arXiv subjects

C. Hoffmann

Publications and source records attributed to C. Hoffmann.

18 recordsLinked to original sources

arXiv2021

Collinear antiferromagnetic order in URu$_2$Si$_{2-x}$P$_x$ revealed by neutron diffraction

The hidden order phase in URu$_2$Si$_2$ is highly sensitive to electronic doping. A special interest in silicon-to-phosphorus substitution is due to the fact that it may allow one, in part, to isolate the effects of tuning the chemical potential from the complexity of the correlated $f$ and $d$ electronic states. We investigate the new antiferromagnetic phase that is induced in URu$_2$Si$_{2-x}$P$_x$ at $x\gtrsim0.27$. Time-of-flight neutron diffraction of a single crystal ($x=0.28$) reveals $c$-axis collinear $\mathbf{q}_\mathrm{m}=(\frac12,\frac12,\frac12)$ magnetic structure with localized magnetic moments ($\approx2.1\,\mu_\mathrm{B}$). This points to an unexpected analogy between the (Si,P) and (Ru,Rh) substitution series. Through further comparisons with other tuning studies of URu$_2$Si$_2$, we are able to delineate the mechanisms by which silicon-to-phosphorus substitution affects the system. In particular, both the localization of itinerant 5$f$ electrons as well as the choice of $\mathbf{q}_m$ appears to be consequences of the increase in chemical potential. Further, enhanced exchange interactions are induced by chemical pressure and lead to magnetic order, in which an increase in inter-layer spacing may play a special role.

cond-mat.str-el↗

arXiv2018

Soft antiphase tilt of oxygen octahedra in the hybrid improper multiferroic Ca3Mn1.9Ti0.1O7

We report a single crystal neutron and x-ray diffraction study of the hybrid improper multiferroic Ca3Mn1.9Ti0.1O7 (CMTO), a prototypical system where the electric polarization arises from the condensation of two lattice distortion modes.With increasing temperature (T ), the out-of-plane, antiphase tilt of MnO6 decreases in amplitude while the in-plane, in-phase rotation remains robust and experiences abrupt changes across the first-order structural transition. Application of hydrostatic pressure (P) to CMTO at room temperature shows a similar effect. The consistent behavior under both T and P reveals the softness of antiphase tilt and highlights the role of the partially occupied d orbital of the transition-metal ions in determining the stability of the octahedral distortion. Polarized neutron analysis indicates the symmetry-allowed canted ferromagnetic moment is less than the 0.04 {\mu}B/Mn site, despite a substantial out-of-plane tilt of the MnO6 octahedra.

cond-mat.str-el↗

arXiv2018

Single crystal growth of Cu4(OH)6BrF and universal behavior in quantum spin liquid candidates synthetic barlowite and herbertsmithite

Synthetic barlowite, Cu4(OH)6BrF, has emerged as a new quantum spin liquid (QSL) host, containing kagome layers of S=1/2 Cu2+ ions separated by interlayer Cu2+ ions. Similar to synthetic herbertsmithite, ZnCu3(OH)6Cl2, it has been reported that Zn2+ substitution for the interlayer Cu2+ induces a QSL ground state. Here we report a scalable synthesis of single crystals of Cu4(OH)6BrF. Through x-ray, neutron, and electron diffraction measurements coupled with magic angle spinning 19F and 1H NMR spectroscopy, we resolve the previously reported positional disorder of the interlayer Cu2+ ions and find that the structure is best described in the orthorhombic space group, Cmcm, with lattice parameters a = 6.665(13) A, b = 11.521(2) A, c = 9.256(18) A and an ordered arrangement of interlayer Cu2+ ions. Infrared spectroscopy measurements of the O-H and F-H stretching frequencies demonstrate that the orthorhombic symmetry persists upon substitution of Zn2+ for Cu2+. Specific heat and magnetic susceptibility measurements of Zn-substituted barlowite, ZnxCu4-x(OH)6BrF, reveal striking similarities with the behavior of ZnxCu4-x(OH)6Cl2. These parallels imply universal behavior of copper kagome lattices even in the presence of small symmetry breaking distortions. Thus synthetic barlowite demonstrates universality of the physics of synthetic Cu2+ kagome minerals and furthers the development of real QSL states.

cond-mat.str-el↗

arXiv2017

Extreme events in near integrable lattices

In the present work, we examine the potential robustness of extreme wave events associated with large amplitude fluctuations of the Peregrine soliton type, upon departure from the integrable analogue of the discrete nonlinear Schr\"odinger (DNLS) equation, namely the Ablowitz-Ladik (AL) model. Our model of choice will be the so-called Salerno model, which interpolates between the AL and the DNLS models. We find that rogue wave events essentially are drastically distorted even for very slight perturbations of the homotopic parameter connecting the two models off of the integrable limit. Our results suggest that the Peregrine soliton structure is a rather sensitive feature of the integrable limit, which may not persist under "generic" perturbations of the limiting integrable case.

nlin.PS↗

arXiv2015

On the Chemistry and Physical Properties of Flux and Floating Zone Grown SmB6 Single Crystals

Recent theoretical and experimental findings suggest that the long-known but not well understood low temperature resistance plateau of SmB6 may originate from protected surface states arising from a topologically non-trivial bulk band structure having strong Kondo hybridization. Yet other studies have ascribed this feature to impurity phases, sample vacancies, and surface reconstructions. Given the typical methods used to prepare SmB6 single crystals, the flux and floating zone procedures, these ascriptions should not be taken lightly. Here, we demonstrate how compositional variations and observable amounts of impurity phases in SmB6 crystals grown by floating zone and flux affect the physical properties. From neutron diffraction and X-ray computed tomography experiments, we observe that a 154Sm11B6 crystal prepared using aluminum flux contains co-crystallized, epitaxial aluminum. A large, nearly stoichiometric crystal of SmB6 was successfully grown using the float-zone technique; upon continuing the zone melting, samarium vacancies are introduced. These samarium vacancies drastically alter the resistance and plateauing magnitude of the low temperature resistance compared to stoichiometric SmB6. These results highlight that small presences of impurity phases and compositional variations must be considered when collecting and analyzing physical property data of SmB6. Finally, a more accurate samarium-154 coherent neutron scattering length value, 8.9(1) fm, is reported.

cond-mat.str-el↗

arXiv2011

A dual-band millimeter-wave kinetic inductance camera for the IRAM 30-meter telescope

Context. The Neel IRAM KIDs Array (NIKA) is a fully-integrated measurement system based on kinetic inductance detectors (KIDs) currently being developed for millimeter wave astronomy. In a first technical run, NIKA was successfully tested in 2009 at the Institute for Millimetric Radio Astronomy (IRAM) 30-meter telescope at Pico Veleta, Spain. This prototype consisted of a 27-42 pixel camera imaging at 150 GHz. Subsequently, an improved system has been developed and tested in October 2010 at the Pico Veleta telescope. The instrument upgrades included dual-band optics allowing simultaneous imaging at 150 GHz and 220 GHz, faster sampling electronics enabling synchronous measurement of up to 112 pixels per measurement band, improved single-pixel sensitivity, and the fabrication of a sky simulator to replicate conditions present at the telescope. Results. The new dual-band NIKA was successfully tested in October 2010, performing in-line with sky simulator predictions. Initially the sources targeted during the 2009 run were re-imaged, verifying the improved system performance. An optical NEP was then calculated to be around 2 \dot 10-16 W/Hz1/2. This improvement in comparison with the 2009 run verifies that NIKA is approaching the target sensitivity for photon-noise limited ground-based detectors. Taking advantage of the larger arrays and increased sensitivity, a number of scientifically-relevant faint and extended objects were then imaged including the Galactic Center SgrB2(FIR1), the radio galaxy Cygnus A and the NGC1068 Seyfert galaxy. These targets were all observed simultaneously in the 150 GHz and 220 GHz atmospheric windows.

astro-ph.IM↗

arXiv2010

NIKA: A millimeter-wave kinetic inductance camera

Current generation millimeter wavelength detectors suffer from scaling limits imposed by complex cryogenic readout electronics. To circumvent this it is imperative to investigate technologies that intrinsically incorporate strong multiplexing. One possible solution is the kinetic inductance detector (KID). In order to assess the potential of this nascent technology, a prototype instrument optimized for the 2 mm atmospheric window was constructed. Known as the Néel IRAM KIDs Array (NIKA), it was recently tested at the Institute for Millimetric Radio Astronomy (IRAM) 30-meter telescope at Pico Veleta, Spain. The measurement resulted in the imaging of a number of sources, including planets, quasars, and galaxies. The images for Mars, radio star MWC349, quasar 3C345, and galaxy M87 are presented. From these results, the optical NEP was calculated to be around $1 \times 10^{-15}$ W$ / $Hz$^{1/2}$. A factor of 10 improvement is expected to be readily feasible by improvements in the detector materials and reduction of performance-degrading spurious radiation.

astro-ph.IM↗

arXiv2008

In-situ measurement of the permittivity of helium using microwave NbN resonators

By measuring the electrical transport properties of superconducting NbN quarter-wave resonators in direct contact with a helium bath, we have demonstrated a high-speed and spatially sensitive sensor for the permittivity of helium. In our implementation a $\sim10^{-3}$ mm$^3$ sensing volume is measured with a bandwidth of 300 kHz in the temperature range 1.8 to 8.8 K. The minimum detectable change of the permittivity of helium is calculated to be $\sim6\times$$10^{-11}$ $ε_0$/Hz$^{1/2}$ with a sensitivity of order $10^{-13}$ $ε_0$/Hz$^{1/2}$ easily achievable. Potential applications include operation as a fast, localized helium thermometer and as a transducer in superfluid hydrodynamic experiments.

cond-mat.other↗

arXiv2008

On-orbit Performance of the Solar Optical Telescope aboard Hinode

On-orbit performance of the Solar Optical Telescope (SOT) aboard Hinode is described with some attentions on its unpredicted aspects. In general, SOT revealed an excellent performance and has been providing outstanding data. Some unexpected features exist, however, in behaviors of the focus position, throughput and structural stability. Most of them are recovered by the daily operation i.e., frequent focus adjustment, careful heater setting and corrections in data analysis. The tunable filter contains air bubbles which degrade the data quality significantly. Schemes for tuning the filter without disturbing the bubbles have been developed and tested, and some useful procedures to obtain Dopplergram and magnetogram are now available. October and March when the orbit of satellite becomes nearly perpendicular to the direction towards the sun provide a favorable condition for continuous runs of the narrow-band filter imager.

astro-ph↗

arXiv2006

Molecular states in carbon nanotube double quantum dots

We report electrical transport measurements through a semiconducting single-walled carbon nanotube (SWNT) with three additional top-gates. At low temperatures the system acts as a double quantum dot with large inter-dot tunnel coupling allowing for the observation of tunnel-coupled molecular states extending over the whole double-dot system. We precisely extract the tunnel coupling and identify the molecular states by the sequential-tunneling line shape of the resonances in differential conductance.

cond-mat.mes-hall↗

arXiv2004

Shot-noise and conductance measurements of transparent superconductor / two-dimensional electron gas junctions

We have measured the conductance and shot-noise of superconductor-normal metal (S-N) junctions between a Niobium (Nb) film and a 2-dimensional electron gas (2DEG), formed in an InAs-based semiconductor heterostructure. Adjacent to the junction, the 2DEG is shaped into a submicrometer beam-splitter. The current shot-noise measured through one arm of the beam-splitter is found to be enhanced due to Andreev reflection. Both noise and conductance measurements indicate that the Nb-2DEG interface is of high quality with a transparency approaching approx. 60-70 %. The present device can be seen as a quasi-ballistic S-N beam-splitter junction.

cond-mat.mes-hall↗

arXiv2004

Mesoscopic transition in the shot noise of diffusive S/N/S junctions

We experimentally investigated the current noise in diffusive Superconductor/Normal metal/Superconductor junctions with lengths between the superconducting coherence length xi_Delta and the phase coherence length L_Phi of the normal metal (xi_Delta < L < L_Phi). We measured the shot noise over a large range of energy covering both the regimes of coherent and incoherent multiple Andreev reflections. The transition between these two regimes occurs at the Thouless energy where a pronounced minimum in the current noise density is observed. Above the Thouless energy, in the regime of incoherent multiple Andreev reflections, the noise is strongly enhanced compared to a normal junction and grows linearly with the bias voltage. Semi-classical theory describes the experimental results accurately, when taking into account the voltage dependence of the resistance which reflects the proximity effect. Below the Thouless energy, the shot noise diverges with decreasing voltage which may indicate the coherent transfer of multiple charges.

cond-mat.mes-hall↗

arXiv2003

Doubled Full Shot Noise in Quantum Coherent Superconductor - Semiconductor Junctions

We performed low temperature shot noise measurements in Superconductor (TiN) - strongly disordered normal metal (heavily doped Si) weakly transparent junctions. We show that the conductance has a maximum due to coherent multiple reflections at low energy and that shot noise is then twice the Poisson noise (S=4eI). The shot noise changes to the normal value (S=2eI) due to a large quasiparticle contribution.

cond-mat.mes-hall↗

arXiv2002

Inelastic relaxation and noise temperature in S/N/S junctions

We studied electronic relaxation in long diffusive superconductor / normal metal / superconductor (S/N/S) junctions by means of current noise and transport measurements down to very low temperature (100mK). Samples with normal metal lengths of 4, 10 and 60 micrometer have been investigated. In all samples the shot noise increases very rapidly with the voltage. This is interpreted in terms of enhanced heating of the electron gas confined between the two S/N interfaces. Experimental results are analyzed quantitatively taking into account electron-phonon interaction and heat transfer through the S/N interfaces. Transport measurements reveal that in all samples the two S/N interfaces are connected incoherently, as shown by the reentrance of the resistance at low temperature. The complementarity of noise and transport measurements allows us to show that the energy dependence of the reentrance at low voltage is essentially due to the increasing effective temperature of the quasiparticles in the normal metal.

cond-mat.mes-hall↗

arXiv2002

Mesoscopic proximity effect in double barrier Superconductor/Normal Metal junctions

We report transport measurements down to T=60mK of SININ and SNIN structures in the diffusive limit. We fabricated Al-AlOx/Cu/AlOx/Cu (SININ) and Al/Cu/AlOx/Cu (SNIN) vertical junctions. For the first time, a zero bias anomaly was observed in a metallic SININ structure. We attribute this peak of conductance to coherent multi-reflections of electrons between the two tunnel barriers. This conductance maximum is quantitatively fitted by the relevant theory of mesoscopic SININ structures. When the barrier at the SN interface is removed (SNIN structure), we observe a peak of conductance at finite voltage accompagnied by an excess of sub-gap conductance.

cond-mat.mes-hall↗

arXiv1999

Carrier relaxation, pseudogap, and superconducting gap in high-Tc cuprates: A Raman scattering study

We describe results of electronic Raman-scattering experiments in differently doped single crystals of Y-123 and Bi-2212. The comparison of AF insulating and metallic samples suggests that at least the low-energy part of the spectra originates predominantly from excitations of free carriers. We therefore propose an analysis of the data in terms of a memory function approach. Dynamical scattering rates and mass-enhancement factors for the carriers are obtained. In B2g symmetry the Raman data compare well to the results obtained from ordinary and optical transport. For underdoped materials the dc scattering rates in B1g symmetry become temperature independent and considerably larger than in B2g symmetry. This increasing anisotropy is accompanied by a loss of spectral weight in B2g symmetry in the range between the superconducting transition at Tc and a characteristic temperature T* of order room temperature which compares well with the pseudogap temperature found in other experiments. The energy range affected by the pseudogap is doping and temperature independent. The integrated spectral loss is approximately 25% in underdoped samples and becomes much weaker towards higher carrier concentration. In underdoped samples, superconductivity related features in the spectra can be observed only in B2g symmetry. The peak frequencies scale with Tc. We do not find a direct relation between the pseudogap and the superconducting gap.

cond-mat.supr-con↗

arXiv1999

Non linear flux flow in TiN superconducting thin film

We have studied the superconducting behavior of 100 nm Titanium Nitride (TiN) thin film in a perpendicular magnetic field. We found a zero field transition temperature of 4.6 K and a slope in the H-T plane of -0.745 T/K. At 4.2 K, we have performed careful transport measurements by measuring both the differential resistivity and voltage as a function of a DC current. Our results are analyzed in the framework of linear and non linear flux flow behavior. In particular, we have observed an electronic instability at high vortex velocities and from its dependence with respect to the applied magnetic field, we can exctract the inelastic scattering time and diffusion length of the quasiparticles.

cond-mat.supr-con↗

arXiv1998

Enhanced Electron-Phonon Coupling and its Irrelevance to High T$_{c}$ Superconductivity

It is argued that the origin of the buckling of the CuO$_{2}$ planes in certain cuprates as well as the strong electron-phonon coupling of the $B_{1g}$ phonon is due to the electric field across the planes induced by atoms with different valence above and below. The magnitude of the electric field is deduced from new Raman results on YBa$_{2}$Cu$_{3}$O$_{6+x}$ and Bi$_{2}$Sr$_{2}$(Ca$_{1-x}$Y$_{x}$)Cu$_{2}$O$_{8}$ with different O and Y doping, respectively. In the latter case it is shown that the symmetry breaking by replacing Ca partially by Y enhances the coupling by an order of magnitude, while the superconducting $T_c$ drops to about two third of its original value.

cond-mat.supr-con↗