arXiv subjects

C. H. Wong

Publications and source records attributed to C. H. Wong.

At least 19 recordsLinked to original sources

arXiv2026

Exotic Pressure-Driven Band Gap Widening in Carbon Chain-Filled KFI Zeolite and Its Pathway to High-Pressure Semiconducting Electronics and High-Temperature Superconductivity

Semiconducting devices face persistent challenges in operating at high pressure, as the band theory predicts that materials transition to a more metallic state under compression. However, our findings with carbon chains in KFI substrates reveal a conditional deviation from this norm. We not only witness the transition from polyyne (semiconductor) to cumulene (metal) at medium pressure, but we also observe an unexpected re-entrance of the polyyne at high pressures, where the band gap in the polyyne increases with pressure. In addition, the synthesis of long cumulene chains has posed a longstanding challenge in the quest for high-temperature organic superconductivity. We have identified critical conditions for synthesizing extended cumulene chains within zeolite frameworks, highlighting the interplay between unconventional charge density waves and significant torsions. The KFI zeolite facilitates the formation of carbon chains exceeding 5,000 atoms, in stark contrast to around 100 other zeolites that are limited to ~10 atoms. The cumulene@KFI system demonstrates a superconducting transition temperature reaching ~62 K, surpassing the highest reported values for bulk iron-based superconductors. This interplay between carbon structures and superconductivity not only advances our understanding of charge density waves but also heralds a new era in the study of novel applications

cond-mat.supr-con↗

arXiv2025

Taste breaking in the minimally doubled Karsten-Wilczek action and its tree-level improvement

Minimally doubled fermion actions offer a discretization for two-flavor Quantum Chromodynamics without rooting, but retaining a U(1) chiral symmetry at the same time. The price to pay is a breaking of the hypercubic symmetry, which requires the inclusion and tuning of new counterterms. Similar to staggered quarks, these actions suffer from taste breaking. We perform a mixed action numerical study with the Karsten-Wilczek formulation of minimally doubled fermions on 4stout staggered configurations, generated with physical quark masses, covering a broad range of lattice spacings. We consider a tree-level spatial Naik improvement to mitigate discretization errors. We carry out a non-perturbative tuning of the KW action with and without improvement, and investigate the taste breaking and the approach to the continuum limit.

hep-lat↗

arXiv2021

The GoogLeNet-assisted phase transition detectors

In the presence of the phase fluctuations in superconducting nanowires array, the electrical resistance of the superconducting nanowires is always non-zero unless the system undergoes Berezinskii-Kosterlitz-Thouless (BKT) transition where the superconducting vortices and anti-vortices form pairs. The two-dimensional XY model can mimic the superconducting transition temperature Tc and the BKT transition at a lower critical temperature TBKT by observing the heat capacity anomalies upon cooling. If the Josephson coupling across the nanowires is strong, the heat capacity anomalies almost overlap with each other so that it is difficult to distinguish between the Tc and the TBKT. To solve this issue, we apply an artificial-intelligence technique to split the nearly overlapped heat capacity anomalies. After the GoogLeNet-assisted phase transition detector is built, the GoogLeNet model can learn from the features of the phase transitions and then interpret the Tc and TBKT in the unseen system precisely. Our work opens a path for the GoogLeNet model to enter the world of magnetism and superconductivity.

cond-mat.supr-con↗

arXiv2021

The effectiveness of data augmentation in porous substrate, nanowire, fiber and tip images at the level of deep learning intelligence

To prepare for identifying the composition of nanowire-fiber mixtures in Scanning Electron Microscope (SEM) images, we optimize the performance of image classification between nanowires, fibers and tips due to their geometric similarities. The SEM images are analyzed by deep learning techniques where the validation accuracies of 11 convolutional neural network (CNN) models are compared. By increasing the diversity of data such as reflection, translation and scale factor approaches, the highest validation accuracy of recognizing nanowires, fibers and tips is 97.1%. We proceed to classify the level of porosity in anodized aluminum oxide for the self-assisted nanowire growth where the validation accuracy is optimized at 93%. Our software allow scientists to count the percentage of fibers in any nanowire-fiber composite and design the porous substrate for embedding different sizes of nanowires automatically, which assists the software development in Nanoscience Foundries & Fine Analysis (NFFA) Europe Projects.

cond-mat.mtrl-sci↗

arXiv2020

Spin and charge distributions in Graphene/Nickel (111) substrate under Rashba spin-orbital coupling

To understand the coupling factor between Rashba spin-orbital interaction and ferromagnetic proximity effect, we design a Monte Carlo algorithm to simulate the spin and charge distributions for the room-temperature Rashba material, Graphene/Nickel(111) substrate, at finite temperature. We observe that the rate of exchange fluctuation is a key player to produce giant Rashba spin-orbit splitting in graphene. More importantly, we monitor the Rashba spin-splitting phenomenon where the spin-polarized electrons may be escaped from two opposite edges upon heating. However, the escaped electrons show Gaussian-like distribution in interior area that is important for spintronic engineers to optimize the efficiency of spin-state detection. In addition, we investigate if our Monte Carlo model can explain why room-temperature Rashba effect is observed in Graphene/Nickel(111) substrate experimentally. All results are presented in physical units.

physics.comp-ph↗

arXiv2019

Enormous enhancement of p-orbital magnetism and band gap in the lightly doped carbyne

This paper presents a path to tailor adapted magnetic and optical properties in carbyne. Although p-orbital magnetism is generally much weaker than d-orbital magnetism, we demonstrate that the charge fluctuation of the free radical electrons triggered by a time-varying electric dipole moment leads to enormous p-orbital magnetism. By introducing 25% arsenic and 12.5% fluorine into the monoatomic carbon chain, the magnetic moment of the arsenic atom reaches 2.9 Bohr Magneton, which is ~1.3 times stronger than magnetic moment of bulk Fe. This magnetically optimized carbyne composite carries an exchange-correlation energy of 22meV (~270K). On the other hand, we convert the carbyne (in beta-form) from metallic to a semiconducting state by using anionic dopants. After doping 12.5% nitrogen and 12.5% oxygen into the beta-carbyne, the semiconducting gap of this composite is optimized at 1.6eV, which is 1.4 times larger than the band gap of bulk silicon.

cond-mat.mes-hall↗

arXiv2019

The interactions between antiferromagnetism, tetrahedral sites and electron-phonon coupling in FeSe1-xTex and FeSe/SrTiO3

We show that the superconducting transition temperature Tc of FeSe1-xTex can be computed to reasonable values in a modified McMillan approach in which the electron-phonon coupling is amplified by the antiferromagnetism and the out-of-plane phonons triggered by the tetrahedral lattice sites. This interplay is not only effective at ambient pressure, but also under hydrostatic compression. According to our model, the theoretical Tc of the compressed FeSe0.5Te0.5 agrees with experiment results. More importantly, by taking into account the interfacial effect between an FeSe monolayer and its SrTiO3 substrate as an additional gain factor, our calculated Tc value is up to 91 K high, and provides evidence that the strong Tc enhancement recently observed in such monolayers with Tc reaching 100 K may be due to an enhanced-electron phonon coupling.

cond-mat.supr-con↗

arXiv2018

Revisiting the semi-flexible entangled chains of polymer in the carbyne model

The Monte Carlo carbyne model is modified to investigate the glass transition of the semi-flexible entangled polymer chains. The stochastic bombardment between monomers are monitored by Metropolis algorithm with help of the consideration of hard potential while the mobility of monomers is governed by its mass, scattering rate and temperature. Our model is capable to show that the glass transition temperature reduces with decreasing film thickness and the formation of critical voids in the thinner polymer contributing to the glass transition that is much easier than the bulk polymer.

physics.comp-ph↗

arXiv2018

Electron-electron interactions of the multi-Cooper-pairs in the 1D limit and their role in the formation of global phase coherence in quasi-one-dimensional superconducting nanowire arrays

Nanostructuring of superconducting materials to form dense arrays of thin parallel nanowires with significantly large transverse Josephson coupling has proven to be an effective way to increase the upper critical field of superconducting elements by as much as two orders of magnitude as compared to the corresponding bulk materials and, in addition, may cause considerable enhancements in their critical temperatures. Such materials have been realized in the linear pores of mesoporous substrates or exist intrinsically in the form of various quasi-1D crystalline materials. The transverse coupling between the superconducting nanowires is determined by the size-dependent coherence length E0. In order to obtain E0 over the Langer-Ambegaokar- McCumber-Halperin (LAMH) theory, extensive experimental fitting parameters have been required over the last 40 years. We propose a novel Monte Carlo algorithm for determining E0 of the multi-Cooper pair system in the 1D limit. The concepts of uncertainty principle, Pauli-limit, spin flip mechanism, electrostatic interaction, thermal perturbation and co-rotating of electrons are considered in the model. We use Pb nanowires as an example to monitor the size effect of E0 as a result of the modified electron-electron interaction without the need for experimental fitting parameters. We investigate how the coherence length determines the transverse coupling of nanowires in dense arrays. This determines whether or not a global phase-coherent state with zero resistance can be formed in such arrays. Our Monte Carlo results are in very good agreement with experimental data from various types of superconducting nanowire arrays

cond-mat.supr-con↗

arXiv2018

High-pressure effects on isotropic superconductivity in the iron-free layered pnictide superconductor BaPd2As2

While the layered 122 iron arsenide superconductors are highly anisotropic, unconventional, and exhibit several forms of electronic orders that coexist or compete with superconductivity in different regions of their phase diagrams, we find in the absence of iron in the structure that the superconducting characteristics of the end member BaPd2As2 are surprisingly conventional. Here we report on complementary measurements of specific heat, magnetic susceptibility, resistivity measurements, Andreev spectroscopy, and synchrotron high pressure x-ray diffraction measurements supplemented with theoretical calculations for BaPd2As2. Its superconducting properties are completely isotropic as demonstrated by the critical fields, which do not depend on the direction of the applied field. Under the application of high pressure, Tc is linearly suppressed, which is the typical behavior of classical phonon-mediated superconductors with some additional effect of a pressure-induced decrease in the electronic density of states and the electron-phonon coupling parameters. Structural changes in the layered BaPd2As2 have been studied by means of angle-dispersive diffraction in a diamond-anvil cell. At 12 GPa and 24.2 GPa we observed pressure induced lattice distortions manifesting as the discontinuity and, hence discontinuity in the Birch-Murnaghan equation of state. The bulk modulus is B0=40(6) GPa below 12 GPa and B0=142(3) GPa below 27.2 GPa.

cond-mat.supr-con↗

arXiv2018

Thermal disorder in finite-length carbon nanowire

Chemisorption is one of the active research areas in carbon materials. The occurrence of the monoatomic carbon chain can be made by surrounding the double walled carbon nanotube and meanwhile worldwide efforts have been made to create the extraction technique for unlashing the carbon chains from the enclosure. Here we report an extensive study of the kink structure in the free standing carbon nanowires. Our Monte Carlo simulation considers the multi-monoatomic carbon chains laterally interacted by the Van der Waal force. Despite the linearity of the carbon nanowires is independent of chain length at low temperatures, the same situation does not hold at high temperatures. Disordered kink structure is observed in the short carbon chains especially above Peierls transition temperature. For instance, the average kink angle of 50-atoms carbon nanowire is as large as 35 degree at 800K. We have provided an important inspection that any physical property of the finite-length carbon chain predicted by ab-initio calculation should reconsider the atomic rearrangement due to the thermal instability. Apart from this, the kink structure in the nanowires likely increases the probability of attaching negatively charged atoms which is an encouragement to find the next generation materials for chemisorption.

cond-mat.mtrl-sci↗

arXiv2017

Superconductivity in ultra-thin carbon nanotubes and carbyne-nanotube composites: an ab-initio approach

The superconductivity of the 4-angstrom single-walled carbon nanotubes (SWCNTs) was discovered more than a decade ago, and marked the breakthrough of finding superconductivity in pure elemental undoped carbon compounds. The van Hove singularities in the electronic density of states at the Fermi level in combination with a large Debye temperature of the SWCNTs are expected to cause an impressively large superconducting gap. We have developed an innovative computational algorithm specially tailored for the investigation of superconductivity in ultrathin SWCNTs. We predict the superconducting transition temperature of various thin carbon nanotubes resulting from electron-phonon coupling by an ab-initio method, taking into account the effect of radial pressure, symmetry, chirality (N,M) and bond lengths. By optimizing the geometry of the carbon nanotubes, a maximum Tc of 60K is found. We also use our method to calculate the Tc of a linear carbon chain embedded in the center of (5,0) SWCNTs. The strong curvature in the (5,0) carbon nanotubes in the presence of the inner carbon chain provides an alternative path to increase the Tc of this carbon composite by a factor of 2.2 with respect to the empty (5,0) SWCNTs.

cond-mat.supr-con↗

arXiv2016

Effect of symmetry on the electronic DOS, charge fluctuations and electron-phonon coupling in carbon chains

A theoretical model is provided to address the parameters influencing the electronic properties of kink-structured carbon chain at 0K. It is studied by the principle of DFT and solving the numerical 1D time-independent Schrödinger equation of electron and phonon simultaneously. Two different lengths of branches A and B, are occupied alternatively to generate the asymmetric carbon chain. The ratio of the asymmetric branch length,RAB=A/B, plays an important role in the electronic density of states DOS around Fermi level Ef . The highest DOS(Ef) occurs if the RAB equals to 2 and while the Fermi level coincides with the Von-Hove singularity at RAB=3. The location of the singularity point relative to the Ef is controllable via branch length interestingly. By comparison with the symmetric case, tuning the branch length asymmetrically shows a stronger impact to shift the Ef to the singularity point. The numerical solution of the 1D time independent Schrodinger equation of phonon indicates that the kink reinforces the charge fluctuations but the fluctuations are minimized when the RAB goes up. Based on the simulation results, the electron phonon coupling of the carbon nanowire decreases with chain length. In comparison to the symmetric structure, the electron phonon coupling of the asymmetric carbon chain is higher. The maximum electron phonon coupling of the asymmetric carbon chain takes place at RAB=2 . However, the weakening of the electron phonon coupling is observed owing to ultrahigh concentration of kinks. The reduction of the electron phonon coupling of the carbon chain is occurred under pressure.

cond-mat.mtrl-sci↗

arXiv2016

Simulation of chemical bond distributions and phase transformation in carbon chains

In the present work we develop a Monte Carlo algorithm of the carbon chains ordered into 2D hexagonal array. The chemical bond of the chained carbon is computed from 1K to 1300K. Our model confirms that the beta phase is more energetic preferable at low temperatures but the system prefers the alpha phase at high temperatures. Based on the thermal effect on the bond distributions and 3D atomic vibrations in the carbon chains, the bond softening temperature is observed at 500K. The bond softening temperature is higher in the presence of interstitial doping but it does not change with the length of nanowire. The elastic modulus of the carbon chains is 1.7TPa at 5K and the thermal expansion is +7 x 10-5 K-1 at 300K via monitoring the collective atomic vibrations and bond distributions. Thermal fluctuation in terms of heat capacity as a function of temperatures is computed in order to study the phase transition across melting point. The heat capacity anomaly initiates around 3800K.

cond-mat.mtrl-sci↗

arXiv2014

Large gap, a pseudogap and proximity effect in the Bi2Te3/Fe1+yTe interfacial superconductor

We report directional point-contact spectroscopy data on the novel Bi2Te3/Fe1+yTe interfacial superconductor for a Bi2Te3 thickness of 9 quintuple layers, bonded by van der Waals epitaxy to a Fe1+yTe film at an atomically sharp interface. Our data show a very large superconducting twin-gap structure with an energy scale exceeding that of bulk FeSe or FeSe1-xTex by a factor of 4. While the larger gap is isotropic and attributed to a thin FeTe layer in proximity of the interface, the smaller gap has a pronounced anisotropy and is associated with proximity-induced superconductivity in the topological insulator Bi2Te3. Zero resistance is lost above 8 K, but superconducting fluctuations are visible up to at least 12 K and the large gap is replaced by a pseudogap that persists up to 40 K. The spectra show a pronounced zero-bias conductance peak in the superconducting state, which may be a signature of an unconventional pairing mechanism.

cond-mat.supr-con↗

arXiv2013

Extended hadron and two-hadron operators of definite momentum for spectrum calculations in lattice QCD

Multi-hadron operators are crucial for reliably extracting the masses of excited states lying above multi-hadron thresholds in lattice QCD Monte Carlo calculations. The construction of multi-hadron operators with significant coupling to the lowest-lying multi-hadron states of interest involves combining single hadron operators of various momenta. The design and implementation of large sets of spatially-extended single-hadron operators of definite momentum and their combinations into two-hadron operators are described. The single hadron operators are all assemblages of gauge-covariantly-displaced, smeared quark fields. Group-theoretical projections onto the irreducible representations of the symmetry group of a cubic spatial lattice are used in all isospin channels. Tests of these operators on 24^3 x 128 and 32^3 x 256 anisotropic lattices using a stochastic method of treating the low-lying modes of quark propagation which exploits Laplacian Heaviside quark-field smearing are presented. The method provides reliable estimates of all needed correlations, even those that are particularly difficult to compute, such as eta eta -> eta eta in the scalar channel, which involves the subtraction of a large vacuum expectation value. A new glueball operator is introduced, and the evaluation of the mixing of this glueball operator with a quark-antiquark operator, pi-pi, and eta-eta operators is shown to be feasible.

hep-lat↗

arXiv2012

Topological transport in a spin-orbit coupled bosonic Mott insulator

We investigate topological transport in a spin-orbit coupled bosonic Mott insulator. We show that interactions can lead to anomalous quasi-particle dynamics even when the spin-orbit coupling is abelian. To illustrate the latter, we consider the spin-orbit coupling realized in the experiment of Lin \textit{et al}. [Nature (London) \textbf{471}, 83 (2011)]. For this spin-orbit coupling, we compute the quasiparticle dispersions and spectral weights, the interaction-induced momentum space Berry curvature, and the momentum space distribution of spin density, and propose experimental signatures. Furthermore, we find that in our approximation for the single-particle propagator, the ground state can in principle support an integer Hall conductivity if the sum of the Chern numbers of the hole bands is nonzero.

cond-mat.str-el↗

arXiv2012

Spin-Seebeck effect in a strongly interacting Fermi gas

We study the spin-Seebeck effect in a strongly interacting, two-component Fermi gas and propose an experiment to measure this effect by relatively displacing spin up and spin down atomic clouds in a trap using spin-dependent temperature gradients. We compute the spin-Seebeck coefficient and related spin-heat transport coefficients as functions of temperature and interaction strength. We find that when the inter-spin scattering length becomes larger than the Fermi wavelength, the spin-Seebeck coefficient changes sign as a function of temperature, and hence so does the direction of the spin-separation. We compute this zero-crossing temperature as a function of interaction strength and in particular in the unitary limit for the inter-spin scattering.

cond-mat.quant-gas↗