arXiv subjects

C. A. Busser

Publications and source records attributed to C. A. Busser.

15 recordsLinked to original sources

arXiv2014

Kondo versus indirect exchange: the role of the lattice and the actual range of RKKY interactions in real materials

Magnetic impurities embedded in a metal interact via an effective Ruderman-Kittel-Kasuya-Yosida (RKKY) coupling mediated by the conduction electrons, which is commonly assumed to be long ranged, with an algebraic decay in the inter-impurity distance. However, they can also form a Kondo screened state that is oblivious to the presence of other impurities. The competition between these effects leads to a critical distance above which Kondo effect dominates, translating into a finite range for the RKKY interaction. We study this mechanism on the square and cubic lattices by introducing an exact mapping onto an effective one-dimensional problem that we can solve with the density matrix renormalization group method (DMRG). We show a clear departure from the conventional RKKY theory, that can be attributed to the dimensionality and different densities of states. In particular, for dimension d>1, Kondo physics dominates even at short distances, while the ferromagnetic RKKY state is energetically unfavorable.

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arXiv2013

Polarized currents and spatial separation of Kondo state: NRG study of spin-orbital effect in a double QD

A double quantum dot device, connected to two channels that only see each other through interdot Coulomb repulsion, is analyzed using the numerical renormalization group technique. By using a two-impurity Anderson model, and parameter values obtained from experiment [S. Amasha {\it et al.}, Phys. Rev. Lett. {\bf 110}, 046604 (2013)], it is shown that, by applying a moderate magnetic field, and adjusting the gate potential of each quantum dot, opposing spin polarizations are created in each channel. Furthermore, through a well defined change in the gate potentials, the polarizations can be reversed. This polarization effect is clearly associated to a spin-orbital Kondo state having a Kondo peak that originates from spatially separated parts of the device. This fact opens the exciting possibility of experimentally probing the internal structure of an SU(2) Kondo state.

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arXiv2013

Lanczos transformation for quantum impurity problems in d-dimensional lattices: application to graphene nanoribbons

We present a completely unbiased and controlled numerical method to solve quantum impurity problems in d-dimensional lattices. This approach is based on a canonical transformation, of the Lanczos form, where the complete lattice Hamiltonian is exactly mapped onto an equivalent one dimensional system, in the same spirit as Wilson's numerical renormalization. The method is particularly suited to study systems that are inhomogeneous, and/or have a boundary. As a proof of concept, we use the density matrix renormalization group to solve the equivalent one-dimensional problem. The resulting dimensional reduction translates into a reduction of the scaling of the entanglement entropy by a factor $L^{d-1}$, where L is the linear dimension of the original d-dimensional lattice. This allows one to calculate the ground state of a magnetic impurity attached to an LxL square lattice and an LxLxL cubic lattice with L up to 140 sites. We also study the localized edge states in graphene nanoribbons by attaching a magnetic impurity to the edge or the center of the system. For armchair metallic nanoribbons we find a slow decay of the spin correlations as a consequence of the delocalized metallic states. In the case of zigzag ribbons, the decay of the spin correlations depends on the position of the impurity. If the impurity is situated in the bulk of the ribbon, the decay is slow as in the metallic case. On the other hand, if the adatom is attached to the edge, the decay is fast, within few sites of the impurity, as a consequence of the localized edge states, and the short correlation length. The mapping can be combined with ab-initio band structure calculations to model the system, and to understand correlation effects in quantum impurity problems from first principles.

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arXiv2011

Reducing entanglement with symmetries: application to persistent currents in impurity problems

We show how canonical transformations can map problems with impurities coupled to non-interacting rings onto a similar problem with open boundary conditions. The consequent reduction of entanglement, and the fact the density matrix renormalization group (DMRG) is optimally suited for open boundary conditions, increases the efficiency of the method exponentially, making it an unprecedented tool to study persistent currents. We demonstrate its application to the case of the one-channel and two-channel Kondo problems, finding interesting connections between the two.

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arXiv2010

Transport in Carbon Nanotubes: 2LSU(2) regime reveals subtle competition between Kondo and Intermediate Valence states

In this work, we use three different numerical techniques to study the charge transport properties of a system in the two-level SU(2) (2LSU2) regime, obtained from an SU(4) model Hamiltonian by introducing orbital mixing of the degenerate orbitals via coupling to the leads. SU(4) Kondo physics has been experimentally observed, and studied in detail, in Carbon Nanotube Quantum Dots. Adopting a two molecular orbital basis, the Hamiltonian is recast into a form where one of the molecular orbitals decouples from the charge reservoir, although still interacting capacitively with the other molecular orbital. This basis transformation explains in a clear way how the charge transport in this system turns from double- to single-channel when it transitions from the SU(4) to the 2LSU2 regime. The charge occupancy of these molecular orbitals displays gate-potential-dependent occupancy oscillations that arise from a competition between the Kondo and Intermediate Valence states. The determination of whether the Kondo or the Intermediate Valence state is more favorable, for a specific value of gate potential, is assessed by the definition of an energy scale $T_0$, which is calculated through DMRG. We speculate that the calculation of $T_0$ may provide experimentalists with a useful tool to analyze correlated charge transport in many other systems. For that, a current work is underway to improve the numerical accuracy of its DRMG calculation and explore different definitions.

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arXiv2009

Kondo regime in triangular arrangements of quantum dots: Molecular orbitals, interference and contact effects

Transport properties of an interacting triple quantum dot system coupled to three leads in a triangular geometry has been studied in the Kondo regime. Applying mean-field finite-U slave boson and embedded cluster approximations to the calculation of transport properties unveils a set of rich features associated to the high symmetry of this system. Results using both calculation techniques yield excellent overall agreement and provide additional insights into the physical behavior of this interesting geometry. In the case when just two current leads are connected to the three-dot system, interference effects between degenerate molecular orbitals are found to strongly affect the overall conductance. An S=1 Kondo effect is also shown to appear for the perfect equilateral triangle symmetry. The introduction of a third current lead results in an `amplitude leakage' phenomenon, akin to that appearing in beam splitters, which alters the interference effects and the overall conductance through the system.

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arXiv2008

Transport through quantum dots: A combined DMRG and cluster-embedding study

The numerical analysis of strongly interacting nanostructures requires powerful techniques. Recently developed methods, such as the time-dependent density matrix renormalization group (tDMRG) approach or the embedded-cluster approximation (ECA), rely on the numerical solution of clusters of finite size. For the interpretation of numerical results, it is therefore crucial to understand finite-size effects in detail. In this work, we present a careful finite-size analysis for the examples of one quantum dot, as well as three serially connected quantum dots. Depending on odd-even effects, physically quite different results may emerge from clusters that do not differ much in their size. We provide a solution to a recent controversy over results obtained with ECA for three quantum dots. In particular, using the optimum clusters discussed in this paper, the parameter range in which ECA can reliably be applied is increased, as we show for the case of three quantum dots. As a practical procedure, we propose that a comparison of results for static quantities against those of quasi-exact methods, such as the ground-state density matrix renormalization group (DMRG) method or exact diagonalization, serves to identify the optimum cluster type. In the examples studied here, we find that to observe signatures of the Kondo effect in finite systems, the best clusters involving dots and leads must have a total z-component of the spin equal to zero.

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arXiv2008

Transport properties and Kondo correlations in nanostructures: the time-dependent DMRG method applied to quantum dots coupled to Wilson chains

We apply the adaptive time-dependent Density Matrix Renormalization Group method (tDMRG) to the study of transport properties of quantum-dot systems connected to metallic leads. Finite-size effects make the usual tDMRG description of the Kondo regime a numerically demanding task. We show that such effects can be attenuated by describing the leads by "Wilson chains", in which the hopping matrix elements decay exponentially away from the impurity ($t_n \propto Λ^{-n/2}$). For a given system size and in the linear response regime, results for $Λ> 1$ show several improvements over the undamped, $Λ=1$ case: perfect conductance is obtained deeper in the strongly interacting regime and current plateaus remain well defined for longer time scales. Similar improvements were obtained in the finite-bias regime up to bias voltages of the order of the Kondo temperature. These results show that, with the proposed modification, the tDMRG characterization of Kondo correlations in the transport properties can be substantially improved, while it turns out to be sufficient to work with much smaller system sizes. We discuss the numerical cost of this approach with respect to the necessary system sizes and the entanglement growth during the time-evolution.

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arXiv2008

A Novel Approach to Study Highly Correlated Nanostructures: The Logarithmic Discretization Embedded Cluster Approximation

This work proposes a new approach to study transport properties of highly correlated local structures. The method, dubbed the Logarithmic Discretization Embedded Cluster Approximation (LDECA), consists of diagonalizing a finite cluster containing the many-body terms of the Hamiltonian and embedding it into the rest of the system, combined with Wilson's idea of a logarithmic discretization of the representation of the Hamiltonian. The physics associated with both one embedded dot and a double-dot side-coupled to leads is discussed in detail. In the former case, the results perfectly agree with Bethe ansatz data, while in the latter, the physics obtained is framed in the conceptual background of a two-stage Kondo problem. A many-body formalism provides a solid theoretical foundation to the method. We argue that LDECA is well suited to study complicated problems such as transport through molecules or quantum dot structures with complex ground states.

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arXiv2006

New Numerical Results Indicate a Half-Filling SU(4) Kondo State in Carbon Nanotubes

Numerical calculations simulate transport experiments in carbon nanotube quantum dots (P. Jarillo-Herrero et al., Nature 434, 484 (2005)), where a strongly enhanced Kondo temperature T_K ~ 8K was associated with the SU(4) symmetry of the Hamiltonian at quarter-filling for an orbitally double-degenerate single-occupied electronic shell. Our results clearly suggest that the Kondo conductance measured for an adjacent shell with T_K ~ 16K, interpreted as a singlet-triplet Kondo effect, can be associated instead to an SU(4) Kondo effect at half-filling. Besides presenting spin-charge Kondo screening similar to the quarter-filling SU(4), the half-filling SU(4) has been recently associated to very rich physical behavior, including a non-Fermi-liquid state (M. R. Galpin et al., Phys. Rev. Lett. 94, 186406 (2005)).

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arXiv2006

Applying Adaptive Time-Dependent DMRG to Calculate the Conductance of Strongly Correlated Nanostructures

A procedure based on the recently developed ``adaptive'' time-dependent density-matrix-renormalization-group (DMRG) technique is presented to calculate the zero temperature conductance of nanostructures, such as a quantum dots (QD's) or molecular conductors, when represented by a small number of active levels. The leads are modeled using non-interacting tight-binding Hamiltonians. The ground state at time zero is calculated at zero bias. Then, a small bias is applied between the two leads, the wave-function is DMRG evolved in time, and currents are measured as a function of time. Typically, the current is expected to present periodicities over long times, involving intermediate well-defined plateaus that resemble steady states. The conductance can be obtained from those steady-state-like currents. To test this approach, several cases of interacting and non-interacting systems have been studied. Our results show excellent agreement with exact results in the non-interacting case. More importantly, the technique also reproduces quantitatively well-established results for the conductance and local density-of-states in both the cases of one and two coupled interacting QD's. The technique also works at finite bias voltages, and it can be extended to include interactions in the leads.

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arXiv2005

Transport properties of strongly correlated electrons in quantum dots using a simple circuit model

Numerical calculations are shown to reproduce the main results of recent experiments involving nonlocal spin control in nanostructures (N. J. Craig et al., Science 304, 565 (2004)). In particular, the splitting of the zero-bias-peak discovered experimentally is clearly observed in our studies. To understand these results, a simple "circuit model" is introduced and shown to provide a good qualitative description of the experiments. The main idea is that the splitting originates in a Fano anti-resonance, which is caused by having one quantum dot side-connected in relation to the current's path. This scenario provides an explanation of Craig et al.'s results that is alternative to the RKKY proposal, which is here also addressed.

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arXiv2004

Prediction of Ferromagnetic Correlations in Coupled Double-Level Quantum Dots

Numerical results are presented for transport properties of two coupled double-level quantum dots. The results strongly suggest that under appropriate circumstances the dots can develop a novel ferromagnetic (FM) correlation at quarter-filling (one electron per dot). In the strong coupling regime (Coulomb repulsion larger than electron hopping) and with the inter-dot tunneling larger than the tunneling to the leads, an S=1 Kondo resonance develops in the density of states, leading to a peak in the conductance. A qualitative 'phase diagram', incorporating the new FM phase, is presented. It is also shown that the conditions necessary for the FM regime are less restrictive than naively believed, leading to its possible experimental observation in real quantum dots.

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arXiv2004

Effect of topology on the transport properties of two interacting dots

The transport properties of a system of two interacting dots, one of them directly connected to the leads constituting a side-coupled configuration (SCD), are studied in the weak and strong tunnel-coupling limits. The conductance behavior of the SCD structure has new and richer physics than the better studied system of two dots aligned with the leads (ACD). In the weak coupling regime and in the case of one electron per dot, the ACD configuration gives rise to two mostly independent Kondo states. In the SCD topology, the inserted dot is in a Kondo state while the side-connected one presents Coulomb blockade properties. Moreover, the dot spins change their behavior, from an antiferromagnetic coupling to a ferromagnetic correlation, as a consequence of the interaction with the conduction electrons. The system is governed by the Kondo effect related to the dot that is embedded into the leads. The role of the side-connected dot is to introduce, when at resonance, a new path for the electrons to go through giving rise to the interferences responsible for the suppression of the conductance. These results depend on the values of the intra-dot Coulomb interactions. In the case where the many-body interaction is restricted to the side-connected dot, its Kondo correlation is responsible for the scattering of the conduction electrons giving rise to the conductance suppression.

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arXiv2001

Effect of a Variable-Spin Quantum Dot on a Wire Conductance

A numerically exact calculation of the T=0 transport properties of a quantum wire interacting with a lateral two-level quantum dot is presented. The wire conductance is calculated for all different states of charge and spin of the quantum dot. For a dot with two electrons we obtain an enhancement of the Kondo temperature at the singlet-triplet transition and a non-universal scaling law for its dependence upon the dot energy spacing. We find that the Kondo correlation is stronger for a dot spin $S_D \sim 1$ than for $S_D \sim 1/2$. In both cases the wire current is totally quenched by the Kondo effect. When the dot is in the mixed-valence regime and $1/2 < S_D < 1$ the wire conductance is partially quenched except in a very small region of gate potential where it reaches the maximum value $e^2/h$.

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