arXiv subjects

C. H. Lee

Publications and source records attributed to C. H. Lee.

At least 19 recordsLinked to original sources

arXiv2026

Preventing quart-NaI adhesion in Bridgman growth using ammonium iodide

Adhesion between NaI(Tl) single crystals and the walls of quartz ampoules remains a major limitation for Bridgman growth under sealed conditions, particularly for applications requiring ultra-radiopure scintillators for dark matter searches, where sealed handling is essential. In this study, ammonium iodide (NH4I) was used as an additive to generate HI in situ, thereby suppressing the NaOH-SiO2 reaction that forms adhesive sodium silicate phases. Small-diameter crystals (8 mm) were first grown to determine the NH4I concentration required to eliminate adhesion. The optimized condition was then applied to the growth of a large NaI(Tl) crystal. A crack-free and bubble-free NaI(Tl) crystal with dimensions of 3 inches in diameter by 3 inches in length was successfully grown. The crystal exhibited a light output of 59,000 photons/MeV, which is higher than that of the commercial NaI(Tl) crystals used as references in this study.

physics.ins-det↗

arXiv2026

A study of neutrinoless double electron capture in $^{40}$Ca from the AMoRE experiment

The search for neutrinoless double electron capture ($0ν\mathrm{2EC}$) provides a sensitive probe of lepton-number violation and the Majorana nature of neutrinos. We investigate the $0ν\mathrm{2EC}$ decay of $^{40}$Ca using cryogenic detectors equipped with metallic magnetic calorimeters in the AMoRE-I experiment. The analysis is based on a physics dataset corresponding to a total exposure of 7.32 kg$\cdot$yr from thirteen $^{40}$Ca$^{100}$MoO$_4$ crystals. No significant excess is observed, and a lower limit on the half-life is obtained as $T^{0ν}_{1/2} > 1.7 \times 10^{22}$ yr at 90$\%$ confidence level. An improved sensitivity is expected for the upcoming AMoRE-II experiment. These results demonstrate the potential of CaMoO$_4$ detectors to explore rare decay processes beyond the primary $^{100}$Mo $0νββ$ search program.

nucl-ex↗

arXiv2025

Translational symmetry breaking in the electronic nematic phase of BaFe2As2

The microscopic origin of the nematicity, namely, four-fold rotational symmetry breaking in iron-based superconductors has been controversial since its discovery. In particular, its relationship with the stripe-type spin-density-wave order and the orthorhombic lattice distortion in the antiferromagnetic orthorhombic (AFO) phase, which exists at temperatures below the electronic nematic phase, has been highly debated. Here, we report on the temperature evolution of angle-resolved photoemission spectra of the parent compound BaFe2As2, ranging from the AFO to nematic to paramagnetic phases. The Dirac cone feature, which is formed in the AFO phase, is found to persist in the nematic phase, suggesting that an antiferroic order of the same periodicity as the AFO phase persists in the nematic phase. Considering the relatively shallow d_xy orbital in BaFe2As2, we propose that an antiferro-orbital order involving the d_xy and other orbitals takes place in the nematic phase.

cond-mat.supr-con↗

arXiv2025

Enhanced superconducting gap in the outer CuO$_2$ plane of the trilayer cuprate (Hg,Re)Ba$_2$Ca$_2$Cu$_3$O$_{8+δ}$

We report the first observation of a momentum-resolved superconducting gap in the Hg-based trilayer cuprate, which holds the highest record of superconducting transition temperature ($T_\mathrm{c}$) at ambient pressure. By angle-resolved photoemission spectroscopy utilizing a micro-focused beam, clear quasiparticle dispersions originating from the inner and outer CuO$_2$ planes (IP and OP, respectively) were separately identified. The magnitude of the superconducting gap for the IP was comparable to that of the Bi-based trilayer cuprate with a lower $T_\mathrm{c}$. In contrast, the superconducting gap for the OP was significantly larger than that of the Bi-based one. While strong pairing in the IP has been highlighted as the key element of trilayer cuprates, the present results suggest that the enhanced pairing energy in the OP is essential for the highest $T_\mathrm{c}$ at ambient pressure realized in the Hg-based trilayer cuprate.

cond-mat.supr-con↗

arXiv2025

Improved limit on neutrinoless double beta decay of $^{100}$Mo from AMoRE-I

AMoRE searches for the signature of neutrinoless double beta decay of $^{100}$Mo with a 100 kg sample of enriched $^{100}$Mo. Scintillating molybdate crystals coupled with a metallic magnetic calorimeter operate at milli-Kelvin temperatures to measure the energy of electrons emitted in the decay. As a demonstration of the full-scale AMoRE, we conducted AMoRE-I, a pre-experiment with 18 molybdate crystals, at the Yangyang Underground Laboratory for over two years. The exposure was 8.02 kg$\cdot$year (or 3.89 kg$_{\mathrm{^{100}Mo}}\cdot$year) and the total background rate near the Q-value was 0.025 $\pm$ 0.002 counts/keV/kg/year. We observed no indication of $0νββ$ decay and report a new lower limit of the half-life of $^{100}$Mo $0νββ$ decay as $ T^{0ν}_{1/2}>2.9\times10^{24}~\mathrm{yr}$ at 90\% confidence level. The effective Majorana mass limit range is $m_{ββ}<$(210--610) meV using nuclear matrix elements estimated in the framework of different models, including the recent shell model calculations.

nucl-ex↗

arXiv2025

Development of MMC-based lithium molybdate cryogenic calorimeters for AMoRE-II

The AMoRE collaboration searches for neutrinoless double beta decay of $^{100}$Mo using molybdate scintillating crystals via low temperature thermal calorimetric detection. The early phases of the experiment, AMoRE-pilot and AMoRE-I, have demonstrated competitive discovery potential. Presently, the AMoRE-II experiment, featuring a large detector array with about 90 kg of $^{100}$Mo isotope, is under construction. This paper discusses the baseline design and characterization of the lithium molybdate cryogenic calorimeters to be used in the AMoRE-II detector modules. The results from prototype setups that incorporate new housing structures and two different crystal masses (316 g and 517 - 521 g), operated at 10 mK temperature, show energy resolutions (FWHM) of 7.55 - 8.82 keV at the 2.615 MeV $^{208}$Tl $γ$ line, and effective light detection of 0.79 - 0.96 keV/MeV. The simultaneous heat and light detection enables clear separation of alpha particles with a discrimination power of 12.37 - 19.50 at the energy region around $^6$Li(n, $α$)$^3$H with Q-value = 4.785 MeV. Promising detector performances were demonstrated at temperatures as high as 30 mK, which relaxes the temperature constraints for operating the large AMoRE-II array.

physics.ins-det↗

arXiv2024

Projected background and sensitivity of AMoRE-II

AMoRE-II aims to search for neutrinoless double beta decay with an array of 423 Li$_2$$^{100}$MoO$_4$ crystals operating in the cryogenic system as the main phase of the Advanced Molybdenum-based Rare process Experiment (AMoRE). AMoRE has been planned to operate in three phases: AMoRE-pilot, AMoRE-I, and AMoRE-II. AMoRE-II is currently being installed at the Yemi Underground Laboratory, located approximately 1000 meters deep in Jeongseon, Korea. The goal of AMoRE-II is to reach up to $T^{0νββ}_{1/2}$ $\sim$ 6 $\times$ 10$^{26}$ years, corresponding to an effective Majorana mass of 15 - 29 meV, covering all the inverted mass hierarchy regions. To achieve this, the background level of the experimental configurations and possible background sources of gamma and beta events should be well understood. We have intensively performed Monte Carlo simulations using the GEANT4 toolkit in all the experimental configurations with potential sources. We report the estimated background level that meets the 10$^{-4}$counts/(keV$\cdot$kg$\cdot$yr) requirement for AMoRE-II in the region of interest (ROI) and show the projected half-life sensitivity based on the simulation study.

physics.ins-det↗

arXiv2024

Background study of the AMoRE-pilot experiment

We report a study on the background of the Advanced Molybdenum-Based Rare process Experiment (AMoRE), a search for neutrinoless double beta decay (\znbb) of $^{100}$Mo. The pilot stage of the experiment was conducted using $\sim$1.9 kg of \CAMOO~ crystals at the Yangyang Underground Laboratory, South Korea, from 2015 to 2018. We compared the measured $β/γ$ energy spectra in three experimental configurations with the results of Monte Carlo simulations and identified the background sources in each configuration. We replaced several detector components and enhanced the neutron shielding to lower the background level between configurations. A limit on the half-life of $0νββ$ decay of $^{100}$Mo was found at $T_{1/2}^{0ν} \ge 3.0\times 10^{23}$ years at 90\% confidence level, based on the measured background and its modeling. Further reduction of the background rate in the AMoRE-I and AMoRE-II are discussed.

nucl-ex↗

arXiv2023

Kondo screening in a Majorana metal

Kondo impurities provide a nontrivial probe to unravel the character of the excitations of a quantum spin liquid. In the S=1/2 Kitaev model on the honeycomb lattice, Kondo impurities embedded in the spin-liquid host can be screened by itinerant Majorana fermions via gauge-flux binding. Here, we report experimental signatures of metallic-like Kondo screening at intermediate temperatures in the Kitaev honeycomb material α-RuCl3 with dilute Cr3+ (S=3/2) impurities. The static magnetic susceptibility, the muon Knight shift, and the muon spin-relaxation rate all feature logarithmic divergences, a hallmark of a metallic Kondo effect. Concurrently, the linear coefficient of the magnetic specific heat is large in the same temperature regime, indicating the presence of a host Majorana metal. This observation opens new avenues for exploring uncharted Kondo physics in insulating quantum magnets.

cond-mat.str-el↗

arXiv2021

New Gelfond-Type Transcendental Numbers

It is well known that value at a non-zero algebraic number of each of the functions $e^{x}, \ln x, \sin x, \cos x, \tan x, \csc x, \sec x, \cot x, \sinh x,$ $ \cosh x,$ $ \tanh x,$ and $\coth x$ is transcendental number (see Theorem 9.11 of \cite{N}). In the work, we show that for any one of the above mentioned functions, $f(x)$, and for a polynomial $g(x)$ with rational coefficients the zero, if any, of the equation $f(x)=g(x)$ is a transcendental number. We also show that if $f(x)$ and $g(x)$ are polynomials with rational coefficients, then a zero of the equation $e^{f(x)}=g(x)$ is a transcendental number. Finally we show that the existence of an abelian group whose non-zero elements are transcendental numbers.

math.NT↗

arXiv2020

Isotropic parallel antiferromagnetism in the magnetic-field-induced charge-ordered state of SmRu$_4$P$_{12}$ caused by $p$-$f$ hybridization

Nature of the field-induced charge ordered phase (phase II) of SmRu$_4$P$_{12}$ has been investigated by resonant x-ray diffraction (RXD) and polarized neutron diffraction (PND), focusing on the relationship between the atomic displacements and the antiferromagnetic (AFM) moments of Sm. From the analysis of the interference between the non-resonant Thomson scattering and the resonant magnetic scattering, combined with the spectral function obtained from x-ray magnetic circular dichroism, it is shown that the AFM moment of Sm prefers to be parallel to the field ($m_{\text{AF}} \parallel H$), giving rise to large and small moment sites around which the P$_{12}$ and Ru cage contract and expand, respectively. This is associated with the formation of the staggered ordering of the $Γ_7$-like and $Γ_8$-like crystal-field states, providing a strong piece of evidence for the charge order. PND was also performed to obtain complementary and unambiguous conclusion. In addition, isotropic and continuous nature of the phase II is demonstrated by the field-direction invariance of the interference spectrum in RXD. Crucial role of the $p$-$f$ hybridization is shown by resonant soft x-ray diffraction at the P $K$-edge ($1s\leftrightarrow 3p$), where we detected a resonance due to the spin polarized $3p$ orbitals reflecting the AFM order of Sm.

cond-mat.str-el↗

arXiv2020

Unconventional scaling at non-Hermitian critical points

Critical phase transitions contain a variety of deep and universal physics, and are intimately tied to thermodynamic quantities through scaling relations. Yet, these notions are challenged in the context of non-Hermiticity, where spatial or temporal divergences render the thermodynamic limit ill-defined. In this work, we show that a thermodynamic grand potential can still be defined in pseudo-Hermitian Hamiltonians, and can be used to characterize aspects of criticality unique to non-Hermitian systems. Using the non-Hermitian Su-Schrieffer-Heeger (SSH) model as a paradigmatic example, we demonstrate the fractional order of topological phase transitions in the complex energy plane. These fractional orders add up to the integer order expected of a Hermitian phase transition when the model is doubled and Hermitianized. More spectacularly, gap preserving highly degenerate critical points known as non-Bloch band collapses possess fractional order that are not constrained by conventional scaling relations, testimony to the emergent extra length scale from the skin mode accumulation. Our work showcases that a thermodynamic approach can prove fruitful in revealing unconventional properties of non-Hermitian critical points.

cond-mat.stat-mech↗

arXiv2020

Development of ultra-pure NaI(Tl) detectors for the COSINE-200 experiment

The annual modulation signal observed by the DAMA experiment is a long-standing question in the community of dark matter direct detection. This necessitates an independent verification of its existence using the same detection technique. The COSINE-100 experiment has been operating with 106~kg of low-background NaI(Tl) detectors providing interesting checks on the DAMA signal. However, due to higher backgrounds in the NaI(Tl) crystals used in COSINE-100 relative to those used for DAMA, it was difficult to reach final conclusions. Since the start of COSINE-100 data taking in 2016, we also have initiated a program to develop ultra-pure NaI(Tl) crystals for COSINE-200, the next phase of the experiment. The program includes efforts of raw powder purification, ultra-pure NaI(Tl) crystal growth, and detector assembly techniques. After extensive research and development of NaI(Tl) crystal growth, we have successfully grown a few small-size (0.61$-$0.78 kg) thallium-doped crystals with high radio-purity. A high light yield has been achieved by improvements of our detector assembly technique. Here we report the ultra-pure NaI(Tl) detector developments at the Institute for Basic Science, Korea. The technique developed here will be applied to the production of NaI(Tl) detectors for the COSINE-200 experiment.

physics.ins-det↗

arXiv2020

Growth and development of pure Li2MoO4 crystals for rare event experiment at CUP

The Center for Underground Physics (CUP) of the Institute for Basic Science (IBS) is searching for the neutrinoless double-beta decay (0ν\b{eta}\b{eta}) of 100Mo in the molybdate crystals of the AMoRE experiment. The experiment requires pure scintillation crystals to minimize internal backgrounds that can affect the 0ν\b{eta}\b{eta} signal. For the last few years, we have been growing and studying Li2MoO4 crystals in a clean-environment facility to minimize external contamination during the crystal growth. Before growing Li2100MoO4 crystal, we have studied Li2natMoO4 crystal growth by a conventional Czochralski (CZ) grower. We grew a few different kinds of Li2natMO4 crystals using different raw materials in a campaign to minimize impurities. We prepared the fused Al2O3 refractories for the growth of ingots. Purities of the grown crystals were measured with high purity germanium detectors and by inductively coupled plasma mass spectrometry. The results show that the Li2MoO4 crystal has purity levels suitable for rare-event experiments. In this study, we present the growth of Li2MoO4 crystals at CUP and their purities.

physics.ins-det↗

arXiv2019

Coexistence of type-I and type-II superconductivity in topological superconductor PdTe$_2$

The type-II Dirac semimetal PdTe2 was recently reported to be a type-I superconductor with a superconducting transition temperature Tc = 1.65 K. However, the recent results from tunneling and point contact spectroscopy suggested the unusual state of a mixture of type-I and type-II superconductivity. These contradictory results mean that there is no clear picture of the superconducting phase diagram and warrants a detailed investigation of the superconducting phase. We report here the muon spin rotation and relaxation ($μ$SR) measurements on the superconducting state of the topological Dirac semimetal PdTe2. From $μ$SR measurements, we find that PdTe2 exhibits mixed type-I/type-II superconductivity. Using these results a phase diagram has been determined. In contrast to previous results where local type-II superconductivity persists up to Hc2 = 600 G, we observed that bulk superconductivity is destroyed above 225 G.

cond-mat.supr-con↗

arXiv2019

Emerging superconductivity with broken time reversal symmetry inside a superconducting $s$-wave state

In general, magnetism and superconductivity are antagonistic to each other. However, there are several families of superconductors, in which superconductivity may coexist with magnetism, and only a few examples are known, when superconductivity itself induces spontaneous magnetism. The most known compounds are Sr$_2$RuO$_4$ and some noncentrosymmetric superconductors. Here, we report the finding of a narrow dome of a novel $s+is'$ superconducting (SC) phase with broken time-reversal symmetry (BTRS) inside the broad $s$-wave SC region of the centrosymmetric multiband superconductor Ba$_{\rm 1-x}$K$_{\rm x}$Fe$_2$As$_2$ ($0.7 \lesssim x \lesssim 0.85$). We observe spontaneous magnetic fields inside this dome using the muon spin relaxation ($μ$SR) technique. Furthermore, our detailed specific heat study reveals that the BTRS dome appears very close to a change in the topology of the Fermi surface (Lifshitz transition). With this, we experimentally demonstrate the emergence of a novel quantum state due to topological changes of the electronic system.

cond-mat.supr-con↗

arXiv2018

Thermoelectric properties of (Ba,K)Cd2As2 crystallized in the CaAl2Si2-type structure

As-Based Zintl compounds Ba1-xKxCd2As2 crystallized in the CaAl2Si2-type structure (space group P3-m1) were prepared using solid-state reactions followed by hot-pressing. We have successfully substituted K for Ba up to x = 0.08, producing hole-carrier doping with concentrations up to 1.60*1020 cm-3. We have determined the band-gap value of non-doped BaCd2As2 to be 0.40 eV from the temperature dependence of the electrical resistivity. Both the electrical resistivity and the Seebeck coefficient decrease with hole doping, leading to a power factor value of 1.28 mW m-1 K-2 at 762 K for x = 0.04. A first-principles band calculation shows that the relatively large power factor mainly originates from the two-fold degeneracy of the bands comprising As px,y orbitals and from the anisotropic band structure at the valence-band maximum. The lattice thermal conductivity is suppressed by the K doping to 0.46 W m-1 K-1 at 773 K for x = 0.08, presumably due to randomness. The effect of randomness is compensated by an increase in the electronic thermal conductivity, which keeps the total thermal conductivity approximately constant. In consequence, the dimensionless figure-of-merit ZT reaches a maximum value of 0.81 at 762 K for x = 0.04.

cond-mat.mtrl-sci↗

arXiv2018

Exotic low-energy excitations emergent in the random Kitaev magnet Cu$_2$IrO$_3$

We report on magnetization $M(H)$, dc/ac magnetic susceptibility $χ(T)$, specific heat $C_{\mathrm{m}}(T)$ and muon spin relaxation ($μ$SR) measurements of the Kitaev honeycomb iridate Cu$_2$IrO$_2$ with quenched disorder. In spite of the chemical disorders, we find no indication of spin glass down to 260~mK from the $C_{\mathrm{m}}(T)$ and $μ$SR data. Furthermore, a persistent spin dynamics observed by the zero-field muon spin relaxation evidences an absence of static magnetism. The remarkable observation is a scaling relation of $χ[H,T]$ and $M[H,T]$ in $H/T$ with the scaling exponent $α=0.26-0.28$, expected from bond randomness. However, $C_{\mathrm{m}}[H,T]/T$ disobeys the predicted universal scaling law, pointing towards the presence of low-lying excitations in addition to random singlets. Our results signify an intriguing role of quenched disorder in a Kitaev spin system in creating low-energy excitations possibly pertaining to Z$_2$ fluxes.

cond-mat.str-el↗