arXiv subjects

C. Chin

Publications and source records attributed to C. Chin.

15 recordsLinked to original sources

arXiv2026

First-order phase transition in atom-molecule quantum degenerate mixtures with coherent three-body recombination

We map the phase diagram of a two-mode atom-molecule Bose-Einstein condensate with Fano-Feshbach and coherent three-body recombination (cTBR) terms. The standard second order phase transition observed as the molecular energy is tuned through the Feshbach resonance, is replaced by a first order transition when cTBR becomes prominent, due to a double-well structure in the free energy landscape. This transition is associated with atom-molecule entanglement, bistability, and molecular metastability. Our results establish cTBR as a powerful knob for quantum state engineering and control of reaction dynamics in ultracold chemistry.

cond-mat.quant-gas↗

arXiv2009

Determination of atomic scattering lengths from measurements of molecular binding energies near Feshbach resonances

We present an analytic model to calculate the atomic scattering length near a Feshbach resonance from data on the molecular binding energy. Our approach considers finite-range square-well potentials and can be applied near broad, narrow, or even overlapping Feshbach resonances. We test our model on Cs$_2$ Feshbach molecules. We measure the binding energy using magnetic-field modulation spectroscopy in a range where one broad and two narrow Feshbach resonances overlap. From the data we accurately determine the Cs atomic scattering length and the positions and widths of two particular resonances.

cond-mat.other↗

arXiv2007

Spectroscopy of Ultracold, Trapped Cesium Feshbach Molecules

We explore the rich internal structure of Cs_2 Feshbach molecules. Pure ultracold molecular samples are prepared in a CO_2-laser trap, and a multitude of weakly bound states is populated by elaborate magnetic-field ramping techniques. Our methods use different Feshbach resonances as input ports and various internal level crossings for controlled state transfer. We populate higher partial-wave states of up to eight units of rotational angular momentum (l-wave states). We investigate the molecular structure by measurements of the magnetic moments for various states. Avoided level crossings between different molecular states are characterized through the changes in magnetic moment and by a Landau-Zener tunneling method. Based on microwave spectroscopy, we present a precise measurement of the magnetic-field dependent binding energy of the weakly bound s-wave state that is responsible for the large background scattering length of Cs. This state is of particular interest because of its quantum-halo character.

cond-mat.other↗

arXiv2007

`Stückelberg interferometry' with ultracold molecules

We report on the realization of a time-domain `Stückelberg interferometer', which is based on the internal state structure of ultracold Feshbach molecules. Two subsequent passages through a weak avoided crossing between two different orbital angular momentum states in combination with a variable hold time lead to high-contrast population oscillations. This allows for a precise determination of the energy difference between the two molecular states. We demonstrate a high degree of control over the interferometer dynamics. The interferometric scheme provides new possibilities for precision measurements with ultracold molecules.

cond-mat.other↗

arXiv2006

Precision Measurements of Collective Oscillations in the BEC-BCS Crossover

We report on precision measurements of the frequency of the radial compression mode in a strongly interacting, optically trapped Fermi gas of Li-6 atoms. Our results allow for a test of theoretical predictions for the equation of state in the BEC-BCS crossover. We confirm recent quantum Monte-Carlo results and rule out simple mean-field BCS theory. Our results show the long-sought beyond-mean-field effects in the strongly interacting BEC regime.

cond-mat.other↗

arXiv2006

Experimental Evidence for Efimov Quantum States

Three interacting particles form a system which is well known for its complex physical behavior. A landmark theoretical result in few-body quantum physics is Efimov's prediction of a universal set of weakly bound trimer states appearing for three identical bosons with a resonant two-body interaction. Surprisingly, these states even exist in the absence of a corresponding two-body bound state and their precise nature is largely independent of the particular type of the two-body interaction potential. Efimov's scenario has attracted great interest in many areas of physics; an experimental test however has not been achieved. We report the observation of an Efimov resonance in an ultracold thermal gas of cesium atoms. The resonance occurs in the range of large negative two-body scattering lengths and arises from the coupling of three free atoms to an Efimov trimer. We observe its signature as a giant three-body recombination loss when the strength of the two-body interaction is varied near a Feshbach resonance. This resonance develops into a continuum resonance at non-zero collision energies, and we observe a shift of the resonance position as a function of temperature. We also report on a minimum in the recombination loss for positive scattering lengths, indicating destructive interference of decay pathways. Our results confirm central theoretical predictions of Efimov physics and represent a starting point from which to explore the universal properties of resonantly interacting few-body systems.

cond-mat.other↗

arXiv2006

Evidence for Efimov quantum states in an ultracold gas of cesium atoms

Systems of three interacting particles are notorious for their complex physical behavior. A landmark theoretical result in few-body quantum physics is Efimov's prediction of a universal set of bound trimer states appearing for three identical bosons with a resonant two-body interaction. Counterintuitively, these states even exist in the absence of a corresponding two-body bound state. Since the formulation of Efimov's problem in the context of nuclear physics 35 years ago, it has attracted great interest in many areas of physics. However, the observation of Efimov quantum states has remained an elusive goal. Here we report the observation of an Efimov resonance in an ultracold gas of cesium atoms. The resonance occurs in the range of large negative two-body scattering lengths, arising from the coupling of three free atoms to an Efimov trimer. Experimentally, we observe its signature as a giant three-body recombination loss when the strength of the two-body interaction is varied. We also detect a minimum in the recombination loss for positive scattering lengths, indicating destructive interference of decay pathways. Our results confirm central theoretical predictions of Efimov physics and represent a starting point with which to explore the universal properties of resonantly interacting few-body systems. While Feshbach resonances have provided the key to control quantum-mechanical interactions on the two-body level, Efimov resonances connect ultracold matter to the world of few-body quantum phenomena.

cond-mat.other↗

arXiv2004

Exploring the BEC-BCS Crossover with an Ultracold Gas of $^6$Li Atoms

We present an overview of our recent measurements on the crossover from a Bose-Einstein condensate of molecules to a Bardeen-Cooper-Schrieffer superfluid. The experiments are performed on a two-component spin-mixture of $^6$Li atoms, where a Fesh\-bach resonance serves as the experimental key to tune the s-wave scattering length and thus to explore the various interaction regimes. In the BEC-BCS crossover, we have characterized the interaction energy by measuring the size of the trapped gas, we have studied collective excitation modes, and we have observed the pairing gap. Our observations provide strong evidence for superfluidity in the strongly interacting Fermi gas.

cond-mat.other↗

arXiv2004

Observation of Feshbach-like resonances in collisions between ultracold molecules

We observe magnetically tuned collision resonances for ultracold Cs2 molecules stored in a CO2-laser trap. By magnetically levitating the molecules against gravity, we precisely measure their magnetic moment. We find an avoided level crossing which allows us to transfer the molecules into another state. In the new state, two Feshbach-like collision resonances show up as strong inelastic loss features. We interpret these resonances as being induced by Cs4 bound states near the molecular scattering continuum. The tunability of the interactions between molecules opens up novel applications such as controlled chemical reactions and synthesis of ultracold complex molecules.

cond-mat.other↗

arXiv2004

Efficient creation of molecules from a cesium Bose-Einstein condensate

We report a new scheme to create weakly bound Cs$_2$ molecules from an atomic Bose-Einstein condensate. The method is based on switching the magnetic field to a narrow Feshbach resonance and yields a high atom-molecule conversion efficiency of more than 30%, a factor of three higher than obtained with conventional magnetic-field ramps. The Cs$_2$ molecules are created in a single $g$-wave rotational quantum state. The observed dependence of the conversion efficiency on the magnetic field and atom density shows scattering processes beyond two-body coupling to occur in the vicinity of the Feshbach resonance.

cond-mat.soft↗

arXiv2004

Precise determination of $^6$Li cold collision parameters by radio-frequency spectroscopy on weakly bound molecules

We employ radio-frequency spectroscopy on weakly bound $^6$Li$_2$ molecules to precisely determine the molecular binding energies and the energy splittings between molecular states for different magnetic fields. These measurements allow us to extract the interaction parameters of ultracold $^6$Li atoms based on a multi-channel quantum scattering model. We determine the singlet and triplet scattering lengths to be $a_s=45.167(8)a_0$ and $a_t=-2140(18)a_0$ (1 $a_0$ = 0.0529177 nm), and the positions of the broad Feshbach resonances in the energetically lowest three $s-$wave scattering channels to be 83.41(15) mT, 69.04(5) mT, and 81.12(10) mT.

cond-mat.other↗

arXiv2004

Observation of the Pairing Gap in a Strongly Interacting Fermi Gas

We study fermionic pairing in an ultracold two-component gas of $^6$Li atoms by observing an energy gap in the radio-frequency excitation spectra. With control of the two-body interactions via a Feshbach resonance we demonstrate the dependence of the pairing gap on coupling strength, temperature, and Fermi energy. The appearance of an energy gap with moderate evaporative cooling suggests that our full evaporation brings the strongly interacting system deep into a superfluid state.

cond-mat.supr-con↗

arXiv2004

Collective excitations of a degenerate gas at the BEC-BCS crossover

We study collective excitation modes of a fermionic gas of $^6$Li atoms in the BEC-BCS crossover regime. While measurements of the axial compression mode in the cigar-shaped trap close to a Feshbach resonance confirm theoretical expectations, the radial compression mode shows surprising features. In the strongly interacting molecular BEC regime we observe a negative frequency shift with increasing coupling strength. In the regime of a strongly interacting Fermi gas, an abrupt change in the collective excitation frequency occurs, which may be a signature for a transition from a superfluid to a collisionless phase.

cond-mat.other↗

arXiv2004

Crossover from a molecular Bose-Einstein condensate to a degenerate Fermi gas

We demonstrate a reversible conversion of a Li2 molecular Bose-Einstein condensate to a degenerate Fermi gas of atoms by adiabatically crossing a Feshbach resonance. By optical in situ imaging, we observe a smooth change of the cloud size in the crossover regime. On the Feshbach resonance, the ensemble is strongly interacting and the measured cloud size is 75(7)% of the one of a non-interacting zero-temperature Fermi gas. The high condensate fraction of more than 90% and the adiabatic crossover suggest our Fermi gas to be cold enough to form a superfluid.

cond-mat.other↗

arXiv2003

Pure Gas of Optically Trapped Molecules Created from Fermionic Atoms

We report on the production of a pure sample of up to 3x10^5 optically trapped molecules from a Fermi gas of 6Li atoms. The dimers are formed by three-body recombination near a Feshbach resonance. For purification a Stern-Gerlach selection technique is used that efficiently removes all trapped atoms from the atom-molecule mixture. The behavior of the purified molecular sample shows a striking dependence on the applied magnetic field. For very weakly bound molecules near the Feshbach resonance, the gas exhibits a remarkable stability with respect to collisional decay.

cond-mat.soft↗