examining the altermagnetic susceptibility and mean field instabilities within a Hubbard model we reveal that these models have altermagnetic ground states and yield a Berry curvature that is linear in the spin-orbit coupling. We apply our models to RuO$_2$, MnF$_2$, FeSb$_2$, $κ$-Cl, CrSb, and MnTe.

cond-mat.str-el↗

Signatures of Amorphous Shiba State in FeTe$_{0.55}$Se$_{0.45}$

The iron-based superconductor FeTe$_{0.55}$Se$_{0.45}$ is a peculiar material: it hosts a surface state with a Dirac dispersion, is a putative topological superconductor hosting Majorana modes in vortices, and has an unusually low Fermi energy. The superconducting state is generally thought to be characterized by three gaps in different bands, with the usual homogenous, spatially extended Bogoliubov excitations -- in this work, we uncover evidence that it is instead of a very different nature. Our scanning tunneling spectroscopy data shows several peaks in the density of states above a full gap, and by analyzing the spatial and junction-resistance dependence of the peaks, we conclude that the peaks above the first one are not coherence peaks from different bands. Instead, comparisons with our simulations indicate that they originate from generalized Shiba states that are spatially overlapping. This can lead to an amorphous state of Bogoliubov quasiparticles, reminiscent of impurity bands in semiconductors. We discuss the origin and implications of this new state.

cond-mat.supr-con↗

Nonlocal electrodynamics and the penetration depth of superconducting Sr$_2$RuO$_4$

The thermal quasiparticles in a clean type-II superconductor with line nodes give rise to a quadratic low-temperature change of the penetration depth, $Δλ\sim T^2$, as first shown by Kosztin and Leggett [I. Kosztin and A. J. Leggett, Phys. Rev. Lett. 79, 135 (1997)]. Here, we generalize this result to multiple nodes and compare it to numerically exact evaluations of the temperature-dependent penetration depth in Sr$_2$RuO$_4$ using a high-precision tight-binding model. We compare the calculations to recent penetration depth measurements in high purity single crystals of Sr$_2$RuO$_4$ [J. F. Landaeta et al., arXiv:2312.05129]. When assuming the order parameter to have $\mathrm{B}_{1\mathrm{g}}$ symmetry, we find that both a simple $d_{x^2-y^2}$-wave and complicated gap structures with contributions from higher harmonics and accidental nodes can accommodate the experimental data.

cond-mat.supr-con↗

Spontaneous time-reversal symmetry breaking by disorder in superconductors

A growing number of superconducting materials display evidence for spontaneous time-reversal symmetry breaking (TRSB) below their critical transition temperatures. Precisely what this implies for the nature of the superconducting ground state of such materials, however, is often not straightforward to infer. We review the experimental status and survey different theoretical mechanisms for the generation of TRSB in superconductors. In cases where a TRSB complex combination of two superconducting order parameter components is realized, defects, dislocations and sample edges may generate superflow patterns that can be picked up by magnetic probes. However, even single-component condensates that do not break time-reversal symmetry in their pure bulk phases can also support signatures of magnetism inside the superconducting state. This includes, for example, the generation of localized orbital current patterns or spin-polarization near atomic-scale impurities, twin boundaries and other defects. Signals of TRSB may also arise from a superconductivity-enhanced Ruderman-Kittel-Kasuya-Yosida exchange coupling between magnetic impurity moments present in the normal state. We discuss the relevance of these different mechanisms for TRSB in light of recent experiments on superconducting materials of current interest.

cond-mat.supr-con↗

Thermodynamic transitions and topology of spin-triplet superconductivity: Application to UTe$_2$

The discovery of unconventional superconductivity in the heavy-fermion material UTe$_2$ has reinvigorated research of spin-triplet superconductivity. We perform a theoretical study of coupled two-component spin-triplet superconducting order parameters and their thermodynamic transitions into the superconducting state. With focus on the behavior of the temperature dependence of the specific heat capacity, we find that two-component time-reversal symmetry breaking superconducting order may feature vanishing or even negative secondary specific heat anomalies. The origin of this unusual specific heat behavior is tied to the non-unitarity of the composite order parameter. Additionally, we supply an analysis of the topological surface states associated with the different possible spin-triplet orders: single-component orders host Dirac Majorana surface states in addition to possible bulk nodes. A second component breaking time-reversal symmetry gaps these surface states producing chiral Majorana hinge modes. DFT+$U$ band-structure calculations support that these topological phases are realized in UTe$_2$ when introducing weak superconducting pairing. Our topological analysis suggests measurable signatures for surface-probe experiments to acquire further evidence of the superconducting pairing symmetry.

cond-mat.supr-con↗

Lateral quantum confinement effect on monolayer high-Tc superconductors

Despite decades of research in spatially confined superconducting systems to understand the modification of superconductivity from reduced length scales, the investigation of the quantum confinement effect on high-temperature superconductors remains an outstanding challenge. Here, we report scanning tunneling spectroscopy measurements on laterally confined FeSe monolayers on SrTiO3 substrates, which are formed by epitaxially growing FeSe films with a coverage less than one unit cell. Comparing to the uniform regions of FeSe monolayers, the peninsula regions at the monolayer boundary exhibit reduced Fermi energy and undiminished superconductivity, leading to a putative crossover from a Bardeen-Cooper-Schrieffer state to a Bose-Einstein condensate state. In isolated FeSe monolayer islands, superconductivity is shown to exist in samples of smaller volume in contrast to conventional superconductors, while the validity of Anderson's criterion remains fulfilled. Our work reveals lateral quantum confinement effects in unconventional superconductors, to enrich the understanding of high-temperature superconductivity in low-dimensional systems.

cond-mat.supr-con↗

Superconducting diodes from magnetization gradients

The superconducting diode effect may exist in bulk systems as well as in junctions when time-reversal and inversion symmetries are simultaneously broken. Magnetization gradients and textures satisfy both requirements and therefore also allow for superconducting diodes. We concretely demonstrate such possibilities in two-dimensional superconductors. We first consider superconducting Rashba metals in the presence of an inhomogeneous out-of-plane exchange field. Using analytical arguments, we reveal that such magnetization gradients stabilize a helical superconducting ground state, similar to homogeneous in-plane magnetic fields. Our predictions are confirmed by employing self-consistent real-space numerical lattice simulations exemplified through the cases of a uniform magnetization gradient or a ferromagnetic domain wall. Furthermore, by considering a phase difference, we determine the nonreciprocal current-phase relations and explore their parameter dependence. Our calculations show that planar devices with out-of-plane magnetization gradients may be as efficient supercurrent rectifiers as their analogs induced by uniform in-plane fields. In addition, they feature the advantage that by means of tailoring the spatial profile of the out-of-plane magnetization, one may optimize and spatially control the diode effect. Finally, we show that superconducting diodes may become also accessible even in the absence of spin-orbit coupling by means of suitable spatially-varying magnetization fields.

cond-mat.supr-con↗

Unconventional superconductivity protected from disorder on the kagome lattice

Motivated by the recent discovery of superconductivity in the kagome $A$V$_3$Sb$_5$ ($A$: K, Rb, Cs) metals, we perform a theoretical study of the symmetry-allowed superconducting orders on the two-dimensional kagome lattice with focus on their response to disorder. We uncover a qualitative difference between the robustness of intraband spin-singlet (even-parity) and spin-triplet (odd-parity) unconventional superconductivity to atomic-scale nonmagnetic disorder. Due to the particular sublattice character of the electronic states on the kagome lattice, disorder in spin-singlet superconducting phases is only weakly pair-breaking despite the fact that the gap structure features sign changes. By contrast, spin-triplet condensates remain fragile to disorder on the kagome lattice. We demonstrate these effects in terms of the absence of impurity bound states and an associated weak disorder-induced $T_c$-suppression for spin-singlet order. We also discuss the consequences for quasi-particle interference and their inherent tendency for momentum-space anisotropy due to sublattice effects on the kagome lattice. For unconventional kagome superconductors, our results imply that any allowed spin-singlet order, including for example $d+id$-wave superconductivity, exhibits a disorder-response qualitatively similar to standard conventional $s$-wave superconductors.

cond-mat.supr-con↗

Anatomy of Spin and Current Generation from Magnetization Gradients in Topological Insulators and Rashba Metals

We explore the spin density and charge currents arising on the surface of a topological insulator and in a 2D Rashba metal due to magnetization gradients. For topological insulators a single interconversion coefficient controls the generation of both quantities. This coefficient is quantized to a value proportional to the vorticity of the Dirac point which constitutes a hallmark of parity anomaly at finite density. As such, it also unveils a robust route to disentangle and detect the protected states of a topological insulator on a given surface. In stark contrast, Rashba metals do not exhibit such anomalies since they contain an even number of helical branches. Nonetheless, also these are governed by quantized responses which, however, are not protected against weak disorder. Furthermore, we find that for Rashba metals the interconversion coefficients demonstrate discontinuities and a nontrivial interplay upon varying the chemical potential, the strength of the spin-orbit coupling, and a pairing gap. Our results have implications for the binding between magnetic skyrmions and superconducting vortices, the emergence of Majorana zero modes, and pave the way for superconducting diode effects mediated by out-of-plane magnetization gradients.

cond-mat.mes-hall↗

Time-reversal symmetry breaking from lattice dislocations in superconductors

Spontaneous generation of time-reversal symmetry breaking in unconventional superconductors is currently a topic of considerable interest. While chiral superconducting order is often assumed to be the source of such signatures, they can sometimes also arise from nonmagnetic disorder. Here we perform a theoretical study of the impact of dislocations on the superconducting order parameter within a microscopic one-band model which, in the homogeneous case, features either extended $s$-wave, $d$-wave, or $s+id$-wave superconductivity depending on the electron concentration. We find that the dislocations minimize their impact on the superconducting condensate by inducing localized supercurrents pinned by the dislocations, even well outside the $s+id$ regime. We map out the parameter and density dependence of the induced currents. From these results we conclude that quite generically unconventional superconductors hosting dislocations tend to break time-reversal symmetry locally.

cond-mat.supr-con↗

Superconductivity from Orbital-Selective Electron-Phonon Coupling in $A\mathrm{V}_3\mathrm{Sb}_5$

Recent experiments have shown that the phase diagrams of the kagome superconductors $A\mathrm{V}_3\mathrm{Sb}_5$ are strongly impacted by changes in the $c$-axis lattice parameter. Here, we show that $c$-axis deformations impact primarily the Sb apical bonds and thus the overlap between their $p_z$ orbitals. Changes in the latter, in turn, substantially affect low-energy electronic states with significant Sb character, most notably the central electron pocket and the van Hove singularities located above the Fermi level. Based on the orbital-selective character of $c$-axis strain, we argue that these electronic states experience a non-negligible attractive electron-phonon pairing interaction mediated by fluctuations in the apical Sb bonds. We thus propose a multi-band model for superconductivity in $A\mathrm{V}_3\mathrm{Sb}_5$ that includes both the Sb pocket and the V-derived van Hove singularities. Upon comparing the theoretical phase diagram with the experimentally observed vanishing of the $T_c$ dome across a Lifshitz transition of the Sb pocket, we propose that either an $s^{+-}$ or an $s^{++}$ state is realized in $A\mathrm{V}_3\mathrm{Sb}_5$.

cond-mat.supr-con↗

Superconducting gap symmetry from Bogoliubov quasiparticle interference analysis on {Sr}$_2${RuO}$_4$

The nature of the superconducting order parameter in {Sr}$_2${RuO}$_4$ has generated intense interest in recent years. Since the superconducting gap is very small, high resolution methods such as scanning tunneling spectroscopy might be the best chance to directly resolve the gap symmetry. Recently, a Bogoliubov quasiparticle interference imaging (BQPI) experiment has suggested that the $d_{x^2-y^2}$ gap symmetry is appropriate for {Sr}$_2${RuO}$_4$. In this work, we use a material-specific theoretical approach based on Wannier functions of the surface of {Sr}$_2${RuO}$_4$ to calculate the continuum density of states as detected in scanning tunneling microscopy experiments. We examine several different proposed gap order parameters, and calculate the expected BQPI pattern for each case. Comparing to the available experimental data, our results suggest that a $s'+id_{xy}$ gap order parameter is the most probable state, but the measured BQPI patterns still display features unaccounted for by the theory for any of the states currently under discussion.

cond-mat.supr-con↗

Interplay of Hidden Orbital Order and Superconductivity in CeCoIn5

Visualizing atomic-orbital degrees of freedom is a frontier challenge in scanned microscopy. Some types of orbital order are virtually imperceptible to normal scattering techniques because they do not reduce the overall crystal lattice symmetry. A good example is dxz/dyz (π,π) orbital order in tetragonal lattices. For enhanced detectability, here we consider the quasiparticle scattering interference (QPI) signature of such (π,π) orbital order in both normal and superconducting phases. The theory reveals that sublattice-specific QPI signatures generated by the orbital order should emerge strongly in the superconducting phase. Sublattice-resolved QPI visualization in superconducting CeCoIn5 then reveals two orthogonal QPI patterns at lattice-substitutional impurity atoms. We analyze the energy dependence of these two orthogonal QPI patterns and find the intensity peaked near E=0, as predicted when such (π) orbital order is inte,πrtwined with d-wave superconductivity. Sublattice-resolved superconductive QPI techniques thus represent a new approach for study of hidden orbital order.

cond-mat.str-el↗