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C. Andreoiu

Publications and source records attributed to C. Andreoiu.

At least 37 records · Page 2Linked to original sources

Collision-Induced Dissociation at TRIUMF's Ion Trap for Atomic and Nuclear science

The performance of high-precision mass spectrometry of radioactive isotopes can often be hindered by large amounts of contamination, including molecular species, stemming from the production of the radioactive beam. In this paper, we report on the development of Collision-Induced Dissociation (CID) as a means of background reduction for experiments at TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). This study was conducted to characterize the quality and purity of radioactive ion beams and the reduction of molecular contaminants to allow for mass measurements of radioactive isotopes to be done further from nuclear stability. This is the first demonstration of CID at an ISOL-type radioactive ion beam facility, and it is shown that molecular contamination can be reduced up to an order of magnitude.

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Improved measurement of the $0_2^+\rightarrow0_1^+$ E0 transition strength for $^{72}$Se using the SPICE spectrometer

The selenium isotopes lie at the heart of a tumultuous region of the nuclear chart where shape coexistence effects grapple with neutron-proton pairing correlations, triaxiality, and the impending proton dripline. In this work a study of $^{72}$Se by internal conversion electron and $γ$-ray spectroscopy was undertaken with the SPICE and TIGRESS arrays. New measurements of the branching ratio and lifetime of the $0_2^+$ state were performed yielding a determination of $ρ^2(E0;0_2^+{\rightarrow}0_1^+)=29(3)$ milliunits. two state mixing calculations were performed that highlighted the importance of interpretation of such $E0$ strength values in the context of shape-coexistence.

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Summit of the N=40 Island of Inversion: precision mass measurements and ab initio calculations of neutron-rich chromium isotopes

Mass measurements continue to provide invaluable information for elucidating nuclear structure and scenarios of astrophysical interest. The transition region between the $Z = 20$ and $28$ proton shell closures is particularly interesting due to the onset and evolution of nuclear deformation as nuclei become more neutron rich. This provides a critical testing ground for emerging ab-initio nuclear structure models. Here, we present high-precision mass measurements of neutron-rich chromium isotopes using the sensitive electrostatic Multiple-Reflection Time-Of-Flight Mass Spectrometer (MR-TOF-MS) at TRIUMF's Ion Trap for Atomic and Nuclear Science (TITAN) facility. Our high-precision mass measurements of $^{59, 61-63}$Cr confirm previous results, and the improved precision in measurements of $^{64-65}$Cr refine the mass surface beyond N=40. With the ab initio in-medium similarity renormalization group, we examine the trends in collectivity in chromium isotopes and give a complete picture of the N=40 island of inversion from calcium to nickel.

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High-precision half-life determination of $^{14}$O via direct $β$ counting

The half-life of the superallowed Fermi $β^+$ emitter $^{14}$O was determined to high precision via a direct $β$ counting experiment performed at the Isotope Separator and Accelerator (ISAC) facility at TRIUMF. The result, $T_{1/2}$($^{14}$O) = 70619.2(76) ms, is consistent with, but is more precise than, the world average obtained from 11 previous measurements. Combining the $^{14}$O half-life deduced in the present work with the previous most precise measurements of this quantity leads to a reduction in the overall uncertainty, by nearly a factor of 2. The new world average is $T_{1/2}$($^{14}$O) = 70619.6(63) ms with a reduced $χ^2$ value of 0.87 obtained from 8 degrees of freedom.

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Coulomb excitation of the $\left|T_z\right|=\frac{1}{2}$, $A=23$ mirror pair

Background: Electric-quadrupole ($E2$) strengths relate to the underlying quadrupole deformation of a nucleus and present a challenge for many nuclear theories. Mirror nuclei in the vicinity of the line of $N=Z$ represent a convenient laboratory for testing deficiencies in such models, making use of the isospin-symmetry of the systems. Purpose: Uncertainties associated with literature $E2$ strengths in \textsuperscript{23}Mg are some of the largest in $T_z=\left|\frac{1}{2}\right|$ nuclei in the $sd$-shell. The purpose of the present work is to improve the precision with which these values are known, to enable better comparison with theoretical models. Methods: Coulomb-excitation measurements of $^{23}$Mg and $^{23}$Na were performed at the TRIUMF-ISAC facility using the TIGRESS spectrometer. They were used to determine the $E2$ matrix elements of mixed $E2$/$M1$ transitions. Results: Reduced $E2$ transition strengths, $B(E2)$, were extracted for \textsuperscript{23}Mg and \textsuperscript{23}Na. Their precision was improved by factors of approximately six for both isotopes, while agreeing within uncertainties with previous measurements. Conclusions: A comparison was made with both shell-model and {\it ab initio} valence-space in-medium similarity renormalization group calculations. Valence-space in-medium similarity-renormalization-group calculations were found to underpredict the absolute $E2$ strength - in agreement with previous studies.

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Structure of $^{83}$As, $^{85}$As and $^{87}$As: from semi-magicity to $γ$-softness

The structure of $^{83}$As, $^{85}$As and $^{87}$As have been studied in fusion-fission reaction $^{238}$U+$^9$Be. Fission fragments were identified in mass and atomic number using the VAMOS++ spectrometer and the coincident $γ$-rays were detected in the $γ$-ray tracking array AGATA. New transitions in $^{83}$As and $^{85}$As are reported and placed in the level schemes. A level scheme of the excited states in $^{87}$As is proposed for the first time. The data are interpreted in frame of Large-Scale Shell-Model calculations, SU3 symmetries and Beyond Mean-Field frameworks. A spherical regime at magic number $N$=50 is predicted and the location of the proton $g_{9/2}$ orbital is proposed for the first time. Development of collectivity in a prolate deformed, $γ$-soft regime in the open shell cases $^{85}$As and $^{87}$As, most neutron-rich isotopes beyond $N$=50, is concluded. Data and theoretical calculations give confidence to a relatively high extrapolated excitation energy about 4 MeV of the $9/2^+$ state in $^{79}$Cu, one proton above $^{78}$Ni.

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Use of Bayesian Optimization to Understand the Structure of Nuclei

Monte Carlo simulations are widely used in nuclear physics to model experimental systems. In cases where there are significant unknown quantities, such as energies of states, an iterative process of simulating and fitting is often required to describe experimental data. We describe a Bayesian approach to fitting experimental data, designed for data from a $^{12}$Be(d,p) reaction measurement, using simulations made with GEANT4. Q-values from the $^{12}$C(d,p) reaction to well-known states in $^{13}$C are compared with simulations using BayesOpt. The energies of the states were not included in the simulation to reproduce the situation for $^{13}$Be where the states are poorly known. Both cases had low statistics and significant resolution broadening owing to large proton energy losses in the solid deuterium target. Excitation energies of the lowest three excited states in $^{13}$C were extracted to better than 90 keV, paving a way for extracting information on $^{13}$Be.

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LEGEND-1000 Preconceptual Design Report

We propose the construction of LEGEND-1000, the ton-scale Large Enriched Germanium Experiment for Neutrinoless $ββ$ Decay. This international experiment is designed to answer one of the highest priority questions in fundamental physics. It consists of 1000 kg of Ge detectors enriched to more than 90% in the $^{76}$Ge isotope operated in a liquid argon active shield at a deep underground laboratory. By combining the lowest background levels with the best energy resolution in the field, LEGEND-1000 will perform a quasi-background-free search and can make an unambiguous discovery of neutrinoless double-beta decay with just a handful of counts at the decay $Q$ value. The experiment is designed to probe this decay with a 99.7%-CL discovery sensitivity in the $^{76}$Ge half-life of $1.3\times10^{28}$ years, corresponding to an effective Majorana mass upper limit in the range of 9-21 meV, to cover the inverted-ordering neutrino mass scale with 10 yr of live time.

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First direct measurement of $^{59}$Cu(p,$α$)$^{56}$Ni: A step towards constraining the Ni-Cu cycle in the Cosmos

Reactions on the proton-rich nuclides drive the nucleosynthesis in Core-Collapse Supernovae (CCSNe) and in X-ray bursts (XRBs). CCSNe eject the nucleosynthesis products to the interstellar medium and hence are a potential inventory of p-nuclei, whereas in XRBs nucleosynthesis powers the light curves. In both astrophysical sites the Ni-Cu cycle, which features a competition between $^{59}$Cu(p,$α$)$^{56}$Ni and $^{59}$Cu(p,$γ$)$^{60}$Zn, could potentially halt the production of heavier elements. Here, we report the first direct measurement of $^{59}$Cu(p,$α$)$^{56}$Ni using a re-accelerated $^{59}$Cu beam and cryogenic solid hydrogen target. Our results show that the reaction proceeds predominantly to the ground state of $^{56}$Ni and the experimental rate has been found to be lower than Hauser-Feshbach-based statistical predictions. New results hint that the $νp$-process could operate at higher temperatures than previously inferred and therefore remains a viable site for synthesizing the heavier elements.

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Evidence against the wobbling nature of low-spin bands in $^{135}$Pr

The electromagnetic character of the $ΔI=1$ transitions connecting the one- to zero-phonon and the two- to one-phonon wobbling bands should be dominated by an $E2$ component, due to the collective motion of the entire nuclear charge. In the present work it is shown, based on combined angular correlation and linear polarization measurements, that the mixing ratios of all analyzed connecting transitions between low-lying bands in $^{135}$Pr interpreted as zero-, one-, and two-phonon wobbling bands, have absolute values smaller than one. This indicates predominant $M1$ magnetic character, which is incompatible with the proposed wobbling nature. All experimental observables are instead in good agreement with quasiparticle-plus-triaxial-rotor model calculations, which describe the bands as resulting from a rapid re-alignment of the total angular momentum from the short to the intermediate nuclear axis.

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Spectroscopic studies of neutron-rich $^{129}$In and its $β$-decay daughter, $^{129}$Sn, using the GRIFFIN spectrometer

The $β$-decay of neutron-rich $^{129}$In into $^{129}$Sn was studied using the GRIFFIN spectrometer at the ISAC facility at TRIUMF. The study observed the half-lives of the ground state and each of the $β$-decaying isomers. The level scheme of $^{129}$Sn has been expanded with thirty-one new $γ$-ray transitions and nine new excited levels, leading to a re-evaluation of the $β$-branching ratios and level spin assignments. The observation of the $β$-decay of the (29/2$^{+}$) 1911-keV isomeric state in $^{129}$In is reported for the first time, with a branching ratio of 2.0(5)$\%$.

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High-Precision Branching Ratio Measurement and Spin Assignment Implications for $^{62}$Ga Superallowed $β$ Decay

A high-precision branching ratio measurement for the superallowed Fermi $β^{+}$ emitter $^{62}$Ga was performed with the Gamma-Ray Infrastructure for Fundamental Investigations of Nuclei (GRIFFIN) spectrometer at the Isotope Separator and Accelerator (ISAC) radioactive ion beam facility at TRIUMF. The high efficiency of the GRIFFIN spectrometer allowed 63 $γ$-ray transitions, with intensities down to $\approx$1 part per million (ppm) per $^{62}$Ga $β^{+}$ decay, to be placed in the level scheme of the daughter nucleus $^{62}$Zn, establishing the superallowed $β$ branching ratio for $^{62}$Ga decay to be 99.8577$^{+0.0023}_{-0.0029}\%$, a factor of 4 more precise than the previous world average. For several cascades, $γ-γ$ angular correlation measurements were performed to assign spins and/or determine the mixing ratios of transitions. In particular, the spin of the 2.342 MeV excited state in the daughter nucleus $^{62}$Zn was definitively assigned as $J = 0$. This assignment resolves a discrepancy between previous measurements and has important implications for the isospin symmetry breaking correction, $δ_{C1}$, in $^{62}$Ga superallowed Fermi $β$ decay.

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Spectroscopic study of $^{47}$Ca from the $β^-$ decay of $^{47}$K

The $β^-$ decay of $^{47}$K to $^{47}$Ca is an appropriate mechanism for benchmarking interactions spanning the $sd$ and $pf$ shells, but current knowledge of the $β^-$-decay scheme is limited. We have performed a high-resolution, high-efficiency study of the $β^-$-decay of $^{47}$K with the GRIFFIN spectrometer at TRIUMF-ISAC. The study revealed 48 new transitions, a more precise value for the $^{47}$K half-life (17.38(3)~s), and new spin and parity assignments for eight excited states. Levels placed for the first time here raise the highest state observed in $β^-$ decay to within 568(3) keV of the $Q$-value and confirm the previously measured large $β^-$-decay branching ratios to the low-lying states. Previously unobserved $β^-$-feeding to 3/2$^+$ states between 4.5 and 6.1~MeV excitation energy was identified with a total $β^-$-feeding intensity of 1.29(2)\%. The sum of the $B(GT)$ values for these states indicates that the $1s_{1/2}$ proton hole strength near this excitation energy is comparable to the previously known $1s_{1/2}$ proton and neutron hole strengths near 2.6 MeV.

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Absence of Low-Energy Shape Coexistence in $^{80}$Ge: The Nonobservation of a Proposed Excited 0$_2^+$ Level at 639 keV

The $^{80}$Ge structure was investigated in a high-statistics $β$-decay experiment of $^{80}$Ga using the GRIFFIN spectrometer at TRIUMF-ISAC through $γ$, $β$-$e$, $e$-$γ$ and $γ$-$γ$ spectroscopy. No evidence was found for the recently reported 0$_2^{+}$ 639-keV level suggested as evidence for low-energy shape coexistence in $^{80}$Ge. Large-scale shell model calculations performed in $^{78,80,82}$Ge place the $0^{+}_{2}$ level in $^{80}$Ge at 2\,MeV. The new experimental evidence combined with shell model predictions indicate that low-energy shape coexistence is not present in $^{80}$Ge.

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Multiple chiral bands in $^{137}$Nd

Two new bands have been identified in $^{137}$Nd from a high-statistics JUROGAM II gamma-ray spectroscopy experiment. Constrained density functional theory and particle rotor model calculations are used to assign configurations and investigate the band properties, which are well described and understood. It is demonstrated that these two new bands can be interpreted as chiral partners of previously known three-quasiparticle positive- and negative-parity bands. The newly observed chiral doublet bands in $^{137}$Nd represent an important support to the existence of multiple chiral bands in nuclei. The present results constitute the missing stone in the series of Nd nuclei showing multiple chiral bands, which becomes the most extended sequence of nuclei presenting multiple chiral bands in the Segré chart.

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Single-particle structure in neutron-rich Sr isotopes approaching the N = 60 shape transition

Background: Neutron-rich nuclei around neutron number N = 60 show a dramatic shape transition from spherical ground states to prolate deformation in 98Sr and heavier nuclei. Purpose: The purpose of this study is to investigate the single-particle structure approaching the shape transitional region. Method: The level structures of neutron-rich 93,94,95Sr were studied via the d(94,95,96Sr,t) one-neutron stripping reactions at TRIUMF using a beam energy of 5.5 AMeV. γ-rays emitted from excited states and recoiling charged particles were detected by using the TIGRESS and SHARC arrays, respectively. States were identified by gating on the excitation energy and, if possible, the coincident γ radiation. Results: Triton angular distributions for the reactions populating states in ejectile nuclei 93,94,95Sr were compared with distorted wave Born approximation calculations to assign and revise spin and parity quantum numbers and extract spectroscopic factors. The results were compared with shell model calculations and the reverse (d,p) reactions and good agreement was obtained. Conclusions: The results for the d(94Sr,t)93Sr and d(95Sr,t)94Sr reactions are in good agreement with shell model calculations. A two level mixing analysis for the 0+ states in 94Sr suggest strong mixing of two shapes. For the d(96Sr,t)95Sr reaction the agreement with the shell model is less good. The configuration of the ground state of 96Sr is already more complex than predicted, and therefore indications for the shape transition can already be observed before N = 60.

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Decay Spectroscopy of $^{129}$Cd

Excited states of $^{129}$In populated following the $β$-decay of $^{129}$Cd were experimentally studied with the GRIFFIN spectrometer at the ISAC facility of TRIUMF, Canada. A 480-MeV proton beam was impinged on a uranium carbide target and $^{129}$Cd was extracted using the Ion Guide Laser Ion Source (IG-LIS). $β$- and $γ$-rays following the decay of $^{129}$Cd were detected with the GRIFFIN spectrometer comprising the plastic scintillator SCEPTAR and 16 high-purity germanium (HPGe) clover-type detectors. %, along with the $β$-particles were detected with SCEPTAR. From the $β$-$γ$-$γ$ coincidence analysis, 32 new transitions and 7 new excited states were established, expanding the previously known level scheme of $^{129}$In. The $\log ft$ values deduced from the $β$-feeding intensities suggest that some of the high-lying states were populated by the $ν0 g_{7/2} \rightarrow π0 g_{9/2}$ allowed Gamow-Teller (GT) transition, which indicates that the allowed GT transition is more dominant in the $^{129}$Cd decay than previously reported. Observation of fragmented Gamow-Teller strengths is consistent with theoretical calculations.

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$β$ Decay of $^{132}$In and Spectroscopy of $^{132}$Sn and $^{131}$Sb with the GRIFFIN Spectrometer

Spectroscopy of doubly magic $^{132}_{50}$Sn$_{82}$ has been performed with the GRIFFIN spectrometer at TRIUMF-ISAC following the $β$ decay of $^{132}_{49}$In$_{83}$. The analysis has allowed for the placement of a total of 70 transitions and 29 excited states in $^{132}$Sn. Detailed spectroscopy has also been performed on $^{131}$Sb, resulting from the $β$ decay of $^{131}$Sn, produced from the $β$-delayed neutron decay of $^{132}$In. Measurement of $γ$-rays in both $^{131}$Sn and $^{131}$Sb has led to the determination of the $β$-delayed neutron emission probability, $P_{n}$, from $^{132}$In. This is the first time the $P_{n}$ has been measured for this nucleus using $γ$ spectroscopy, and the new value of 12.3(4)% is consistent with the most recent $β-n$ counting experiment. Additionally, $γ$-$γ$ angular correlations have been performed in $^{132}$Sn, supporting the spin assignments of several excited states. Novel ab initio calculations are presented which describe several of the excited states, and these are compared to the experimental spectrum.

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