arXiv subjects

C. Fougères

Publications and source records attributed to C. Fougères.

11 recordsLinked to original sources

arXiv2026

Direct transfer to $^{46,48}$K as a survey of the $π(s_{1/2})$$-ν(sdpf)$ interaction

The collapse of the canonical $N=28$ magic number in nuclei with $Z<20$ has drawn significant interest as it relates to the emergence of an island of inversion centered on $^{42}$Si and $^{44}$S. In particular, interactions between the $πs_{1/2}$ orbital -- empty in $^{42}$Si and full in $^{44}$S -- and the neutron orbitals just above and below the $N=28$ gap are expected to be critical in this region, but remain relatively unexplored. In this paper, we expand upon the results of our previous study of the direct transfer reaction $^{47}$K(d,p$γ$)$^{48}$K [C.\,J.~Paxman \textit{et al.}, Phys. Rev. Lett. 134, 162504 (2025)] with the results of the complementary $^{47}$K(d,t$γ$)$^{46}$K reaction. Through this study, we present a comprehensive scan of the interaction between the critical $πs_{1/2}$ orbital and a broad range of neutron orbitals spanning nearly two full shells. We identify several discrepancies between the experimental results and state-of-the-art shell model calculations, which suggest a deficiency of the shell model to fully capture the complex proton configuration mixing in this region, highlighting a significant challenge for single-particle descriptions of the island of inversion.

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arXiv2025

First experimental determination of the $^{40}$Ar($n,2n$)$^{39}$Ar reaction cross section and $^{39}$Ar production in Earth's atmosphere

The cosmogenic $^{39}$Ar(t$_{1/2}$= 268 years) isotope of argon is used for geophysical dating and tracing owing to its appropriate half-life and chemical inertness as a noble gas; $^{39}$Ar serves also in nuclear weapon test monitoring. We measured for the first time the total cross section of the main $^{39}$Ar cosmogenic production reaction in the atmosphere, namely $^{40}$Ar$(n,2n)^{39}$Ar, using 14.8$\pm0.3$ MeV neutrons. The neutrons, produced by a deuterium-tritium generator, impinged on a stainless steel sphere filled with Ar gas highly enriched in the $^{40}$Ar isotope. The reaction yield was measured by atom counting of $^{39}$Ar with noble gas accelerator mass spectrometry and, independently, by decay counting relative to atmospheric argon. A total $^{40}$Ar$(n,2n)^{39}$Ar cross section of 610$\pm100$ mb was determined. This result serves as a benchmark for recent theoretical calculations and evaluations, found to reproduce well the experimental total cross section. We use these energy-dependent theoretical cross sections together with experimental spectra of cosmogenic neutrons at different altitudes to calculate the global average rate of neutron-induced $^{39}$Ar atmospheric production, resulting in $770\pm240$ $^{39}$Ar atoms/cm$^2$/day. The secular equilibrium between the $^{39}$Ar calculated production rate and radioactive decay rate leads to a partial isotopic abundance $^{39}$Ar/Ar$= (5.9\pm 1.8) \times 10^{-16}$, showing that $\approx$73% of atmospheric $^{39}$Ar is produced by cosmogenic neutrons. The $^{40}$Ar($n,2n$)$^{39}$Ar cross section at 14 MeV is also a key parameter for quantifying the anthropogenic contribution to atmospheric $^{39}$Ar produced during the thermonuclear tests of the 1960s. We estimate that anthropogenic $^{39}$Ar accounts for roughly 20% of the present atmospheric inventory.

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arXiv2025

First measurement of 87Rb(α, xn) cross sections at weak r-process energies in supernova ν-driven ejecta to investigate elemental abundances in low-metallicity stars

Observed abundances of Z ~ 40 elements in metal-poor stars vary from star to star, indicating that the rapid and slow neutron capture processes may not contribute alone to the synthesis of elements beyond iron. The weak r-process was proposed to produce Z ~ 40 elements in a subset of old stars. Thought to occur in the ν-driven ejecta of a core-collapse supernova, (α, xn) reactions would drive the nuclear flow toward heavier masses at T = 2-5 GK. However, current comparisons between modelled and observed yields do not bring satisfactory insights into the stellar environment, mainly due to the uncertainties of the nuclear physics inputs where the dispersion in a given reaction rate often exceeds one order of magnitude. Involved rates are calculated with the statistical model where the choice of an α-optical-model potential (αOMP) leads to such a poor precision. The first experiment on 87Rb(α, xn) reactions at weak r-process energies is reported here. Total inclusive cross sections were assessed at Ec.m. = 8.1 - 13 MeV (3.7 - 7.6 GK) with the active target MUlti-Sampling Ionization Chamber (MUSIC). With a N = 50 seed nucleus, the measured values agree with statistical model estimates using the αOMP Atomki-V2. A re-evaluated reaction rate was incorporated into new nucleosynthesis calculations, focusing on ν-driven ejecta conditions known to be sensitive to this specific rate. These conditions were found to fail to reproduce the lighter-heavy element abundances in metal-poor stars.

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arXiv2025

Probing exotic cross-shell interactions at N=28 with single-neutron transfer on 47K

We present the first measurement of the $^{47}$K($d,pγ$)$^{48}$K transfer reaction, performed in inverse kinematics using a reaccelerated beam of $^{47}$K. The level scheme of $^{48}$K has been greatly extended with nine new bound excited states identified and spectroscopic factors deduced. Detailed comparisons with SDPF-U and SDPF-MU shell-model calculations reveal a number of discrepancies with these results, and a preference for SDPF-MU is found. Intriguingly, an apparent systematic overestimation of spectroscopic factors and a poor reproduction of the energies for 1$^-$ states suggests that the mixing between the $πs^{\,\,\,1}_{1/2} d^{\,\,\,4}_{3/2}$ and $πs^{\,\,\,2}_{1/2} d^{\,\,\,3}_{3/2}$ proton configurations in $^{48}$K is not correctly described using current interactions, challenging our descriptions of light $N=28$ nuclei.

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arXiv2024

Meaurement of spin vs. TKE of $^{144}$Ba produced in spontaneous fission of $^{252}$Cf

We measure the average spin of $^{144}$Ba, a common fragment produced in $^{252}$Cf(sf), as a function of the total kinetic energy (TKE). We combined for the first time a twin Frisch-gridded ionization chamber with a world-class $γ$-ray spectrometer that was designed to measure high-multiplicity $γ$-ray events, Gammasphere. The chamber, loaded with a $^{252}$Cf(sf) source, provides a fission trigger, the TKE of the fragments, the approximate fragment masses, and the polar angle of the fission axis. Gammasphere provides the total $γ$-ray yield, fragment identification through the tagging of decay $γ$ rays, and the feeding of rotational bands in the fragments. We determine the dependence of the average spin of $^{144}$Ba on the fragments' TKE by correlating the fragment properties with the distribution of discrete levels that are fed. We find that the average spin only changes by about $0.5$ $\hbar$ across the TKE range of 158-203 MeV. The virtual independence of the spin on TKE suggests that spin is not solely generated through the statistical excitation of rotational modes, and more complex mechanisms are required.

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arXiv2024

High-precision spectroscopy of $^{20}$O benchmarking ab-initio calculations in light nuclei

The excited states of unstable $^{20}$O were investigated via $γ$-ray spectroscopy following the $^{19}$O$(d,p)^{20}$O reaction at 8 $A$MeV. By exploiting the Doppler Shift Attenuation Method, the lifetime of the 2$^+_2$ and 3$^+_1$ states were firmly established. From the $γ$-ray branching and E2/M1 mixing ratios for transitions deexciting the 2$^+_2$ and 3$^+_1$ states, the B(E2) and B(M1) were determined. Various chiral effective field theory Hamiltonians, describing the nuclear properties beyond ground states, along with a standard USDB interaction, were compared with the experimentally obtained data. Such a comparison for a large set of $γ$-ray transition probabilities with the valence space in medium similarity renormalization group ab-initio calculations was performed for the first time in a nucleus far from stability. It was shown that the ab-initio approaches using chiral EFT forces are challenged by detailed high-precision spectroscopic properties of nuclei. The reduced transition probabilities were found to be a very constraining test of the performance of the ab-initio models.

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arXiv2024

Direct cross-section measurement of the weak r-process 88Sr(α,n)91Zr reaction in ν-driven winds of core collapse supernovae

About half of the heavy elements beyond iron are known to be produced by the rapid neutron capture process, known as r-process. However, the astrophysical site producing the r-process is still uncertain. Chemical abundances observed in several cosmic sites indicate that different mechanisms should be at play. For instance, the abundances around silver measured in a subset of metal-poor stars indicate the presence of a weak r-process. This process may be active in neutrino-driven winds of core collapse supernovae where ($α$,n) reactions dominate the synthesis of Z ~ 40 elements in the expelled materials. Scarcely measured, the rates of ($α$,n) reactions are determined from statistical Hauser-Feshbach calculations with $α$-optical-model potentials, which are still poorly constrained. The uncertainties of the ($α$,n) reaction rates therefore make a significant contribution to the uncertainties of the abundances determined from stellar modeling. In this work, the $^{88}$Sr($α$,n)$^{91}$Zr reaction which impacts the weak r-process abundances has been probed at astrophysics energy for the first time; directly measuring the total cross sections at astrophysical energies of 8.37 - 13.09 MeV in the center of mass (3.8 - 7.5 GK). Two measurements were performed at ATLAS with the electrically-segmented ionization chamber MUSIC, in inverse kinematics, while following the active target technique. The cross sections of this $α$-induced reaction on $^{88}$Sr, located at the shell closure N = 50, have been found to be lower than expected, by a factor of 3, despite recent statistical calculations validated by measurements on neighboring nuclei. This result encourages more experimental investigations of ($α$,n) reactions, at N = 50 and towards the neutron-rich side, to further test the predictive power and reliability of such calculations.

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arXiv2022

Search for $^{22}$Na in novae supported by a novel method for measuring femtosecond nuclear lifetimes

Classical novae are thermonuclear explosions in stellar binary systems, and important sources of $^{26}$Al and $^{22}$Na. While gamma rays from the decay of the former radioisotope have been observed throughout the Galaxy, $^{22}$Na remains untraceable. The half-life of $^{22}$Na (2.6 yr) would allow the observation of its 1.275 MeV gamma-ray line from a cosmic source. However, the prediction of such an observation requires good knowledge of the nuclear reactions involved in the production and destruction of this nucleus. The $^{22}$Na($p,γ$)$^{23}$Mg reaction remains the only source of large uncertainty about the amount of $^{22}$Na ejected. Its rate is dominated by a single resonance on the short-lived state at 7785.0(7) keV in $^{23}$Mg. In the present work, a combined analysis of particle-particle correlations and velocity-difference profiles is proposed to measure femtosecond nuclear lifetimes. The application of this novel method to the study of the $^{23}$Mg states, combining magnetic and highly-segmented tracking gamma-ray spectrometers, places strong limits on the amount of $^{22}$Na produced in novae, explains its non-observation to date in gamma rays (flux < 2.5x$10^{-4}$ ph/(cm$^2$s)), and constrains its detectability with future space-borne observatories.

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arXiv2022

Understanding the cosmic abundance of $^{22}$Na: lifetime measurements in $^{23}$Mg

Simulations of explosive nucleosynthesis in novae predict the production of $^{22}$Na, a key astronomical observable to constrain nova models. Its gamma-ray line at 1.275 MeV has not yet been observed by the gamma-ray space telescopes. The $^{20}$Ne/$^{22}$Ne ratio in presolar grains, a possible tool to identify nova grains, also depends on $^{22}$Na produced. Uncertainties on its yield in classical novae currently originate from the rate of the $^{22}$Na(p, $γ$)$^{23}$Mg reaction. At peak novae temperatures, this reaction is dominated by a resonance at E$_{\text{R}}$=0.204 MeV, corresponding to the $E_x$=7.785 MeV excited state in $^{23}$Mg. The resonance strengths measured so far disagree by one order of magnitude. An experiment has been performed at GANIL to measure the lifetime and the proton branching ratio of this key state, with a femtosecond resolution for the former. The reactions populating states in $^{23}$Mg have been studied with a high resolution detection set-up, i.e. the particle VAMOS, SPIDER and gamma tracking AGATA spectrometers, allowing the measurements of lifetimes and proton branchings. We present here a comparison between experimental results and shell-model calculations, that allowed us to assign the spin and parity of the key state. Rather small values obtained for reduced $M1$ matrix elements, $|M(M1)|\lesssim 0.5$ $μ_N$, and proton spectroscopic factors, $C^{2}S_{\text{p}}$<10$^{-2}$, seem to be beyond the accuracy of the shell model. With the reevaluated $^{22}$Na(p, $γ$)$^{23}$Mg rate, the $^{22}$Na detectability limit and its observation frequency from novae are found promising for the future space telescopes.

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arXiv2021

Narrow resonances in the continuum of the unbound nucleus $^{15}$F

The structure of the unbound $^{15}$F nucleus is investigated using the inverse kinematics resonant scattering of a radioactive $^{14}$O beam impinging on a CH$_2$ target. The analysis of $^{1}$H($^{14}$O,p)$^{14}$O and $^{1}$H($^{14}$O,2p)$^{13}$N reactions allowed the confirmation of the previously observed narrow $1/2^{-}$ resonance, near the two-proton decay threshold, and the identification of two new narrow 5/2$^{-}$ and 3/2$^{-}$ resonances. The newly observed levels decay by 1p emission to the ground of $^{14}$O, and by sequential 2p emission to the ground state (g.s.) of $^{13}$N via the $1^-$ resonance of $^{14}$O. Gamow shell model (GSM) analysis of the experimental data suggests that the wave functions of the 5/2$^{-}$ and 3/2$^{-}$ resonances may be collectivized by the continuum coupling to nearby 2p- and 1p- decay channels. The observed excitation function $^{1}$H($^{14}$O,p)$^{14}$O and resonance spectrum in $^{15}$F are well reproduced in the unified framework of the GSM.

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arXiv2021

The MUGAST-AGATA-VAMOS campaign : set-up and performance

The MUGAST-AGATA-VAMOS set-up at GANIL combines the MUGAST highly-segmented silicon array with the state-of-the-art AGATA array and the large acceptance VAMOS spectrometer. The mechanical and electronics integration copes with the constraints of maximum efficiency for each device, in particular γ-ray transparency for the silicon array. This complete set-up offers a unique opportunity to perform exclusive measurements of direct reactions with the radioactive beams from the SPIRAL1 facility. The performance of the set-up is described through its commissioning and two examples of transfer reactions measured during the campaign. High accuracy spectroscopy of the nuclei of interest, including cross-sections and angular distributions, is achieved through the triple-coincidence measurement. In addition, the correction from Doppler effect of the γ-ray energies is improved by the detection of the light particles and the use of two-body kinematics and a full rejection of the background contributions is obtained through the identification of heavy residues. Moreover, the system can handle high intensity beams (up to 108 pps). The particle identification based on the measurement of the time-of-flight between MUGAST and VAMOS and the reconstruction of the trajectories is investigated.

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