arXiv subjects

Bulbul Chakraborty

Publications and source records attributed to Bulbul Chakraborty.

At least 73 records · Page 4Linked to original sources

arXiv2009

Entropic origin of stress correlations in granular materials

We study the response of granular materials to external stress using experiment, simulation, and theory. We derive an entropic, Ginzburg-Landau functional that enforces mechanical stability and positivity of contact forces. In this framework, the elastic moduli depend only on the applied stress. A combination of this feature and the positivity constraint leads to stress correlations whose shape and magnitude are extremely sensitive to the applied stress. The predictions from the theory describe the stress correlations for both simulations and experiments semiquantitatively.

cond-mat.stat-mech↗

arXiv2008

Jamming in Systems Composed of Frictionless Ellipse-Shaped Particles

We study the structural and mechanical properties of jammed ellipse packings, and find that the nature of the jamming transition in these systems is fundamentally different from that for spherical particles. Ellipse packings are generically hypostatic with more degrees of freedom than constraints. The spectra of low energy excitations possess two gaps and three distinct branches over a range of aspect ratios. In the zero compression limit, the energy of the modes in the lowest branch increases {\it quartically} with deformation amplitude, and the density of states possesses a $δ$-function at zero frequency. We identify scaling relations that collapse the low-frequency part of the spectra for different aspect ratios. Finally, we find that the degree of hypostaticity is determined by the number of quartic modes of the packing.

cond-mat.soft↗

arXiv2008

Dynamics in the Metabasin Space of a Lennard-Jones Glass Former: Connectivity and Transition Rates

Using simulations, we construct the effective dynamics in metabasin space for a Lennard-Jones glass-former. Metabasins are identified via a scheme that measures transition rates between inherent structures, and generates clusters of inherent structures by drawing in branches that have the largest transition rates. The effective dynamics is shown to be Markovian but differs significantly from the simplest trap models. We specifically show that retaining information about the connectivity in metabasin space is crucial for reproducing the slow dynamics observed in this system.

cond-mat.soft↗

arXiv2008

Why Do Granular Materials Stiffen with Shear Rate? A Test of Novel Stress-Based Statistics

Recent experiments exhibit a rate-dependence for granular shear such that the stress grows linearly in the logarithm of the shear rate, \dotγ. Assuming a generalized activated process mechanism, we show that these observations are consistent with a recent proposal for a stress-based statistical ensemble. By contrast, predictions for rate-dependence using conventional energy-based statistical mechanics to describe activated processes, predicts a rate dependence that of (\ln (\dotγ))^{1/2}.

cond-mat.soft↗

arXiv2008

Growing length scale in gravity-driven dense granular flow

We report simulations of a two-dimensional, dense, bidisperse system of inelastic hard disks falling down a vertical tube under the influence of gravity. We examine the approach to jamming as the average flow of particles down the tube is slowed by making the outlet narrower. Defining coarse-grained velocity and stress fields, we study two-point temporal and spatial correlation functions of these fields in a region of the tube where the time-averaged velocity is spatially uniform. We find that fluctuations in both velocity and stress become increasingly correlated as the system approaches jamming. We extract a growing length scale and time scale from these correlations.

cond-mat.soft↗

arXiv2008

Single Polymer Confinement in a Slit: Correlation between structure and dynamics

In this paper, we construct an effective model for the dynamics of an excluded-volume chain under confinement, by extending the formalism of Rouse modes. We make specific predictions about the behavior of the modes for a single polymer confined to a slit. The results are tested against Monte Carlo simulations using the bond-fluctuation algorithm which uses a lattice representation of the polymer chain with excluded-volume effects.

cond-mat.soft↗

arXiv2007

Spatially heterogenous dynamics in dense, driven granular flows

Interest in the dynamical arrest leading to a fluid --> solid transition in thermal and athermal systems has led to questions about the nature of these transitions. These jamming transitions may be dependent on the influence of extended structures on the dynamics of the system. Here we show results from a simple driven, dissipative, non-equilibrium system which exhibits dynamical heterogeneities similar to those observed in a supercooled liquid which is a system in thermal equilibrium. Observations of the time $τ_R(r)$ required for a particular particle to move a distance $r$ reveal the existence of large-scale correlated dynamical regions with characteristic timescales chosen from a broad distribution. The mean squared displacement of ensembles of particles with varying characteristic $τ_R(r)$ reveals an intriguing spatially heterogenous mobility. This suggests that a unified framework for jamming will have to be based on the connection between the nature of these heterogeneities and the effective dynamics.

cond-mat.soft↗

arXiv2007

Entropy and Temperature of a Static Granular Assembly

Granular matter is comprised of a large number of particles whose collective behavior determines macroscopic properties such as flow and mechanical strength. A comprehensive theory of the properties of granular matter, therefore, requires a statistical framework. In molecular matter, equilibrium statistical mechanics, which is founded on the principle of conservation of energy, provides this framework. Grains, however, are small but macroscopic objects whose interactions are dissipative since energy can be lost through excitations of the internal degrees of freedom. In this work, we construct a statistical framework for static, mechanically stable packings of grains, which parallels that of equilibrium statistical mechanics but with conservation of energy replaced by the conservation of a function related to the mechanical stress tensor. Our analysis demonstrates the existence of a state function that has all the attributes of entropy. In particular, maximizing this state function leads to a well-defined granular temperature for these systems. Predictions of the ensemble are verified against simulated packings of frictionless, deformable disks. Our demonstration that a statistical ensemble can be constructed through the identification of conserved quantities other than energy is a new approach that is expected to open up avenues for statistical descriptions of other non-equilibrium systems.

cond-mat.stat-mech↗

arXiv2005

Numerical Studies of the Compressible Ising Spin Glass

We study a two-dimensional compressible Ising spin glass at constant volume. The spin interactions are coupled to the distance between neighboring particles in the Edwards-Anderson model with +/- J interactions. We find that the energy of a given spin configuration is shifted from its incompressible value, E_0, by an amount quadratic in E_0 and proportional to the coupling strength. We then construct a simple model expressed only in terms of spin variables that predicts the existence of a critical value of the coupling above which the spin-glass transition disappears.

cond-mat.dis-nn↗

arXiv2005

Critical Dynamics of Dimers: Implications for the Glass Transition

The Adam-Gibbs view of the glass transition relates the relaxation time to the configurational entropy, which goes continuously to zero at the so-called Kauzmann temperature. We examine this scenario in the context of a dimer model with an entropy vanishing phase transition, and stochastic loop dynamics. We propose a coarse-grained master equation for the order parameter dynamics which is used to compute the time-dependent autocorrelation function and the associated relaxation time. Using a combination of exact results, scaling arguments and numerical diagonalizations of the master equation, we find non-exponential relaxation and a Vogel-Fulcher divergence of the relaxation time in the vicinity of the phase transition. Since in the dimer model the entropy stays finite all the way to the phase transition point, and then jumps discontinuously to zero, we demonstrate a clear departure from the Adam-Gibbs scenario. Dimer coverings are the "inherent structures" of the canonical frustrated system, the triangular Ising antiferromagnet. Therefore, our results provide a new scenario for the glass transition in supercooled liquids in terms of inherent structure dynamics.

cond-mat.stat-mech↗

arXiv2005

Stress and large-scale spatial structures in dense, driven granular flows

We study the appearance of large-scale dynamical heterogeneities in a simplified model of a driven, dissipative granular system. Simulations of steady-state gravity-driven flows of inelastically colliding hard disks show the formation of large-scale linear structures of particles with a high collision frequency. These chains can be shown to carry much of the collisional stress in the system due to a dynamical correlation that develops between the momentum transfer and time between collisions in these "frequently-colliding" particles. The lifetime of these dynamical stress heterogeneities is seen to grow as the flow velocity decreases towards jamming, leading to slowly decaying stress correlations reminiscent of the slow dynamics observed in supercooled liquids.

cond-mat.soft↗

arXiv2005

Jamming as a critical phenomenon: a field theory of zero-temperature grain packings

A field theory of frictionless grain packings in two dimensions is shown to exhibit a zero-temperature critical point at a non-zero value of the packing fraction. The zero-temperature constraint of force-balance plays a crucial role in determining the nature of the transition. Two order parameters, , the deviation of the average number of contacts from the isostatic value and, , the average magnitude of the force per contact, characterize the transition from the jammed (high packing fraction) to the unjammed (low packing fraction state). The critical point has a mixed character with the order parameters showing a jump discontinuity but with fluctuations of the contact force diverging. At the critical point, the distribution of F shows the characteristic plateau observed in static granular piles. The theory makes falsifiable predictions about the spatial fluctuations of the contact forces. Implications for finite temperature dynamics and generalizations to frictional packings and higher dimensions are discussed

cond-mat.stat-mech↗

arXiv2004

Landau theory of glassy dynamics

An exact solution of a Landau model of an order-disorder transition with activated critical dynamics is presented. The model describes a funnel-shaped topography of the order parameter space in which the number of energy lowering trajectories rapidly diminishes as the ordered ground-state is approached. This leads to an asymmetry in the effective transition rates which results in a non-exponential relaxation of the order-parameter fluctuations and a Vogel-Fulcher-Tammann divergence of the relaxation times, typical of a glass transition. We argue that the Landau model provides a general framework for studying glassy dynamics in a variety of systems.

cond-mat.stat-mech↗

arXiv2002

Trap dominated dynamics of classical dimer models

We consider dynamics of classical dimer models undergoing a phase transition to an ordered, frozen state. Relaxation processes are dominated by traps which are entropic in origin and can be traced to the locally jammed nature of the dimer states. Depending on the nature of the phase transition, critical dynamics are characterized either by an exponential, or sub-exponential in time relaxation of the order parameter. In the latter case relaxation time scales diverge {\em exponentially} as the critical point is approached, following the Vogel-Fulcher law.

cond-mat.stat-mech↗

arXiv2002

Aggregate formation in a system of coagulating and fragmenting particles with mass-dependent diffusion rates

The effect of introducing a mass dependent diffusion rate ~ m^{-alpha} in a model of coagulation with single-particle break up is studied both analytically and numerically. The model with alpha=0 is known to undergo a nonequilibrium phase transition as the mass density in the system is varied from a phase with an exponential distribution of mass to a phase with a power-law distribution of masses in addition to a single infinite aggregate. This transition is shown to be curbed, at finite densities, for all alpha > 0 in any dimension. However, a signature of this transition is seen in finite systems in the form of a large aggregate and the finite size scaling implications of this are characterized. The exponents characterizing the steady state probability that a randomly chosen site has mass m are calculated using scaling arguments. The full probability distribution is obtained within a mean field approximation and found to compare well with the results from numerical simulations in one dimension.

cond-mat.stat-mech↗

arXiv2001

Topological jamming of extended structures and the glass transition

We propose a new scenario for glassy dynamics in frustrated systems with no quenched-in randomness, based on jamming of extended dynamical structures near a critical point. This route to a glassy state is demonstrated in a lattice model of fluctuating lines. Numerical simulations of the model show non-exponential relaxations and diverging energy barriers in the vicinity of a thermodynamic phase transition. A master equation for the coarse grained dynamics is constructed. It shows how topological jamming leads to the observed glassy dynamics.

cond-mat.stat-mech↗

arXiv2001

Slow dynamics and aging in a non-randomly frustrated spin system

A simple, non-disordered spin model has been studied in an effort to understand the origin of the precipitous slowing down of dynamics observed in supercooled liquids approaching the glass transition. A combination of Monte Carlo simulations and exact calculations indicates that this model exhibits an entropy vanishing transition accompanied by a rapid divergence of time scales. Measurements of various correlation functions show that the system displays a hierarchy of time scales associated with different degrees of freedom. Extended structures, arising from the frustration in the system, are identified as the source of the slow dynamics. In the simulations, the system falls out of equilibrium at a temperature $T_{g}$ higher than the entropy-vanishing transition temperature and the dynamics below $T_{g}$ exhibits aging as distinct from coarsening. The cooling rate dependence of the energy is also consistent with the usual glass formation scenario.

cond-mat.stat-mech↗

arXiv2001

Entropy-vanishing transition and glassy dynamics in frustrated spins

In an effort to understand the glass transition, the dynamics of a non-randomly frustrated spin model has been analyzed. The phenomenology of the spin model is similar to that of a supercooled liquid undergoing the glass transition. The slow dynamics can be associated with the presence of extended string-like structures which demarcate regions of fast spin flips. An entropy-vanishing transition, with the string density as the order parameter, is related to the observed glass transition in the spin model.

cond-mat.stat-mech↗