arXiv subjects

C. Delafosse

Publications and source records attributed to C. Delafosse.

18 recordsLinked to original sources

arXiv2025

Data sorting modes of phoswich detector array

The different data-sorting modes of the phoswich detector array PARIS used for detecting high-energy (4$-$10 MeV) $\gamma$ rays are investigated. The characteristics including time resolution, energy resolution and detection efficiency under various modes are studied. The present study shows that PARIS has capabilities of rejecting escape and pileup events when used for decay spectroscopy. Notably, the methods presented in this work refer specifically to the $\beta$-decay experiment of $^{80g+m}$Ga conducted with three PARIS clusters comprising 27 phoswich detectors, rather than to a general report on the PARIS array or its overall performance for in-beam spectroscopy. Compared with the 2"$\times$2"$\times$2" LaBr$_3$(Ce) detector (Ciema{\l}a et al., 2009), even in individual mode, PARIS provides significant suppression of single- and double-escape peaks and reduces background via vetoing function of the outer-volume NaI(Tl) crystals. In contrast to the common approach of adding back the energies in LaBr$_3$(Ce) and NaI(Tl) to increase the detection efficiency of the full-energy peak, using NaI(Tl) as a veto shield provides a superior trade-off for applications where spectral purity is essential. Employing add-back analysis within each cluster of nine phoswiches or between all phoswiches could enhance full-energy peak efficiency and further suppress escape peaks and background. Applying a multiplicity condition provides a further suppression but simultaneously lowers the statistics of full-energy peaks.

physics.ins-det↗

arXiv2025

$\beta$-delayed spectroscopy of $^{80}$Ge$_{48}$ and competition between Gamow-Teller and first-forbidden transitions in $^{80g+m}$Ga$_{49}$ $\beta$ decay

The $\beta$-delayed spectroscopy of $^{80}$Ge has been studied using sources of ground and low-lying isomeric states of $^{80}$Ga. A hybrid $\gamma$-ray spectrometer was used, composed of high-purity germanium (HPGe) detectors for low-energy $\gamma$-ray detection, phoswich detectors from the PARIS array for high-energy $\gamma$ rays and a plastic detector for $\beta$ tagging. The new decay level schemes are presented, with 13 and 14 states $\beta$ populated by $^{80g}$Ga and $^{80m}$Ga, respectively, being reported for the first time. We quantitatively compare summed intensities of first-forbidden and previously reported Gamow-Teller $\beta$ transitions [R. Li et al., \href{https://doi.org/10.1103/PhysRevC.111.034303}{Phys. Rev. C 111, 034303 (2025)}]. The upper-limit fractions of first-forbidden transitions contributing to the decays of $^{80g}$Ga and $^{80m}$Ga are (48.0 $\pm$ 2.7)$\%$ and (47.9 $\pm$ 3.3)$\%$ of the observed total $\beta$ transition intensities of (78.2 $\pm$ 2.5)$\%$ and (82.2 $\pm$ 3.7)$\%$, respectively. Notably, the half-lives decrease in accordance with the upper limits of (48.0 $\pm$ 6.0)$\%$ [3.67(20) s $\rightarrow$ 1.91(3) s] and (47.9 $\pm$ 7.2)$\%$ [3.01(19) s $\rightarrow$ 1.57(1) s] for $^{80g}$Ga and $^{80m}$Ga, respectively, when including first-forbidden transitions, in contrast to those by Gamow-Teller transitions only.

nucl-ex↗

arXiv2025

$\beta$-delayed neutron spectroscopy of $^{85, 86}$As with MONSTER at IGISOL

The $\beta$-delayed neutron emission in the $^{85, 86}$As $\beta$-decays has been measured at the Ion Guide Isotope Separator On Line facility of the Accelerator Laboratory of the University of Jyv\"askyl\"a. The complete $\beta$-decays have been studied with a complex setup that consists of a plastic scintillator for $\beta$-particles, MONSTER -- the MOdular Neutron time-of-flight SpectromeTER -- for neutrons, and a high-purity germanium and four LaBr$_3$ crystals for $\gamma$-rays. The $\beta$-delayed neutron energy distributions have been determined by unfolding the time-of-flight spectra with an innovative methodology based on the iterative Bayesian unfolding method and accurate Monte Carlo simulations. The results obtained for $^{85}$As are in excellent agreement with the existing evaluated data, validating the proposed methodology. In the case of $^{86}$As, a stronger neutron intensity at higher energies than previously predicted is discovered.

nucl-ex↗

arXiv2024

Binding energies, charge radii, spins and moments: odd-odd Ag isotopes and discovery of a new isomer

We report on the masses and hyperfine structure of ground and isomeric states in $^{114,116,118,120}$Ag isotopes, measured with the phase-imaging ion-cyclotron-resonance technique (PI-ICR) with the JYFLTRAP mass spectrometer and the collinear laser spectroscopy beamline at the Ion Guide Isotope Separator On-Line (IGISOL) facility, Jyv\"askyl\"a, Finland. We measured the masses and excitation energies, electromagnetic moments, and charge radii, and firmly established the nuclear spins of the long-lived states. A new isomer was discovered in $^{118}$Ag and the half-lives of $^{118}$Ag long-lived states were reevaluated. We unambiguously pinned down the level ordering of all long-lived states, placing the inversion of the $I = 0^-$ and $I = 4^+$ states at $A = 118$ $(N = 71)$. Lastly, we compared the electromagnetic moments of each state to empirical single-particle moments to identify the dominant configuration where possible.

nucl-ex↗

arXiv2024

Simultaneous impacts of nuclear shell structure and collectivity on $\beta$ decay: Evidence from $^{80}$Ga$_{49}$

The Gamow-Teller strength distribution covering the entire $\beta$-decay window, up to 10.312(4) MeV, of $^{80g+m}$Ga was measured for the first time in photo fission of UC$_x$ induced by a 50 MeV electron beam. The new data show significant enhancement in the high-energy region with a jump structure. Simultaneously, the $\gamma$ deexciting behavior of $\beta$-populated states presents a competition between deexcitation to 2$_1^+$ [$\beta_2$ = 0.155(9)] and to 2$_2^+$ [$\beta_2$ = 0.053$_{0.009}^{0.008}$)] in $^{80}$Ge. To understand these data, we performed a realistic shell-model calculation and systematic analysis of log $\it{ft}$ ratios between precursors' $\beta$ decay to 2$_2^+$ and to 2$_1^+$ of Ga isotopes. We conclude that these phenomena evidence simultaneous impacts of nuclear shell structure and collectivity on $\it{B}$(GT) distribution and therefore the half-life of the precursor.

nucl-ex↗

arXiv2024

High-resolution spectroscopy of neutron-rich Br isotopes and signatures for a prolate-to-oblate shape transition at N=56

The first systematic experimental study of the neutron-rich Br isotopes with two complementary state-of-the-art techniques is presented. These isotopes have been populated in the fission process at two different facilities, GANIL and ILL. New spectroscopic information has been obtained for odd-even $^{87-93}$Br isotopes and the experimental results have been compared with state-of-the-art Large-Scale Shell-Model and DNO Shell-Model calculations. As a result of such theoretical approaches, a transition from prolate ($^{87,89}$Br) to oblate ($^{91,93}$Br) shapes is obtained from the subtle balance between proton and neutron quadrupole deformations, as a clear signature of pseudo-SU3 quadrupole regime.

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arXiv2024

Isomeric states of fission fragments explored via Penning trap mass spectrometry at IGISOL

The masses of $^{84}$Br, $^{105}$Mo, $^{115,119,121}$Pd, $^{122}$Ag, $^{127,129}$In, $^{132}$Sb and their respective isomeric states have been measured with the JYFLTRAP Penning trap mass spectrometer using the phase-imaging ion-cyclotron-resonance technique. The excitation energies of the isomeric states in $^{132}$Sb and $^{119}$Pd were experimentally determined for the first time, while for $^{84}$Br, $^{115}$Pd and $^{127,129}$In, the precision of the mass values was substantially improved. In $^{105}$Mo and $^{121}$Pd there were no signs of a long-lived isomeric state. The ground-state measurements of $^{119}$Pd and $^{122}$Ag indicated that both are significantly more bound than the literature values. For $^{122}$Ag, there was no indication of a proposed third long-lived state. The results for the $N=49$ nucleus $^{84}$Br and isomers close to doubly magic $^{132}$Sn have been compared to the shell-model and the microscopic quasiparticle-phonon model calculations.

nucl-ex↗

arXiv2024

Mass measurements in the $^{132}$Sn region with the JYFLTRAP double Penning trap mass spectrometer

We report on new precision mass measurements of neutron-rich $^{137}$Sb and $^{136-142}$I isotopes from the JYFLTRAP double Penning trap mass spectrometer. We confirm the value from the previous Penning-trap measurement of $^{137}$Sb at the Canadian Penning Trap and therefore rule out the conflicting result from the Experimental Storage Ring. The ground state and isomer in $^{136}$I were resolved and measured directly for the first time. The isomer excitation energy, $E_x = 215.1(43)$ keV, agrees with the literature but is three times more precise. The measurements have improved the precision of the mass values and confirmed previous results in the majority of cases. However, for $^{138,140}$I the results differ by 17(6) keV and 23(12) keV, respectively. This could be explained by an unresolved contamination or different ratio of unresolved isomeric states in the case of $^{140}$I.

nucl-ex↗

arXiv2024

First investigation on the isomeric ratio in multinucleon transfer reactions: Entrance channel effects on the spin distribution

The multinucleon transfer (MNT) reaction approach was successfully employed for the first time to measure the isomeric ratios (IRs) of $^{211}$Po (25/2$^+$) isomer and its (9/2$^+$) ground state at the IGISOL facility using a 945 MeV $^{136}$Xe beam impinged on $^{209}$Bi and $^{\rm nat}$Pb targets. The dominant production of isomers compared to the corresponding ground states was consistently revealed in the $\alpha$-decay spectra. Deduced IR of $^{211}$Po populated through the $^{136}$Xe+$^{\rm nat}$Pb reaction was found to enhance $\approx$1.8-times than observed for $^{136}$Xe+$^{209}$Bi. State-of-the-art Langevin-type model calculations have been utilized to estimate the spin distribution of an MNT residue. The computations qualitatively corroborate with the considerable increase in IRs of $^{211}$Po produced from $^{136}$Xe+$^{\rm nat}$Pb compared to $^{136}$Xe+$^{209}$Bi. Theoretical investigations indicate a weak influence of target spin on IRs. The enhancement of the $^{211}$Po isomer in the $^{136}$Xe+$^{\rm nat}$Pb over $^{136}$Xe+$^{209}$Bi can be attributed to the different proton ($p$)-transfer production routes. Estimations demonstrate an increment in the angular momentum transfer, favorable for isomer production, with increasing projectile energy. Comparative analysis indicates the two entrance channel parameters, projectile mass and $p$-transfer channels, strongly influencing the population of the high-spin isomer of $^{211}$Po (25/2$^+$). This is the first experimental and theoretical investigation on the IRs of nuclei produced via different channels of MNT reactions, with the latter quantitatively underestimating the former by a factor of two.

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arXiv2023

Isospin symmetry in the $T = 1, A = 62$ triplet

Excited states in the $T_z = 0, -1$ nuclei $^{62}$Ga and $^{62}$Ge were populated in direct reactions of relativistic radioactive ion beams at the RIBF. Coincident \grays were measured with the DALI2$^+$ array and uniquely assigned to the $A=62$ isobars. In addition, $^{62}$Ge was also studied independently at JYFL-ACCLAB using the ${}^{24}$Mg(${}^{40}$Ca,$2n$)${}^{62}$Ge fusion-evaporation reaction. The first excited $T=1, J^π=2^+$ states in $^{62}$Ga and $^{62}$Ge were identified at $979(1)$ and $965(1)$~keV, respectively, resolving discrepant interpretations in the literature. States beyond the first $2^+$ state in $^{62}$Ge were also identified for the first time in the present work. The results are compared with shell-model calculations in the $fp$ model space. Mirror and triplet energy differences are analyzed in terms of individual charge-symmetry and charge-independence breaking contributions. The MED results confirm the shrinkage of the $p$-orbits' radii when they are occupied by at least one nucleon on average.

nucl-ex↗

arXiv2023

Binding energies of ground and isomeric states in neutron-rich ruthenium isotopes: measurements at JYFLTRAP and comparison to theory

We report on precision mass measurements of $^{113,115,117}$Ru performed with the JYFLTRAP double Penning trap mass spectrometer at the Accelerator Laboratory of University of Jyväskylä. The phase-imaging ion-cyclotron-resonance technique was used to resolve the ground and isomeric states in $^{113,115}$Ru and enabled for the first time a measurement of the isomer excitation energies, $E_x(^{113}$Ru$^{m})=100.5(8)$ keV and $E_x(^{115}$Ru$^{m})=129(5)$ keV. The ground state of $^{117}$Ru was measured using the time-of-flight ion-cyclotron-resonance technique. The new mass-excess value for $^{117}$Ru is around 36 keV lower and 7 times more precise than the previous literature value. With the more precise ground-state mass values, the evolution of the two-neutron separation energies is further constrained and a similar trend as predicted by the BSkG1 model is obtained up to the neutron number $N=71$.

nucl-ex↗

arXiv2023

Probing Earth's Missing Potassium using the Unique Antimatter Signature of Geoneutrinos

The formation of the Earth remains an epoch with mysterious puzzles extending to our still incomplete understanding of the planet's potential origin and bulk composition. Direct confirmation of the Earth's internal heat engine was accomplished by the successful observation of geoneutrinos originating from uranium (U) and thorium (Th) progenies, manifestations of the planet's natural radioactivity dominated by potassium (40K) and the decay chains of uranium (238U) and thorium (232Th). This radiogenic energy output is critical to planetary dynamics and must be accurately measured for a complete understanding of the overall heat budget and thermal history of the Earth. Detecting geoneutrinos remains the only direct probe to do so and constitutes a challenging objective in modern neutrino physics. In particular, the intriguing potassium geoneutrinos have never been observed and thus far have been considered impractical to measure. We propose here a novel approach for potassium geoneutrino detection using the unique antimatter signature of antineutrinos to reduce the otherwise overwhelming backgrounds to observing this rarest signal. The proposed detection framework relies on the innovative LiquidO detection technique to enable positron (e+) identification and antineutrino interactions with ideal isotope targets identified here for the first time. We also provide the complete experimental methodology to yield the first potassium geoneutrino discovery.

physics.geo-ph↗

arXiv2022

Search for $^{22}$Na in novae supported by a novel method for measuring femtosecond nuclear lifetimes

Classical novae are thermonuclear explosions in stellar binary systems, and important sources of $^{26}$Al and $^{22}$Na. While gamma rays from the decay of the former radioisotope have been observed throughout the Galaxy, $^{22}$Na remains untraceable. The half-life of $^{22}$Na (2.6 yr) would allow the observation of its 1.275 MeV gamma-ray line from a cosmic source. However, the prediction of such an observation requires good knowledge of the nuclear reactions involved in the production and destruction of this nucleus. The $^{22}$Na($p,γ$)$^{23}$Mg reaction remains the only source of large uncertainty about the amount of $^{22}$Na ejected. Its rate is dominated by a single resonance on the short-lived state at 7785.0(7) keV in $^{23}$Mg. In the present work, a combined analysis of particle-particle correlations and velocity-difference profiles is proposed to measure femtosecond nuclear lifetimes. The application of this novel method to the study of the $^{23}$Mg states, combining magnetic and highly-segmented tracking gamma-ray spectrometers, places strong limits on the amount of $^{22}$Na produced in novae, explains its non-observation to date in gamma rays (flux < 2.5x$10^{-4}$ ph/(cm$^2$s)), and constrains its detectability with future space-borne observatories.

nucl-ex↗

arXiv2022

Odd-odd neutron-rich rhodium isotopes studied with the double Penning trap JYFLTRAP

Precision mass measurements of neutron-rich rhodium isotopes have been performed at the JYFLTRAP Penning trap mass spectrometer at the Ion Guide Isotope Separator On-Line (IGISOL) facility. We report results on ground- and isomeric-state masses in $^{110,112,114,116,118}$Rh and the very first mass measurement of $^{120}$Rh. The isomeric states were separated and measured for the first time using the phase-imaging ion-cyclotron-resonance (PI-ICR) technique. For $^{112}$Rh, we also report new half-lives for both the ground state and the isomer. The results are compared to theoretical predictions using the BSkG1 mass model and discussed in terms of triaxial deformation.

nucl-ex↗

arXiv2022

Structure of $^{83}$As, $^{85}$As and $^{87}$As: from semi-magicity to $γ$-softness

The structure of $^{83}$As, $^{85}$As and $^{87}$As have been studied in fusion-fission reaction $^{238}$U+$^9$Be. Fission fragments were identified in mass and atomic number using the VAMOS++ spectrometer and the coincident $γ$-rays were detected in the $γ$-ray tracking array AGATA. New transitions in $^{83}$As and $^{85}$As are reported and placed in the level schemes. A level scheme of the excited states in $^{87}$As is proposed for the first time. The data are interpreted in frame of Large-Scale Shell-Model calculations, SU3 symmetries and Beyond Mean-Field frameworks. A spherical regime at magic number $N$=50 is predicted and the location of the proton $g_{9/2}$ orbital is proposed for the first time. Development of collectivity in a prolate deformed, $γ$-soft regime in the open shell cases $^{85}$As and $^{87}$As, most neutron-rich isotopes beyond $N$=50, is concluded. Data and theoretical calculations give confidence to a relatively high extrapolated excitation energy about 4 MeV of the $9/2^+$ state in $^{79}$Cu, one proton above $^{78}$Ni.

nucl-ex↗

arXiv2022

Direct determination of the atomic mass difference of the pairs $^{76}$As-$^{76}$Se and $^{155}$Tb-$^{155}$Gd rules out $^{76}$As and $^{155}$Tb as possible candidates for electron (anti)neutrino mass measurements

The first direct determination of the ground-state-to-ground-state $Q$ values of the $β^-$ decay $^{76}$As $\rightarrow$ $^{76}$Se and the electron-capture decay $^{155}$Tb $\rightarrow$ $^{155}$Gd was performed utilizing the double Penning trap mass spectrometer JYFLTRAP. By measuring the atomic mass difference of the decay pairs via the phase-imaging ion-cyclotron-resonance (PI-ICR) technique, the $Q$ values of $^{76}$As $\rightarrow$ $^{76}$Se and $^{155}$Tb $\rightarrow$ $^{155}$Gd were determined to be 2959.265(74) keV and 814.94(18) keV, respectively. The precision was increased relative to earlier measurements by factors of 12 and 57, respectively. The new $Q$ values are 1.33 keV and 5 keV lower compared to the values adopted in the most recent Atomic Mass Evaluation 2020. With the newly determined ground-state-to-ground-state $Q$ values combined with the excitation energy from $γ$-ray spectroscopy, the $Q$ values for ground-state-to-excited-state transitions $^{76}$As (ground state) $\rightarrow$ $^{76}$Se$^*$ (2968.4(7) keV) and $^{155}$Tb (ground state) $\rightarrow$ $^{155}$Gd$^*$ (815.731(3) keV) were derived to be -9.13(70) keV and -0.79(18) keV. Thus we have confirmed that both of the $β^{-}$-decay and EC-decay candidate transitions are energetically forbidden at a level of at least 4$σ$, thus definitely excluding these two cases from the list of potential candidates for the search of low-$Q$-value $β^-$ or EC decays to determine the electron-(anti)neutrino mass.

nucl-ex↗

arXiv2021

Charged-particle branching ratios above the neutron threshold in $^{19}$F: constraining $^{15}$N production in core-collapse supernovae

Spatially-correlated overabundances of $^{15}$N and $^{18}$O observed in some low-density graphite meteoritic grains have been connected to nucleosynthesis taking place in the helium-burning shell during core-collapse supernovae. Two of the reactions which have been identified as important to the final abundances of $^{15}$N and $^{18}$O are $^{18}$F($n,α$)$^{15}$N and $^{18}$F($n,p$)$^{18}$O. The relative strengths of the $^{18}$F($n,α$)$^{15}$N and $^{18}$F($n,p$)$^{18}$O reactions depend on the relative $α_0$ and $p_0$ decays from states above the neutron threshold in $^{19}$F in addition to other properties. Experimental data on the charged-particle decays from these highly excited states are lacking or inconsistent. Two experiments were performed using proton inelastic scattering from LiF targets and magnetic spectrographs. The first experiment used the high-resolution Q3D spectrograph at Munich to constrain properties of levels in $^{19}$F. A second experiment using the Orsay Split-Pole spectrograph and an array of silicon detectors was performed in order to measure the charged-particle decays of neutron-unbound levels in $^{19}$F. A number of levels in $^{19}$F have been identified along with their corresponding charged-particle decays. The first state above the neutron threshold which has an observed proton-decay branch to the ground state of $^{18}$O lies 68 keV above the neutron threshold while the $α$-particle decays from the neutron-unbound levels are generally observed to be much stronger than the proton decays. Neutron-unbound levels in $^{19}$F are observed to decay predominantly by $α$-particle emission, supporting the role of $^{18}$F($n,α$)$^{15}$N in the production of $^{15}$N in the helium-burning shell of supernovae. Improved resonant-scattering reaction data are required in order to be able to determine the reaction rates accurately.

nucl-ex↗

arXiv2018

Charged-particle decays of highly excited states in $^{19}$F

Neutron-capture reactions on $^{18}$F in the helium-burning shell play an important role in the production of $^{15}$N during core-collapse supernovae. The competition between the $^{18}$F($n,p/α$)$^{18}$O/$^{15}$N reactions controls the amount of $^{15}$N produced. The strengths of these reactions depend on the decay branching ratios of states in $^{19}$F above the neutron threshold. We report on an experiment investigating the decay branching ratios of these states in order to better constrain the strengths of the reactions.

nucl-ex↗