arXiv subjects

C. C. Tsuei

Publications and source records attributed to C. C. Tsuei.

17 recordsLinked to original sources

arXiv2020

Observation of triplet superconductivity in CoSi$_2$/TiSi$_2$ heterostructures

Unconventional superconductivity and in particular triplet superconductivity have been front and center of topological materials and quantum technology research. Here we report our observation of triplet superconductivity in nonmagnetic CoSi$_2$/TiSi$_2$ heterostructures on silicon. CoSi$_2$ undergoes a sharp superconducting transition at a critical temperature $T_c \approx$ 1.5 K, while TiSi$_2$ is a normal metal. We investigate conductance spectra of both two-terminal CoSi$_2$/TiSi$_2$ tunnel junctions and three-terminal T-shaped CoSi$_2$/TiSi$_2$ superconducting proximity structures. We report an unexpectedly large spin-orbit coupling in CoSi$_2$ heterostructures. Below $T_c$, we observe (1) a narrow zero-bias conductance peak on top of a broad hump, accompanied by two symmetric side dips in the tunnel junctions, (2) a narrow zero-bias conductance peak in T-shaped structures, and (3) hysteresis in the junction magnetoresistance. These three independent and complementary observations are indicative of chiral $p$-wave pairing in CoSi$_2$/TiSi$_2$ heterostructures. This chiral triplet superconductivity and the excellent fabrication compatibility of CoSi$_2$ and TiSi$_2$ with present-day silicon integrated-circuit technology facilitate full scalability for potential use in quantum-computing devices.

cond-mat.supr-con↗

arXiv2015

Tunneling spectroscopy and Majorana modes emergent from topological gapless phases in high-Tc cuprate superconductors

We explore possible signatures for observing Majorana Fermions in the tunneling spectroscopy of high-Tc cuprate superconductors. We find that as long as the Rashba spin orbit interaction is in presence either through proximity effect due to an electrode made by heavy metal or by the intrinsic nature of cuprates, in addition to the Heisenberg spin exchange interaction, the Dzyaloshinskii-Moriya and spin dipole-dipole interactions are induced. As a result, $p$-wave superconductivity is induced with the gap function $d$-vector being not aligned with the internal magnetic field of the spin-orbit interaction. Most importantly, the ground state goes through transitions into gapless phases with split nodal points. The split nodal structure always results in Majorana modes for any interfaces that are not exactly in (100) or (010) directions. Hence for general interfaces, existence of Majorana bound edge states is a robust feature. Our results indicate that these Majorana modes would result in a small plateau in tunneling spectrum near zero bias peak and in 4 $π$ periodicity in typical SIS$'$ junctions . As a result, it is easy for a $π$-ring in tricrystal experiments to hold Majorana Ferimions and exhibit periods of two flux quanta in external magnetic fields. These phenomena may have been already observed in experiments and their connections to experimental results are discussed.

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arXiv2011

Superconducting to spin glass state transformation in ß-pyrochlore KxOs2O6

ß-pyrochore KOs2O6, which shows superconductivity below ~ 9.7K, has been converted into KxOs2O6 (x < 2/3 - 1/2) electrochemically to show spin glass-like behavior below ~ 6.1K. Room temperature sample surface potential versus charge transfer scan indicates that there are at least two two-phase regions for x between 1 and 0.5. Rattling model of superconductivity for the title compound has been examined using electrochemical potassium de-intercalation. The significant reduction of superconducting volume fraction due to minor potassium reduction suggests the importance of defect and phase coherence in the rattling model. Magnetic susceptibility, resistivity, and specific heat measurement results have been compared between the superconducting and spin glass-like samples.

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arXiv2011

Half-Integer Flux Quantization in Unconventional Superconductors

In this article, we wish to give a historical and personal account of the advent of our tricrystal phase-sensitive symmetry experiments using scanning SQUID microscope for establishing d-wave pairing symmetry in the cuprate superconductors. On the occasion of commemorating the 100th anniversary of the discovery of superconductivity by Kamerlingh Onnes, we are honored to present this article as part of the Jubilee Celebration.

cond-mat.supr-con↗

arXiv2010

Ab initio Understanding of the Pseudogap in Cuprate High Temperature Superconductors via the Fluctuating Bond Model

Understanding the origin of the pseudogap is an essential step towards elucidating the pairing mechanism in the cuprate superconductors. Recently there has been strong experimental evidence showing that C4 symmetry breaking occurs on formation of the pseudogap. This form of symmetry breaking was predicted by the Fluctuating Bond Model (FBM), an empirical model based on a strong, local coupling of electrons to the square of the planar oxygen vibrator amplitudes. In this paper we approach the FBM theory from a new direction, starting from {\it ab initio} molecular dynamics simulations. The simulations demonstrate a doping-dependent instability of the in-plane oxygens towards displacement off the Cu-O-Cu bond axis. From these results and perturbation theory we derive an improved and quantitative form of the Fluctuating Bond Model. A mean field solution of the FBM leads to C4 symmetry breaking in the oxygen vibrational amplitudes, and to a d-type pseudogap in the electronic spectrum, the features linked by recent experimental data. The phase diagram of the pseudogap derived from mean field theory, its doping- and temperature-dependences, including the phase boundary T$^*$, agree well with experimental data. We extend the theory to include the long range Coulomb interaction on the same basis as the FBM interaction. When the long-range Coulomb interaction is included in the FBM, a CDW instability in the charge channel is predicted which explains the nanoscale, rather than spatially uniform, behavior of the C4 symmetry-breaking. Taking the CDW into account, with the theoretical k-dependence of the pseudogap, enables the Fermi Surface arc phenomenon to be understood.

cond-mat.supr-con↗

arXiv2010

Integer and half-integer flux-quantum transitions in a niobium/iron-pnictide loop

The recent discovery of iron-based superconductors challenges the existing paradigm of high-temperature superconductivity. Owing to their unusual multi-orbital band structure, magnetism, and electron correlation, theories propose a unique sign reversed s-wave pairing state, with the order parameter changing sign between the electron and hole Fermi pockets. However, because of the complex Fermi surface topology and material related issues, the predicted sign reversal remains unconfirmed. Here we report a novel phase-sensitive technique for probing unconventional pairing symmetry in the polycrystalline iron-pnictides. Through the observation of both integer and half-integer flux-quantum transitions in composite niobium/iron-pnictide loops, we provide the first phase-sensitive evidence of the sign change of the order parameter in NdFeAsO0.88F0.12, lending strong support for microscopic models predicting unconventional s-wave pairing symmetry. These findings have important implications on the mechanism of pnictide superconductivity, and lay the groundwork for future studies of new physics arising from the exotic order in the FeAs-based superconductors.

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arXiv2009

Giant Nonlinear Electron-lattice Interaction in Cuprate Superconductors, and Origin of the Pseudogap

The pseudogap is a key property of the cuprate superconductors, whose understanding should illuminate the pairing mechanism. Recent experimental data support a close connection between the pseudogap and an oxygen-driven C4 symmetry breaking within the CuO2 plane unit cell. Using ab initio Molecular Dynamics, we demonstrate the existence of a strong nonlinear electron-oxygen vibrator coupling in two cuprates. In a mean field approach applied to this coupling within a model Hamiltonian, we derive a C4 splitting/pseudogap phase diagram in agreement with experiment - providing an explanation for the pseudogap phenomenon from first principles. The implications for superconductivity and the Fermi surface arc effect are discussed.

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arXiv2006

Experiments using high-Tc/low-Tc Josephson contacts

Remarkably rich physics is involved in the behavior of hybrid Josephson junctions, connecting high-Tc and low-Tc superconductors. This relates in particular to the different order parameter symmetries underlying the formation of the superconducting states in these materials. Experiments on high-Tc/low-Tc contacts have also played a crucial role in settling the decade-long d-wave versus s-wave debate in cuprate superconductors. Recently, such hybrid junctions have enabled more detailed pairing symmetry tests. Furthermore, with these junctions, complex arrays of pi-rings have been realized, enabling studies on spontaneously generated fractional flux quanta and their mutual interactions. Steps toward novel superconducting electronic devices are taken, utilizing the phase-shifts inherent to the d-wave superconducting order parameter. This paper is intended to reflect the current status of experiments using high-Tc and low-Tc Josephson contacts.

cond-mat.supr-con↗

arXiv2006

Fluctuating Cu-O-Cu Bond model of high temperature superconductivity in cuprates

Twenty years of extensive research has yet to produce a general consensus on the origin of high temperature superconductivity (HTS). However, several generic characteristics of the cuprate superconductors have emerged as the essential ingredients of and/or constraints on any viable microscopic model of HTS. Besides a Tc of order 100K, the most prominent on the list include a d-wave superconducting gap with Fermi liquid nodal excitations, a d-wave pseudogap with the characteristic temperature scale T*, an anomalous doping-dependent oxygen isotope shift, nanometer-scale gap inhomogeneity, etc.. The key role of planar oxygen vibrations implied by the isotope shift and other evidence, in the context of CuO2 plane symmetry and charge constraints from the strong intra-3d Coulomb repulsion U, enforces an anharmonic mechanism in which the oxygen vibrational amplitude modulates the strength of the in-plane Cu-Cu bond. We show, within a Fermi liquid framework, that this mechanism can lead to strong d-wave pairing and to a natural explanation of the salient features of HTS.

cond-mat.supr-con↗

arXiv2005

Anti-ferromagnetic ordering in arrays of superconducting pi-rings

We report experiments in which one dimensional (1D) and two dimensional (2D) arrays of YBa2Cu3O7-x-Nb pi-rings are cooled through the superconducting transition temperature of the Nb in various magnetic fields. These pi-rings have degenerate ground states with either clockwise or counter-clockwise spontaneous circulating supercurrents. The final flux state of each ring in the arrays was determined using scanning SQUID microscopy. In the 1D arrays, fabricated as a single junction with facets alternating between alignment parallel to a [100] axis of the YBCO and rotated 90 degrees to that axis, half-fluxon Josephson vortices order strongly into an arrangement with alternating signs of their magnetic flux. We demonstrate that this ordering is driven by phase coupling and model the cooling process with a numerical solution of the Sine-Gordon equation. The 2D ring arrays couple to each other through the magnetic flux generated by the spontaneous supercurrents. Using pi-rings for the 2D flux coupling experiments eliminates one source of disorder seen in similar experiments using conventional superconducting rings, since pi-rings have doubly degenerate ground states in the absence of an applied field. Although anti-ferromagnetic ordering occurs, with larger negative bond orders than previously reported for arrays of conventional rings, long-range order is never observed, even in geometries without geometric frustration. This may be due to dynamical effects. Monte-Carlo simulations of the 2D array cooling process are presented and compared with experiment.

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arXiv2004

Low-bandwidth control scheme for an oscillator stabilized Josephson qubit

We introduce a new Josephson junction circuit for which quantum operations are realized by low-bandwidth, nearly adiabatic magnetic-flux pulses. Coupling to the fundamental mode of a superconducting transmission line permits a stabilization of the rotation angle of the quantum operation against flux noise. A complete scheme for one-qubit rotations, and high-visibility Ramsey-fringe oscillations, is given. We show that high visibility depends on passing through a portal in the space of applied fluxes, where the width of the portal is proportional to the ramp-up rate of the flux pulse.

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arXiv2004

Robust dx2-y2 pairing symmetry in high-temperature superconductors

Although initially quite controversial, it has been widely accepted that the Cooper pairs in optimally doped cuprate superconductors have predominantly dx2-y2 wavefunction symmetry. The controversy has now shifted to whether the high-Tc pairing symmetry changes away from optimal doping. Here we present phase-sensitive tricrystal experiments on three cuprate systems: Y0.7Ca0.3Ba2Cu3O7-x (Ca-doped Y-123), La2-xSrxCuO4 (La-214) and Bi2Sr2CaCu2O8+x (Bi-2212),with doping levels covering the underdoped, optimal and overdoped regions. Our work implies that time-reversal invariant, predominantly dx2-y2 pairing symmetry is robust over a large variation in doping, and underscores the important role of on-site Coulomb repulsion in the making of high-temperature superconductivity.

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arXiv2003

Fluxoid dynamics in superconducting thin film rings

We have measured the dynamics of individual magnetic fluxoids entering and leaving photolithographically patterned thin film rings of the underdoped high-temperature superconductor Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$, using a variable sample temperature scanning SQUID microscope. These results can be qualitatively described using a model in which the fluxoid number changes by thermally activated nucleation of a Pearl vortex in, and transport of the Pearl vortex across, the ring wall.

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arXiv2003

Evidence for Thermally Activated Spontaneous Fluxoid Formation in Superconducting Thin-Film Rings

We have observed spontaneous fluxoid generation in thin-film rings of the amorphous superconductor Mo$_3$Si, cooled through the normal-superconducting transition, as a function of quench rate and externally applied magnetic field, using a variable sample temperature scanning SQUID microscope. Our results can be explained using a model of freezout of thermally activated fluxoids, mediated by the transport of bulk vortices across the ring walls. This mechanism is complementary to a mechanism proposed by Kibble and Zurek, which only relies on causality to produce a freezout of order parameter fluctuations.

cond-mat.supr-con↗

arXiv2001

Direct measurement of single fluxoid dynamics in superconducting rings

We have measured the dynamics of individual magnetic fluxoids entering and leaving thin film, photolithographically patterned rings of underdoped high-temperature superconductor BSCCO using a variable sample temperature scanning SQUID microscope. These measurements can be understood within a phenomenological model in which the fluxoid number changes by thermal activation of a Pearl vortex in the ring wall. We place upper limits on the "vison" binding energy in these samples from these measurements.

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arXiv2000

Phase-sensitive Evidence for d-wave Pairing Symmetry in Electron-doped Cuprate Superconductors

We present phase-sensitive evidence that the electron-doped cuprates Nd1.85Ce0.15CuO4-y (NCCO) and Pr1.85Ce0.15CuO4-y (PCCO) have d-wave pairing symmetry. This evidence was obtained by observing the half-flux quantum effect, using a scanning SQUID microscope, in c-axis oriented films of NCCO or PCCO epitaxially grown on tricrystal [100] SrTiO3 substrates designed to be frustrated for a d(x2-y2) order parameter. Samples with two other configurations, designed to b unfrustrated for a d-wave superconductor, do not show the half-flux quantum effect.

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arXiv2000

d-wave pairing symmetry in cuprate superconductors

Phase-sensitive tests of pairing symmetry have provided strong evidence for predominantly d-wave pairing symmetry in both hole- and electron-doped high-Tc cuprate superconductors. Temperature dependent measurements in YBCO indicate that the d-wave pairing dominates, with little if any imaginary component, at all temperatures from 0.5K through Tc. In this article we review some of this evidence and discuss the implications of the universal d-wave pairing symmetry in the cuprates.

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