arXiv subjects

C. H. Keitel

Publications and source records attributed to C. H. Keitel.

At least 55 records · Page 3Linked to original sources

arXiv2020

Coherent x-ray-optical control of nuclear excitons with zeptosecond phase-stability

Coherent control of quantum dynamics is key to a multitude of fundamental studies and applications alike. In the visible or longer-wavelength domains, near-resonant light fields have become the primary tool to control electron dynamics. Recently, coherent control in the extreme-ultraviolet range was demonstrated, with timing stability of the applied light fields in the few-attosecond range. At hard x-ray energies, Mössbauer nuclei feature narrow nuclear resonances, and spectroscopy of these resonances is a widespread tool to study magnetic, structural and dynamical properties of matter. It has been shown that the power and scope of Mössbauer spectroscopy can be significantly advanced using various control techniques. However, the coherent control of atomic nuclei using near-resonant x-ray fields remains an open challenge, also because of the extreme stability requirements on the x-ray light in the few-zeptosecond range. Here, we demonstrate such control, and use the relative phase of two x-ray pulses to switch the nuclear dynamics between stimulated emission and enhanced coherent excitation. For this, we suggest and implement a method to shape single pulses delivered by modern x-ray facilities into tunable double-pulses, with the desired stability on the few-zeptosecond level. Our results unlock coherent optical control for nuclei, and pave the way for nuclear Ramsey spectroscopy and spin-echo-like techniques, which not only provide key concepts for advancing nuclear quantum optics, but also essential ingredients for possible x-ray clocks and frequency standards. As a long-term perspective, we envision time-resolved studies of nuclear out-of-equilibrium dynamics, which is a long-standing open challenge in Mössbauer science.

quant-ph↗

arXiv2020

The measurement of the quadrupole moment of 185-Re and 187-Re from the hyperfine structure of muonic X rays

The hyperfine splitting of the 5g -> 4f transitions in muonic 185,187-Re has been measured using high resolution HPGe detectors and compared to state-of-the-art atomic theoretical predictions. The spectroscopic quadrupole moment has been extracted using modern fitting procedures and compared to the values available in literature obtained from muonic X rays of natural rhenium. The extracted values of the nuclear spectroscopic quadrupole moment are 2.07(5) barn and 1.94(5) barn, respectively for 185-Re and 187-Re. This work is part of a larger effort at the Paul Scherrer Institut towards the measurement of the nuclear charge radii of radioactive elements.

nucl-ex↗

arXiv2019

Detection of the $5p-4f$ orbital crossing and its optical clock transition in Pr$^{9+}$

Recent theoretical works have proposed atomic clocks based on narrow optical transitions in highly charged ions. The most interesting candidates for searches of new physics are those which occur at rare orbital crossings where the shell structure of the periodic table is reordered. There are only three such crossings expected to be accessible in highly charged ions, and hitherto none have been observed as both experiment and theory have proven difficult. In this work we observe an orbital crossing in highly charged ions for the first time, in a system chosen to be tractable from both sides: Pr$^{9+}$. We present electron beam ion trap measurements of its spectra, including the inter-configuration lines that reveal the sought-after crossing. The proposed nHz-wide clock line, found to be at 452.334(1) nm, proceeds through hyperfine admixture of its upper state with an E2-decaying level. With state-of-the-art calculations we show that it has a very high sensitivity to new physics and extremely low sensitivity to external perturbations, making it a unique candidate for proposed precision studies.

physics.atom-ph↗

arXiv2019

Parametric Mössbauer radiation source

Numerous applications of Mössbauer spectroscopy are related to a unique resolution of absorption spectra of resonant radiation in crystals, when the nucleus absorbs a photon without a recoil. However, the narrow nuclear linewidth renders efficient driving of the nuclei challenging, restricting precision spectroscopy, nuclear inelastic scattering and nuclear quantum optics. Moreover, the need for dedicated X-ray optics restricts access to only few isotopes, impeding precision spectroscopy of a wider class of systems. Here, we put forward a novel Mössbauer source, which offers a high resonant photon flux for a large variety of Mössbauer isotopes, based on relativistic electrons moving through a crystal and emitting parametric Mössbauer radiation essentially unattenuated by electronic absorption. As a result, a collimated beam of resonant photons is formed, without the need for additional monochromatization. We envision the extension of high-precision Mössbauer spectroscopy to a wide range of isotopes at accelerator facilities using dumped electron beams.

physics.acc-ph↗

arXiv2019

$g$-factor of Boronlike Argon $^{40}\textrm{Ar}^{13+}$

We have measured the ground-state $g$-factor of boronlike argon $^{40}\textrm{Ar}^{13+}$ with a fractional uncertainty of \SI{1.4e-9}{} with a single ion in the newly developed ALPHATRAP double Penning-trap setup. The here obtained value of $g=0.663\,648\,455\,32(93)$ is in agreement with our theoretical prediction of $0.663\,648\,12(58)$. The latter is obtained accounting for quantum electrodynamics, electron correlation, and nuclear effects within the state-of-the-art theoretical methods. Our experimental result distinguishes between existing predictions that are in disagreement, and lays the foundations for an independent determination of the fine-structure constant.

physics.atom-ph↗

arXiv2019

Improved local-constant-field approximation for strong-field QED codes

The local-constant-field approximation (LCFA) is an essential theoretical tool for investigating strong-field QED phenomena in background electromagnetic fields with complex spacetime structure. In our previous work [Phys.~Rev.~A~\textbf{98}, 012134 (2018)] we have analyzed the shortcomings of the LCFA in nonlinear Compton scattering at low emitted photon energies for the case of a background plane-wave field. Here, we generalize that analysis to background fields, which can feature a virtually arbitrary spacetime structure. In addition, we provide an explicit and simple implementation of an improved expression of the nonlinear Compton scattering differential probability that solves the main shortcomings of the standard LCFA in the infrared region, and is suitable for background electromagnetic fields with arbitrary spacetime structure such as those occurring in particle-in-cell simulations. Finally, we carry out a systematic procedure to calculate the probability of nonlinear Compton scattering per unit of emitted photon light-cone energy and of nonlinear Breit-Wheeler pair production per unit of produced positron light-cone energy beyond the LCFA in a plane-wave background field, which allows us to identify the limits of validity of this approximation quantitatively.

hep-ph↗

arXiv2019

The $g$ factor of bound electrons as a test for physics beyond the Standard Model

The use of high-precision measurements of the $g$ factor of few-electron ions and its isotope shifts is put forward as a probe for physics beyond the Standard Model. The contribution of a hypothetical fifth fundamental force to the $g$ factor is calculated for the ground state of H-like, Li-like and B-like ions, and employed to derive bounds on the parameters of that force. The weighted difference and especially the isotope shift of $g$ factors are used in order to increase the experimental sensitivity to the new physics contribution. It is found that, combining measurements from four different isotopes of H-like, Li-like and B-like calcium ions at currently accessible accuracy levels, experimental results compatible with King planarity would constrain the new physics coupling constant more than one order of magnitude further than the best current atomic data.

physics.atom-ph↗

arXiv2018

Semi-classical limitations for photon emission in strong external fields

The semi-classical heuristic emission formula of Baier-Katkov [Sov. Phys. JETP \textbf{26}, 854 (1968)] is well-known to describe radiation of an ultrarelativistic electron in strong external fields employing the electron's classical trajectory. To find the limitations of the Baier-Katkov approach, we investigate electron radiation in a strong rotating electric field quantum mechanically using the Wentzel-Kramers-Brillouin approximation. Except for an ultrarelativistic velocity, it is shown that an additional condition is required in order to recover the widely used semi-classical result. A violation of this condition leads to two consequences. First, it gives rise to qualitative discrepancy in harmonic spectra between the two approaches. Second, the quantum harmonic spectra are determined not only by the classical trajectory but also by the dispersion relation of the effective photons of the external field.

hep-ph↗

arXiv2018

Nonlinear Compton scattering of an ultra-intense laser pulse in a plasma

Laser pulses traveling through a plasma can feature group velocities significantly differing from the speed of light in vacuum. This modifies the well-known Volkov states of an electron inside a strong laser-field from the vacuum case and consequently all quantum electrodynamical effects triggered by the electron. Here we present an in-depth study of the basic process of photon emission by an electron scattered from an intense short laser pulse inside a plasma, labeled nonlinear Compton scattering, based on modified Volkov solutions derived from first principles. Consequences of the nonlinear, plasma-dressed laser dispersion on the Compton spectra of emitted photons and implications for high-intensity laser-plasma experiments are pointed out.

physics.plasm-ph↗

arXiv2018

Experimental signatures of the quantum nature of radiation reaction in the field of an ultra-intense laser

The description of the dynamics of an electron in an external electromagnetic field of arbitrary intensity is one of the most fundamental outstanding problems in electrodynamics. Remarkably, to date there is no unanimously accepted theoretical solution for ultra-high intensities and little or no experimental data. The basic challenge is the inclusion of the self-interaction of the electron with the field emitted by the electron itself - the so-called radiation reaction force. We report here on the experimental evidence of strong radiation reaction, in an all-optical experiment, during the propagation of highly relativistic electrons (maximum energy exceeding 2 GeV) through the field of an ultra-intense laser (peak intensity of $4\times10^{20}$ W/cm$^2$). In their own rest frame, the highest energy electrons experience an electric field as high as one quarter of the critical field of quantum electrodynamics and are seen to lose up to 30% of their kinetic energy during the propagation through the laser field. The experimental data show signatures of quantum effects in the electron dynamics in the external laser field, potentially showing departures from the constant cross field approximation.

physics.plasm-ph↗

arXiv2018

Implementing nonlinear Compton scattering beyond the local constant field approximation

In the calculation of probabilities of physical processes occurring in a background classical field, the local constant field approximation (LCFA) relies on the possibility of neglecting the space-time variation of the external field within the region of formation of the process. This approximation is widely employed in strong-field QED as it allows to evaluate probabilities of processes occurring in arbitrary electromagnetic fields starting from the corresponding quantities computed in a constant electromagnetic field. Here, we demonstrate in the case of nonlinear single Compton scattering that the LCFA is quantitatively and qualitatively insufficient for describing the low-energy part of the emitted photon probability. In addition, we provide a simple recipe to implement an improved expression of the photon emission probability beyond the LCFA in numerical codes, which are an essential tool to interpret present and upcoming experiments in strong-field QED.

hep-ph↗

arXiv2018

Theory of the two-loop self-energy correction to the $\boldsymbol g$ factor in non-perturbative Coulomb fields

Two-loop self-energy corrections to the bound-electron $g$ factor are investigated theoretically to all orders in the nuclear binding strength parameter $Zα$. The separation of divergences is performed by dimensional regularization, and the contributing diagrams are regrouped into specific categories to yield finite results. We evaluate numerically the loop-after-loop terms, and the remaining diagrams by treating the Coulomb interaction in the electron propagators up to first order. The results show that such two-loop terms are mandatory to take into account for projected near-future stringent tests of quantum electrodynamics and for the determination of fundamental constants through the $g$ factor.

physics.atom-ph↗

arXiv2018

Access to improve the muon mass and magnetic moment anomaly via the bound-muon $g$ factor

A theoretical description of the $g$ factor of a muon bound in a nuclear potential is presented. One-loop self-energy and multi-loop vacuum polarization corrections are calculated, taking into account the interaction with the binding potential exactly. Nuclear effects on the bound-muon $g$ factor are also evaluated. We put forward the measurement of the bound-muon $g$ factor via the continuous Stern-Gerlach effect as an independent means to determine the free muons magnetic moment anomaly and mass. The scheme presented enables to increase the accuracy of the mass by more than an order of magnitude.

hep-ph↗

arXiv2017

Analytic model of a multi-electron atom

A fully analytical approximation for the observable characteristics of many-electron atoms is developed via a complete and orthonormal hydrogen-like basis with a single-effective charge parameter for all electrons of a given atom. The basis completeness allows us to employ the secondary-quantized representation for the construction of regular perturbation theory, which includes in a natural way correlation effects, converges fast and enables an effective calculation of the subsequent corrections. The hydrogen-like basis set provides a possibility to perform all summations over intermediate states in closed form, including both the discrete and continuous spectra. This is achieved with the help of the decomposition of the multi-particle Green function in a convolution of single-electronic Coulomb Green functions. We demonstrate that our fully analytical zeroth-order approximation describes the whole spectrum of the system, provides accuracy, which is independent of the number of electrons and is important for applications where the Thomas-Fermi model is still utilized. In addition already in second-order perturbation theory our results become comparable with those via a multi-configuration Hartree-Fock approach.

quant-ph↗

arXiv2017

Electron-correlation effects in the $g$-factor of light Li-like ions

We investigate electron-correlation effects in the $g$-factor of the ground state of Li-like ions. Our calculations are performed within the nonrelativistic quantum electrodynamics (NRQED) expansion up to two leading orders in the fine-structure constant $α$, $α^2$ and $α^3$. The dependence of the NRQED results on the nuclear charge number $Z$ is studied and the individual $1/Z$-expansion contributions are identified. Combining the obtained data with the results of the all-order (in $Zα$) calculations performed within the $1/Z$ expansion, we derive the unified theoretical predictions for the $g$-factor of light Li-like ions.

physics.atom-ph↗

arXiv2017

Extraction of the electron mass from $g$ factor measurements on light hydrogenlike ions

The determination of the electron mass from Penning-trap measurements with $^{12}$C$^{5+}$ ions and from theoretical results for the bound-electron $g$ factor is described in detail. Some recently calculated contributions slightly shift the extracted mass value. Prospects of a further improvement of the electron mass are discussed both from the experimental and from the theoretical point of view. Measurements with $^4$He$^+$ ions will enable a consistency check of the electron mass value, and in future an improvement of the $^4$He nuclear mass and a determination of the fine-structure constant.

physics.atom-ph↗

arXiv2017

Interplay between Coulomb-focusing and non-dipole effects in strong-field ionization with elliptical polarization

Strong-field ionization and rescattering beyond the long-wavelength limit of the dipole approximation is studied with elliptically polarized mid-IR pulses. We have measured the full three-dimensional photoelectron momentum distributions (3D PMDs) with velocity map imaging and tomographic reconstruction. The ellipticity-dependent 3D-PMD measurements revealed an unexpected sharp, thin line-shaped ridge structure in the polarization plane for low momentum photoelectrons. With classical trajectory Monte Carlo (CTMC) simulations and analytical methods we identified the associated ionization dynamics for this sharp ridge to be due to Coulomb focusing of slow recollisions of electrons with a momentum approaching zero. This ridge is another example of the many different ways how the Coulomb field of the parent ion influences the different parts of the momentum space of the ionized electron wave packet. Building on this new understanding of the PMD, we extend our studies on the role played by the magnetic field component of the laser beam when operating beyond the long-wavelength limit of the dipole approximation. In this regime, we find that the PMD exhibits an ellipticity-dependent asymmetry along the beam propagation direction: the peak of the projection of the PMD onto the beam propagation axis is shifted from negative to positive values with increasing ellipticity. This turnover occurs rapidly once the ellipticity exceeds $\sim$0.1. We identify the sharp, thin line-shaped ridge structure in the polarization plane as the origin of the ellipticity-dependent PMD asymmetry in the beam propagation direction. These results yield fundamental insights into strong-field ionization processes, and should increase the precision of the emerging applications relying on this technique, including time-resolved holography and molecular imaging.

physics.atom-ph↗

arXiv2017

Soliton-like solution in quantum electrodynamics

A novel soliton-like solution in quantum electrodynamics is obtained via a self-consistent field method. By writing the Hamiltonian of quantum electrodynamics in the Coulomb gauge, we separate out a classical component in the density operator of the electron-positron field. Then, by modeling the state vector in analogy with the theory of superconductivity, we minimize the functional for the energy of the system. This results in the equations of the self-consistent field, where the solutions are associated with the collective excitation of the electron-positron field---the soliton-like solution. In addition, the canonical transformation of the variables allowed us to separate out the total momentum of the system and, consequently, to find the relativistic energy dispersion relation for the moving soliton.

hep-th↗