arXiv subjects

C. D. Pruitt

Publications and source records attributed to C. D. Pruitt.

12 recordsLinked to original sources

arXiv2024

The role of the likelihood for elastic scattering uncertainty quantification

Background: Analyses of elastic scattering with the optical model (OMP) are widely used in nuclear reactions. Purpose: Previous work compared a traditional frequentist approach and a Bayesian approach to quantify uncertainties in the OMP. In this study, we revisit this comparison and consider the role of the likelihood used in the analysis. Method: We compare the Levenberg-Marquardt algorithm for $χ^{2}$ minimization with Markov Chain Monte Carlo sampling to obtain parameter posteriors. Following previous work, we consider how results are affected when $χ^{2}$/N is used for the likelihood function, N being the number of data points, to account for possible correlations in the model and underestimation of the error in the data. Results: We analyze a simple linear model and then move to OMP analysis of elastic angular distributions using a) a 5-parameter model and b) a 6-parameter model. In the linear model, the frequentist and Bayesian approaches yield consistent optima and uncertainty estimates. The same is qualitatively true for the 5-parameter OMP analysis. For the 6-parameter OMP analysis, the parameter posterior is no longer well-approximated by a Gaussian and a covariance-based frequentist prediction becomes unreliable. In all cases, when the Bayesian approach uses $χ^{2}$/N in the likelihood, uncertainties increase by $\sqrt{N}$. Conclusions: When the parameter posterior is near-Gaussian and the same likelihood is used, the frequentist and Bayesian approaches recover consistent parameter uncertainty estimates. If the parameter posterior has significant higher moments, the covariance-only frequentist approach becomes unreliable and the Bayesian approach should be used. Empirical coverage can serve as an important internal check for uncertainty estimation, providing red flags for uncertainty analyses.

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arXiv2023

Strong evidence for 9N and the limits of existence of atomic nuclei

The boundaries of the Chart of Nuclides contain exotic isotopes that possess extreme proton-toneutron asymmetries. Here we report on strong evidence of 9N, one of the most exotic proton-rich isotopes where more than one half of its constitute nucleons are unbound. With seven protons and two neutrons, this extremely proton-rich system would represent the first-known example of a ground-state five-proton emitter. The invariant-mass spectrum of its decay products can be fit with two peaks whose energies are consistent with the theoretical predictions of an open-quantum-system approach, however we cannot rule out the possibility that only a single resonance-like peak is present in the spectrum.

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arXiv2023

Optical potentials for the rare-isotope beam era

We review recent progress and motivate the need for further developments in nuclear optical potentials that are widely used in the theoretical analysis of nucleon elastic scattering and reaction cross sections. In regions of the nuclear chart away from stability, which represent a frontier in nuclear science over the coming decade and which will be probed at new rare-isotope beam facilities worldwide, there is a targeted need to quantify and reduce theoretical reaction model uncertainties, especially with respect to nuclear optical potentials. We first describe the primary physics motivations for an improved description of nuclear reactions involving short-lived isotopes, focusing on its benefits for fundamental science discoveries and applications to medicine, energy, and security. We then outline the various methods in use today to build optical potentials starting from phenomenological, microscopic, and ab initio methods, highlighting in particular the strengths and weaknesses of each approach. We then discuss publicly-available tools and resources facilitating the propagation of recent progresses in the field to practitioners. Finally, we provide a set of open challenges and recommendations for the field to advance the fundamental science goals of nuclear reaction studies in the rare-isotope beam era.

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arXiv2022

Uncertainty-quantified phenomenological optical potentials for single-nucleon scattering

Optical-model potentials (OMPs) continue to play a key role in nuclear reaction calculations. However, the uncertainty of phenomenological OMPs in widespread use -- inherent to any parametric model trained on data -- has not been fully characterized, and its impact on downstream users of OMPs remains unclear. Here we assign well-calibrated uncertainties for two representative global OMPs, those of Koning-Delaroche and Chapel Hill '89, using Markov-Chain Monte Carlo for parameter inference. By comparing the canonical versions of these OMPs against the experimental data originally used to constrain them, we show how a lack of outlier rejection and a systematic underestimation of experimental uncertainties contributes to bias of, and overconfidence in, best-fit parameter values. Our updated, uncertainty-quantified versions of these OMPs address these issues and yield complete covariance information for potential parameters. Scattering predictions generated from our ensembles show improved performance both against the original training corpora of experimental data and against a new "test" corpus comprising many of the experimental single-nucleon scattering data collected over the last twenty years. Finally, we apply our uncertainty-quantified OMPs to two case studies of application-relevant cross sections. We conclude that, for many common applications of OMPs, including OMP uncertainty should become standard practice. To facilitate their immediate use, digital versions of our updated OMPs and related tools for forward uncertainty propagation are included as Supplementary Material.

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arXiv2021

Using spin alignment of inelastically-excited fast beams to make spin assignments: the spectroscopy of 13O as a test case

Excited states in 13O were investigated using inelastic scattering of an E/A=69.5-MeV 13O beam off of a 9Be target. The excited states were identified in the invariant-mass spectra of the decay products. Both single proton and sequential two-proton decays of the excited states were examined. For a number of the excited states, the protons were emitted with strong anisotropy where emissions transverse to the beam axis are favored. The measured proton-decay angular distributions were compared to predictions from distorted-wave born-approximation (DWBA) calculations of the spin alignment which was shown to be largely independent of the excitation mechanism. The deduced $^{13}$O level scheme is compared to ab initio no-core shell model with continuum (NCSMC) predictions. The lowest-energy excited states decay isotropically consistent with predictions of strong proton 1s1/2 structure. Above these states in the level scheme, we observed a number of higher-spin states not predicted within the model. Possibly these are associated with rotational bands built on deformed cluster configurations predicted by antisymmetrized molecular dynamics (AMD) calculations. The spin alignment mechanism is shown to be useful for making spin assignments and may have widespread use.

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arXiv2021

Evidence against the Efimov effect in $^{12}\mathrm{C}$ from spectroscopy and astrophysics

Background: The Efimov effect is a universal phenomenon in physics whereby three-body systems are stabilized via the interaction of an unbound two-body sub-systems. A hypothetical state in $^{12}\mathrm{C}$ at 7.458 MeV excitation energy, comprising of a loose structure of three $α$-particles in mutual two-body resonance, has been suggested in the literature to correspond to an Efimov state in nuclear physics. The existence of such a state has not been demonstrated experimentally. Method: Using the combined data sets from two recent experiments, one with the TexAT TPC to measure $α$-decay and the other with Gammasphere to measure $γ$-decay of states in $^{12}\mathrm{C}$ populated by $^{12}\mathrm{N}$ and $^{12}\mathrm{B}$ $β$-decay respectively, we achieve high sensitivity to states in close-proximity to the $α$-threshold in $^{12}\mathrm{C}$. Results: No evidence of a state at 7.458 MeV is seen in either data set. Using a likelihood method, the 95\% C.L. $γ$-decay branching ratio is determined as a function of the $β$-decay feeding strength relative to the Hoyle state. In parallel, calculations of the triple-alpha reaction rate show the inclusion of the Efimov corresponds to a large increase in the reaction rate around $5 \times 10^{7}$ K. Conclusion: From decay spectroscopy - at the 95\% C.L., the Efimov state cannot exist at 7.458 MeV with any $γ$-decay branching ratio unless the $β$-strength is less than 0.7\% of the Hoyle state. This limit is evaluated for a range of different excitation energies and the results are not favorable for existence of the hypothetical Efimov state in $^{12}\mathrm{C}$. Furthermore, the triple-alpha reaction rate with the inclusion of a state between 7.43 and 7.53 MeV exceeds the rate required for stars to undergo the red giant phase.

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arXiv2020

Almost medium-free measurement of the Hoyle state direct-decay component with a TPC

Background: The structure of the Hoyle state, a highly $α$-clustered state at 7.65 MeV in $^{12}\mathrm{C}$, has long been the subject of debate. Understanding if the system comprises of three weakly-interacting $α$-particles in the 0s orbital, known as an $α$-condensate state, is possible by studying the decay branches of the Hoyle state. Purpose: The direct decay of the Hoyle state into three $α$-particles, rather than through the $^{8}\mathrm{Be}$ ground state, can be identified by studying the energy partition of the 3 $α$-particles arising from the decay. This paper provides details on the break-up mechanism of the Hoyle stating using a new experimental technique. Method: By using beta-delayed charged-particle spectroscopy of $^{12}\mathrm{N}$ using the TexAT (Texas Active Target) TPC, a high-sensitivity measurement of the direct 3 $α$ decay ratio can be performed without contributions from pile-up events. Results: A Bayesian approach to understanding the contribution of the direct components via a likelihood function shows that the direct component is $<0.043\%$ at the 95\% confidence level (C.L.). This value is in agreement with several other studies and here we can demonstrate that a small non-sequential component with a decay fraction of about $10^{-4}$ is most likely. Conclusion: The measurement of the non-sequential component of the Hoyle state decay is performed in an almost medium-free reaction for the first time. The derived upper-limit is in agreement with previous studies and demonstrates sensitivity to the absolute branching ratio. Further experimental studies would need to be combined with robust microscopic theoretical understanding of the decay dynamics to provide additional insight into the idea of the Hoyle state as an $α$-condensate.

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arXiv2020

Isotopically resolved neutron total cross sections at intermediate energies

The neutron total cross sections $σ_{tot}$ of $^{16,18}$O, $^{58,64}$Ni, $^{103}$Rh, and $^{112,124}$Sn have been measured at the Los Alamos Neutron Science Center (LANSCE) from low to intermediate energies (3 $\leq E_{lab} \leq$ 450 MeV) by leveraging waveform-digitizer technology. The $σ_{tot}$ relative differences between isotopes are presented, revealing additional information about the isovector components needed for an accurate optical-model description away from stability. Digitizer-enabled $σ_{tot}$-measurement techniques are discussed and a series of uncertainty-quantified dispersive optical model (DOM) analyses using these new data is presented, validating the use of the DOM for modeling light systems ($^{16,18}$O) and systems with open neutron shells ($^{58,64}$Ni and $^{112,124}$Sn). The valence-nucleon spectroscopic factors extracted for each isotope reaffirm the usefulness of high-energy proton reaction cross sections for characterizing depletion from the mean-field expectation.

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arXiv2020

Systematic Matter and Binding-Energy Distributions from a Dispersive Optical Model Analysis

We present the first systematic nonlocal dispersive optical model analysis using both bound-state and scattering data of $^{16,18}$O, $^{40,48}$Ca, $^{58,64}$Ni, $^{112,124}$Sn, and $^{208}$Pb. In all systems, roughly half the total nuclear binding energy is associated with the most-bound 10% of the total nucleon density. The extracted neutron skins reveal the interplay of asymmetry, Coulomb, and shell effects on the skin thickness. Our results indicate that simultaneous optical model fits of inelastic scattering and structural data on isotopic pairs are effective for constraining asymmetry-dependent nuclear structural quantities otherwise difficult to observe experimentally.

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arXiv2020

A dispersive optical model analysis of $^{208}$Pb generating a neutron-skin prediction beyond the mean field

A nonlocal dispersive-optical-model analysis has been carried out for neutrons and protons in $^{208}$Pb. Elastic-scattering angular distributions, total and reaction cross sections, single-particle energies, the neutron and proton numbers, the charge distribution, and the binding energy have been fitted to extract the neutron and proton self-energies both above and below the Fermi energy. From the single-particle propagator derived from these self-energies, we have determined the charge and matter distributions in $^{208}$Pb. The predicted spectroscopic factors are consistent with results from the $(e,e'p)$ reaction and inelastic-electron-scattering data to very high spin states. Sensible results for the high-momentum content of neutrons and protons are obtained with protons appearing more correlated, in agreement with experiment and \textit{ab initio} calculations of asymmetric matter. A neutron skin of $0.25\pm0.05$ fm is deduced. An analysis of several nuclei leads to the conclusion that finite-size effects play a non-negligible role in the formation of the neutron skin in finite nuclei.

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arXiv2020

Particle decays of levels in $^{11,12}$N and $^{12}$O investigated with the invariant-mass method

Particle-decaying states of the light nuclei $^{11,12}$N and $^{12}$O were studied using the invariant-mass method. The decay energies and intrinsic widths of a number of states were measured, and the momentum correlations of three-body decaying states were considered. A second 2$p$-decaying 2$^+$ state of $^{12}$O was observed for the first time, and a higher energy $^{12}$O state was observed in the 4$p$+2$α$ decay channel. This 4$p$+2$α$ channel also contains contributions from fission-like decay paths, including $^6$Be$_{g.s.}$+$^{6}$Be$_{g.s.}$. Analogs to these states in $^{12}$O were found in $^{12}$N in the 2$p$+$^{10}$B and 2$p$+$α$+$^6$Li channels. The momentum correlations for the prompt 2$p$ decay of $^{12}$O$_{g.s.}$ were found to be nearly identical to those of $^{16}$Ne$_{g.s.}$, and the correlations for the new 2$^+$ state were found to be consistent with sequential decay through excited states in $^{11}$N. The momentum correlations for the 2$^+_1$ state in $^{12}$O provide a new value for the $^{11}$N ground-state energy. The states in $^{12}$N/$^{12}$O that belong to the $A$=12 isobaric sextet do not deviate from the quadratic isobaric multiplet mass equation (IMME) form.

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arXiv2019

First observation of unbound $^{11}$O, the mirror of the halo nucleus $^{11}$Li

The structure of the extremely proton-rich nucleus $^{11}_{~8}$O$_3$, the mirror of the two-neutron halo nucleus $^{11}_{~3}$Li$_8$, has been studied experimentally for the first time. Following two-neutron knockout reactions with a $^{13}$O beam, the $^{11}$O decay products were detected after two-proton emission and used to construct an invariant-mass spectrum. A broad peak of width $\sim$3\,MeV was observed. Within the Gamow coupled-channel approach, it was concluded that this peak is a multiplet with contributions from the four-lowest $^{11}$O resonant states: $J^π$=3/2$^-_1$, 3/2$^-_2$, 5/2$^+_1$, and 5/2$^+_2$. The widths and configurations of these states show strong, non-monotonic dependencies on the depth of the $p$-$^9$C potential. This unusual behavior is due to the presence of a broad threshold resonant state in $^{10}$N, which is an analog of the virtual state in $^{10}$Li in the presence of the Coulomb potential. After optimizing the model to the data, only a moderate isospin asymmetry between ground states of $^{11}$O and $^{11}$Li was found.

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