arXiv subjects

C. Bray

Publications and source records attributed to C. Bray.

18 recordsLinked to original sources

arXiv2026

Electron spin resonance driven photogalvanic effect in graphene-based structures

We report an electron-spin-resonance-driven linear photogalvanic effect (LPGE) in unbiased monolayer graphene and WSe_2/graphene heterostructures. Under linearly polarized 45--75 GHz radiation, the photovoltage exhibits pronounced resonant features in both Faraday and Voigt geometries. Multiple resonances associated with the electron spin resonance in graphene are observed for both out-of-plane and in-plane magnetic-field orientations. Their magnetic-field positions vary linearly with frequency, their amplitudes reverse sign across the charge-neutrality point, and the resonant contribution has the opposite sign to the nonresonant Drude photogalvanic background. We develop a microscopic theory in which radiation-induced momentum alignment followed by skew scattering generates both contributions. Their opposite signs originate from the orthogonal momentum alignments produced by indirect Drude absorption and direct spin-resonant transitions. The theory describes well the main features of the observed resonant photocurrent and provides a microscopic description of ESR-induced LPGE in two-dimensional systems. These results establish the photogalvanic response as a probe of ESR in unbiased micron-scale graphene-based devices.

cond-mat.mtrl-sci↗

arXiv2025

Nonlinear Terahertz Electroluminescence from Dirac Landau Polaritons

We report Dirac Landau polaritons observed by terahertz (THz) magnetoreflectivity spectroscopy, demonstrating strong coupling between cyclotron transitions of two-dimensional (2D) Dirac fermions in HgTe quantum wells and optical cavity modes. Under pulsed electrical injection we observe efficient nonlinear electroluminescence, with a strongly out-of-equilibrium polariton distribution dominated by emission from the upper polariton branches. Model analysis of the bias-dependent emission intensity and spectral narrowing indicates a polariton occupancy per mode approaching unity, with a possible contribution from stimulated polariton emission in the spectral region of the upper anticrossing. These results open prospects toward Dirac Landau polariton condensates and low-threshold, tunable THz polariton lasers based on cyclotron emission.

cond-mat.mes-hall↗

arXiv2024

Spin-dependent photovoltage in graphene/MoS2-based field-effect transistors

It has recently been shown that Terahertz sensors can effectively detect the spin resonances of Dirac fermions in graphene. The associated photovoltaic measurement technique allows for the investigation of the intrinsic spin-orbit coupling in graphene as well as its topological properties from microwave to Terahertz frequencies. In this work, using graphene/MoS2-based Field-Effect Transistors, we observed a magnetic resonance photovoltage signal in the Gigahertz range that is independent of the gate bias. The dispersion of the associated spin-flip transitions remains intriguingly unaffected by the MoS2 layer. In parallel, the spin-related signal consistently appears as a drop in photovoltage, regardless of the signal's polarity or origin, whether it arises from plasma wave rectification or thermoelectric effects. This behavior is interpreted as a decrease in the system's spin polarization due to spin-dependent recombination or scattering of photocarriers. Understanding the various photovoltaic signals in highly sensitive Gigahertz/Terahertz sensors paves the way for exploring spin-dependent mechanisms in two-dimensional quantum materials, influenced by proximity effects such as spin-orbit coupling, topology, and magnetism.

cond-mat.mes-hall↗

arXiv2024

High-Precision Excited-State Nuclear Recoil Spectroscopy with Superconducting Sensors

Superconducting sensors doped with rare isotopes have recently demonstrated powerful sensing performance for sub-keV radiation from nuclear decay. Here, we report the first high-resolution recoil spectroscopy of a single, selected nuclear state using superconducting tunnel junction (STJ) sensors. The STJ sensors were used to measure the eV-scale nuclear recoils produced in $^7$Be electron capture decay in coincidence with a 478 keV $\gamma$-ray emitted in decays to the lowest-lying excited nuclear state in $^7$Li. Details of the Doppler broadened recoil spectrum depend on the slow-down dynamics of the recoil ion. The measured spectral broadening is compared to empirical stopping power models as well as modern molecular dynamics simulations at low energy. The results have implications in several areas from nuclear structure and stopping powers at eV-scale energies to direct searches for dark matter, neutrino mass measurements, and other physics beyond the standard model.

physics.ins-det↗

arXiv2024

Multi-probe analysis to separate edge currents from bulk currents in quantum spin Hall insulators and to analyze their temperature dependence

We present a multi-probe transport analysis that effectively separates bulk and edge currents in large Hall bar devices with standard geometries. Applied to transport measurements on all possible four-probe configurations of six-probe Hall bar devices made of inverted three-layer InAs/GaInSb quantum wells (QWs), our analysis not only reveals the presence of dissipative edge currents in the topological gap, but also allows the temperature dependence of bulk and edge conductivity to be evaluated separately. The temperature dependence of the edge conductivity for Hall bar channels from 10 $\mu$m to 70~$\mu$m in the range of 1.5 K to 45 K is consistent with the theoretical expectation of weakly interacting helical edge electrons with backscattering due to localized magnetic moments of charge impurities. We argue that these charge impurities are naturally associated with intrinsic Ga-antisite defects, which act as double acceptors in InAs/Ga(In)Sb-based QWs.

cond-mat.mes-hall↗

arXiv2023

The Data Acquisition System for Phase-III of the BeEST Experiment

The BeEST experiment is a precision laboratory search for physics beyond the standard model that measures the electron capture decay of $^7$Be implanted into superconducting tunnel junction (STJ) detectors. For Phase-III of the experiment, we constructed a continuously sampling data acquisition system to extract pulse shape and timing information from 16 STJ pixels offline. Four additional pixels are read out with a fast list-mode digitizer, and one with a nuclear MCA already used in the earlier limit-setting phases of the experiment. We present the performance of the data acquisition system and discuss the relative advantages of the different digitizers.

physics.ins-det↗

arXiv2023

Gate tunable terahertz cyclotron emission from two-dimensional Dirac fermions

Two-dimensional Dirac fermions in HgTe quantum wells close to the topological phase transition can generate significant cyclotron emission that is magnetic field tunable in the Terahertz (THz) frequency range. Due to their relativistic-like dynamics, their cyclotron mass is strongly dependent on their electron concentration in the quantum well, providing a second tunability lever and paving the way for a gate-tunable, permanent-magnet Landau laser. In this work, we demonstrate the proof-of-concept of such a back-gate tunable THz cyclotron emitter at fixed magnetic field. The emission frequency detected at 1.5 Tesla is centered on 2.2 THz and can already be electrically tuned over 250 GHz. With an optimized gate and a realistic permanent magnet of 1.0 Tesla, we estimate that the cyclotron emission could be continuously and rapidly tunable by the gate bias between 1 and 3 THz, that is to say on the less covered part of the THz gap.

cond-mat.mes-hall↗

arXiv2023

Terahertz cyclotron emission from two-dimensional Dirac fermions

Since the emergence of graphene, we have seen several proposals for the realization of Landau lasers tunable over the terahertz frequency range. The hope was that the non-equidistance of the Landau levels from Dirac fermions would suppress the harmful non-radiative Auger recombination. Unfortunately, even with this non-equidistance an unfavorable non-radiative process persists in Landau-quantized graphene, and so far no cyclotron emission from Dirac fermions has been reported. One way to eliminate this last non-radiative process is to sufficiently modify the dispersion of the Landau levels by opening a small gap in the linear band structure. A proven example of such gapped graphene-like materials are HgTe quantum wells close to the topological phase transition. In this work, we experimentally demonstrate Landau emission from Dirac fermions in such HgTe quantum wells, where the emission is tunable by both the magnetic field and the carrier concentration. Consequently, these results represent an advance in the realization of terahertz Landau lasers tunable by magnetic field and gate-voltage.

cond-mat.mes-hall↗

arXiv2022

Current-induced enhancement of photo-response in graphene THz radiation detectors

Thermoelectric readout in a graphene THz radiation detector requires a p-n junction across the graphene channel. Even without an intentional p-n junction, two latent junctions can exist in the vicinity of the electrodes/antennas through the proximity to metal. In a symmetrical structure, these junctions are connected back-to-back and therefore counterbalance each other with regard to rectification of the ac signal. Because of the Peltier effect, a small dc current results in additional heating in one- and cooling in another p-n junction, thereby breaking the symmetry. The p-n junctions then no longer cancel, resulting in a greatly enhanced rectified signal. This allows to simplify the design and effectively control the sensitivity of the THz-radiation detectors.

cond-mat.mes-hall↗

arXiv2022

Temperature Dependent Zero-Field Splittings in Graphene

Graphene is a quantum spin Hall insulator with a 45 $\mu$eV wide non-trivial topological gap induced by the intrinsic spin-orbit coupling. Even though this zero-field spin splitting is weak, it makes graphene an attractive candidate for applications in quantum technologies, given the resulting long spin relaxation time. On the other side, the staggered sub-lattice potential, resulting from the coupling of graphene with its boron nitride substrate, compensates intrinsic spin-orbit coupling and decreases the non-trivial topological gap, which may lead to the phase transition into trivial band insulator state. In this work, we present extensive experimental studies of the zero-field splittings in monolayer and bilayer graphene in a temperature range 2K-12K by means of sub-Terahertz photoconductivity-based electron spin resonance technique. Surprisingly, we observe a decrease of the spin splittings with increasing temperature. We discuss the origin of this phenomenon by considering possible physical mechanisms likely to induce a temperature dependence of the spin-orbit coupling. These include the difference in the expansion coefficients between the graphene and the boron nitride substrate or the metal contacts, the electron-phonon interactions, and the presence of a magnetic order at low temperature. Our experimental observation expands knowledge about the non-trivial topological gap in graphene.

cond-mat.mtrl-sci↗

arXiv2022

Large inverted band-gap in strained three-layer InAs/GaInSb quantum wells

Quantum spin Hall insulators (QSHIs) based on HgTe and three-layer InAs/GaSb quantum wells (QWs) have comparable bulk band-gaps of about 10--18~meV. The former however features a band-gap vanishing with temperature, while the gap in InAs/GaSb QSHIs is rather temperature-independent.Here, we report on the realization of large inverted band-gap in strained three-layer InAs/GaInSb QWs. By temperature-dependent magnetotransport measurements of gated Hall bar devices, we extract a gap as high as 45 meV. Combining local and non-local measurements, we attribute the edge conductivity observed at temperatures up to 40 K to the topological edge channels with equilibration lengths of a few micrometers. Our findings pave the way toward manipulating edge transport at high temperatures in QW heterostructures.

cond-mat.mes-hall↗

arXiv2021

Kiloton-scale xenon detectors for neutrinoless double beta decay and other new physics searches

Large detectors employing xenon are a leading technology in existing and planned searches for new physics, including searches for neutrinoless double beta decay ($0\nu\beta\beta$) and dark matter. While upcoming detectors will employ target masses of a ton or more, further extending gas or liquid phase Xe detectors to the kton scale would enable extremely sensitive next-generation searches for rare phenomena. The key challenge to extending this technology to detectors well beyond the ton scale is the acquisition of the Xe itself. We describe the motivation for extending Xe time projection chambers (TPCs) to the kton scale and possible avenues for Xe acquisition that avoid existing supply chains. If acquisition of Xe in the required quantities is successful, kton-scale detectors of this type could enable a new generation of experiments, including searches for $0\nu\beta\beta$ at half-life sensitivities as long as $10^{30}$ yr.

physics.ins-det↗

arXiv2021

Photo-induced plasmon-phonon coupling in PbTe

We report the observation of photo-induced plasmon-phonon coupled modes in the group IV-VI semiconductor PbTe using Fourier-transform inelastic X-ray scattering at the Linac Coherent Light Source (LCLS). We measure the near-zone-center dispersion of the heavily screened longitudinal optical (LO) phonon branch as extracted from differential changes in x-ray diffuse scattering intensity following above band gap photoexcitation.

cond-mat.mtrl-sci↗

arXiv2020

Limits on the Existence of sub-MeV Sterile Neutrinos from the Decay of $^7$Be in Superconducting Quantum Sensors

Sterile neutrinos are natural extensions to the standard model of particle physics and provide a possible portal to the dark sector. We report a new search for the existence of sub-MeV sterile neutrinos using the decay-momentum reconstruction technique in the decay of $^7$Be. The experiment measures the total energy of the $^7$Li daughter atom from the electron capture decay of $^7$Be implanted into sensitive superconducting tunnel junction (STJ) quantum sensors. This first experiment presents data from a single STJ operated at a low count rate for a net total of 28 days, and provides exclusion limits on sterile neutrinos in the mass range from 100 to 850 keV that improve upon previous work by up to an order of magnitude.

nucl-ex↗

arXiv2020

Direct measurement of the $^7$Be $L/K$ capture ratio in Ta-based superconducting tunnel junctions

We report a high-statistics measurement of the $L/K$ orbital electron capture (EC) ratio in $^7$Be embedded in cryogenic Ta. The thin Ta film formed part of a high-resolution superconducting tunnel junction (STJ) radiation detector that was used to identify the signals from different decay channels. The measured $L/K$ capture ratio of 0.070(7) is significantly larger than the only previous measurement of this quantity and the theoretical predictions that include in-medium effects. This value is a uniquely sensitive probe of the 1s and 2s orbital overlaps with the nucleus, and is of relevance to nuclear and atomic physics, as well as Li production in novae and other astrophysical scenarios. This is the first experiment that uses STJs for nuclear-recoil detection, opening a new experimental avenue for low-energy precision measurements with rare isotopes.

nucl-ex↗

arXiv2018

A nearby superluminous supernova with a long pre-maximum 'plateau' and strong CII features

Super-luminous supernovae (SLSNe) are rare events defined as being significantly more luminous than normal terminal stellar explosions. The source of the extra powering needed to achieve such luminosities is still unclear. Discoveries in the local Universe (i.e. $z<0.1$) are scarce, but afford dense multi-wavelength observations. Additional low-redshift objects are therefore extremely valuable. We present early-time observations of the type I SLSN ASASSN-18km/SN~2018bsz. These data are used to characterise the event and compare to literature SLSNe and spectral models. Host galaxy properties are also analysed. Optical and near-IR photometry and spectroscopy were analysed. Early-time ATLAS photometry was used to constrain the rising light curve. We identified a number of spectral features in optical-wavelength spectra and tracked their time evolution. Finally, we used archival host galaxy photometry together with HII region spectra to constrain the host environment. ASASSN-18km/SN~2018bsz is found to be a type I SLSN in a galaxy at a redshift of 0.0267 (111 Mpc), making it the lowest-redshift event discovered to date. Strong CII lines are identified in the spectra. Spectral models produced by exploding a Wolf-Rayet progenitor and injecting a magnetar power source are shown to be qualitatively similar to ASASSN-18km/SN~2018bsz, contrary to most SLSNe-I that display weak/non-existent CII lines. ASASSN-18km/SN~2018bsz displays a long, slowly rising, red 'plateau' of $>$26 days, before a steeper, faster rise to maximum. The host has an absolute magnitude of --19.8 mag ($r$), a mass of M$_{*}$ = 1.5$^{+0.08}_{-0.33}$ $\times$10$^{9}$ M$_{\odot}$ , and a star formation rate of = 0.50$^{+2.22}_{-0.19}$ M$_{\odot}$ yr$^{-1}$. A nearby HII region has an oxygen abundance (O3N2) of 8.31$\pm$0.01 dex.

astro-ph.HE↗

arXiv2015

Photoinduced suppression of the ferroelectric instability in PbTe

The interactions between electrons and phonons drive a large array of technologically relevant material properties including ferroelectricity, thermoelectricity, and phase-change behaviour. In the case of many group IV-VI, V, and related materials, these interactions are strong and the materials exist near electronic and structural phase transitions. Their close proximity to phase instability produces a fragile balance among the various properties. The prototypical example is PbTe whose incipient ferroelectric behaviour has been associated with large phonon anharmonicity and thermoelectricity. Experimental measurements on PbTe reveal anomalous lattice dynamics, especially in the soft transverse optical phonon branch. This has been interpreted in terms of both giant anharmonicity and local symmetry breaking due to off-centering of the Pb ions. The observed anomalies have prompted renewed theoretical and computational interest, which has in turn revived focus on the extent that electron-phonon interactions drive lattice instabilities in PbTe and related materials. Here, we use Fourier-transform inelastic x-ray scattering (FT-IXS) to show that photo-injection of free carriers stabilizes the paraelectric state. With support from constrained density functional theory (CDFT) calculations, we find that photoexcitation weakens the long-range forces along the cubic direction tied to resonant bonding and incipient ferroelectricity. This demonstrates the importance of electronic states near the band edges in determining the equilibrium structure.

cond-mat.mtrl-sci↗

arXiv2010

Antihydrogen formation dynamics in a multipolar neutral anti-atom trap

Antihydrogen production in a neutral atom trap formed by an octupole-based magnetic field minimum is demonstrated using field-ionization of weakly bound anti-atoms. Using our unique annihilation imaging detector, we correlate antihydrogen detection by imaging and by field-ionization for the first time. We further establish how field-ionization causes radial redistribution of the antiprotons during antihydrogen formation and use this effect for the first simultaneous measurements of strongly and weakly bound antihydrogen atoms. Distinguishing between these provides critical information needed in the process of optimizing for trappable antihydrogen. These observations are of crucial importance to the ultimate goal of performing CPT tests involving antihydrogen, which likely depends upon trapping the anti-atom.

hep-ex↗