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C. -C. Chen

Publications and source records attributed to C. -C. Chen.

49 records · Page 3Linked to original sources

Numerical exploration of spontaneous broken symmetries in multi-orbital Hubbard models

We study three proposals for broken symmetry in the cuprate pseudogap - oxygen antiferromagnetism, $Θ_{II}$ orbital loop currents, and circulating currents involving apex oxygens - through numerical exploration of multi-orbital Hubbard models. Our numerically exact results show no evidence for the existence of oxygen antiferromagnetic order or the $Θ_{II}$ phase in the three-orbital Hubbard model. The model also fails to sustain an ordered current pattern even with the presence of additional apex oxygen orbitals. We thereby conclude that it is difficult to stabilize the aforementioned phases in the multi-orbital Hubbard models for parameters relevant to cuprate superconductors. However, the $Θ_{II}$ phase might be stabilized through explicit flux terms. We find an enhanced propensity for circulating currents with such terms in calculations simulating applied stress or strain, which skew the copper-oxygen plane to resemble a kagome lattice. We propose an experimental viewpoint to shed additional light on this problem.

cond-mat.supr-con↗

Is There a Maximum Star Formation Rate in High-Redshift Galaxies?

We use the James Clerk Maxwell Telescope's SCUBA-2 camera to image a 400 arcmin^2 area surrounding the GOODS-N field. The 850 micron rms noise ranges from a value of 0.49 mJy in the central region to 3.5 mJy at the outside edge. From these data, we construct an 850 micron source catalog to 2 mJy containing 49 sources detected above the 4-sigma level. We use an ultradeep (11.5 uJy at 5-sigma) 1.4 GHz image obtained with the Karl G. Jansky Very Large Array together with observations made with the Submillimeter Array to identify counterparts to the submillimeter galaxies. For most cases of multiple radio counterparts, we can identify the correct counterpart from new and existing Submillimeter Array data. We have spectroscopic redshifts for 62% of the radio sources in the 9 arcmin radius highest sensitivity region (556/894) and 67% of the radio sources in the GOODS-N region (367/543). We supplement these with a modest number of additional photometric redshifts in the GOODS-N region (30). We measure millimetric redshifts from the radio to submillimeter flux ratios for the unidentified submillimeter sample, assuming an Arp 220 spectral energy distribution. We find a radio flux dependent K-z relation for the radio sources, which we use to estimate redshifts for the remaining radio sources. We determine the star formation rates (SFRs) of the submillimeter sources based on their radio powers and their submillimeter and find that they agree well. The radio data are deep enough to detect star-forming galaxies with SFRs >2000 solar masses per year to z~6. We find galaxies with SFRs up to ~6,000 solar masses per year over the redshift range z=1.5-6, but we see evidence for a turn-down in the SFR distribution function above 2000 solar masses per year.

astro-ph.GA↗

Time-Dependent Charge-Order and Spin-Order Recovery in Striped Systems

Using time-dependent Ginzburg-Landau theory, we study the role of amplitude and phase fluctuations in the recovery of charge and spin stripe phases in response to a pump pulse that melts the orders. For parameters relevant to the case where charge order precedes spin order thermodynamically, amplitude recovery governs the initial time scales, while phase recovery controls behavior at longer times. In addition to these intrinsic effects, there is a longer spin re-orientation time scale related to the scattering geometry that dominates the recovery of the spin phase. Coupling between the charge and spin orders locks the amplitude and similarly the phase recovery, reducing the number of distinct time scales. Our results well reproduce the major experimental features of pump-probe x-ray diffraction measurements on the striped nickelate La$_{1.75}$Sr$_{0.25}$NiO$_4$. They highlight the main idea of this work, which is the use of time-dependent Ginzburg-Landau theory to study systems with multiple coexisting order parameters.

cond-mat.str-el↗

Doping Evolution of Oxygen K-edge X-ray Absorption Spectra in Cuprate Superconductors

We study oxygen K-edge x-ray absorption spectroscopy (XAS) and investigate the validity of the Zhang-Rice singlet (ZRS) picture in overdoped cuprate superconductors. Using large-scale exact diagonalization of the three-orbital Hubbard model, we observe the effect of strong correlations manifesting in a dynamical spectral weight transfer from the upper Hubbard band to the ZRS band. The quantitative agreement between theory and experiment highlights an additional spectral weight reshuffling due to core-hole interaction. Our results confirm the important correlated nature of the cuprates and elucidate the changing orbital character of the low-energy quasi-particles, but also demonstrate the continued relevance of the ZRS even in the overdoped region.

cond-mat.supr-con↗

Precise Identifications of Submillimeter Galaxies: Measuring the History of Massive Star-Forming Galaxies to z>5

We carried out extremely sensitive Submillimeter Array (SMA) 340 GHz (860 micron) continuum imaging of a complete sample of SCUBA 850 micron sources (>4 sigma) with fluxes >3 mJy in the GOODS-N. Using these data and new SCUBA-2 data, we do not detect 4 of the 16 SCUBA sources, and we rule out the original SCUBA fluxes at the 4 sigma level. Three more resolve into multiple fainter SMA galaxies, suggesting that our understanding of the most luminous high-redshift dusty galaxies may not be as reliable as we thought. 10 of the 16 independent SMA sources have spectroscopic redshifts (optical/infrared or CO) to z=5.18. Using a new, ultradeep 20 cm image obtained with the Karl G. Jansky Very Large Array (rms of 2.5 microJy), we find that all 16 of the SMA sources are detected at >5 sigma. Using Herschel far-infrared (FIR) data, we show that the five isolated SMA sources with Herschel detections are well described by an Arp 220 spectral energy distribution template in the FIR. They also closely obey the local FIR-radio correlation, a result that does not suffer from a radio bias. We compute the contribution from the 16 SMA sources to the universal star formation rate (SFR) per comoving volume. With individual SFRs in the range 700-5000 solar masses per year, they contribute ~30% of the extinction-corrected ultraviolet-selected SFR density from z=1 to at least z=5. Star formation histories determined from extinction-corrected ultraviolet populations and from submillimeter galaxy populations only partially overlap, due to the extreme ultraviolet faintness of some submillimeter galaxies.

astro-ph.CO↗

Uncovering selective excitations using the resonant profile of indirect inelastic x-ray scattering in correlated materials: Observing two-magnon scattering and relation to the dynamical structure factor

Resonant inelastic x-ray scattering (RIXS) is a spectroscopic technique which has been widely used to study various elementary excitations in correlated and other condensed matter systems. For strongly correlated materials, besides boosting the overall signal the dependence of the resonant profile on incident photon energy is still not fully understood. Previous endeavors in connecting indirect RIXS, such as Cu K-edge for example where scattering takes place only via the core-hole created as an intermediate state, with the charge dynamical structure factor S(q,ω) neglected complicated dependence on the intermediate state configuration. To resolve this issue, we performed an exact diagonalization study of the RIXS cross-section using the single-band Hubbard model by fully addressing the intermediate state contribution. Our results are relevant to indirect RIXS in correlated materials, such as high Tc cuprates. We demonstrate that RIXS spectra can be reduced to S(q,ω) when there is no screening channel for the core-hole potential in the intermediate state. We also show that two-magnon excitations are highlighted at the resonant photon energy when the core-hole potential in the corresponding intermediate state is poorly screened. Our results demonstrate that different elementary excitations can be emphasized at different intermediate states, such that selecting the exact incident energy is critical when trying to capture a particular elementary excitation.

cond-mat.str-el↗

Existence of Orbital Order and its Fluctuation in Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ Revealed by X-ray Absorption Spectroscopy

We performed temperature dependent X-ray linear dichroism (XLD) experiments on an iron pnictide system, Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ with $x$=0.00 and 0.05, to experimentally verify existence of orbital ordering (OO). We observed clear XLD in polarization dependent X-ray absorption spectra of Fe $L$ edges. By exploiting the difference in the temperature dependent behaviors, we were able to separate OO and structure contributions to XLD. The observed OO signal indicates different occupation numbers for $d_{yz}$ and $d_{zx}$ orbitals and supports existence of a ferro-OO. The results are also consistent with the theoretical prediction. Moreover, we find substantial OO signal above the transition temperature, which suggests that OO fluctuation exists well above the transition temperature.

cond-mat.supr-con↗

A Fidelity Study of the Superconducting Phase Diagram in the 2D Single-band Hubbard Model

Extensive numerical studies have demonstrated that the two-dimensional single-band Hubbard model contains much of the key physics in cuprate high-temperature superconductors. However, there is no definitive proof that the Hubbard model truly possesses a superconducting ground state or, if it does, of how it depends on model parameters. To answer these longstanding questions, we study an extension of the Hubbard model including an infinite-range d-wave pair field term, which precipitates a superconducting state in the d-wave channel. Using exact diagonalization on 16-site square clusters, we study the evolution of the ground state as a function of the strength of the pairing term. This is achieved by monitoring the fidelity metric of the ground state, as well as determining the ratio between the two largest eigenvalues of the d-wave pair/spin/charge-density matrices. The calculations show a d-wave superconducting ground state in doped clusters bracketed by a strong antiferromagnetic state at half filling controlled by the Coulomb repulsion U and a weak short-range checkerboard charge ordered state at larger hole doping controlled by the next-nearest-neighbor hopping t'. We also demonstrate that negative t' plays an important role in facilitating d-wave superconductivity.

cond-mat.supr-con↗

Revealing the degree of magnetic frustration by non-magnetic impurities

Imaging the magnetic fields around a non-magnetic impurity can provide a clear benchmark for quantifying the degree of magnetic frustration. Focusing on the strongly frustrated $J_1$-$J_2$ model and the spatially anisotropic $J_{1a}$-$J_{1b}$-$J_2$ model, very distinct low energy behaviors reflect different levels of magnetic frustration. In the $J_1$-$J_2$ model, bound magnons appear trapped near the impurity in the ground state and strongly reduce the ordered moments for sites proximal to the impurity. In contrast, local moments in the $J_{1a}$-$J_{1b}$-$J_2$ model are enhanced on the impurity neighboring sites. These theoretical predictions can be probed by experiments such as nuclear magnetic resonance and scanning tunneling microscopy, and the results can elucidate the role of frustration in antiferromagnets and help narrow the possible models to understand magnetism in the iron pnictdies.

cond-mat.str-el↗

Theory of two magnon Raman scattering in antiferromagnetic iron pnictides

Although the parent iron-based pnictides and chalcogenides are itinerant antiferromagnets, the use of local moment picture to understand their magnetic properties is still widespread. We study magnetic Raman scattering from a local moment perspective for various quantum spin models proposed for this new class of superconductors. These models vary greatly in the level of magnetic frustration and show a vastly different two-magnon Raman response. Light scattering by two-magnon excitations thus provides a robust and independent measure of the underlying spin interactions. In accord with other recent experiments, our results indicate that the amount of magnetic frustration in these systems may be small.

cond-mat.str-el↗

Unraveling the Nature of Charge Excitations in La$_2$CuO$_4$ with Momentum-Resolved Cu $K$-edge Resonant Inelastic X-ray Scattering

Results of model calculations using exact diagonalization reveal the orbital character of states associated with different Raman loss peaks in Cu $K$-edge resonant inelastic X-ray scattering (RIXS) from La$_{2}$CuO$_{4}$. The model includes electronic orbitals necessary to highlight non-local Zhang-Rice singlet, charge transfer and $d$-$d$ excitations, as well as states with apical oxygen 2$p_z$ character. The dispersion of these excitations is discussed with prospects for resonant final state wave-function mapping. A good agreement with experiments emphasizes the substantial multi-orbital character of RIXS profiles in the energy transfer range 1-6 eV.

cond-mat.str-el↗

Orbital Order and Spontaneous Orthorhombicity in Iron Pnictides

A growing list of experiments show orthorhombic electronic anisotropy in the iron pnictides, in some cases at temperatures well above the spin density wave transition. These experiments include neutron scattering, resistivity and magnetoresistance measurements, and a variety of spectroscopies. We explore the idea that these anisotropies stem from a common underlying cause: orbital order manifest in an unequal occupation of $d_{xz}$ and $d_{yz}$ orbitals, arising from the coupled spin-orbital degrees of freedom. We emphasize the distinction between the total orbital occupation (the integrated density of states), where the order parameter may be small, and the orbital polarization near the Fermi level which can be more pronounced. We also discuss light-polarization studies of angle-resolved photoemission, and demonstrate how x-ray absorption linear dichroism may be used as a method to detect an orbital order parameter.

cond-mat.supr-con↗

Finite temperature spin-dynamics and phase transitions in spin-orbital models

We study finite temperature properties of a generic spin-orbital model relevant to transition metal compounds, having coupled quantum Heisenberg-spin and Ising-orbital degrees of freedom. The model system undergoes a phase transition, consistent with that of a 2D Ising model, to an orbitally ordered state at a temperature set by short-range magnetic order. At low temperatures the orbital degrees of freedom freeze-out and the model maps on to a quantum Heisenberg model. The onset of orbital excitations causes a rapid scrambling of the spin spectral weight away from coherent spin-waves, which leads to a sharp increase in uniform magnetic susceptibility just below the phase transition, reminiscent of the observed behavior in the Fe-pnictide materials.

cond-mat.str-el↗