arXiv subjects

C. Faber

Publications and source records attributed to C. Faber.

10 recordsLinked to original sources

arXiv2015

Polaronic metal state at the LaAlO3/SrTiO3 interface

Interplay of spin, charge, orbital and lattice degrees of freedom in oxide heterostructures results in a plethora of fascinating properties, which can be exploited in new generations of electronic devices with enhanced functionalities. The paradigm example is the interface between the two band insulators LaAlO3 and SrTiO3 (LAO/STO) that hosts two-dimensional electron system (2DES). Apart from the mobile charge carriers, this system exhibits a range of intriguing properties such as field effect, superconductivity and ferromagnetism, whose fundamental origins are still debated. Here, we use soft-X-ray angle-resolved photoelectron spectroscopy to penetrate through the LAO overlayer and access charge carriers at the buried interface. The experimental spectral function directly identifies the interface charge carriers as large polarons, emerging from coupling of charge and lattice degrees of freedom, and involving two phonons of different energy and thermal activity. This phenomenon fundamentally limits the carrier mobility and explains its puzzling drop at high temperatures.

cond-mat.mtrl-sci↗

arXiv2015

Exploring approximations to the GW self-energy ionic gradients

The accuracy of the many-body perturbation theory GW formalism to calculate electron-phonon coupling matrix elements has been recently demonstrated in the case of a few important systems. However, the related computational costs are high and thus represent strong limitations to its widespread application. In the present study, we explore two less demanding alternatives for the calculation of electron-phonon coupling matrix elements on the many-body perturbation theory level. Namely, we test the accuracy of the static Coulomb-hole plus screened-exchange (COHSEX) approximation and further of the constant screening approach, where variations of the screened Coulomb potential W upon small changes of the atomic positions along the vibrational eigenmodes are neglected. We find this latter approximation to be the most reliable, whereas the static COHSEX ansatz leads to substantial errors. Our conclusions are validated in a few paradigmatic cases: diamond, graphene and the C60 fullerene. These findings open the way for combining the present many-body perturbation approach with efficient linear-response theories.

physics.comp-ph↗

arXiv2012

Many-body Green's function study of coumarins for dye-sensitized solar cells

We study within the many-body Green's function $GW$ and Bethe-Salpeter formalisms the excitation energies of several coumarin dyes proposed as an efficient alternative to ruthenium complexes for dye-sensitized solar cells. Due to their internal donor-acceptor structure, these chromophores present low-lying excitations showing a strong intramolecular charge-transfer character. We show that combining $GW$ and Bethe-Salpeter calculations leads to charge-transfer excitation energies and oscillator strengths in excellent agreement with reference range-separated functional studies or coupled-cluster calculations. The present results confirm the ability of this family of approaches to describe accurately Frenkel and charge-transfer photo-excitations in both extended and finite size systems without any system-dependent adjustable parameter, paving the way to the study of dye-sensitized semiconducting surfaces.

cond-mat.mtrl-sci↗

arXiv2012

Molecular fingerprints in the electronic properties of crystalline organic semiconductors: from experiment to theory

By comparing photoemission spectroscopy with a non-perturbative dynamical mean field theory extension to many-body ab initio calculations, we show in the prominent case of pentacene crystals that an excellent agreement with experiment for the bandwidth, dispersion and lifetime of the hole carrier bands can be achieved in organic semiconductors provided that one properly accounts for the coupling to molecular vibrational modes and the presence of disorder. Our findings rationalize the growing experimental evidence that even the best band structure theories based on a many-body treatment of electronic interactions cannot reproduce the experimental photoemission data in this important class of materials.

cond-mat.mtrl-sci↗

arXiv2011

Tautological and non-tautological cohomology of the moduli space of curves

After a short exposition of the basic properties of the tautological ring of the moduli space of genus g Deligne-Mumford stable curves with n markings, we explain three methods of detecting non-tautological classes in cohomology. The first is via curve counting over finite fields. The second is by obtaining length bounds on the action of the symmetric group S_n on tautological classes. The third is via classical boundary geometry. Several new non-tautological classes are found.

math.AG↗

arXiv2006

On the cusp form motives in genus 1 and level 1

We prove that the moduli space of stable n-pointed curves of genus one and the projector associated to the alternating representation of the symmetric group on n letters define (for n>1) the Chow motive corresponding to cusp forms of weight n+1 for SL(2,Z). This provides an alternative (in level one) to the construction of Scholl.

math.AG↗

arXiv2004

Hodge integrals, partition matrices, and the lambda_g conjecture

We prove a closed formula for integrals of the cotangent line classes against the top Chern class of the Hodge bundle on the moduli space of stable pointed curves. These integrals are computed via relations obtained from virtual localization in Gromov-Witten theory. An analysis of several natural matrices indexed by partitions is required.

math.AG↗

arXiv2003

Relative maps and tautological classes

The moduli space of stable relative maps to the projective line combines features of stable maps and admissible covers. We prove all standard Gromov-Witten classes on these moduli spaces of stable relative maps have tautological push-forwards to the moduli space of curves. In particular, the fundamental classes of all moduli spaces of admissible covers push-forward to tautological classes. Consequences for the tautological rings of the moduli spaces of curves include methods for generating new relations, uniform derivations of the socle and vanishing statements of the Gorenstein conjectures for the complete, compact type, and rational tail cases, tautological boundary terms for Ionel's, Looijenga's, and Getzler's vanishings, and applications to Gromov-Witten theory.

math.AG↗

arXiv2000

Logarithmic series and Hodge integrals in the tautological ring (with an appendix by D. Zagier)

We describe a new perspective on the intersection theory of the moduli space of curves involving both Virasoro constraints and Gorenstein conditions. The main result of the paper is the computation of a basic 1-point Hodge integral series occurring in the tautological ring of the moduli space of nonsingular curves. In the appendix by D. Zagier, "Polynomials arising from the tautological ring", a detailed study is made of certain polynomials whose coefficients are intersection numbers on moduli space. The paper and the appendix together provide proofs of all previously conjectured formulas for 1-point integrals in the tautological ring, and of natural extensions of these formulas as well.

math.AG↗

arXiv1998

Hodge integrals and Gromov-Witten theory

Integrals of the Chern classes of the Hodge bundle in Gromov-Witten theory are studied. We find a universal system of differential equations which determines the generating function of these integrals from the standard descendent potential (for any target X). We use virtual localization and classical degeneracy calculations to find trigonometric closed form solutions for special Hodge integrals over the moduli space of pointed curves. These formulas are applied to two computations in Gromov-Witten theory for Calabi-Yau 3-folds. The genus g, degree d multiple cover contribution of a rational curve is found to be simply proportional to the Euler characteristic of M_g. The genus g, degree 0 Gromov-Witten invariant is calculated (in agreement with recent string theoretic calculations of Gopakumar-Vafa and Marino-Moore). Finally, with Zagier's help, our Hodge integral formulas imply a general genus prediction of the punctual Virasoro constraints applied to the projective line.

math.AG↗