arXiv subjects

C. -T. Chen

Publications and source records attributed to C. -T. Chen.

At least 37 records · Page 2Linked to original sources

arXiv2012

Evidence for a cos(4φ) Modulation of the Superconducting Energy Gap of Optimally Doped FeTe_{0.6}Se_{0.4} Single Crystals Using Laser Angle-Resolved Photoemission Spectroscopy

We study the superconducting(SC)-gap anisotropy of the Γ-centered hole Fermi surface in optimally doped FeTe_{0.6}Se_{0.4} (T_c = 14.5 K), using laser-excited angle-resolved photoemission spectroscopy (ARPES). We observe sharp superconducting coherence peaks at T = 2.5 K. In contrast to earlier ARPES studies but consistent with thermodynamic results, the momentum dependence shows a \cos(4φ) modulation of the SC-gap anisotropy. The observed SC-gap anisotropy strongly indicates that the pairing interaction is not a conventional phonon-mediated isotropic one. Instead, the results suggest the importance of second-nearest-neighbor electronic interactions between the iron sites in the framework of s_\pm-wave superconductivity.

cond-mat.supr-con↗

arXiv2012

Abrupt change in the energy gap of superconducting Ba1-xKxFe2As2 single crystals with hole doping

We performed a Laser angle-resolved photoemission spectroscopy (ARPES) study on a wide doping range of Ba1-xKxFe2As2 (BaK) and precisely determined the doping evolution of the superconducting (SC) gaps in this compound. The gap size of the outer hole Fermi surface (FS) sheet around the Brillioun zone (BZ) center shows an abrupt drop with overdoping (for x > 0.6) while the inner and middle FS gaps roughly scale with Tc. This is accompanied by the simultaneous disappearance of the electron FS sheet with similar orbital character at the BZ corner. These results browse the different contributions of X2-Y2 and XZ/YZ orbitals to superconductivity in BaK and can be hardly completely reproduced by the available theories on iron-based superconductors.

cond-mat.supr-con↗

arXiv2011

Common Origin of the Circular-dichroism Pattern in ARPES of SrTiO3 and CuxBi2Se3

Circular dichroism in the angular distribution (CDAD) of photoelectrons from SrTiO3:Nb and CuxBi2Se3 is investigated by 7-eV laser ARPES. In addition to the well-known node that occurs in CDAD when the incidence plane matches the mirror plane of the crystal, we show that another type of node occurs when the mirror plane of the crystal is vertical to the incidence plane and the electronic state is two dimensional. The flower-shaped CDAD's occurring around the Fermi level of SrTiO3:Nb and around the Dirac point of CuxBi2Se3 are explained on equal footings. We point out that the penetration depth of the topological states of CuxBi2Se3 depends on momentum.

cond-mat.mtrl-sci↗

arXiv2010

Integer and half-integer flux-quantum transitions in a niobium/iron-pnictide loop

The recent discovery of iron-based superconductors challenges the existing paradigm of high-temperature superconductivity. Owing to their unusual multi-orbital band structure, magnetism, and electron correlation, theories propose a unique sign reversed s-wave pairing state, with the order parameter changing sign between the electron and hole Fermi pockets. However, because of the complex Fermi surface topology and material related issues, the predicted sign reversal remains unconfirmed. Here we report a novel phase-sensitive technique for probing unconventional pairing symmetry in the polycrystalline iron-pnictides. Through the observation of both integer and half-integer flux-quantum transitions in composite niobium/iron-pnictide loops, we provide the first phase-sensitive evidence of the sign change of the order parameter in NdFeAsO0.88F0.12, lending strong support for microscopic models predicting unconventional s-wave pairing symmetry. These findings have important implications on the mechanism of pnictide superconductivity, and lay the groundwork for future studies of new physics arising from the exotic order in the FeAs-based superconductors.

cond-mat.supr-con↗

arXiv2010

Orbital-dependent modifications of electronic structure across magneto-structural transition in BaFe2As2

Laser angle-resolved photoemission spectroscopy (ARPES) is employed to investigate the temperature (T) dependence of the electronic structure in BaFe2As2 across the magneto-structural transition at TN ~ 140 K. A drastic transformation in Fermi surface (FS) shape across TN is observed, as expected by first-principles band calculations. Polarization-dependent ARPES and band calculations consistently indicate that the observed FSs at kz ~ pi in the low-T antiferromagnetic (AF) state are dominated by the Fe3dzx orbital, leading to the two-fold electronic structure. These results indicate that magneto-structural transition in BaFe2As2 accompanies orbital-dependent modifications in the electronic structure.

cond-mat.supr-con↗

arXiv2009

Superconducting electronic state in optimally doped YBa2Cu3O7-d observed with laser-excited angle-resolved photoemission spectroscopy

Low energy electronic structure of optimally doped YBa2Cu3O7-d is investigated using laser-excited angle-resolved photoemission spectroscopy. The surface state and the CuO chain band that usually overlap the CuO2 plane derived bands are not detected, thus enabling a clear observation of the bulk superconducting state. The observed bilayer splitting of the Fermi surface is ~0.08 angstrom^{-1} along the (0,0)-(pi,pi) direction, significantly larger than Bi2Sr2CaCu2O8+d. The kink structure of the band dispersion reflecting the renormalization effect at ~60 meV shows up similarly as in other hole-doped cuprates. The momentum-dependence of the superconducting gap shows d_{x^2-y^2}-wave like amplitude, but exhibits a nonzero minimum of ~12 meV along the (0,0)-(pi,pi) direction. Possible origins of such an unexpected "nodeless" gap behavior are discussed.

cond-mat.supr-con↗

arXiv2009

Anomalous State Sandwiched between Fermi Liquid and Charge Ordered Mott-Insulating Phases of Ti4O7

The Magneli phase Ti4O7 exhibits two sharp jumps in resistivity with coupled structural transitions as a function of temperature at Tc1=142 K and Tc2=154 K. We have studied electronic structure changes across the two transitions using 7 eV laser, soft x-ray and hard x-ray (HX) photoemission spectroscopy (PES). Ti 2p-3d resonant PES and HX-PES show a clear metallic Fermi-edge and mixed valency above Tc2. The low temperature phase below Tc1 shows a clear insulating gap of 100 meV. The intermediate phase between Tc1 and Tc2 indicates a pseudogap coexisting with remnant coherent states. HX-PES and complementary calculations have confirmed the coherent screening in the strongly correlated intermediate phase. The results suggest existence of a highly anomalous state sandwiched between the mixed-valent Fermi liquid and charge ordered Mott-insulating phase in Ti4O7.

cond-mat.str-el↗

arXiv2009

Unusual Pseudogap-like Features Observed in Iron Oxypnictide Superconductors

We have performed a temperature-dependent angle-integrated laser photoemission study of iron oxypnictide superconductors LaFeAsO:F and LaFePO:F exhibiting critical transition temperatures (Tc's) of 26 K and 5 K, respectively. We find that high-Tc LaFeAsO:F exhibits a temperature-dependent pseudogap-like feature extending over ~0.1 eV about the Fermi level at 250 K, whereas such a feature is absent in low-Tc LaFePO:F. We also find ~20-meV pseudogap-like features and signatures of superconducting gaps both in LaFeAsO:F and LaFePO:F. We discuss the possible origins of the unusual pseudogap-like features through comparison with the high-Tc cuprates.

cond-mat.supr-con↗

arXiv2008

Competing orders and the doping and momentum dependent quasiparticle excitations in cuprate superconductors

The low-energy quasiparticle excitations in hole- and electron-type cuprate superconductors are investigated via both experimental and theoretical means. It is found that the doping and momentum dependence of the empirical low-energy quasiparticle excitations is consistent with a scenario of coexisting competing orders and superconductivity in the ground state of the cuprates. This finding, based on zero-field quasiparticle spectra, is further corrobarated by the patially resolved vortex-state scanning tunneling spectroscopy, which reveals pseudogap-like features consistent with a remaining competing order inside the vortex core upon the suppression of superconductivity. The competing orders compatible with empirical observations include the charge-density wave and spin-density wave. In contrast, spectral characteristics derived from incorporating the $d$-density wave as a competing order appear unfavorable in comparison with experiments.

cond-mat.supr-con↗

arXiv2007

Doping-dependence of nodal quasiparticle properties in high-$T_{\rm c}$ cuprates studied by laser-excited angle-resolved photoemission spectroscopy

We investigate the doping dependent low energy, low temperature ($T$ = 5 K) properties of nodal quasiparticles in the d-wave superconductor Bi$_{2.1}$Sr$_{1.9}$CaCu$_2$O$_{8+δ}$ (Bi2212). By utilizing ultrahigh resolution laser-excited angle-resolved photoemission spectroscopy, we obtain precise band dispersions near $E_{F}$, mean free paths and scattering rates ($Γ$) of quasiparticles. For optimally and overdoped, we obtain very sharp quasiparticle peaks of 8 meV and 6 meV full-width at half-maximum, respectively, in accord with terahertz conductivity. For all doping levels, we find the energy-dependence of $Γ\sim |ω|$, while $Γ$($ω=0$) shows a monotonic increase from overdoping to underdoping. The doping dependence suggests the role of electronic inhomogeneity on the nodal quasiparticle scattering at low temperature (5 K $\lsim 0.07T_{\rm c}$), pronounced in the underdoped region.

cond-mat.supr-con↗

arXiv2007

Competing Orders and Quantum Phase Fluctuations on the Low-Energy Excitations and Pseudogap Phenomena of Cuprate Superconductors

We investigate the low-energy quasiparticle excitation spectra of cuprate superconductors by incorporating both superconductivity (SC) and competing orders (CO) in the bare Green's function and quantum phase fluctuations in the proper self-energy. Our approach provides consistent explanations for various empirical observations, including the excess subgap quasiparticle density of states, ``dichotomy'' in the momentum-dependent quasiparticle coherence and the temperature-dependent gap evolution, and the presence (absence) of the low-energy pseudogap in hole- (electron-) type cuprates depending on the relative scale of the CO and SC energy gaps.

cond-mat.supr-con↗

arXiv2006

Valence, spin, and orbital state of the Co ions in the one-dimensional Ca3Co2O6: an x-ray absorption and magnetic circular dichroism study

We have investigated the valence, spin, and orbital state of the Co ions in the one-dimensional cobaltate Ca3Co2O6 using x-ray absorption and x-ray magnetic circular dichroism at the Co-L2,3 edges. The Co ions at both the octahedral Co_oct and trigonal Co_trig sites are found to be in a 3+ state. From the analysis of the dichroism we established a low-spin state for the Co_oct and a high-spin state with an anomalously large orbital moment of 1.7 muB at the Co3+ trig ions. This large orbital moment along the c-axis chain and the unusually large magnetocrystalline anisotropy can be traced back to the double occupancy of the d2 orbital in trigonal crystal field.

cond-mat.str-el↗

arXiv2006

Investigating the Physical Origin of Unconventional Low-Energy Excitations and Pseudogap Phenomena in Cuprate Superconductors

We investigate the physical origin of unconventional low-energy excitations in cuprate superconductors by considering the effect of coexisting competing orders (CO) and superconductivity (SC) and of quantum fluctuations and other bosonic modes on the low-energy charge excitation spectra. By incorporating both SC and CO in the bare Green's function and quantum phase fluctuations in the self-energy, we can consistently account for various empirical findings in both the hole- and electron-type cuprates, including the excess subgap quasiparticle density of states, ``dichotomy'' in the fluctuation-renormalized quasiparticle spectral density in momentum space, and the occurrence and magnitude of a low-energy pseudogap being dependent on the relative gap strength of CO and SC. Comparing these calculated results with experiments of ours and others, we suggest that there are two energy scales associated with the pseudogap phenomena, with the high-energy pseudogap probably of magnetic origin and the low-energy pseudogap associated with competing orders.

cond-mat.supr-con↗

arXiv2006

Observation of superconducting gap in boron-doped diamond by laser-excited photoemission spectroscopy

We have investigated the low energy electronic state of a boron-doped diamond thin film by the ultrahigh resolution laser-excited photoemission spectroscopy. We observed a clear shift of the leading edge below 11 K indicative of a superconducting gap opening ($Δ\sim 0.78$ meV at 4.5 K). The gap feature is significantly broad and the well-defined quasiparticle peak is not recognizable even at the lowest temperature of measurement 4.5 K. We discuss our result in terms of possible disorder effect on superconductivity in this system.

cond-mat.supr-con↗

arXiv2004

Experimental Investigation of the Competing Orders and Quantum Criticality in Hole- and Electron-Doped Cuprate Superconductors

We investigate the issues of competing orders and quantum criticality in cuprate superconductors via experimental studies of the high-field thermodynamic phase diagrams and the quasiparticle tunneling spectroscopy. Our results suggest substantial field-induced quantum fluctuations in all cuprates investigated, and their correlation with quasiparticle spectra implies that both electron- (n-type) and hole-doped (p-type) cuprate superconductors are in close proximity to a quantum critical point that separates a pure superconducting (SC) phase from a phase consisting of coexisting SC and a competing order. We further suggests that the relevant competing order is likely a spin-density wave (SDW) or a charge density wave (CDW), which can couple to an in-plane Cu-O bond stretching longitudinal optical (LO) phonon mode in the p-type cuprates but not in the n-type cuprates. This cooperative interaction may account for the pseudogap phenomenon above Tc only in the p-type cuprate superconductors.

cond-mat.supr-con↗

arXiv2004

Quasiparticle spectroscopy and high-field phase diagrams of cuprate superconductors -- An investigation of competing orders and quantum criticality

We present scanning tunneling spectroscopic and high-field thermodynamic studies of hole- and electron-doped (p- and n-type) cuprate superconductors. Our experimental results are consistent with the notion that the ground state of cuprates is in proximity to a quantum critical point (QCP) that separates a pure superconducting (SC) phase from a phase comprised of coexisting SC and a competing order, and the competing order is likely a spin-density wave (SDW). The effect of applied magnetic field, tunneling current, and disorder on the revelation of competing orders and on the low-energy excitations of the cuprates is discussed.

cond-mat.supr-con↗

arXiv2004

Experimental investigation of the asymmetric spectroscopic characteristics of electron- and hole-doped cuprates

Quasiparticle tunneling spectroscopic studies of electron- (n-type) and hole-doped (p-type) cuprates reveal that the pairing symmetry, pseudogap phenomenon and spatial homogeneity of the superconducting order parameter are all non-universal. We compare our studies of p-type YBa_2Cu_3O_{7-x} and n-type infinite-layer Sr_{0.9}Ln_{0.1}CuO_2 (Ln = La, Gd) systems with results from p-type Bi_2Sr_2CaCu_2O_x and n-type one-layer Nd_{1.85}Ce_{0.15}CuO_4 cuprates, and attribute various non-universal behavior to different competing orders in p-type and n-type cuprates.

cond-mat.supr-con↗

arXiv2003

Collective modes and quasiparticle interference on the local density of states of cuprate superconductors

The energy, momentum and temperature dependence of the quasiparticle local density of states (LDOS) of a two-dimensional $d_{x^2-y^2}$-wave superconductor with random disorder is investigated using the first-order T-matrix approximation. The results suggest that collective modes such as spin/charge density waves are relevant low-energy excitations of the cuprates that contribute to the observed LDOS modulations in recent scanning tunneling microscopy studies of $\rm Bi_2Sr_2CaCu_2O_x$.

cond-mat.supr-con↗