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C. Aa. Diget

Publications and source records attributed to C. Aa. Diget.

At least 19 recordsLinked to original sources

The impact of $^{17}$O$+α$ reaction rate uncertainties on the s-process in rotating massive stars

Massive stars are crucial to galactic chemical evolution for elements heavier than iron. Their contribution at early times in the evolution of the Universe, however, is unclear due to poorly constrained nuclear reaction rates. The competing $^{17}$O($α,γ$)$^{21}$Ne and $^{17}$O($α,n$)$^{20}$Ne reactions strongly impact weak s-process yields from rotating massive stars at low metallicities. Abundant $^{16}$O absorbs neutrons, removing flux from the s-process, and producing $^{17}$O. The $^{17}$O($α,n$)$^{20}$Ne reaction releases neutrons, allowing continued s-process nucleosynthesis, if the $^{17}$O($α,γ$)$^{21}$Ne reaction is sufficiently weak. While published rates are available, they are based on limited indirect experimental data for the relevant temperatures and, more importantly, no uncertainties are provided. The available nuclear physics has been evaluated, and combined with data from a new study of astrophysically relevant $^{21}$Ne states using the $^{20}$Ne($d,p$)$^{21}$Ne reaction. Constraints are placed on the ratio of the ($α,n$)/($α,γ$) reaction rates with uncertainties on the rates provided for the first time. The new rates favour the ($α,n$) reaction and suggest that the weak s-process in rotating low-metallicity stars is likely to continue up to barium and, within the computed uncertainties, even to lead.

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The MUGAST-AGATA-VAMOS campaign : set-up and performance

The MUGAST-AGATA-VAMOS set-up at GANIL combines the MUGAST highly-segmented silicon array with the state-of-the-art AGATA array and the large acceptance VAMOS spectrometer. The mechanical and electronics integration copes with the constraints of maximum efficiency for each device, in particular γ-ray transparency for the silicon array. This complete set-up offers a unique opportunity to perform exclusive measurements of direct reactions with the radioactive beams from the SPIRAL1 facility. The performance of the set-up is described through its commissioning and two examples of transfer reactions measured during the campaign. High accuracy spectroscopy of the nuclei of interest, including cross-sections and angular distributions, is achieved through the triple-coincidence measurement. In addition, the correction from Doppler effect of the γ-ray energies is improved by the detection of the light particles and the use of two-body kinematics and a full rejection of the background contributions is obtained through the identification of heavy residues. Moreover, the system can handle high intensity beams (up to 108 pps). The particle identification based on the measurement of the time-of-flight between MUGAST and VAMOS and the reconstruction of the trajectories is investigated.

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New experimental $^{23}$Na($α,p$)$^{26}$Mg Reaction Rate for Massive Star and Type-Ia Supernova models

The $^{23}$Na($α,p$)$^{26}$Mg reaction has been identified as having a significant impact on the nucleosynthesis of several nuclei between Ne and Ti in type-Ia supernovae, and of $^{23}$Na and $^{26}$Al in massive stars. The reaction has been subjected to renewed experimental interest recently, motivated by high uncertainties in early experimental data and in the statistical Hauser-Feshbach models used in reaction rate compilations. Early experiments were affected by target deterioration issues and unquantifiable uncertainties. Three new independent measurements instead are utilizing inverse kinematics and Rutherford scattering monitoring to resolve this. In this work we present directly measured angular distributions of the emitted protons to eliminate a discrepancy in the assumptions made in the recent reaction rate measurements, which results in cross sections differing by a factor of 3. We derive a new combined experimental reaction rate for the $^{23}$Na($α,p$)$^{26}$Mg reaction with a total uncertainty of 30% at relevant temperatures. Using our new $^{23}$Na($α,p$)$^{26}$Mg rate, the $^{26}$Al and $^{23}$Na production uncertainty is reduced to within 8%. In comparison, using the factor of 10 uncertainty previously recommended by the rate compilation STARLIB, $^{26}$Al and $^{23}$Na production was changing by more than a factor of 2. In type-Ia supernova conditions, the impact on production of $^{23}$Na is constrained to within 15%.

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Single-particle structure in neutron-rich Sr isotopes approaching the N = 60 shape transition

Background: Neutron-rich nuclei around neutron number N = 60 show a dramatic shape transition from spherical ground states to prolate deformation in 98Sr and heavier nuclei. Purpose: The purpose of this study is to investigate the single-particle structure approaching the shape transitional region. Method: The level structures of neutron-rich 93,94,95Sr were studied via the d(94,95,96Sr,t) one-neutron stripping reactions at TRIUMF using a beam energy of 5.5 AMeV. γ-rays emitted from excited states and recoiling charged particles were detected by using the TIGRESS and SHARC arrays, respectively. States were identified by gating on the excitation energy and, if possible, the coincident γ radiation. Results: Triton angular distributions for the reactions populating states in ejectile nuclei 93,94,95Sr were compared with distorted wave Born approximation calculations to assign and revise spin and parity quantum numbers and extract spectroscopic factors. The results were compared with shell model calculations and the reverse (d,p) reactions and good agreement was obtained. Conclusions: The results for the d(94Sr,t)93Sr and d(95Sr,t)94Sr reactions are in good agreement with shell model calculations. A two level mixing analysis for the 0+ states in 94Sr suggest strong mixing of two shapes. For the d(96Sr,t)95Sr reaction the agreement with the shell model is less good. The configuration of the ground state of 96Sr is already more complex than predicted, and therefore indications for the shape transition can already be observed before N = 60.

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Experimental identification of the $T = 1$, $J^π = 6^+$ state of $^{54}$Co and isospin symmetry in $A = 54$ studied via one-nucleon knockout reactions

New experimental data obtained from $γ$-ray tagged one-neutron and one-proton knockout from $^{55}$Co is presented. A candidate for the sought-after $T=1, T_z = 0, J^π = 6^+$ state in $^{54}$Co is proposed based on a comparison to the new data on $^{54}$Fe, the corresponding observables predicted by large-scale-shell-model (LSSM) calculations in the full $fp$-model space employing charge-dependent contributions, and isospin-symmetry arguments. Furthermore, possible isospin-symmetry breaking in the $A=54$, $T=1$ triplet is studied by calculating the experimental $c$ coefficients of the isobaric mass multiplet equation (IMME) up to the maximum possible spin $J=6$ expected for the $(1f_{7/2})^{-2}$ two-hole configuration relative to the doubly-magic nucleus $^{56}$Ni. The experimental quantities are compared to the theoretically predicted $c$ coefficients from LSSM calculations using two-body matrix elements obtained from a realistic chiral effective field theory potential at next-to-next-to-next-to-leading order (N$^3$LO).

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Single-Particle Structure of Neutron-Rich Sr Isotopes Via d( 94,95,96 Sr, p) Reactions

The region around neutron number N = 60 in the neutron-rich Sr and Zr nuclei is one of the most dramatic examples of a ground state shape transition from (near) spherical below N = 60 to strongly deformed shapes in the heavier isotopes. The single-particle structure of 95-97Sr approaching the ground state shape transition at 98 Sr has been investigated via single-neutron transfer reactions using the (d, p) reaction in inverse kinematics. These reactions selectively populate states with a large overlap of the projectile ground state coupled to a neutron in a single-particle orbital. Radioactive 94,95,96Sr nuclei with energies of 5.5 AMeV were used to bombard a CD 2 target. Recoiling light charged particles and γ rays were detected using a quasi-4π silicon strip detector array and a 12 element Ge array. The excitation energy of states populated was reconstructed employing the missing mass method combined with γ-ray tagging and differential cross sections for final states were extracted. A reaction model analysis of the angular distributions allowed for firm spin assignments to be made for the low-lying 352, 556 and 681 keV excited states in 95Sr and a constraint has been placed on the spin of the higher-lying 1666 keV state. Angular distributions have been extracted for 10 states populated in the d(95Sr,p)96Sr reaction, and constraints have been provided for the spins and parities of several final states. Results are compared to shell model calculations in several model spaces and the structure of low-lying states in 94Sr and 95Sr is well-described. The spectroscopic strength of the 0+ and 2 states in 96Sr is significantly more fragmented than predicted.

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A direct measurement of the 17O(a,g)21Ne reaction in inverse kinematics and its impact on heavy element production

During the slow neutron capture process in massive stars, reactions on light elements can both produce and absorb neutrons thereby influencing the final heavy element abundances. At low metallicities, the high neutron capture rate of 16-O can inhibit s-process nucleosynthesis unless the neutrons are recycled via the 17O(a,n)20Ne reaction. The efficiency of this neutron recycling is determined by competition between the 17O(a,n)20Ne and 17O(a,g)21Ne reactions. While some experimental data are available on the former reaction, no data exist for the radiative capture channel at the relevant astrophysical energies. The 17O(a,g)21Ne reaction has been studied directly using the DRAGON recoil separator at the TRIUMF Laboratory. The reaction cross section has been determined at energies between 0.6 and 1.6 MeV Ecm, reaching into the Gamow window for core helium burning for the first time. Resonance strengths for resonances at 0.63, 0.721, 0.81 and 1.122 MeV Ecm have been extracted. The experimentally based reaction rate calculated represents a lower limit, but suggests that significant s-process nucleosynthesis occurs in low metallicity massive stars.

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One-proton and one-neutron knockout reactions from $N = Z = 28$ $^{56}$Ni to the $A = 55$ mirror pair $^{55}$Co and $^{55}$Ni

We present a high-resolution in-beam $γ$-ray spectroscopy study of excited states in the mirror nuclei $^{55}$Co and $^{55}$Ni following one-nucleon knockout from a projectile beam of $^{56}$Ni. The newly determined partial cross sections and the $γ$-decay properties of excited states provide a test of state-of-the-art nuclear structure models and probe mirror symmetry in unique ways. A mirror asymmetry for the partial cross sections leading to the two lowest $3/2^-$ states in the $A = 55$ mirror pair was identified as well as a significant difference in the $E1$ decays from the $1/2^+_1$ state to the same two $3/2^-$ states. The mirror asymmetry in the partial cross sections cannot be reconciled with the present shell-model picture or small mixing introduced in a two-state model. The observed mirror asymmetry in the $E1$ decay pattern, however, points at stronger mixing between the two lowest $3/2^-$ states in $^{55}$Co than in its mirror $^{55}$Ni.

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Shell evolution approaching the N=20 island of inversion: Structure of 29Mg

The "Island of Inversion" for neutron-rich nuclei in the vicinity of N=20 has become the testing ground par excellence for our understanding and modelling of shell evolution with isospin. In this context, the structure of the transitional nucleus 29Mg is critical. The first quantitative measurements of the single particle structure of 29Mg are reported, using data from the d(28Mg,p gamma)29Mg reaction. Two key states carrying significant ell=3 (f-wave) strength were identified at 2.40 +/- 0.10 (Jpi = 5/2-) and 4.28 +/- 0.04 MeV (7/2-). New state-of-the-art shell model calculations have been performed and the predictions are compared in detail with the experimental results. Whilst the two lowest 7/2- levels are well described, the sharing of single-particle strength disagrees with experiment for both the 3/2- and 5/2- levels and there appear to be general problems with configurations involving the p3/2 neutron orbital and core-excited components. These conclusions are supported by an analysis of the neutron occupancies in the shell model calculations.

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Shape Coexistence and Mixing of Low-Lying $0^+$ States in $^{96}$Sr

The low energy excited $0_{2,3}^+$ states in $^{96}$Sr are amongst the most prominent examples of shape coexistence across the nuclear landscape. In this work, the neutron $[2s_{1/2}]^2$ content of the $0_{1,2,3}^+$ states in $^{96}$Sr was determined by means of the d($^{95}$Sr,p) transfer reaction at the TRIUMF-ISAC2 facility using the SHARC and TIGRESS arrays. Spectroscopic factors of 0.19(3) and 0.22(3) were extracted for the $^{96}$Sr ground and 1229~keV $0^+$ states, respectively, by fitting the experimental angular distributions to DWBA reaction model calculations. A detailed analysis of the $γ$-decay of the isomeric $0_3^+$ state was used to determine a spectroscopic factor of 0.33(13). The experimental results are compared to shell model calculations, which predict negligible spectroscopic strength for the excited $0^+$ states in $^{96}$Sr. The strengths of the excited $0_{2,3}^+$ states were also analyzed within a two-level mixing model and are consistent with a mixing strength of $a^2$=0.40(14) and a difference in intrinsic deformations of $|Δβ|=0.31(3)$. These results suggest coexistence of three different configurations in $^{96}$Sr and strong shape mixing of the two excited $0^+$ states.

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CAKE: The Coincidence Array for K600 Experiments

The combination of a magnetic spectrometer and ancillary detectors such as silicon detectors is a powerful tool for the study of nuclear reactions and nuclear structure. This paper discusses the recently commissioned silicon array called the CAKE which is designed for use with the K600 magnetic spectrometer at iThemba LABS.

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Characterization of the proposed 4-α cluster state candidate in 16O

The $\mathrm{^{16}O}(α, α^{\prime})$ reaction was studied at $θ_{lab} = 0^\circ$ at an incident energy of $\textrm{E}_{lab}$ = 200 MeV using the K600 magnetic spectrometer at iThemba LABS. Proton and $α$-decay from the natural parity states were observed in a large-acceptance silicon-strip detector array at backward angles. The coincident charged particle measurements were used to characterize the decay channels of the $0_{6}^{+}$ state in $\mathrm{^{16}O}$ located at $E_{x} = 15.097(5)$ MeV. This state is identified by several theoretical cluster calculations to be a good candidate for the 4-$α$ cluster state. The results of this work suggest the presence of a previously unidentified resonance at $E_{x}\approx15$ MeV that does not exhibit a $0^{+}$ character. This unresolved resonance may have contaminated previous observations of the $0_{6}^{+}$ state.

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Binding Blocks: building the Universe one nucleus at the time

We present a new teaching and outreach activity based around the construction of a three-dimensional chart of isotopes using LEGO$^{\circledR}$ bricks. The activity, \emph{Binding Blocks}, demonstrates nuclear and astrophysical processes through a seven-meter chart of all nuclear isotopes, built from over 26,000 LEGO$^{\circledR}$ bricks. It integrates A-level and GCSE curricula across areas of nuclear physics, astrophysics, and chemistry, including: nuclear decays (through the colours in the chart); nuclear binding energy (through tower heights); production of chemical elements in the cosmos; fusion processes in stars and fusion energy on Earth; as well as links to medical physics, particularly diagnostics and radiotherapy.

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Shell evolution approaching the N=20 island of inversion: structure of 26Na

The levels in 26Na with single particle character have been observed for the first time using the d(25Na,p gamma) reaction at 5 MeV/nucleon. The measured excitation energies and the deduced spectroscopic factors are in good overall agreement with (0+1) hbar-omega shell model calculations performed in a complete spsdfp basis and incorporating a reduction in the N=20 gap. Notably, the 1p3/2 neutron configuration was found to play an enhanced role in the structure of the low-lying negative parity states in 26Na, compared to the isotone 28Al. Thus, the lowering of the 1p3/2 orbital relative to the 0f7/2 occurring in the neighbouring Z=10 and 12 nuclei -- 25,27Ne and 27,29Mg -- is seen also to occur at Z=11 and further strengthens the constraints on the modelling of the transition into the island of inversion.

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The 23Na(α,p) 26Mg reaction rate at astrophysically relevant energies

The production of 26 Al in massive stars is sensitive to the 23 Na(a,p) 26 Mg cross section. Recent experimental data suggest the currently recommended cross sections are underestimated by a factor of 40. We present here differential cross sections for the 23 Na(a,p) 26 Mg reaction measured in the energy range E c.m. = 1.7 - 2.5 MeV. Concurrent measurements of Rutherford scattering provide absolute normalisations which are independent of variations in target properties. Angular distributions were measured for both p 0 and p 1 permitting the determination of total cross sections. The results show no significant deviation from the statistical model calculations upon which the recommended rates are based. We therefore retain the previous recommendation without the increase in cross section and resulting stellar reaction rates of a factor of 40, impacting on the 26 Al yield from massive stars by more than a factor of three.

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Two-neutron transfer reaction mechanisms in $^{12}$C($^6$He,$^{4}$He)$^{14}$C using a realistic three-body $^{6}$He model

The reaction mechanisms of the two-neutron transfer reaction $^{12}$C($^6$He,$^4$He) have been studied at 30 MeV at the TRIUMF ISAC-II facility using the SHARC charged-particle detector array. Optical potential parameters have been extracted from the analysis of the elastic scattering angular distribution. The new potential has been applied to the study of the transfer angular distribution to the 2$^+_2$ 8.32 MeV state in $^{14}$C, using a realistic 3-body $^6$He model and advanced shell model calculations for the carbon structure, allowing to calculate the relative contributions of the simultaneous and sequential two-neutron transfer. The reaction model provides a good description of the 30 MeV data set and shows that the simultaneous process is the dominant transfer mechanism. Sensitivity tests of optical potential parameters show that the final results can be considerably affected by the choice of optical potentials. A reanalysis of data measured previously at 18 MeV however, is not as well described by the same reaction model, suggesting that one needs to include higher order effects in the reaction mechanism.

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Mirror Energy Differences at Large Isospin Studied through Direct Two-Nucleon Knockout

The first spectroscopy of excited states in 52Ni (Tz=2) and 51Co (Tz=-3/2) has been obtained using the highly selective two-neutron knockout reaction. Mirror energy differences between isobaric analogue states in these nuclei and their mirror partners are interpreted in terms of isospin nonconserving effects. A comparison between large scale shell-model calculations and data provides the most compelling evidence to date that both electromagnetic and an additional isospin nonconserving interactions for J=2 couplings, of unknown origin, are required to obtain good agreement.

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In-beam gamma-ray spectroscopy of very neutron-rich nuclei: Excited states in 46S and 48Ar

We report on the first in-beam gamma-ray spectroscopy study of the very neutron-rich nucleus 46S. The N=30 isotones 46S and 48Ar were produced in a novel way in two steps that both necessarily involve nucleon exchange and neutron pickup reactions, 9Be(48Ca,48K)X followed by 9Be(48K,48Ar+gamma)X at 85.7 MeV/u mid-target energy and 9Be(48Ca,46Cl)X followed by 9Be(46Cl,46S+gamma)X at 87.0 MeV/u mid-target energy, respectively. The results are compared to large-scale shell-model calculations in the sdpf shell using the SDPF-NR effective interaction and Z-dependent modifications.

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