arXiv subjects

C. Grimaldi

Publications and source records attributed to C. Grimaldi.

At least 55 records · Page 3Linked to original sources

arXiv2002

High $T_c$ superconductivity in MgB$_2$ by nonadiabatic pairing

The evidence for the key role of the $σ$ bands in the electronic properties of MgB$_2$ points to the possibility of nonadiabatic effects in the superconductivity of these materials. These are governed by the small value of the Fermi energy due to the vicinity of the hole doping level to the top of the $σ$ bands. We show that the nonadiabatic theory leads to a coherent interpretation of $T_c = 39$ K and the boron isotope coefficient $α_{\rm B} = 0.30$ without invoking very large couplings and it naturally explains the role of the disorder on $T_c$. It also leads to various specific predictions for the properties of MgB$_2$ and for the material optimization of these type of compounds.

cond-mat.supr-con↗

arXiv2002

Zeeman effects on the impurity-induced resonances in d-wave superconductors

It is shown how the resonant states induced by a single spinless impurity in a d-wave superconductor evolve under the effect of an applied Zeeman magnetic field. Moreover, it is demonstrated that the spin-orbit coupling to the impurity potential can have important and characteristic effects on the resonant states and their response to the Zeeman field, especially when the impurity is close to the unitary limit. For zero or very small spin-orbit interaction, the resonant states becomes Zeeman splitted by the magnetic field while when the spin-orbit coupling is important, new low-lying resonances arise which do not show any Zeeman splitting.

cond-mat.supr-con↗

arXiv2001

Unitary Limit of Spin-orbit scattering in two-dimensional s- and d-wave superconductors

Non-magnetic impurities affect the paramagnetic response of superconductors via the associated spin-orbit interaction which, when the non-magnetic impurity is close to the unitary limit, must be treated beyond the classical Born approximation. Here the Zeeman response of two-dimensional s- and d-wave superconductors is calculated within the self-consistent T-matrix formulation for both impurity and spin-orbit scatterings. It is shown that at the unitary limit, for which the spin-orbit scattering is maximum, the spin-up and spin-down channels becomes decoupled implying full Zeeman splitting of the quasiparticle excitations. These results could be used to test the unitary scattering hypothesis in high-Tc superconductors.

cond-mat.supr-con↗

arXiv2001

Nonadiabatic Superconductivity and Vertex Corrections in Uncorrelated Systems

We investigate the issue of the nonadiabatic superconductivity in uncorrelated systems. A local approximation is employed coherently with the weak dependence on the involved momenta. Our results show that nonadiabatic vertex corrections are never negligible, but lead to a strong suppression of $T_c$ with respect to the conventional theory. This feature is understood in terms of the momentum-frequency dependence of the vertex function. In contrast to strongly correlated systems, where the small ${\bf q}$-selection probes the positive part of vertex function, vertex corrections in uncorrelated systems are essentially negative resulting in an effective reduction of the superconducting pairing. Our analysis shows that vertex corrections in nonadiabatic regime can be never disregarded independently of the degree of electronic correlation in the system.

cond-mat.supr-con↗

arXiv2001

Breakdown of Migdal-Eliashberg Theory in Rb$_3$C$_{60}$

This paper has been withdrawn. An extended version of this work can be found in E. Cappelluti, C. Grimaldi, L. Pietronero, S. Straessler: Phys. Rev. Lett. 85, 4771 (2000) [cond-mat/0105560] and E. Cappelluti, C. Grimaldi, L. Pietronero, S. Straessler, G.A. Ummarino: Eur. Phys. J. B 21, 383 (2001) [cond-mat/0104457]

cond-mat.supr-con↗

arXiv2001

Nonadiabatic Channels in the Superconducting Pairing of Fullerides

We show the intrinsic inconsistency of the conventional phonon mediated theory of superconductivity in relation to the observed properties of Rb$_3$C$_{60}$. The recent, highly accurate measurement of the carbon isotope coefficient $α_{\rm C}=0.21$, together with the high value of $T_c$ (30 K) and the very small Fermi energy $E_{\rm F}$ (0.25 eV), unavoidably implies the opening of nonadiabatic channels in the superconducting pairing. We estimate these effects and show that they are actually the key elements for the high value of $T_c$ in these materials compared to the very low values of graphite intercalation compounds.

cond-mat.supr-con↗

arXiv2001

Superconductivity of Rb$_3$C$_{60}$: breakdown of the Migdal-Eliashberg theory

In this paper, through an exhaustive analysis within the Migdal-Eliashberg theory, we show the incompatibility of experimental data of Rb$_3$C$_{60}$ with the basic assumptions of the standard theory of superconductivity. For different models of the electron-phonon spectral function $α^2F(Ω)$ we solve numerically the Eliashberg equations to find which values of the electron-phonon coupling $λ$, of the logarithmic phonon frequency $Ω_{ln}$ and of the Coulomb pseudopotential $μ^*$ reproduce the experimental data of Rb$_3$C$_{60}$. We find that the solutions are essentially independent of the particular shape of $α^2F(Ω)$ and that, to explain the experimental data of Rb$_3$C$_{60}$, one has to resort to extremely large couplings: $λ=3.0\pm 0.8$. This results differs from the usual partial analyses reported up to now and we claim that this value exceeds the maximum allowed $λ$ compatible with the crystal lattice stability. Moreover, we show quantitatively that the obtained values of $λ$ and $Ω_{ln}$ strongly violate Migdal's theorem and consequently are incompatible with the Migdal-Eliashberg theory. One has therefore to consider the generalization of the theory of superconductivity in the nonadiabatic regime to account for the experimental properties of fullerides.

cond-mat.supr-con↗

arXiv2001

Nonadiabatic Pauli susceptibility in fullerene compounds

Pauli paramagnetic susceptibility $χ$ is unaffected by the electron-phonon interaction in the Migdal-Eliashberg context. Fullerene compounds however do not fulfill the adiabatic assumption of Migdal's theorem and nonadiabatic effects are expected to be relevant in these materials. In this paper we investigate the Pauli spin susceptibility in nonadiabatic regime by following a conserving approach based on Ward's identity. We find that a sizable renormalization of $χ$ due to electron-phonon coupling appears when nonadiabatic effects are taken into account. The intrinsic dependence of $χ$ on the electron-phonon interaction gives rise to a finite and negative isotope effect which could be experimentally detected in fullerides. In addition, we find an enhancement of the spin susceptibility with temperature increasing, in agreement with the temperature dependence of $χ$ observed in fullerene compounds. The role of electronic correlation is also discussed.

cond-mat.supr-con↗

arXiv2001

Longitudinal and transversal piezoresistive response of granular metals

In this paper, we study the piezoresistive response and its anisotropy for a bond percolation model of granular metals. Both effective medium results and numerical Monte Carlo calculations of finite simple cubic networks show that the piezoresistive anisotropy is a strongly dependent function of bond probability p and of bond conductance distribution width Δg. We find that piezoresistive anisotropy is strongly suppressed as p is reduced and/or Δg is enhanced and that it vanishes at the percolation thresold p=p_c. We argue that a measurement of the piezoresistive anisotropy could be a sensitive tool to estimate critical metallic concentrations in real granular metals.

cond-mat.dis-nn↗

arXiv2000

Gauge factor enhancement driven by heterogeneity in thick-film resistors

We present a simple picture of the gauge factor (GF) enhancement in highly heterogeneous materials such as thick-film resistors. We show that when the conducting phase is stiffer than the insulating one, the local strains within this latter are enhanced with respect to the averaged macroscopic strain. Within a simple model of electron tunneling processes, we show that the enhanced local strain leads to values of GF higher than those expected for a homogeneous system. Moreover we provide formulas relating the enhancement of GF to the elastic and microstructural characteristics of TFRs.

cond-mat.dis-nn↗

arXiv2000

s- and d-wave Symmetries in Nonadiabatic Theory of Superconductivity

High-$T_c$ superconductors have Fermi energies $E_F$ much smaller than conventional metals comparable to phonon frequencies. In such a situation nonadiabatic effects are important. A generalization of Eliashberg theory in the nonadiabatic regime has previously been shown to reproduce some anomalous features of the high-$T_c$ superconductors as for istance the enhancement of $T_c$ or the isotopic effects on $T_c$ and $m^*$. In this contribution we address the issue of the symmetry of the gap in the context of nonadiabatic superconductivity. We show that vertex corrections have a momentum structure which favours d-wave superconductivity when forward scattering is predominant. An additional increase of $T_c$ is also found.

cond-mat.supr-con↗

arXiv2000

A survey of nonadiabatic superconductivity in cuprates and fullerides

High-$T_c$ superconductors are characterized by very low carrier densities. This feature leads to two fundamental consequences: on one hand the Fermi energies are correspondingly small and they can be of the same order of phonon frequencies. In such a situation nonadiabatic corrections arising from the breakdown of Migdal's theorem can not be longer neglected. In addition, small carrier densities imply poor screening and correlation effects have to be taken into account. We present a comprehensive overview of the theory of superconductivity generalized into the nonadiabatic regime which is qualitatively different from the conventional one. In this framework some of the observed properties of the cuprates and the fullerene compounds can be naturally accounted for, and a number of theoretical predictions are proposed that can be experimentally tested.

cond-mat.supr-con↗

arXiv2000

Effect of Strong Correlation on the Electron-Phonon Interaction

High-$T_c$ superconductors are usually described as strongly correlated electronic systems. This feature deeply affects the one-particle and two-particle properties of the system. In particular, a large incoherent background developes on the top of a narrow quasi-particle peak in the one-electron spectral function. We schematize this structure with a simple phenomenological form. The corresponding Green's function is employed to calculate the charge response of the system taking into account in a proper way strong correlation effects. The effective charge interaction acquires a structure in the exchanged momentum space with a predominance of forward scattering, in agreement with previous numerical calculations. The consequences of the momentum dependence of the interaction are discussed in the framework of the nonadiabatic theory of superconductivity proposed for the high-$T_c$ materials.

cond-mat.supr-con↗

arXiv2000

Nonadiabatic theory of the superconducting state

Fermi energies in fullerene compounds and cuprates are extremely small as consequence of the small number of charge carriers and are comparable to the phonon frequency scale. In this situation the conventional Migdal-Eliashberg theory does not hold anymore and nonadiabatic effects need to be taken into account. In previous studies, a generalization of Eliashberg theory in the nonadiabatic regime has been proposed to calculate normal state properties and the onset temperature $T_c$ of the superconductive phase. Here we extend the nonadiabatic theory below $T_c$ where the opening of the superconducting order parameter affects the nonadiabatic correction. The superconducting gap $Δ$ is calculated in a self-consistent way. We find that large values of the ratio $2 Δ/T_c$ are obtained in the nonadiabatic theory by smaller electron-phonon coupling $λ$ than in Migdal-Eliashberg theory. This agrees with the picture that strong-coupling phenomenology can be achieved in nonadiabatic theory by ``reasonable'' values of $λ$. We apply our analysis to the case of the fullerene compounds.

cond-mat.supr-con↗

arXiv2000

Failure of the Migdal-Eliashberg Theory of Superconductivity in Rb_3C_60

We discuss the compatibility of the most accurate experimental data with the ordinary Migdal-Eliashberg theory of superconductivity in the fullerene compound Rb_3C_60. By using different model phonon spectra we conclude that the experimental data can be fitted only by invoking an electron-phonon coupling of order λ\simeq 3. This exceedingly high value is unphysical and it is not consistent with the basic assumptions of the Migdal-Eliashberg theory. On the contrary, by relaxing the adiabatic hypothesis on which the Migdal-Eliashberg theory rests, the experimental data can be fitted by much more realistic values of λ. This generalized theory predicts also characteristic features absent in the Migdal-Eliashberg framework which can be experimentally tested.

cond-mat.supr-con↗

arXiv2000

d-wave nonadiabatic superconductivity

The inclusion of nonadiabatic corrections to the electron-phonon interaction leads to a strong momentum dependence in the generalized Eliashberg equations beyond Migdal's limit. For a s-wave symmetry of the order parameter, this induced momentum dependence leads to an enhancement of Tc when small momentum transfer is dominant. Here we study how the d-wave symmetry affects the above behavior. We find that the nonadiabatic corrections depend only weakly on the symmetry of the order parameter provided that only small momentum scatterings are allowed for the electron-phonon interaction. In this situation, We show that also for a d-wave symmetry of the order parameter, the nonadiabatic corrections enhance Tc. We also discuss the possible interplay and crossover between s- and d-wave depending on the material's parameters.

cond-mat.supr-con↗

arXiv2000

Gauge factor of thick film resistors: outcomes of the variable range hopping model

Despite a large amount of data and numerous theoretical proposals, the microscopic mechanism of transport in thick film resistors remains unclear. However, recent low temperature measurements point toward a possible variable range hopping mechanism of transport. Here we examine how such a mechanism affects the gauge factor of thick film resistors. We find that at sufficiently low temperatures $T$, for which the resistivity follows the Mott's law $R(T)\sim \exp(T_0/T)^{1/4}$, the gauge factor GF is proportional to $(T_0/T)^{1/4}$. Moreover, the inclusion of Coulomb gap effects leads to ${\rm GF}\sim (T_0'/T)^{1/2}$ at lower temperatures. In addition, we study a simple model which generalizes the variable range hopping mechanism by taking into account the finite mean inter-grain spacing. Our results suggest a possible experimental verification of the validity of the variable range hopping in thick film resistors.

cond-mat.dis-nn↗

arXiv1999

Anomalous impurity effects in nonadiabatic superconductors

We show that, in contrast with the usual electron-phonon Migdal-Eliashberg theory, the critical temperature Tc of an isotropic s-wave nonadiabatic superconductor is strongly reduced by the presence of diluted non-magnetic impurities. Our results suggest that the recently observed Tc-suppression driven by disorder in K3C60 [Phys. Rev. B vol.55, 3866 (1997)] and in Nd(2-x)CexCuO(4-delta) [Phys. Rev. B vol.58, 8800 (1998)] could be explained in terms of a nonadiabatic electron-phonon coupling. Moreover, we predict that the isotope effect on Tc has an impurity dependence qualitatively different from the one expected for anisotropic superconductors.

cond-mat.supr-con↗