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C. Figueira de Morisson Faria

Publications and source records attributed to C. Figueira de Morisson Faria.

At least 19 recordsLinked to original sources

Ultrafast quantum gate operations in a Kramers-Henneberger atom Qubit

We propose and demonstrate the Kramers-Henneberger KH) atom as a novel qubit platform for ultrafast single-qubit gate operations. In the KH frame, the time-averaged strong laser field engineers a double-well potential whose two lowest eigenstates define the qubit basis, so that the computational structure is created and maintained by the driving field itself. A weak resonant control field drives coherent gate operations: full time-dependent Schrödinger equation simulations with the complete time-dependent KH potential confirm a Z gate and S gate of the order of femtoseconds, six orders of magnitude faster than laser-driven superconducting qubit gates. Decoherence characterisation gives longer decoherence times than those required for the gate operations. The complete six-gate single-qubit set is demonstrated in the time-averaged two-level limit, with strong agreement between the full and time-averaged descriptions confirming that fidelity is limited by structured leakage rather than stochastic decoherence. In principle, this is an error channel suppressible through pulse engineering. These results constitute the first demonstration of coherent single-qubit gates in a strong-field setting, with a clear pathway toward attosecond-scale operations.

quant-ph↗

Erasing photons from bright squeezed vacuum light via above-threshold ionization

While the interface between strong-field physics and quantum optics offers a unique regime for combining extreme nonlinearity with quantum optical resources, its potential for generating non-classical states of light remains largely unexplored. Standard protocols for generating optical Schrödinger cat states, such as photon subtraction from squeezed light, are inherently limited in the achievable macroscopicity of the state and its scalability. In this work, we bridge this gap by demonstrating that above-threshold ionization driven by bright squeezed light provides a strong-field analogue of photon subtraction, where photoelectron detection acts as a high-intensity heralding mechanism, enabling the generation of large amplitude optical Schrödinger cat states. We characterize the resulting non-Gaussian features and show that they can be tuned via the detected photoelectron momentum, and study their robustness against the experimental imperfections arising from finite momentum resolution at the heralding step. Despite the noise, we show that the generated states can be manipulated to violate a Bell inequality, thereby highlighting their potential for foundational and practical applications. Our results establish strong-field processes as a scalable platform for macroscopic quantum state engineering, opening a route to quantum optics in previously inaccessible regimes.

quant-ph↗

Interferometrically Enhanced Asymmetry in Strong-field Ionization with Bright Squeezed Vacuum

We demonstrate that quantum light statistics can be used to control strong-field ionization at the tunneling step. Using a bichromatic linearly polarized field composed of a strong coherent driver and a weak bright squeezed vacuum (BSV), we show through simulation that photoelectron momentum distributions (PMDs) exhibit asymmetries that exceed those obtained with classical fields of comparable intensity by orders of magnitude. This enhancement is uniquely linked to the nonclassical statistics of the BSV field. A semiclassical analysis based on the strong-field approximation (SFA) reveals that the effect originates from fluctuations in the instantaneous field amplitude, which strongly modify the tunneling ionization probability while leaving the electron's continuum dynamics essentially unchanged. This selective control enables reconstruction of ionization pathways and provides a robust route to extract sub-cycle dynamics from strong-field observables.

quant-ph↗

Unravelling inter-channel quantum interference in below-threshold nonsequential double ionization with statistical measures

We present a systematic study of interchannel quantum interference in laser-induced nonsequential double ionization (NSDI) within the strong-field approximation. Focusing on the below-threshold intensity regime where the recollision-excitation with subsequent ionization (RESI) pathway dominates, we derive analytical phase conditions governing interference between distinct excitation channels for arbitrary driving fields. To quantify the interplay between channels resulting from a vast number of interfering processes, we introduce statistical metrics based on the Earth Mover's Distance, allowing us to assess the relative weight of each channel's contribution to the two-electron photoelectron momentum distributions (PMDs). We identify key factors that determine whether interchannel interference is appreciable such as comparable channel intensities, strong spatial overlap between the excited-state wavefunctions and the energy difference between contributing channels. We demonstrate that for linearly polarized few-cycle pulses, the typical intrachannel interference features associated with exchange, temporal shifts and combined exchange-temporal interference are retained with interchannel interference. Our findings establish a hierarchy of interference mechanisms in RESI and may provide practical guidelines for enhancing or suppressing interference in different regions of the momentum plane. The toolkit presented in this work is transferable to a wide range of interferometric schemes involving different excitation channels.

physics.atom-ph↗

Microscopic analysis of above-threshold ionization driven by squeezed light

Above-threshold ionization (ATI) is a strong-field-driven process where electrons absorb more photons than required for ionization. While ATI dynamics and outputs are well-understood when driven by classical, perfectly coherent light, the recent development of non-classical light sources for strong-field phenomena has spurred interest in their effect on the involved electron dynamics. In this work, we present a microscopic quantum optical theory describing ATI under the influence of strong squeezed light. We observe that squeezed light significantly enhances the coupling between light and matter, making their mutual backaction more important than under classical driving. This backaction profoundly impacts the electronic ionization times, as well as the non-classical properties of the joint electron-light state. This results in pronounced entanglement features, both immediately after ionization, and at later times. These entanglement features are reflected in the properties of the quantum optical state of the driving field revealing notable non-Gaussian features that depend on both, the amount of squeezing, and the number of ionization events occurring during the interaction.

quant-ph↗

Below threshold nonsequential double ionization with linearly polarized two-color fields I: symmetry and dominance

We investigate laser-induced nonsequential double ionization with linearly polarized bichromatic fields, focusing on the recollision-excitation with subsequent ionization (RESI) mechanism. Using the strong-field approximation, we assess how the symmetries of the field influence the dominant events. Furthermore, we show that, by manipulating the field parameters such as the field frequencies and relative phase between the two driving waves, one can influence the correlated electron-momentum distributions. Specific features of a linearly polarized bichromatic field are that the momentum distributions of the second electron are no longer centered around vanishing momenta and that there may be more than one ionization event per half cycle. This can be used to confine the RESI distributions to specific momentum regions and to determine a hierarchy of parameters that make an event dominant.

physics.atom-ph↗

Below threshold nonsequential double ionization with linearly polarized two-color fields II: Quantum interference

We perform a systematic analysis of intra-channel quantum interference in laser-induced nonsequential double ionization with linearly polarized bichromatic fields, focusing on the recollision-excitation with subsequent ionization (RESI) mechanism, and employing the strong-field approximation. We generalize and elaborate several analytic interference conditions for RESI in arbitrary driving fields, with a focus on the interference arising from the specific symmetries of bichromatic fields. For example, for waves of comparable strengths, multiple events per half cycle for the direct electron must be considered. Furthermore, interference breaks some of the symmetries arising from the field. We detangle the superimposed interference fringes originating from phase differences related to symmetrization due to electron exchange, temporal shifts and a combination of exchange and event interference. We show that the hierarchy between exchange-only and exchange-temporal interference is fluid and can be manipulated by an appropriate choice of driving-field parameters. This is enabled by different types of interference occupying specific regions of the plane spanned by the electron momentum components parallel to the driving-field polarization.

physics.atom-ph↗

Quantum beating and cyclic structures in the phase-space dynamics of the Kramers-Henneberger atom

We investigate the phase-space dynamics of the Kramers Henneberger (KH) atom solving the time-dependent Schrödinger equation for reduced-dimensionality models and using Wigner quasiprobability distributions. We find that, for the time-averaged KH potential, coherent superpositions of eigenstates perform a cyclic motion confined in momentum space, whose frequency is proportional to the energy difference between the two KH eigenstates. This cyclic motion is also present if the full time dependent dynamics are taken into consideration. However, there are time delays regarding the time-averaged potential, and some tail-shaped spilling of the quasiprobability flow towards higher momentum regions. These tails are signatures of ionization, indicating that, for the potential studied in this work, a small momentum spread is associated with stabilization. A comparison of the quasiprobability flow with classical phase-space constraints shows that, for the KH atom, the momentum must be bounded from above. This is a major difference from a molecule, for which the quasiprobability flow is confined in position space for small internuclear separation. Furthermore, we assess the stability of different propagation strategies and find that the most stable scenario for the full dynamics is obtained if the system is initially prepared in the KH ground state.

quant-ph↗

Energy-conservation conditions in saddle-point approximation for the strong-field-ionization of atoms

Orbit-based methods are widespread in strong-field laser-matter interaction. They provide a framework in which photoelectron momentum distributions can be interpreted as the quantum interference between different semi-classical pathways the electron can take on its way to the detector, which brings with it great predictive power. The transition amplitude of an electron going from a bound state to a final continuum state is often written as multiple integrals, which can be computed either numerically, or by employing the saddle-point method. If one computes the momentum distribution via a saddle-point method, the obtained distribution is highly dependent on the time window from which the saddle points are selected for inclusion in the "sum over paths". In many cases, this leads to the distributions not even satisfying the basic symmetry requirements and often containing many more oscillations and interference fringes than their numerically integrated counterparts. Using the strong-field approximation, we find that the manual enforcement of the energy-conservation condition on the momentum distribution calculated via the saddle-point method provides a unique momentum distribution which satisfies the symmetry requirements of the system and which is in a good agreement with the numerical results. We illustrate our findings using the example of the Ar atom ionized by a selection of monochromatic and bichromatic linearly polarized fields.

physics.atom-ph↗

Influence of catastrophes and hidden dynamical symmetries on ultrafast backscattered photoelectrons

We discuss the effect of using potentials with a Coulomb tail and different degrees of softening in the photoelectron momentum distributions (PMDs) using the recently implemented hybrid forward-boundary CQSFA (H-CQSFA). We show that introducing a softening in the Coulomb interaction influences the ridges observed in the PMDs associated with backscattered electron trajectories. In the limit of a hard-core Coulomb interaction, the re-scattering ridges close along the polarization axis, while for a soft-core potential, they are interrupted at ridge-specific angles. We analyze the momentum mapping of the different orbits leading to the ridges. For the hard-core potential, there exist two types of saddle-point solutions that coalesce at the ridge. By increasing the softening, we show that two additional solutions emerge as the result of breaking a hidden dynamical symmetry associated exclusively with the Coulomb potential. Further signatures of this symmetry breaking are encountered in subsets of momentum-space trajectories. Finally, we use scattering theory to show how the softening affects the maximal scattering angle and provide estimates that agree with our observations from the CQSFA. This implies that, in the presence of residual binding potentials in the electron's continuum propagation, the distinction between purely kinematic and dynamic caustics becomes blurred.

physics.atom-ph↗

Detangling the quantum tapestry of intra-channel interference in below-threshold nonsequential double ionization with few-cycle laser pulses

We perform a systematic analysis of single-channel quantum interference in laser-induced nonsequential double ionization with few-cycle pulses, using the strong-field approximation. We focus on a below-threshold intensity for which the recollision-excitation with subsequent ionization (RESI) mechanism is prevalent. We derive and classify several analytic interference conditions for single-channel RESI in arbitrary driving fields, and address specific issues for few-cycle pulses. Since the cycles in a short pulse are no longer equivalent, there are several events whose dominance varies. We quantify this dominance for single excitation channels by proposing a dominance parameter. Moreover, there will be many more types of superimposed interference fringes that must be taken into consideration. We find an intricate tapestry of patterns arising from phase differences related to symmetrization, temporal shifts and a combination of exchange and event interference.

physics.atom-ph↗

Impact of the continuum Coulomb interaction in quantum-orbit-based treatments of high-order above-threshold ionization

We perform a systematic comparison between photoelectron momentum distributions computed with the rescattered-quantum orbit strong-field approximation (RQSFA) and the Coulomb-quantum orbit strong-field approximation (CQSFA). We exclude direct, hybrid, and multiple scattered CQSFA trajectories, and focus on the contributions of trajectories that undergo a single act of rescattering. For this orbit subset, one may establish a one-to-one correspondence between the RQSFA and CQSFA contributions for backscattered and forward-scattered trajectory pairs. We assess the influence of the Coulomb potential on the ionization and rescattering times of specific trajectory pairs, kinematic constraints determined by rescattering, and quantum interference between specific pairs of trajectories. We analyze how the Coulomb potential alters their ionization and return times, and their interference in photoelectron momentum distributions. We show that Coulomb effects are not significant for high or medium photoelectron energies and shorter orbits, while, for lower momentum ranges or longer electron excursion times in the continuum, the residual Coulomb potential is more important. We also assess the agreement of both theories for different field parameters, and show that it improves with the increase of the wavelength.

physics.atom-ph↗

Forward and hybrid path-integral methods in photoelectron holography: sub-barrier corrections, initial sampling and momentum mapping

We construct two strong-field path integral methods with full Coulomb distortion, in which the quantum pathways are mimicked by interfering electron orbits: the rate-based CQSFA (R-CQSFA) and the hybrid forward-boundary CQSFA (H-CQSFA). The methods have the same starting point as the standard Coulomb quantum-orbit strong-field approximation (CQSFA), but their implementation does not require pre-knowledge of the orbits' dynamics. These methods are applied to ultrafast photoelectron holography. In the rate-based method, electron orbits are forward propagated and we derive a non-adiabatic ionization rate from the CQSFA, which includes sub-barrier Coulomb corrections and is used to weight the initial orbit ensemble. In the H-CQSFA, the initial ensemble provides initial guesses for a subsequent boundary problem and serves to include or exclude specific momentum regions, but the ionization probabilities associated with individual trajectories are computed from sub-barrier complex integrals. We perform comparisons with the standard CQSFA and \textit{ab-initio} methods, which show that the standard, purely boundary-type implementation of the CQSFA leaves out whole sets of trajectories. We show that the sub-barrier Coulomb corrections broaden the resulting photoelectron momentum distributions (PMDs) and improve the agreement of the R-CQSFA with the H-CQSFA and other approaches. We probe different initial sampling distributions, uniform and otherwise, and their influence on the PMDs. We find that initial biased sampling emphasizes rescattering ridges and interference patterns in high-energy ranges, while an initial uniform sampling guarantees accurate modeling of the holographic patterns near the ionization threshold or polarization axis. Our results are explained using the initial to final momentum mapping for different types of interfering trajectories.

physics.atom-ph↗

Twisted quantum interference in photoelectron holography with elliptically polarized fields

We perform a systematic analysis of how ultrafast photoelectron holography is influenced by an elliptically polarized field, with emphasis on quantum interference effects. We find that the interplay of the external field and the binding potential leads to twisted holographic patterns for low ellipticities and recover well-known angular offsets for high ellipticities. Using the Coulomb quantum-orbit strong-field approximation (CQSFA), we assess how the field ellipticity affects specific holographic patterns, such as the fan and the spider. The interplay of the external field and the binding potential leads to twisted holographic patterns in the fan, and to loss of contrast in the spider. This behavior can be traced back to interfering electron trajectories, and unequal changes in tunneling probability due to non-vanishing ellipticity. We also derive tunneling times analytically using the strong-field approximation (SFA), provide estimates for ellipticy ranges for which interference is expected to be prominent, and discuss how to construct continuous electron momentum distributions exploring the rotation symmetry around the origin.

quant-ph↗

Exploring symmetries in photoelectron holography with two-color linearly polarized fields

We investigate photoelectron holography in bichromatic linearly polarized fields of commensurate frequencies $rω$ and $sω$, with emphasis on the existing symmetries and for which values of the relative phase between the two driving waves they are kept or broken. Using group-theoretical methods, we show that, additionally to the well-known half-cycle symmetry, which is broken for $r+s$ odd, there are reflection symmetries around the field zero crossings and maxima, which may or may not be kept, depending on how both waves are dephased. The three symmetries are always present for monochromatic fields, while for bichromatic fields this is not guaranteed, even if $r+s$ is even and the half-cycle symmetry is retained. Breaking the half-cycle symmetry automatically breaks one of the other two, while, if the half-cycle symmetry is retained, the other two symmetries are either \textit{both} kept or broken. We analyze how these features affect the ionization times and saddle-point equations for different bichromatic fields. We also provide general expressions for the relative phases $ϕ$ which retain specific symmetries. As an application, we compute photoelectron momentum distributions for $ω-2ω$ fields with the Coulomb Quantum Orbit Strong-Field approximation and assess how holographic structures such as the fan, the spider and interference carpets behave, focusing on the reflection symmetries. The features encountered can be traced back to the field gradient and amplitude affecting ionization probabilities and quantum interference in different momentum regions.

physics.atom-ph↗

Attoscience in Phase Space

We provide a brief review of how phase space techniques are explored within strong-field and attosecond science. This includes a broad overview of the existing landscape, with focus on strong-field ionisation and rescattering, high-order harmonic generation, stabilisation and free-electron lasers. Furthermore, using our work on the subject, which deals with ionisation dynamics in atoms and diatomic molecules as well as high-order harmonic generation in inhomogeneous fields, we exemplify how such tools can be employed. One may for instance determine qualitatively different phase space dynamics, explore how bifurcations influence ionisation and high-harmonic generation, establish for which regimes classical and quantum correspondence works or fails, and what role different time scales play. Finally, we conclude the review highlighting the importance of the tools available in quantum optics, quantum information and physical chemistry to strong-field laser-matter interaction.

physics.atom-ph↗

Quantum Estimation in Strong Fields: in situ ponderomotive sensing

We develop a new framework to optimize and understand uncertainty from in situ strong field measurements of laser field parameters. We present the first derivation of quantum and classical Fisher information for an electron undergoing strong-field ionization. This is used for parameter estimation and to characterize the uncertainty of the ponderomotive energy, directly proportional to laser intensity. In particular, the quantum and classical Fisher information for the momentum basis displays quadratic scaling over time. This can be linked to above-threshold ionization interference rings for measurements in the momentum basis and to the `ponderomotive phase' for the `ideal' quantum measurements. Preferential scaling is found for increasing laser pulse length and intensity. We use this to demonstrate for in situ measurements of laser intensity, that high resolution momentum spectroscopy has the capacity to reduce the uncertainty by over $25$ times compared to measurements employing the ionization rate, while using the `ideal' quantum measurement would reduce it by a further factor of $2.6$. A minimum uncertainty of the order $2.8 \times 10^{-3}~\%$ is theorized for this framework. Finally, we examine previous in situ measurements formulating a measurement that matches the experimental procedure and suggest how to improve this.

quant-ph↗

Manipulating Twisted Electrons in Strong-Field Ionization

We investigate the discrete orbital angular momentum (OAM) of photoelectrons freed in strongfield ionization. We use these `twisted' electrons to provide an alternative interpretation on existing experimental work of vortex interferences caused by strong field ionization mediated by two counterrotating circularly polarized pulses separated by a delay. Using the strong field approximation, we derive an interference condition for the vortices. In computations for a neon target we find very good agreement of the vortex condition with photoelectron momentum distributions computed with the strong field approximation, as well as with the time-dependent methods Qprop and R-Matrix. For each of these approaches we examine the OAM of the photoelectrons, finding a small number of vortex states localized in separate energy regions. We demonstrate that the vortices arise from the interference of pairs of twisted electron states. The OAM of each twisted electron state can be directly related to the number of arms of the spiral in that region. We gain further understanding by recreating the vortices with pairs of twisted electrons and use this to determine a semiclassical relation for the OAM. A discussion is included on measuring the OAM in strong field ionization directly or by employing specific laser pulse schemes as well as utilizing the OAM in time-resolved imaging of photo-induced dynamics.

physics.atom-ph↗