arXiv subjects
Publications and source records attributed to C. Antón.
In this manuscript we will gather clear experimental evidences of remote coherence between two polariton condensate droplets that have never overlapped in real space and discuss how these interferences in momentum space can be used to estimate the critical temperature for the BEC like transition.
Developing future quantum communication may rely on the ability to engineer cavity-mediated interactions between photons and solid-state artificial atoms, in a deterministic way. Here, we report a set of technological and experimental developments for the deterministic coupling between the optical mode of a micropillar cavity and a quantum dot trion transition. We first identify a charged transition through in-plane magnetic field spectroscopy, and then tune the optical cavity mode to its energy via in-situ lithography. In addition, we design an asymmetric tunneling barrier to allow the optical trapping of the charge, assisted by a quasi-resonant pumping scheme, in order to control its occupation probability. We evaluate the generation of a positively-charged quantum dot through second order auto-correlation measurements of its resonance fluorescence, and the quality of light-matter interaction for these spin-photon interfaces is assessed by measuring the performance of the device as a single-photon source.
Light states composed of multiple entangled photons - such as cluster states - are essential for developing and scaling-up quantum computing networks. Photonic cluster states with discrete variables can be obtained from single-photon sources and entangling gates, but so far this has only been done with probabilistic sources constrained to intrinsically-low efficiencies, and an increasing hardware overhead. Here, we report the resource-efficient generation of polarization-encoded, individually-addressable, photons in linear cluster states occupying a single spatial mode. We employ a single entangling-gate in a fiber loop configuration to sequentially entangle an ever-growing stream of photons originating from the currently most efficient single-photon source technology - a semiconductor quantum dot. With this apparatus, we demonstrate the generation of linear cluster states up to four photons in a single-mode fiber. The reported architecture can be programmed to generate linear-cluster states of any number of photons with record scaling ratios, potentially enabling practical implementation of photonic quantum computing schemes.
Scaling-up optical quantum technologies requires to combine highly efficient multi-photon sources and integrated waveguide components. Here, we interface these scalable platforms: a quantum dot based multi-photon source and a reconfigurable photonic chip on glass are combined to demonstrate high-rate three-photon interference. The temporal train of single-photons obtained from a quantum emitter is actively demultiplexed to generate a 3.8 kHz three-photon source, which is then sent to the input of a tuneable tritter circuit, demonstrating the on-chip quantum interference of three indistinguishable single-photons. Pseudo number-resolving photon detection characterising the output distribution shows that this first combination of scalable sources and reconfigurable photonic circuits compares favourably in performance with respect to previous implementations. A detailed loss-budget shows that merging solid-state based multi-photon sources and reconfigurable photonic chips could allow ten-photon experiments on chip at ${\sim}40$ Hz rate in a foreseeable future.
The ability to generate light in a pure quantum state is essential for advances in optical quantum technologies. However, obtaining quantum states with control in the photon-number has remained elusive. Optical light fields with zero and one photon can be produced by single atoms, but so far it has been limited to generating incoherent mixtures, or coherent superpositions with a very small one-photon term. Here, we report on the on-demand generation of quantum superpositions of zero, one, and even two photons, via pulsed coherent control of a single artificial atom. Driving the system up to full atomic inversion leads to the generation of quantum superpositions of vacuum and one photon, with their relative populations controlled by the driving laser intensity. A stronger driving of the system, with $2π$-pulses, results in a coherent superposition of vacuum, one and two photons, with the two-photon term exceeding the one-photon component, a state allowing phase super-resolving interferometry. Our results open new paths for optical quantum technologies with access to the photon-number degree-of-freedom.
Pillar microcavities are excellent light-matter interfaces providing an electromagnetic confinement in small mode volumes with high quality factors. They also allow the efficient injection and extraction of photons, into and from the cavity, with potentially near-unity input and output-coupling efficiencies. Optimizing the input and output coupling is essential, in particular, in the development of solid-state quantum networks where artificial atoms are manipulated with single incoming photons. Here we propose a technique to accurately measure input and output coupling efficiencies using polarization tomography of the light reflected by the cavity. We use the residual birefringence of pillar microcavities to distinguish the light coupled to the cavity from the uncoupled light: the former participates to rotating the polarization of the reflected beam, while the latter decreases the polarization purity. Applying this technique to a micropillar cavity, we measure a $53 \pm2 \% $ output coupling and a $96 \pm 1\%$ input coupling with unprecedented precision.
Path-entangled N-photon states can be obtained through the coalescence of indistinguishable photons inside linear networks. They are key resources for quantum enhanced metrology, quantum imaging, as well as quantum computation based on quantum walks. However, the quantum tomography of path-entangled indistinguishable photons is still in its infancy as it requires multiple phase estimations increasing rapidly with N. Here, we propose and implement a method to measure the quantum tomography of path-entangled two-photon states. A two-photon state is generated through the Hong-Ou-Mandel interference of highly indistinguishable single photons emitted by a semiconductor quantum dot-cavity device. To access both the populations and the coherences of the path-encoded density matrix, we introduce an ancilla spatial mode and perform photon correlations as a function of a single phase in a split Mach-Zehnder interferometer. We discuss the accuracy of standard quantum tomography techniques and show that an overcomplete data set can reveal spatial coherences that could be otherwise hidden due to limited or noisy statistics. Finally, we extend our analysis to extract the truly indistinguishable part of the density matrix, which allows us to identify the main origin for the imperfect fidelity to the maximally entangled state.
We introduce a tomography approach to describe the optical response of a cavity quantum electrodynamics device, beyond the semiclassical image of polarization rotation, by analyzing the polarization density matrix of the reflected photons in the Poincaré sphere. Applying this approach to an electrically-controlled quantum dot-cavity device, we show that a single resonantly-excited quantum dot induces a large optical polarization rotation by $20^\circ$ in latitude and longitude in the Poincaré sphere, with a polarization purity remaining above $84\%$. The quantum dot resonance fluorescence is shown to contribute to the polarization rotation via its coherent part, whereas its incoherent part contributes to degrading the polarization purity.
A strong limitation of linear optical quantum computing is the probabilistic operation of two-quantum bit gates based on the coalescence of indistinguishable photons. A route to deterministic operation is to exploit the single-photon nonlinearity of an atomic transition. Through engineering of the atom-photon interaction, phase shifters, photon filters and photon- photon gates have been demonstrated with natural atoms. Proofs of concept have been reported with semiconductor quantum dots, yet limited by inefficient atom-photon interfaces and dephasing. Here we report on a highly efficient single-photon filter based on a large optical non-linearity at the single photon level, in a near-optimal quantum-dot cavity interface. When probed with coherent light wavepackets, the device shows a record nonlinearity threshold around $0.3 \pm 0.1$ incident photons. We demonstrate that directly reflected pulses consist of 80% single-photon Fock state and that the two- and three-photon components are strongly suppressed compared to the single-photon one.
Quantum dots in cavities have been shown to be very bright sources of indistinguishable single photons. Yet the quantum interference between two bright quantum dot sources, a critical step for photon based quantum computation, has never been investigated. Here we report on such a measurement, taking advantage of a deterministic fabrication of the devices. We show that cavity quantum electrodynamics can efficiently improve the quantum interference between remote quantum dot sources: poorly indistinguishable photons can still interfere with good contrast with high quality photons emitted by a source in the strong Purcell regime. Our measurements and calculations show that cavity quantum electrodynamics is a powerful tool for interconnecting several devices.
Spin-selective spatial filtering of propagating polariton condensates, using a controllable spin-dependent gating barrier, in a one-dimensional semiconductor microcavity ridge waveguide is reported. A nonresonant laser beam provides the source of propagating polaritons while a second circularly polarized weak beam imprints a spin dependent potential barrier, which gates the polariton flow and generates polariton spin currents. A complete spin-based control over the blocked and transmitted polaritons is obtained by varying the gate polarization.
We investigate, through polarization-resolved spectroscopy, the spin transport by propagating polariton condensates in a quasi one-dimensional microcavity ridge along macroscopic distances. Under circularly polarized, continuous-wave, non-resonant excitation, a sinusoidal precession of the spin in real space is observed, whose phase depends on the emission energy. The experiments are compared with simulations of the spinor-polariton condensate dynamics based on a generalized Gross-Pitaevskii equation, modified to account for incoherent pumping, decay and energy relaxation within the condensate.
We present an experimental study on the ignition and decay of a polariton optical parametric oscillator (OPO) in a semiconductor microcavity pillar. The combination of a continuous wave laser pump, under quasi-phase matching conditions, and a non-resonant, 2 ps-long pulse probe allows us to obtain the full dynamics of the system. The arrival of the probe induces a blue-shift in the polariton emission, bringing the OPO process into resonance with the pump, which triggers the OPO-process. We time-resolve the polariton OPO signal emission for more than 1 nanosecond in both real and momentum-space. We fully characterize the emission of the OPO signal with spectral tomography techniques. Our interpretations are backed up by theoretical simulations based on the 2D coupled Gross-Pitaevskii equation for excitons and photons.
We show that the use of momentum-space optical interferometry, which avoids any spatial overlap between two parts of a macroscopic quantum state, presents a unique way to study coherence phenomena in polariton condensates. In this way, we address the longstanding question in quantum mechanics: "\emph{Do two components of a condensate, which have never seen each other, possess a definitive phase?}" [P. W. Anderson, \emph{Basic Notions of Condensed Matter Physics} (Benjamin, 1984)]. A positive answer to this question is experimentally obtained here for light-matter condensates, created under precise symmetry conditions, in semiconductor microcavities taking advantage of the direct relation between the angle of emission and the in-plane momentum of polaritons.
We present a time-resolved photoluminescence (PL) study in real- and momentum-space of a polariton condensate switch in a quasi-1D semiconductor microcavity. The polariton flow across the ridge is gated by excitons inducing a barrier potential due to repulsive interactions. A study of the device operation dependence on the power of the pulsed gate beam obtains a satisfactory compromise for the ON/OFF-signal ratio and -switching time of the order of 0.3 and $\thicksim50$ ps, respectively. The opposite transition is governed by the long-lived gate excitons, consequently the OFF/ON-switching time is $\thicksim200$ ps, limiting the overall operation speed of the device to $\thicksim3$ GHz. The experimental results are compared to numerical simulations based on a generalized Gross-Pitaevskii equation, taking into account incoherent pumping, decay and energy relaxation within the condensate.
We study the dynamics of polariton condensate wave trains that propagate along a quasi one-dimensional waveguide. Through the application of tuneable potential barriers the propagation can be reflected and multiple reflections used to confine and store a propagating state. Energy-relaxation processes allow the delayed relaxation into a long-living coherent ground state. Aside the potential routing of polariton condensate signals, the system forms an AND-type logic gate compatible with incoherent inputs.
We present a time-resolved study of energy relaxation and trapping dynamics of polariton condensates in a semiconductor microcavity ridge. The combination of two non-resonant, pulsed laser sources in a GaAs ridge-shaped microcavity gives rise to profuse quantum phenomena where the repulsive potentials created by the lasers allow the modulation and control of the polariton flow. We analyze in detail the dependence of the dynamics on the power of both lasers and determine the optimum conditions for realizing an all-optical polariton condensate transistor switch. The experimental results are interpreted in the light of simulations based on a generalized Gross-Pitaevskii equation, including incoherent pumping, decay and energy relaxation within the condensate.