arXiv subjects

C. Bernhard

Publications and source records attributed to C. Bernhard.

At least 91 records · Page 5Linked to original sources

arXiv2004

Spin-controlled Mott-Hubbard bands in LaMnO_3 probed by optical ellipsometry

Spectral ellipsometry has been used to determine the dielectric function of an untwinned crystal of LaMnO_3 in the spectral range 0.5-5.6 eV at temperatures 50 K < T < 300 K. A pronounced redistribution of spectral weight is found at the Neel temperature T_N = 140 K. The anisotropy of the spectral weight transfer matches the magnetic ordering pattern. A superexchange model quantitatively describes spectral weight transfer induced by spin correlations. This analysis implies that the lowest-energy transitions around 2 eV are intersite d-d transitions, and that LaMnO_3 is a Mott-Hubbard insulator.

cond-mat.str-el↗

arXiv2004

In-Plane Spectral Weight Shift of Charge Carriers in $YBa_2Cu_3O_{6.9}$

The temperature dependent redistribution of the spectral weight of the $CuO_2$ plane derived conduction band of the $YBa_2Cu_3O_{6.9}$ high temperature superconductor (T_c = 92.7 K) was studied with wide-band (from 0.01 to 5.6 eV) spectroscopic ellipsometry. A superconductivity - induced transfer of the spectral weight involving a high energy scale in excess of 1 eV was observed. Correspondingly, the charge carrier spectral weight was shown to decrease in the superconducting state. The ellipsometric data also provide detailed information about the evolution of the optical self-energy in the normal and superconducting states.

cond-mat.supr-con↗

arXiv2004

Bulk antiferromagnetism in $\bf Na_{0.82}CoO_2$ single crystals

Susceptibility, specific heat, and muon spin rotation measurements on high-quality single crystals of $\rm Na_{0.82}CoO_2$ have revealed bulk antiferromagnetism with Néel temperature $\rm T_N = 19.8 \pm 0.1$ K and an ordered moment perpendicular to the $\rm CoO_2$ layers. The magnetic order encompasses nearly 100% of the crystal volume. The susceptibility exhibits a broad peak around 30 K, characteristic of two-dimensional antiferromagnetic fluctuations. The in-plane resistivity is metallic at high temperatures and exhibits a minimum at $\rm T_N$.

cond-mat.str-el↗

arXiv2004

Charge ordering and magneto-polarons in Na$_{0.82}$CoO$_2$

Using spectral ellipsometry, we have measured the dielectric function of a Na$_{0.82(2)}$CoO$_2$ crystal that exhibits bulk antiferromagnetism with T$_{N}$=19.8 K. We identify two prominent transitions as a function of temperature. The first one at 280 K involves marked changes of the electronic and the lattice response that are indicative of charge ordering in the CoO$_{2}$ layers. The second transition coincides with T$_{N}$=19.8 K and reveals a sizeable spin-charge coupling. The data are discussed in terms of charge ordering and formation of magneto-polarons due to a charge-induced spin-state transition of adjacent Co$^{3+}$ ions.

cond-mat.str-el↗

arXiv2004

Magnetism, Charge Order and Giant Magnetoresistance in SrFeO$_{3-δ}$ Single Crystals

The electronic and magnetic properties of SrFeO$_{3-δ}$ single crystals with controlled oxygen content ($0 \leq δ\leq 0.19$) have been studied systematically by susceptibility, transport and spectroscopic techniques. An intimate correlation between the spin-charge ordering and the electronic transport behavior is found. Giant negative as well as positive magnetoresistance are observed.

cond-mat.str-el↗

arXiv2004

Intrinsic Josephson Effects in the Magnetic Superconductor RuSr2GdCu2O8

We have measured interlayer current transport in small sized RuSr2GdCu2O8 single crystals. We find a clear intrinsic Josephson effect showing that the material acts as a natural superconductor-insulator-ferromagnet-insulator-superconductor superlattice. So far, we detected no unconventional behavior due to the magnetism of the RuO2 layers.

cond-mat.supr-con↗

arXiv2003

On the origin of the A$_{1g}$ and B$_{1g}$ electronic Raman scattering peaks in the superconducting state of YBa$_{2}$Cu$_{3}$O$_{7-δ}$

The electronic Raman scattering has been investigated in optimally oxygen doped YBa$_{2}$Cu$_{3}$O$_{7-δ}$ single crystals as well as in crystals with non-magnetic, Zn, and magnetic, Ni, impurities. We found that the intensity of the A$_{1g}$ peak is impurity independent and their energy to $T_{c}$ ratio is almost constant ($2Δ/k_{B}T_{c}\sim5$). Moreover, the signal at the B$_{1g}$ channel is completely smeared out when non-magnetic Zn impurities are present. These results are qualitatively interpreted in terms of the Zeyher and Greco's theory that relates the electronic Raman scattering in the A$_{1g}$ and B$_{1g}$ channels to \textit{d}-CDW and superconducting order parameters fluctuations, respectively.

cond-mat.supr-con↗

arXiv2003

Oxygen superstructures throughout the phase diagram of $\bf (Y,Ca)Ba_2 Cu_3 O_{6+x}$

Short-range lattice superstructures have been studied with high-energy x-ray diffuse scattering in underdoped, optimally doped, and overdoped $\rm (Y,Ca)Ba_2 Cu_3 O_{6+x}$. A new four-unit-cell superstructure was observed in compounds with $x\sim 0.95$. Its temperature, doping, and material dependence was used to attribute its origin to short-range oxygen vacancy ordering, rather than electronic instabilities in the $\rm CuO_2$ layers. No significant diffuse scattering is observed in YBa$_2$Cu$_4$O$_{8}$. The oxygen superstructures must be taken into account when interpreting spectral anomalies in $\rm (Y,Ca)Ba_2 Cu_3 O_{6+x}$.

cond-mat.supr-con↗

arXiv2003

Two resonant magnetic modes in an overdoped high-$\bf T_c$ superconductor

A detailed inelastic neutron scattering study of the overdoped high temperature copper oxide superconductor ${Y_{0.9}Ca_{0.1}Ba_{2}Cu_3O_{7}}$ reveals two distinct magnetic resonant modes in the superconducting state. The modes differ in their symmetry with respect to exchange between adjacent copper oxide layers. Counterparts of the mode with odd symmetry, but not the one with even symmetry, had been observed before at lower doping levels. The observation of the even mode resolves a long-standing puzzle, and the spectral weight ratio of both modes yields an estimate of the onset of particle-hole spin-flip excitations.

cond-mat.supr-con↗

arXiv2003

C-axis lattice dynamics in Bi-based cuprate superconductors

We present results of a systematic study of the c axis lattice dynamics in single layer Bi2Sr2CuO6 (Bi2201), bilayer Bi2Sr2CaCu2O8 (Bi2212) and trilayer Bi2Sr2Ca2Cu3O10 (Bi2223) cuprate superconductors. Our study is based on both experimental data obtained by spectral ellipsometry on single crystals and theoretical calculations. The calculations are carried out within the framework of a classical shell model, which includes long-range Coulomb interactions and short-range interactions of the Buckingham form in a system of polarizable ions. Using the same set of the shell model parameters for Bi2201, Bi2212 and Bi2223, we calculate the frequencies of the Brillouin-zone center phonon modes of A2u symmetry and suggest the phonon mode eigenvector patterns. We achieve good agreement between the calculated A2u eigenfrequencies and the experimental values of the c axis TO phonon frequencies which allows us to make a reliable phonon mode assignment for all three Bi-based cuprate superconductors. We also present the results of our shell model calculations for the Gamma-point A1g symmetry modes in Bi2201, Bi2212 and Bi2223 and suggest an assignment that is based on the published experimental Raman spectra. The superconductivity-induced phonon anomalies recently observed in the c axis infrared and resonant Raman scattering spectra in trilayer Bi2223 are consistently explained with the suggested assignment.

cond-mat.supr-con↗

arXiv2003

Anomalous oxygen isotope effect on the in-plane FIR conductivity of detwinned YBa2Cu3$^{16,18}$O$_{6.9}$

We observe an anomalous oxygen isotope effect on the a-axis component of the far-infrared electronic response of detwinned YBa2Cu3$^{16,18}$O$_{6.9}$. For $^{18}$O a pronounced low-energy electronic mode (LEM) appears around 240 cm$^{-1}$. This a-axis LEM exhibits a clear aging effect, after one year it is shifted to 190 cm$^{-1}$. For $^{16}$O we cannot resolve a corresponding a-axis LEM above 120 cm$^{-1}$. We interpret the LEM in terms of a collective electronic mode that is pinned by `isotopic defects', i.e. by the residual $^{16}$O in the matrix of $^{18}$O.

cond-mat.supr-con↗

arXiv2003

Proximity induced metal/insulator transition in $Y Ba_2 Cu_3 O_7 / La_{2/3} Ca_{1/3} Mn O_3$ superlattices

The far-infrared dielectric response of superlattices (SL) composed of superconducting YBa$_{2}$Cu$_{3}$O$_{7}$ (YBCO) and ferromagnetic La$_{0.67}$% Ca$_{0.33}$MnO$_{3}$ (LCMO) has been investigated by ellipsometry. A drastic decrease of the free carrier response is observed which involves an unusually large length scale of d$^{crit}\approx $20 nm in YBCO and d$^{crit}\approx $10 nm in LCMO. A corresponding suppression of metallicity is not observed in SLs where LCMO is replaced by the paramagnetic metal LaNiO$_{3}$. Our data suggest that either a long range charge transfer from the YBCO to the LCMO layers or alternatively a strong coupling of the charge carriers to the different and competitive kind of magnetic correlations in the LCMO and YBCO layers are at the heart of the observed metal/insulator transition. The low free carrier response observed in the far-infrared dielectric response of the magnetic superconductor RuSr$_{2}$GdCu$_{2}$O$_{8}$ is possibly related to this effect.

cond-mat.supr-con↗

arXiv2003

Magneto-Transport Properties of Doped RuSr$_2$GdCu$_2$O$_8$

RuSr$_2$GdCu$_2$O$_8$, in which magnetic order and superconductivity coexist with $T_{Magnetic}$$\gg$$T_c$, is a complex material which poses new and important questions to our understanding of the interplay between magnetic and superconducting (SC) order. Resistivity, Hall effect and thermopower measurements on sintered ceramic RuSr$_2$GdCu$_2$O$_8$ are presented, together with results on a broad range of substituted analogues. The Hall effect and thermopower both show anomalous decreases below $T_{Magnetic}$ which may be explained within a simple two-band model by a transition from localized to more itinerant behavior in the RuO$_2$ layer at $T_{Magnetic}$.

cond-mat.supr-con↗

arXiv2002

The superfluid density in cuprate high-Tc superconductors - a new paradigm

The doping dependence of the superfluid density, r_s, of high-Tc superconductors is usually considered in the context of the Uemura relation, namely Tc proportional to rs, which is generally assumed to apply in the underdoped regime. We show that a modified plot of Tc/Do versus rs, where Do is the maximum d-wave gap at T=0, exhibits universal features that point to an alternative interpretation of the underlying physics. In the underdoped region this plot exhibits the canonical negative curvature expected when a ground-state correlation competes with superconductivity (SC) by opening up a gap in the normal-state DOS. In particular rs is suppressed much faster than Tc/Do or indeed Tc. The pseudogap is found to strongly modify the SC ground state.

cond-mat.supr-con↗

arXiv2002

Structural and Magnetic Instabilities of La$_{2-x}$Sr$_x$CaCu$_2$O$_6$

A neutron scattering study of nonsuperconducting La$_{2-x}$Sr$_x$CaCu$_2$O$_6$ (x=0 and 0.2), a bilayer copper oxide without CuO chains, has revealed an unexpected tetragonal-to-orthorhombic transition with a doping dependent transition temperature. The predominant structural modification below the transition is an in-plane shift of the apical oxygen. In the doped sample, the orthorhombic superstructure is strongly disordered, and a glassy state involving both magnetic and structural degrees of freedom develops at low temperature. The spin correlations are commensurate.

cond-mat.supr-con↗

arXiv2002

Josephson plasma resonance and phonon anomalies in trilayer Bi_2Sr_2Ca_2Cu_3O_10 superconductor

The far-infrared (FIR) c axis conductivity of a Bi2223 crystal has been measured by ellipsometry. Below T$_c$ a strong absorption band develops near 500 cm $^{-1}$, corresponding to a transverse Josephson-plasmon. The related increase in FIR spectral weight leads to a giant violation of the Ferrell-Glover-Tinkham sum-rule. The gain in c axis kinetic energy accounts for a sizeable part of the condensation energy. We also observe phonon anomalies which suggest that the Josephson-currents lead to a drastic variation of the local electric field within the block of closely spaced CuO$_2$ planes.

cond-mat.supr-con↗

arXiv2001

Muon-spin-relaxation study of the magnetic penetration depth in MgB2

The magnetic vortex lattice (VL) of polycrystalline MgB2 has been investigated by transverse-field muon-spin-relaxation (TF-MuSR). The evolution of TF-MuSR depolarization rate, sigma, that is proportional to the second moment of the field distribution of the VL has been studied as a function of temperature and applied magnetic field. The low temperature value s exhibits a pronounced peak near Hext = 75 mT. This behavior is characteristic of strong pinning induced distortions of the VL which put into question the interpretation of the low-field TF-MuSR data in terms of the magnetic penetration depth lambda(T). An approximately constant value of sigma, such as expected for an ideal VL in the London-limit, is observed at higher fields of Hext > 0.4 T. The TF-MuSR data at Hext = 0.6 T are analyzed in terms of a two-gap model. We obtain values for the gap size of D1 = 6.0 meV (2D1/kBTc = 3.6), D2 = 2.6 meV (2D2/kBTc = 1.6), a comparable spectral weight of the two bands and a zero temperature value for the magnetic penetration depth of lambda = 100 nm. In addition, we performed MuSR-measurements in zero external field (ZF-MuSR). We obtain evidence that the muon site (at low temperature) is located on a ring surrounding the center of the boron hexagon. Muon diffusion sets in already at rather low temperature of T > 10 K. The nuclear magnetic moments can account for the observed relaxation rate and no evidence for electronic magnetic moments has been obtained.

cond-mat.supr-con↗

arXiv2001

In-plane polarized collective modes in detwinned YBa$_{2}$Cu$_{3}$O$_{6.95}$ observed by spectral ellipsometry

The in-plane dielectric response of detwinned YBa$_{2}$Cu$_{3}$O$_{6.95}$ has been studied by far-infared ellipsometry. A surprisingly lare number of in-plane polarized modes are observed. Some of them correspond to pure phonon modes. Others posses a large electronic contribution which strongly increases in the superconducting state. The free carrier response and the collective modes exhibit a pronounced a-b anisotropy. We discuss our results in terms of a CDW state in the 1-d CuO chains and induced charge density fluctuations within the 2-d CuO$_{2}$ planes.

cond-mat.supr-con↗